高能质子在散裂靶中的能量沉积计算与实验验证

高能质子在散裂靶中的能量沉积是散裂靶中子学研究的重要内容之一,准确掌握高能质子在散裂靶中引起的能量沉积分布与瞬态变化是开展散裂靶热工流体设计的重要前提.本文采用MCNPX,PHITS与FLUKA三种蒙特卡罗模拟程序,计算并比较了高能质子入射重金属铅靶、钨靶的能量沉积分布及不同粒子对总能量沉积的占比贡献;针对高能质子入射金属钨靶的能量沉积实验数据空白,采用热释光探测器阵列测量了250 MeV质子束入射厚钨靶的能量沉积分布,实验结果表明蒙特卡罗模拟程序在散裂靶中能量沉积的计算结果具有较高的可靠性.     

中高能质子入射碎片质量分布研究

中高能质子轰击靶的碎片的质量分布是了解散裂中子靶的放射性累积和对靶材料性能的影响的一个重要方面.利用在级联-激子模型(CEM)的基础上发展起来的“多步动力学”模型(MSDM,Many Stage Dynamical Model)分别研究了入射质子能量为334,572,775,1200,1500和2600MeV轰击Nb靶,329,555,760,1200,1500和2600MeV轰击¹⁹⁷Au靶,160,230,271,322,533,660,759,1400,1600和2600MeV轰击Pb靶引起的碎片的质量分布,并和实验测量数据进行了比较.     

400~1500 MeV质子轰击铅靶和钨靶的出射中子能谱的FLUKA和Geant4模拟研究

在ADS散裂靶系统的优化设计中,蒙特卡罗方法结合可靠的散裂反应理论模型进行中子学计算具有重要的作用。本工作利用Geant4程序中的INCLXX模型、BIC模型以及BERT模型和FLUKA程序分别模拟了597 MeV和1 500 MeV质子轰击薄铅靶不同出射角度的中子双微分截面,500,1 500 MeV质子轰击厚铅靶不同出射角度的中子双微分产额,以及400,600,800,1 000和1 200 MeV质子轰击厚钨靶在反角方向（175 °）的中子双微分产额,并与实验数据进行比较。研究表明,对于薄铅靶,Geant4程序的INCLXX模型和FLUKA程序模拟结果与实验符合得更好。能量在10～40 MeV范围内,BIC模型模拟结果明显高于实验数据,而BERT模型模拟结果略微低于实验数据。对于厚铅靶,在40 MeV左右所有的模拟结果都低于实验数据。对于厚钨靶,Geant4程序的BIC模型和FLUKA程序与实验数据符合得较好,INCLXX模型在能量高于60 MeV时模拟结果低于实验数据,BERT模型与实验数据差异较大。总体来看,Geant4程序的INCLXX模型和FLUKA程序进行ADS散裂靶相关的中子学的计算是合理和可靠的。The reliable Monte Carlo simulation codes coupled with nuclear reaction models play an important role in the neutronic calculation for the design and optimization of the ADS spallation target. In this work, the double differential cross sections at different angles produced from a thin lead target bombarded with 597 and 1 500 MeV protons, the neutron energy spectra at different angles produced from a thick lead target bombarded with 500 and 1 500 MeV protons, and the neutron energy spectra in the backward direction(175°) produced from a thick tungsten target bombarded with 400, 600, 800, 1 000 and 1 200 MeV protons are calculated with the Geant4 code coupled INCLXX, BIC and BERT models and the FLUKA code. The calculations are compared with the available experimental data. The results show that, for the thin lead target, the calculations with the Geant4 coupled INCLXX model and FLUKA code well reproduce the experimental results. In a energy range from 10 to 40 MeV, BIC model obviously overestimates the experimental results, and BERT model slightly underestimates the experimental results. For the thick lead target, all of the calculations underestimate the experimental results around 40MeV. For the thick tungsten target, the Geant4 coupled BIC model and FLUKA code well reproduce the experimental results. INCLXX model underestimates the experimental results above 60 MeV. BERT model bad reproduces the experimental results. Overall, the neutronic calculations with the Geant4 code coupled INCLXX model and FLUKA code for the ADS spallation target is reasonable and reliable.     

