强流高电荷态Pb离子束的产生与优化研究

随着原子物理及表面物理研究的发展,电荷态金属离子束的需求日益增多. 近来,中国科学院近代物理研究所,14.5GHz LECR3,离子源实验平台上, 以炉子法产生的铅离子束作为研究对象, 进行了一系列,ECR,离子源关键参数(如：磁场、炉子功率、掺气等)影响高电荷态铅离子束产额的实验研究, 在此基础上, 调整优化了,LECR3,离子源的状态参数, 从而获得了强流高电荷态铅离子束,18eμa ²⁰⁷Pb³⁰⁺,和6.7eμa ²⁰⁷Pb³⁷⁺.     

Afterglow工作模式下ECR离子源脉冲束的产生

为满足国家大科学工程兰州重离子冷却储存环的要求,在14.5GHz ECR 离子源上进行afterglow工作模式的实验,首次产生了高电荷态脉冲束流Ar¹¹⁺和Ar¹²⁺,给出了初步实验结果,并对结果进行了分析和解释.     

高离化态硫离子光谱的理论分析

 在考虑组态相互作用的基础上,利用包含相对论修正的Hartree-Fock(HFR)理论对S⁸⁺-S¹³⁺离子的谱线波长及加权振子强度等有关原子参数进行了系统计算,并与最新的实验观测和其它理论计算结果进行了比较。计算结果表明：S⁸⁺-S¹¹⁺的各个原子态在LS耦合下纯度很高,随着离化度的增大,S¹²⁺和S¹³⁺离子的部分原子态能级出现混合,组态相互作用逐渐增强。通过对实验结果的分析,识别出32条实验谱线,其中大多数谱线来自S⁸⁺-S¹³⁺离子的2s²2p^k-2s2p^k+1和2s2p^k+1-2s2p^k+2(k=0,1,2,3,4)之间的跃迁,理论计算结果与实验谱线波长之间的绝对误差大多数都在实验的有效分辨力以内。     

中能区86Kr+197Au反应中的能量耗散、π介子阈下产生和流角

用扩展BUU模型计算了中能区⁸⁶Kr+¹⁹⁷Au重系统的能量耗散、π介子阈下产生和流角,定量地拟合了43MeV/u ⁸⁶Kr+¹⁹⁷Au实验的能量耗散和类弹碎片核电荷数的关系及类弹类靶碎片核电荷数的关联.     

ECR离子源金属离子的产生

讨论了ECR离子源金属供料方法,在145GHzECR离子源上应用炉子加热和MIVOC法获得了⁴⁰Ca¹¹⁺140eμA和⁵⁶Fe¹⁰⁺65eμA,并对实验过程和结果作了分析.     

相对论效应对类锂离子能级结构及辐射跃迁性质的影响

利用基于多组态Dirac-Hartree-Fock(MCDHF) 理论方法的相对论原子结构计算程序包GRASP2K, 细致计算了中性锂原子、类锂Be⁺, C³⁺, O⁵⁺, Ne⁷⁺, Ar¹⁵⁺, Fe²³⁺, Mo³⁹⁺, W⁷¹⁺及U^{89 +} 离子基组态及较低的激发组态1s²nl (n = 2---4, l =s,p,d,f) 的精细结构能级, 以及各能级间发生电偶极(E1) 自发辐射跃迁的能量、概率及振子强度. 同时, 在非相对论极限下, 计算了其相关原子参数. 通过对相对论及非相对论计算结果的比较, 系统研究了相对论效应对类锂等电子系列离子能级结构及E1跃迁性质的影响, 揭示了随原子核电荷数Z变化时, 跃迁能、振子强度强烈依赖于量子数n, l, j变化的规律; 同时, 目前的计算结果与其他已有的理论计算及实验测量结果进行了比较.     

纳秒激光电离分子团簇产生高离化离子的激光波长效应

 利用脉冲分子束-激光电离-飞行时间质谱仪，在10⁹～10¹² W·cm^-2激光功率密度条件下，考察了Nd：YAG激光器输出的1 064，532，266 nm波长的激光与苯、氨、硫化氢等团簇的相互作用。发现1 064 nm的激光可以电离分子束产生高离化态的C⁴⁺，N⁵⁺，S⁶⁺等离子；波长为532 nm的激光则电离产生价态较低的C³⁺，C²⁺，N³⁺，N²⁺， S⁴⁺，S³⁺以及S²⁺ 等离子；在266 nm波长条件下进行实验，没有产生任何高价离子。提出了一个“多光子电离引发-逆轫致吸收加热-电子碰撞电离”模型来解释高价离子的产生。激光场下电子在团簇内部的逆轫致加热是整个过程的关键步骤，电子被加热的速度正比于激光波长的平方。这可以解释为何长波长的激光有利于更高价态离子的产生。     

变形核的电荷密度分布

本文应用原子核的宏观模型提出了一种比较简单的计算变形核电荷密度的方法.具体计算了¹⁹²Os、¹⁵⁴Gd、¹⁵²Sm、¹⁷⁴Yb、及^{144,148,150,152}Sm等原子核的电荷密度分布.结果表明,宏观模型计算的结果能较好地与实验测量结果相符合.因此,只要根据变形核基态到各转动态跃迁几率或电多极矩的实验值,则可按本文方法,从理论上预言变形核的电荷密度分布.     

