汞蒸汽中利用四波和频产生125nm附近可调谐真空紫外激光

以氩为匹配气体的汞蒸汽四波和频实验中,一束泵浦光(ω₁)与汞原子6¹S₀—7¹S₀严格双光子共振,当另一束泵浦光(ω₃)在汞原子7¹S₀—9¹P₁跃迁的蓝端调频时,产生可调谐的真空紫外(VUV)激光(ω₄=2ω₁+ω₃),其 关键词：     

3S1–3D1 coupled channel ΛcN interactions:chiral effective field theory versus lattice QCD

We study the lattice QCD Λ_cN phase shifts for the ³S₁-³D₁ coupled channel using both the leading order covariant chiral effective theory and the next-to-leading order non-relativistic chiral effective field theory(ChEFT).We show that although it is possible to describe simultaneously the ³S₁ and ³D₁ phase shifts and the inelasticity η₁,the fitted energy range is quite small,only up to E<...     

镱原子超精细诱导5d6s 3D1,3→6s2 1S0 E2跃迁及超精细常数的精确计算

在镱原子中,利用5d6s³D₁→6s²¹S₀跃迁探索宇称破缺效应已经得到了深入的研究.但是5d6s³D₁态与基态6s²¹S₀之间的M1跃迁和超精细诱导E2跃迁很大程度上影响了宇称破缺信号的探测.因此,很有必要精确计算5d6s³D₁态与基态6s²¹S₀之间的M1跃迁和超精细诱导E2跃迁的跃迁概率.本文利用多组态Dirac-Hartree-Fock理论精确计算了5d6s³D₁→6s²¹S₀ M1跃迁和超精细诱导5d6s³D_1,3→6s²¹S₀ E2跃...     

GdB3O6中Gd3+的级联发射特性

报道了Gd³⁺离子在GdB₃O₆基质中的光子级联发射特性。用Hitachi M850荧光分光光度计测定了Gd^{3+ 6}G_J能态的位置和Gd³⁺离子的光子级联发射光谱,Gd³⁺离子的第一个光子发射为⁶G_J→⁶P_J(～600nm)和⁶G_J→⁶I_J(～780nm),第二个光子的发射为⁶P_J→⁸S_7/2(～310nm)。由于⁶D_9/2与⁶I_11/2间能级差(～2900cm^-1)和⁶I_7/2与⁶P_J间能级差(～3900cm^-1)较小,多声子弛豫的几率明显超过辐射跃迁几率。因此,当用⁸S_7/2→⁶G_J(202nm)的紫外光激发时,只能观察到⁶P_J→⁸S_7/2(～310nm)、⁶G_J→⁶P_J(～600nm)和⁶G_J→⁶I_J(～780nm)的发射跃迁,未能观察到⁶I_J→⁸S_7/2(～275nm)和⁶D_J→⁸S_7/2(～250nm)的发射跃迁。     

THE 82S1/2→62D EXCITATION TRANSFER OF RUBIDIUM ATOMS INDUCED BY COLLISIONS WITH GROUND-STATE RUBIDIUM AND HYDROGEN MOLECULES

The processes of excitation transfer from the 8²S_1/2 state to the 6²D state of rubidium in Rb(8²S_1/2)-Rb(5²S_1/2) and Rb(8²S_1/2)-H₂ collisions have been studied experimentally. During irradiating the Rb vapor, mixed with H₂, by two light beams for selective stepwise excitation, the Rb 8²S_1/2→5²P_3/2 direct fluorescence and the Rb 6²D_3/2→5²P_1/2 sensitized fluorescence have been measured as a function of H₂ gas pressure. The measurements yielded the cross-sections σ(8²S_1/2→6²D) and σ^*(8²S_1/2→6²D) of Rb 8²S_1/2→6²D excitation tranfer induced by collisions with 5²S_1/2 atom and H₂ molecules respectively. The results are discussed in detail.     

Regarding the 21S0 and 23S1 multiplets

<正>This paper discusses the masses and possible members of 2¹S₀ and 2³S₁ meson multiplets in the framework of meson-meson mixing and Regge phenomenology.For the 2¹S₀ meson nonet,K^*（1460） may be the observed state of the 2¹S₀ isodoublet with a mass of 1400 MeV and the mass ofω（1420） is 1412 MeV.For the 2³S₁ meson nonet,K^*（1410） seems too light to be the 2³S₁ ns member.The fact that the agreement between the present findings and those given by experiments and other different approaches is satisfactory implies that the assignments in this paper may be reasonable.     