GEANT4和FLUKA计算256 MeV质子诱发散裂中子能谱

散裂反应产生的中子能谱等数据是ADS系统设计中的关键参数。由于涉及到的能量范围大、反应道复杂,目前没有完善的评价核数据库可供使用,需要使用合适的核理论模型来进行计算。CiADS （Chinainitiative Accelerator Driven System）即将开始建设,在第一阶段将使用能量约为250 MeV的质子束。利用FLUKA及GEANT4中的BERT_HP、BIC_HP和INCLXX_HP等物理模型列表分别计算了256 MeV质子轰击薄的铝、铁、铅和铀靶后,在7.5°,30°,60°和150°等方向出射的中子双微分截面及轰击厚的铝、铁和铀靶后,在30°,60°,120°和150°等方向出射的中子双微分产额,并与已有的实验数据进行对比。结果表明,FLUKA和INCLXX_HP的计算结果整体上能够更好地符合实验数据。BIC_HP计算的薄靶结果,除铝靶的150°和铅靶的30°外,在5~30 MeV能量范围内要明显高于实验结果,能够达到实验结果的2倍以上。BIC_HP计算的厚铀靶结果在30°和60°方向的5~30 MeV能量范围内要比实验结果高出70%以上,在120°和150°方向的5 MeV以上要高于实验结果的2倍。BERT_HP计算的7.5°和30°方向上铝、铁和铅靶结果在20s100 MeV要比实验结果低40%以上,计算的铀靶结果在20 MeV以下能够达到实验结果的2倍以上。Neutron spectra produced through spallation reaction are key parameters in the design of Accelerator Driven Subcritical Systems. Since the energy span is large and reaction channels are complicated, no complete evaluated nuclear data library is ready for use. Suitable theoretical models are required to calculate the data. The CiADS (China initiative Accelerator Driven System) is going to be constructed in China. At the first stage, the adopted proton energy is about 250 MeV. FLUKA and GEANT4 are used to calculate the double differential cross sections at 7.5°, 30°, 60° and 150° induced by 256 MeV protons bombarding on thin aluminum, iron, lead and uranium targets, respectively. The double differential neutron yields at 30°, 60°, 120° and 150° are also calculated for 256 MeV protons bombarding on thick aluminum, iron and uranium targets, respectively. Three model lists INCLXX_HP, BIC_HP and BERT_HP implemented in GEANT4 are used separately. The calculation results are compared with corresponding experimental data. It is shown that results calculated with FLUKA and INCLXX_HP in GEANT4 fit the corresponding experimental data much better. The calculation results with BIC_HP overestimate the experimental data for thin targets in 5~30 MeV for more than 100%, except for aluminum at 150° and lead at 30°. For uranium target, the results calculated with BIC_HP is greater than the experimental results by more than 70% in the energy range 5~30 MeV at 30° and 60° and by more than 100% in the energy range above 5 MeV at 120° and 150°. In 20~100 MeV for aluminum, iron and lead targets, calculation results at 7.5° and 30° with BERT_HP underestimate the experimental data by more than 40%. And for uranium target, the experimental data up to 20 MeV are overestimated by more than 100%.     

A Bayesian-neural-network prediction for fragment production in proton induced spallation reaction

Fragment production in spallation reactions yields key infrastructure data for various applications. Based on the empirical SPACS parameterizations, a Bayesian-neural-network (BNN) approach is established to predict the fragment cross sections in proton-induced spallation reactions. A systematic investigation has been performed for the measured proton-induced spallation reactions of systems ranging from intermediate to heavy nuclei systems and incident energies ranging from 168 MeV/u to 1500 MeV/u. By learning the residuals between the experimental measurements and SPACS predictions, it is found that the BNN-predicted results are in good agreement with the measured results. The established method is suggested to benefit the related research on nuclear astrophysics, nuclear radioactive beam sources, accelerator driven systems, proton therapy, etc.     