ψ(2S)→ρπ及ψ(2S)→KK衰变的研究

利用在北京谱仪上获取的1.27×10⁶ψ(2S)事例研究了末态为矢量介子与赝标量分子的ψ(2S)两体衰变过程,ψ(2S)→ρπ及KK,得到它们的衰变分支比上限在90%置信度下分别为3.6×10^－5(ρπ),2.5×10^－5(K+K-+C.C.)(C.C.代表电荷共轭态)及1.2×10^－4(K0K0+C.C.).这些结果在新的实验灵敏度水平上证实了ψ(2S)相对于J/ψ强衰变中的反常压制现象的存在.     

谷氨酰胺与碱金属及碱土金属离子络合物的构象和金属离子亲和势：第一性原理研究

利用第一性原理对谷氨酰胺和碱金属及碱土金属络合物的构象与金属离子亲和势做了系统性计算,提出一种搜索络合物低能构象的高效方法,并将其应用于Gln.M^+/++ (M^+/++=Li⁺、Na⁺、K⁺、Rb⁺、Cs⁺、Be⁺⁺、Mg⁺⁺、Ca⁺⁺、Sr⁺⁺和Ba⁺⁺)．应用该方法不仅找到了已经报道的所有结构,还发现了许多新的重要构象,表明了该方法的可靠性与必要性．使用B3LYP、BHandHLYP以及MP2计算了各种重要构象的金属络合模式、偶极矩以及平衡构象分布,给出了相应的红外谱以及金属离子结合的焓变和吉布斯自由能的变化,并与现有实验结果作了对比．     

高电荷态ECR离子源的金属离子产生

简单介绍了采用炉子加热、 挥发性金属化合物和溅射产生ECR离子源的金属离子的3种方法和实验结果, 主要研究了铜、 锌、 镍和铁等多种电荷态离子的产生．　对3种方法分别进行了探讨．To satisfy the requirements of HIRFL (Heavy Ion Research Facility in Lanzhou), series of experiments have been done to produce metallic ion beams. By now, numerous methods have been tested, in which MIVOC (Metallic Ion from Volatile Compounds), heating oven methods and plasma sputter methods are all included. According to the experiments, the results of using MIVOC methods and heating oven methods are very good. In most of our researches, emphasis was put upon the ion production of iron, Nickel, Tantanum, copper of different charge states. Among the ion beams we have obtained, 210 μA Fe11+, 175 μA Fe12+, 142 μA Fe13+, 25 μA Fe16+, 64 μA Ni10+, 57 μA Ni13+, 31 μA Ni15+ and 15 μA Ni16+ are representative results.     

近物所在产生金属离子束方面的研究

Since 1998,many experiments for metallic ion production have been done on LECR2(Lanzhou ECR ion source NO.2),LECR3(Lanzhou ECR ion source NO.3)and SECRAL(Superconductiong ECB ion source Advanced design in Lanzhou)at Institute of Modern Physics.The very heavy metallic ion beams such as those of uranium were also produced by the plasma sputtering method,and supplied for HIRFL(Heavy Ion Research Facility in Lanzhou)accelerators successfully.During the test,11.SeμAU~(28 ),9eμAU~(24 ) were obtained.Some ion beams of the metal having lower melting temperature such as Ni and Mg ion beams were produced by oven method on LECR3 too.The consumption rate was controlled to be lower for ~(26)Mg ion beams production,and the minimum consumption was about 0.3mg per hour.In this paper,the main experimental results are given.Some discussions are made for some experimental phenomena and results,and some conclusions are drawn.     

LBNL14GHz离子源AECR-U的最新进展

A radial sputter probe has been developed for the AECR-U as an additional method of producing metal ion beams.Negative voltage is applied to the probe to incite collisions with target atoms,thereby sputtering material into the plasma.The sputter probe is positioned through one of the 6 radial access slots between the permanent hexapole structure of the AECR-U.The probe position can be varied with respect to the inner edge of the hexapole magnet structure.Charge state distributions and peak beam intensities at bias voltages up to-5kV were obtained for gold samples at varying distances of the probe with respect to the plasma.For high charge states production the radial position with respect to the plasma was more sensitive than for the medium and lower charge states.For high charge state ion production the probe was optimized at a distance of 0.6cm inside the chamber wall(4.1cm from the center of the chamber).Stable beams with peak intensities of up to 28eμA of Au~(24 ) and 1.42eμA of Au~(41 ) have been produced using the sputter probe technique. In addition,a solid state circuit under development by Scientific Solutions,Inc which provides a bandwidth up to 100MHz was used to drive the 14GHz klystron amplifier for the LBNL AECR-U ion source.Various broadband and discrete heating modes were tested and the results for high charge state ion production were compared with single frequency heating.     