NaLa(MoO4)2∶Eu3+的水热调控合成与发光特性研究

采用水热法合成了不同粒径的NaLa(MoO₄)₂∶Eu³⁺微晶.通过调节乙二醇浓度和反应时间,研究了NaLa(MoO₄)₂∶Eu³⁺微晶的形貌演变过程,在水热条件下180 ℃反应16 h获得了均一梭子形NaLa(MoO₄)₂∶Eu³⁺微晶,其晶粒长度约为2.0 μm.荧光光谱分析表明,Eu³⁺取代了NaLa(MoO₄)₂中La³⁺的格位, Eu³⁺在613 nm处红光发射(⁵D₀–⁷F₂跃迁)的浓度猝灭机理是电偶极-电四极相互作用,并发生了Eu³⁺( ⁵D₁ ) + Eu³⁺(⁷F₀ )→ Eu³⁺( ⁵D₀ ) + Eu³⁺(⁷F₃) 交叉弛豫,由此导致浓度猝灭. 关键词： 钼酸盐 水热法 稀土离子 发光     

关于一级近似Tc级数解的收敛问题

本文通过一个实例说明:μ^*=0时,一级近似T_c级数解的收敛半径既不是由z_ph=-∫₀^(ω_ph)dωg(ω)dω·ω²/(ω_ph²-ω²),也不是由z_ph=∫₀^(ω_ph)dωg(ω)dω·ω^{2< 关键词：}     

Au原子高Rydberg态场致电离的实验研究

利用电热法将含金物质加热,产生Au原子束,再以两束UV脉冲激光垂直照射,将处于基态的Au原子共振激发至高Rydberg态。滞后于激光脉冲200ns的高压脉冲电场(6500V/cm)加到反应区,使处于Rydberg态的Au原子电离。激光波长在一定范围内扫描,共测出了Au原子的n²D_3/2(n=18—38)和n²S_1/2(n=21—34;36—38)两通道的38条能级的位置。用参数拟合得到²D_3/2和²S_1/2两系列的极限分别为:E_D=74409.8(3)cm^-1,E_S=74410.0(2)cm^-1,计算了每条能级的量子亏损。我们的实验还证明了场电离是一种十分有效的电离手段,比用通常的激光光电离效率要高得多。这在共振电离谱学(RIS)的研究中是一种很有效的方法。 关键词：     

ZnS:Ho3+的辐射跃迁和无辐射过程

本工作研究了Ho³⁺离子在宽禁带半导体ZnS中的辐射跃迁和无辐射过程。用发射谱线的积分光强和激发态寿命获得ZnS:Ho³⁺的强度参数Ω_λ,同时计算了九个激发态的辐射跃迁几率和能级寿命。另外,通过在不同温度下测定Ho³⁺离子⁵G₆,³K₈,⁵F₂,⁵F₃和⁵S₂(⁵F₄)能级的发射光强和寿命的方法,研究了这几个激发态间的无辐射过程,其中⁵G₆,³K₈,⁵F₂和⁵F₃这四个能级是处于热平衡状态,而⁵F₃与⁵S₂(⁵F₄)能级间存在五个声子((1/n)ω_Lo=351cm^-1)参与的多声子弛豫过程。 关键词：     

Double resonance interference in third-order light mixing

The first observation of interference effects between two sharp resonant contributions to the third-order nonlinear susceptibility χ₍₃₎ (ω₃=ω₀+ω₁?ω₂) is reported. Using two tunable near ir frequencies, ω₀=ω₁ and ω₂, the was seen in crystalline CuCl when 2ω₁ and ω₁?ω₂ were close to the sharp Z₃ exciton at 3.21 eV and the 210 cm^-1 Raman line, respectively. Three different tunable visible frequencies were used to observe similar interference effects in a benzene-cyclohexane mixture when ω₀?ω₂ and ω₁?ω₂ were close to the 992 cm^-1 Raman line of benzene and the 801 cm^-1 Raman line of cyclohexane, respectively.     

Saturation spectroscopy of ultraviolet transitions in mercury with a frequency-doubled cw ring dye laser

Doppler-free saturated absorption spectroscopy has been used to study the ultraviolet HgI transitions 6³P₀-6³D₁ at 296.73 nm and 6³P₀-6¹D₂ at 296.76 nm. The required tunable ultraviolet radiation was produced by a ring cavity cw dye laser with intracavity ADA frequency doubler. The isotope shifts of the 6³P⁰ -6³D₁ line for naturally abundant mercury have been measured to within a few MHz.     

Generation of coherent radiation at 89.6 nm through two-photon resonant phase-matched tripling of fourth-harmonic Nd: Glass laser radiation in Hg vapors

Coherent radiation at 89.6 nm has been obtained through third-harmonic conversion of the 268.8 nm pulses in mercury vapors. Tunability of the fourth-harmonic frequency of the Nd: glass laser radiation to the 6s ¹ S ₀–8s ¹ S ₀ double quantum resonance of Hg atoms has been used for the resonant enhancement of the twelfth-harmonic output. Possibility to phase match the generated radiation and driving polarisation in pure vapors without employing of bufer gas has been demonstrated.     