Intense high-energy proton beams from Petawatt-laser irradiation of solids

An intense collimated beam of high-energy protons is emitted normal to the rear surface of thin solid targets irradiated at 1 PW power and peak intensity 3x10(20) W cm(-2). Up to 48 J ( 12%) of the laser energy is transferred to 2x10(13) protons of energy >10 MeV. The energy spectrum exhibits a sharp high-energy cutoff as high as 58 MeV on the axis of the beam which decreases in energy with increasing off axis angle. Proton induced nuclear processes have been observed and used to characterize the beam.     

Das Spektrum der energiereichen Protonen aus der Reaktion O16(γ,p)N15

Oxygen gas was irradiated with 34·5 MeV bremsstrahlung. The spectrum of protons between 6 MeV and 22 MeV was measured with a Na I(Tl) scintillation spectrometer. The energy resolution was equivalent to that obtainable with nuclear photoplates, but the number of protons registered was much higher. The differential cross section for (γ, p) reactions that leave the residual nucleus in the ground state was found to be 0·13 mbarn/steradian at 30 MeV gamma ray energy and at 90° with respect to the direction of the incident beam.     

Features of the Formation of Correlated Coherent States and Nuclear Fusion Induced by the Interaction of Slow Particles with Crystals and Free Molecules

The results of the experiments, where the intense generation of alpha particles with an energy of about 8.6 MeV was observed at the interaction of 400–600-eV slow protons with a thin lithium foil or lithium vapors, have been analyzed. It has been shown that the high efficiency of these reactions at such a low energy cannot be explained within standard models of accelerator nuclear fusion. A model has been proposed and considered for the initiation of these reactions by correlated coherent states of protons, which are formed at the electrostatic interaction of these moving particles with the fields of surface lithium atoms in a solid target, as well as with atoms in molecules of lithium vapor. It has been shown that the formation of such states is accompanied by a sharp increase in short-term fluctuations of the energy of protons, which are due to the Schrödinger–Robertson uncertainty relation, to an amplitude of 30–80 keV. The calculation has shown that the optimal energy of the initial motion of protons, at which these processes occur and the probability of the (Li, p) reactions involving these protons is large, is near 500 eV in complete agreement with the experimental data.     

Characterisation of the high-energy neutron beam at iThemba LABS

Monoenergetic and white neutron beams with a maximum energy of 200 MeV are produced at the neutron beam facility of the iThemba Laboratory for Accelerator-Based Sciences (iTL) by (p, n) reactions on Li, Be and C targets. The iTL separated-sector cyclotron can accelerate protons from 25 MeV to 200 MeV. Time of flight (TOF) measurements can be carried out by increasing the time separation between proton bunches up to 500 ns with a beam pulse selector. In the present work, the methods of beam characterisation used at this facility are discussed. Comparisons with metrological standards are presented. Specific issues related to monitoring the neutron fields at different accelerator settings are analysed.     

SHIELD程序靶设计的实用化及其在W靶参数设计中的应用

将GEANT3.21中的几何设计和图示技术移植到SHIELD程序中,并在此基础上对几种具有复杂构造的W靶进行参数设计的初步研究.     

Short-laser-pulse-driven emission of energetic ions into a solid target from a surface layer spalled by a laser prepulse

An efficient emission of picosecond bunches of energetic protons and carbon ions from a thin layer spalled from a organic solid by a laser prepulse is demonstrated numerically. We combine the molecular dynamics technique and multi-component collisional particle-in-cell method with plasma ionization to simulate the laser spallation and ejection of a thin (∼20–30 nm) solid layer from an organic target and its further interaction with an intense femtosecond laser pulse. In spite of its small thickness, a layer produced by laser spallation efficiently absorbs ultrashort laser pulses with the generation of hot electrons that convert their energy to ion energy. The efficiency of the conversion of the laser energy to ions can be as high as 20%, and 10% to MeV ions. A transient electrostatic field created between the layer and surface of the target is up to 10 GV/cm. Received: 13 March 2001 / Accepted: 20 March 2001 / Published online: 20 June 2001     