Argonne国家实验室ECR离子源在固体材料离子束流产生方面的研究进展

Development work with solid materials at the Argonne National Laboratory ECR ion sources has been focused on two areas-introduction of materials with low vapour pressures,and increasing the beam intensities of heavy beams(i.e.-lead and uranium).An induction oven,with a demonstrated operating temperature extending to 2000℃,has been utilized to produce a Ti-50 beam with an intensity of 5.5eμA (12 ).In addition,a refinement of the sputter technique has been employed which has resulted in a 42% improvement in lead beam intensities.Details of the induction oven as well as the refined sputter technique will be presented.     

SECRAL在18GHz频率下产生强流高电荷态离子束的初步结果

A Superconducting ECR ion source with Advanced design in Lanzhou (SECRAL) was successfully built to produce intense beams of highly charged ions for Heavy Ion Research Facility in Lanzhou (HIRFL).The ion source has been optimized to be operated at 28GHz for its maximum performance.The superconducting magnet confinement configuration of the ion source consists of three axial solenoid coils and six sextupole coils with a cold iron structure as field booster and clamping.For 28GHz operation,the magnet assembly can produce peak mirror fields on axis 3.6T at injection,2.2T at extraction and a radial sextupole field of 2.0T at plasma chamber wall.A unique feature of SECRAL is that the three axial solenoid coils are located inside of the sextupole bore in order to reduce the interaction forces between the sextupole coils and the solenoid coils. During the ongoing commissioning phase at 18GHz with a stainless steel chamber,tests with various gases and some metals have been conducted with microwave power less than 3.2kW and it turned out the performance is very promising.Some record ion beam intensities have been produced,for instance,810eμA of O~(7 ),505eμA of Xe~(20 ),306eμA of Xe~(27 ),21eμA of Xe~(34 ),2.4eμA of Xe~(38 ) and so on.To reach better results for highly charged ion beams,further modifications such as an aluminium chamber with better cooling,higher microwave power and a movable extraction system will be done,and also emittance measurements are being prepared.     

强脉冲离子束辐照金属材料表面热力学效应计算

 简要讨论了强脉冲离子束与金属靶材料相互作用的理论模型,以此为基础应用数值计算的方法模拟计算了离子能量为1.0 MeV和300 keV,束流密度分别为10 A/cm²、50 A/cm²、100 A/cm²的质子束与金属铝靶材料相互作用时的热力学效应,给出了铝在辐照后内部的温度分布、温度梯度分布,以及温度变化速率（加热速率与冷却速率）、热激波的产生与传播过程及与应力等模拟计算结果。     

Discharge characteristics of the DUHOCAMIS with a high magnetic bottle-shaped field

For the purpose of producing high intensity, multiply charged metal ion beams, the dual hollow cathode ion source for metal ions (DUHOCAMIS) was derived from the hot cathode Penning ion source combined with the hollow cathode sputtering experiments in 2007. To investigate the behavior of this discharge geometry in a stronger magnetic bottle-shaped field, a new test bench for DUHOCAMIS with a high magnetic bottle-shaped field up to 0.6 T has been set up at the Peking University. The experiments with magnetic fields from 0.13 T to 0.52 T have indicated that the discharge behavior is very sensitive to the magnetic flux densities. The slope of discharge curves in a very wide range can be controlled by changing the magnetic field as well as regulated by adjusting the cathode heating power; the production of metallic ions would be much greater than gas ions with the increased magnetic flux density; and the magnetic field has a much higher influence on the DHCD mode than on the PIG mode.     

兰州全永磁ECR离子源——LAPECR1

The Lanzhou All Permanent magnet ECR ion source NO.1(LAPECR1)is the first all permanent magnet multiple ECRIS made in IMP.This ECRIS is running at 14.5GHz and can provide intense low charge state ion beams(varying from several to hundreds of eμA)or medium charge state ion beams(varying from several to tens of eμA).The size of source body is (?)102mm×296mm,the compactness and economical features enable the source suitable to be put on a HV platform or equipped by a small laboratory.This article gives the main parameters of the ion source.     

Ultrafine particle formation by resonant laser excitation of potassium molecules

In a heat pipe oven containing potassium and a noble gas we have observed a large production of metallic potassium particles upon resonant laser excitation of the K₂ molecules. This is a new method for particle production, based on the strong local heating of the vapor due to the high absorption rate of the laser light. As a consequence of the disequilibrium caused at the gas/vapour boundary by this heating, a supersaturated region is created where the vapor condenses and produces ultrafine particles.     

环糊精锌(Ⅱ)荧光试剂在水分析中的应用研究

合成高水溶性的锌()荧光试剂-修饰环糊精的N-(8-对氨基苯磺酰)胺基喹啉(HQAS-1-CD)。该试剂在水溶液中与Zn2+形成2:1配合物而使荧光增强,并且碱金属或碱土金属离子几乎不干扰Zn2+的荧光。利用此配位反应建立了一个荧光测定痕量锌的新方法,测定锌的线性范围为0—13μg/L,检出限0.57μg/L,方法成功的应用于矿泉水中痕量锌的测定。