Development of a Lyman-α laser system for spectroscopy and laser cooling of antihydrogen

Hydrogen Lyman-α radiation (121.56 nm) is important because it allows for the excitation and detection of ground-state hydrogen atoms by a one-photon process. The trapping of antihydrogen, recently reported by the ALPHA collaboration at CERN, has revived interest in Lyman-α lasers. In order to perform high precision tests of matter-antimatter symmetry violations or gravity-antimatter interactions with antihydrogen, laser cooling using the 1s ? 2p single photon transition is essential. Recent theoretical simulations predict that even with a pulsed Lyman-α source, laser cooling of antihydrogen would be possible. Here we describe the implementation of a high power vacuum-ultraviolet (VUV) laser at the Lyman-α transition of hydrogen. The VUV light was generated using a two-photon-resonant four-wave mixing process in a phase-matched mixture of krypton and argon. Two wavelengths (ω _R → 202.31 and ω _T → 602.56 nm) were mixed in a sum-difference scheme (ω _VUV = 2ω _R ? ω _T ) with a two-photon resonance at (4s ²4p ⁵5p[1/2]₀ ← 4s ²4p ⁶(1S ₀)) transition in Kr. With an Ar/Kr mixture of 3.9:1 we obtained 10 ns pulses of 0.1 μJ of energy at a repetition rate of 10 Hz.     

Tunable coherent vacuum ultraviolet generation in carbon monoxide in the 1150 Å range

Coherent and tunable over 500 cm^-1 radiation in the vacuum ultraviolet (VUV) in the 1150 Å region has been generated by resonantly enhanced 4-wave sum frequency mixing in carbon monoxide. Theoretical estimates of the third-order nonlinear susceptibility are shown to be in reasonable agreement with the observed conversion efficiency in CO.     

小分子在真空紫外波段从量子态到量子态的光解离动力学

本文主要描述小分子在真空紫外波段(VUV,6-20 eV)光解离动力学的最新实验和理论研究进展.得益于基于商业化激光器的真空紫外光源技术,以及离子速度成像、高分辨氢原子-里德堡态标记-飞行时间测量和VUV-VUV泵浦-探测等方法的发展,研究人员现在可以对很多小分子在真空紫外波段的光解离动力学进行量子态到量子态层面的测量和研究,本文重点综述H_2(D_2,HD),CO,N_2,NO,O_2,H_2O(D_2O,HOD),CO_2,N_2O以及一些多原子分子在真空紫外波段光解离动力学的最新研究进展.这些小分子在真空紫外波段的光解离在天体化学以及大气化学中有着非常重要的应用.分子吸收一个VUV光子以后,通常会被直接激发到比较高的电子激发态,解离过程会涉及到多个电子态势能面之间的复杂非绝热相互作用.在实验上对解离截面等参数进行从量子态到量子态层面的精细测量对于深入了解这些复杂的势能面之间的相互作用有非常重要的意义.最近建成的大连相干光源是目前世界上唯一一台在真空紫外波段工作的自由电子激光,具有脉冲能量高、扫描范围宽(50～150 nm)等优越的性能,它的建成必将会大大促进小分子真空紫外光解离研究的发展.     

Phase-matched second-harmonic generation at 440 nm in a LiNbO3 -Gd3Ga5O12 waveguide with a tunable stimulated Raman source

Using a tunable stimulated Raman source, we have observed second-harmonic generation in the blue in a sputtered LiNbO₃ film deposited on Gd₃Ga₅O₁₂. With the choice of Gd₃Ga₅O₁₂ as a substrate, it becomes possible to both phase-match a large range of fundamental wavelengths as well as have an excellent epitaxial quality surface. The SHG efficiency for the TM^ω₀ → TM^2ω₂ phase matched conversion process is estimated to be ～ 10^-4.     

The effect of the electric field on the spectral line shape

The effect of the external electric field on the spectral line shape under conditions of a uniform population of magnetic sublevels is studied in the density matrix formalism. The line shapes of spontaneous radiation for the atomic 4¹P₁-2¹S₀, 4³D₁-2³P₀, 4³S₁-2³P₀, 4³P₁-2³S₁, 4³D₁-2³P₁, and 4³S₁-2³P₁ transitions ofHe are calculated. The electric field is shown to be responsible for the spectral line shape asymmetry. Tomsk State University. Translated from Izvestiya Vysshikh Uchebnykh Zavedenii, Fizika, No. 11, pp. 23–28, November, 1999.     

Spin resonant optical mixing in InSb — CW-measurements and transient effects

Optical four-wave mixing due to the resonant spin nonlinearity in n-InSb was observed in magnetic fields up to 1.4 T. The mixing of two CO-laser frequencies ω₁ and ω₂ = ω₁ - Δω yields radiation with frequencies ω₁ + 2Δω, ω₁ + Δω, ω₁ - 2Δω, and ω₁ - 3Δω. We found the resonant contribution to the third order nonlinear susceptibility arising from the spin-flip interaction to increase by more than two orders of magnitude when ω₁ is varied from 1760 cm^-1 to 1896 cm^-1. With the lasers working simultaneously Q-switched we observed radiation at ω₁ + Δω and ω₁ - 2Δω due to the mixing caused by the nonparabolicity of the conduction electrons even without an external magnetic field. At the resonant magnetic field the intensity of the mixed radiation is increased by more than one order of magnitude and is also observed when the laser pulses do not hit the sample simultaneously as long as the time difference between the two pulses does not exceed 450 ns. This points to a spin dephasing time T₂ of about 100 ns.