CMOS图像传感器在质子辐照下热像素的产生和变化规律

应用于空间的图像传感器在辐射影响下产生的热像素严重影响空间光电探测性能,本文通过质子辐照试验研究了热像素的产生和变化规律。首先,使用3 MeV和10 MeV两种能量的质子对图像传感器进行辐照,分析不同能量、不同注量的质子辐照产生热像素的性质;其次,再对辐照后的器件进行退火试验,分析热像素的退火规律。对于相同注量辐照,3 MeV质子辐照下热像素产生率大约是10 MeV质子辐照下的2.3倍,但是10 MeV质子辐照产生热像素的灰度值高于3 MeV质子;辐照过程中热像素的数量都是随着注量的增加线性增加。退火过程中,热像素数量都不断减少,而3 MeV质子辐照产生的热像素相比于10 MeV质子,退火更为显著。结果表明,质子辐照下每个质子与器件之间的作用过程及产生缺陷的机制是相对独立的,不同质子的作用过程之间没有相关性。不同能量的质子辐照产生缺陷的类型不同,导致热像素具有不同特性。     

Preequilibrium α-particle emission in heavy-ion reactions

The α-particle emission following ¹⁴N-induced reactions on various heavy targets at 85–115 MeV has been studied. Cross sections of heavy residual nuclei produced after α-emission were measured in the case of the ²⁰⁹Bi target and were found to be close to the angle-integrated cross sections of α-particles, indicating that the α-emission mainly takes place in a binary process. The measured angular distributions of α-particles are pronouncedly forward-peaked, while the energy spectra are always characterized by the Maxwellian distribution even at forward angles and reproduced excellently by the statistical evaporation formula when nuclear temperature is treated as a free parameter. The resultant value of the temperature is high (4–6 MeV) at forward angles and decreases monotonically with increasing emission angles.The energy and angular distributions of protons, deuterons and tritons were also measured in the ¹⁸¹Ta + ¹⁴N reaction at 115 MeV. The results are similar to those of α-particles. In particular, nuclear temperatures turned out nearly equal to each other, being consistent with the hot-spot interpretation for the relevant preequilibrium light-particle emission.     

Recoil properties of spallation products from bombardment of Z = 13–29 targets with 150,300 and 600 MeV protons

A semi-empirical relation developed using the classical model of high-energy nuclear reactions has been applied to spallation data obtained from thick-target — thick-collector recoil experiments. The ²⁴Na, ⁴²K, ⁴³K, ^44mSc, ⁴⁶Sc, ⁴⁷Sc ranges produced in Al, Sc, Ti, V, Fe, Co, Cu targets by 150, 300 and 600 MeV protons were determined. The excitation energies of the residual nuclei, deduced from the ranges, have been compared with theoretical calculations. The analysis shows that if the mass difference of the target and product nucleus is ΔA ? 10 the cascade plays a privileged role. If ΔA>10 an averaging effect is observed. In this case the number of prompt nucleons is about one-third of the total number and the excitation energy per evaporated nucleon is about 11 MeV.     

Production of exotic nuclei in peripheral nucleus-nucleus collisions below 10 A MeV

Experimental data from the literature concerning nucleus-nucleus collisions at beam energies of few A MeV above the Coulomb barrier are investigated in this work with emphasis on projectile-like fragment distributions. In peripheral collisions at beam energies below 10 A MeV, deep-inelastic transfer is shown to be the dominant reaction mechanism. In addition, the mechanism may involve an extension of the nuclear profile in the window (neck) region, observed primarily in reactions with very heavy target nuclei. Isoscaling observed at these energies can be used as a tool to predict the production rates of exotic nuclei in reactions induced by exotic secondary beams.     

CP violation and the search for new physics

Beta-delayed proton decay of ⁵⁷Zn has been investigated at the GSI on-line isotope separator. The studied ⁵⁷Zn nuclei were produced in fusion evaporation reactions by using a 150 MeV ³²S beam on a ²⁸Si target. Beta-delayed protons were measured by a charged-particle telescope detector. The observed decay pattern was used to construct the level scheme of ⁵⁷Cu and to extract the beta feeding distribution. The experimental results are compared with shell-model calculations. An erratum to this article is available at .     

A system for measuring a low-intensity proton beam

A system for measuring proton beam intensity and energy for the medical channel of the Institute for Nuclear Research, Russian Academy of Sciences, at energies of 70–280 MeV and an average current of about 1 nA is presented. The reaction of elastic scattering of primary beam protons on the polyethylene target is used in the system to determine the intensity and energy of a therapeutic proton beam with accuracies of 1% and 1 MeV, respectively.     

质子与金属布线层核反应对微纳级静态随机存储器单粒子效应的影响分析

金属布线层对微纳级静态随机存储器(static random access memory, SRAM) 质子单粒子效应敏感性的影响值得关注. 利用Geant4针对不同能量(30 MeV, 100 MeV, 200 MeV和500 MeV)的质子与微纳级SRAM器件的核反应过程开展计算, 研究了核反应次级粒子的种类、线性能量传输值(linear energy transfer, LET)及射程情况, 尤其对高LET 值的核反应次级粒子及其射程开展了详细分析. 研究表明, 金属布线层的存在和质子能量的增大为原子序数大于或等于30的重核次级粒子的产生创造了条件, 器件体硅区中原子序数大于60的重核离子来源于质子与钨材料的核反应, 核反应过程中的特殊作用机理会生成原子序数在30至50之间的次级粒子, 且质子能量的增大有助于这种作用机理的发生, 原子序数在30至50之间的次级粒子在器件体硅区的LET值最大约为37 MeV·cm²/mg, 相应射程可达到几微米, 对于阱深在微米量级的微纳级SRAM器件而言, 有引发单粒子闩锁的可能. 研究结果为空间辐射环境中宇航器件的质子单粒子效应研究提供理论支撑.     

利用GEANT4和FLUKA研究质子诱发散裂反应出射中子双微分截面

在中高能质子诱发散裂反应相关核工程设计中,可靠的蒙特卡罗模拟程序结合核反应理论模型具有较好的理论指导意义。本工作中,利用GEANT4耦合INCL4和ABLA理论模型以及FLUKA耦合PEANUT模型模拟计算了几百MeV至几个GeV质子轰击Be,Al,Fe,W,U等靶后30°,60°,120°,150°出射角产生的散裂中子双微分截面,并与现有实验数据进行了比较。结果发现,FLUKA和GEANT4模拟计算较好地再现了Al,Fe,W,U等靶实验测量数据。然而,模拟结果明显低估了Be靶出射中子能量小于10 MeV能区的实验数据。For the design of nuclear engineering related with medium-high energy proton induced spallation reaction,the reliable Monte Carlo simulation codes coupled with nuclear reaction models have a good theoretical guidance.In this work,the production spallation neutron double differential cross sections at 30°,60°,120°,150°emission angle for Be,Al,Fe,W,U target materials at incident proton energies between several hundred MeV and GeV are theoretically calculated by using the GEANT4 coupled INCL4 and ABLA,and the FLUKA coupled PEANUT.The calculated results were compared with the available experimental data.It is found that the GEANT4 and FLUKA calculations well reproduced the experimental measurement of Al,Fe,W,U target materials.However,calculations obviously underestimated the emission neutrons of Be target for lower than 10 MeV energy range.     

Large-angle proton emission in the 9Be(p, 2p) reaction at 300 MeV

A ⁹Be(p, 2p) coincidence experiment performed to further elucidate the reaction mechanism for the production of energetic wide-angle protons in intermediate-energy proton-induced reac- tions is reported. Detectors in a coplanar geometry were used to measure coincidences between trigger protons at 90° to the beam and forward-angle protons on the opposite side of the beam. The incident proton energy was 300 MeV. We report both the inclusive spectra for the trigger protons and the differential mean multiplicities for the coincidence events.The outgoing proton energies were measured using NaI detectors. Trigger protons were grouped into 10 MeV bins covering the kinetic energy range from 55 to 155 MeV. The forward protons were measured over a kinetic energy range of 65–280 MeV and an angular range of 14–60° with respect to the beam.The present results are compared with two previous experiments which covered a more restrictive kinematical range. Calculations are performed with both phase-space and direct knockout models, and compared with experiment. Observation of angle and energy correlation effects suggested by knockout models indicate that such direct mechanisms provide a significant contribution to energetic wide-angle inclusive proton spectra.