CS_2飞秒超快非线性特性的实验研究

采用中心波长800 nm、脉宽30 fs的超短激光脉冲,通过飞秒光开关技术对CS_2的飞秒超快非线性特性进行了实验研究.在探测光强与抽运光强比为1∶10时,得到了较理想的光克尔时间分辨曲线.通过实验测定的光克尔信号强度与激发光和探测光偏振方向夹角的依赖关系表明:30 fs的超短激光脉冲激发CS_2的克尔信号主要是源于光诱导双折射效应,而非用200 fs的超短激光脉冲时来自瞬态栅的自衍射效应.     

ZnTe晶体中光学整流产生的THz辐射及其电光探测研究

借助抽运-探测技术研究了ZnTe晶体中光学整流产生的太赫兹(THz)辐射，利用ZnTe晶体的线性电光效应探测THz辐射场分布，观察到了较窄(约为0.2 ps)的THz场分布及相应较宽(响应超过4 THz，半峰宽约为2.4 THz)的THz频谱，并运用琼斯矩阵对实验结果进行了理论拟合. 研究了飞秒激光脉冲波长(750—850 nm)、脉冲宽度(56—225 fs)和晶体旋转与THz辐射产生的关系. 同时改变探测光偏振方向进行偏振调制，并从理论上分析了偏振调制对THz辐射探测的影响. 关键词： THz辐射 光学整流 电光探测 ZnTe     

飞秒光诱导铽镓石榴石晶体中的磁化响应研究

运用时间分辨抽运-探测光谱技术,研究了磁光晶体铽镓石榴石(TGG)在不同椭圆偏振态的飞秒激光脉冲诱导下的极化和磁化响应.研究表明,当仅存在逆法拉第效应时,探测光旋转角信号和椭圆率信号的变化方向与圆偏振抽运光的旋向相关.这是由于圆偏振光在TGG晶体中产生的瞬态有效磁场的方向依赖于圆偏振光的旋向所致.光诱导磁化过程与材料的性质有关,TGG晶体的顺磁特性决定了其自旋弛豫时间为几十飞秒.由于探测光旋转角信号和椭圆率信号的半高全宽均为500 fs左右,加之信号强度随着抽运光脉冲能量密度的增加呈线性增长,表明TGG晶 关键词： 铽镓石榴石晶体 抽运-探测光谱技术 逆法拉第效应     

光磁相互作用及自旋极化的光学调控

近年来,超短激光脉冲的发展为人们在极端时间尺度上研究光与物质的相互作用提供了有 效工具。皮秒时间尺度上研究磁有序材料中的自旋动力学过程已经成为凝聚态物理研究的热点, 促进了自旋电子学的发展。本论文基于飞秒激光抽运–探测技术,介绍了半导体及其纳米结构中 光注入自旋极化及其弛豫过程;综述了铁磁性薄膜中的超快退磁,激光诱导磁阻尼进动和逆法拉 第效应; 利用太赫兹脉冲的磁场分量,研究了反铁磁晶体中自旋共振模式的激发,相干控制以 及自旋重取向的探测; 最后介绍了超快光谱用于研究多铁性材料中电子、晶格和自旋间的耦合。 了解不同材料在超快时间尺度上的磁光、光磁效应的最新进展,有助于在磁有序的超快光控制研 究领域做出原创性的工作。     

高非线性光子晶体光纤中飞秒脉冲的传输特性和超连续谱产生机制的实验研究及模拟分析

用实验和数值模拟两种方法研究了高非线性光子晶体光纤中飞秒激光脉冲的传输特性和超连续谱的产生机理，给出了抽运脉冲在三种不同中心波长情况下输出光谱展宽并形成超连续谱的实际测量及理论模拟结果.研究表明：在零色散波长抽运时，光谱展宽以自相位调制为主，同时三阶色散的影响明显，传输脉冲在时域内出现振荡次峰.而在反常色散区抽运时，光谱展宽的初期以自相位调制为主，随后根据抽运功率的不同孤子自频移、高阶光孤子的裂变和四波混频效应会逐渐增强，进而成为光谱展宽的主要原因.与此相应，在时域中能明显看到孤子的形成和红移，飞秒传输脉 关键词： 光子晶体光纤 高非线性光子晶体光纤 飞秒脉冲激光 超连续谱     

GaP波导型发射器产生频率可调谐太赫兹脉冲

报道了利用脉宽可调的光子晶体光纤飞秒激光放大器抽运矩形波导结构的GaP晶体太赫兹(THz) 发射器产生频率可调谐的超快THz脉冲.非线性晶体中光整流过程产生的THz辐射频率随抽运光脉冲宽度而 变化. GaP波导THz发射器可通过波导的几何尺寸来控制色散,以达到增加有效作用长度和提高输出功率的目的. 不同横截面尺寸的波导型发射器的THz辐射峰值频率随相位匹配条件的改变而改变,加以脉宽调节技术, 可以在大频谱范围获得频谱精细可调的THz脉冲.实验中在1 mm×0.7 mm的波导型THz发射器中获得了 频率可调谐的THz脉冲.提出实现THz辐射频率大范围调谐的GaP波导型阵列发射器的实施方案.     

空气飞秒激光成丝现象中产生的椭圆偏振单周期太赫兹脉冲

飞秒激光在空气中形成的等离子体细丝会辐射出太赫兹(THz)信号.实验利用1 mJ,800 nm,50 fs的飞秒激光脉冲产生等离子体细丝.应用光电取样方法探测了激光成丝现象中前向辐射的THz脉冲,得到了持续时间为0.1 ps、光谱峰值在1 THz左右的单周期THz脉冲.转动抽运光的偏振态,分析了电光取样信号的变化.通过比较实验数据和计算结果,证明了成丝辐射THz脉冲的偏振态为椭圆偏振态.     

基于液晶空间光调制器的太赫兹波频谱调制

频谱可调制的太赫兹波具有广泛的应用价值。利用一台纯相位式的液晶空间光调制器对飞秒激光脉冲进行空间整形,通过改变飞秒激光脉冲的横向空间分布,实现太赫兹波频谱的调制。在实验中,利用光泵浦整流方式产生太赫兹波,并利用太赫兹时域光谱系统对太赫兹信号进行探测。通过GS算法在液晶空间光调制器上加载不同的相位图,获得了不同的飞秒激光脉冲横向空间分布。通过改变探测距离和飞秒脉冲的空间分布参数,实现了太赫兹波频谱的调制。还利用菲涅尔衍射算法对这一过程进行了理论模拟,理论模拟结果与实验结果吻合的较好,这充分说明了基于飞秒脉冲空间整形的太赫兹光谱调制技术的可行性。     

飞秒脉冲正交位相压缩光的产生

利用锁模飞秒脉冲激光二次谐波为抽运源, 同步抽运单共振光学参量振荡器, 抽运光中心波长为425 nm, 重复率为76 MHz, 脉宽180 fs, 光学振荡器下转换晶体采用Ⅰ类共线PPKTP, 实验上实现了压缩度为2.58 dB的正交位相压缩光.考虑到实验系统的效率, 可以推知光学参量振荡器输出的下转换光压缩度为 4.48 dB. 关键词： 同步抽运光学参量振荡器 压缩光 锁模飞秒脉冲     

基于瞬态光栅频率分辨光学开关法测量飞秒脉冲的研究

超宽光谱的飞秒脉冲测量一直是超快激光领域的重要研究方向之一.常规的飞秒脉冲自相关方法是通过测量自相关倍频信号来获得,而倍频信号具有波长选择性,不同中心波长的飞秒脉冲测量需要更换不同的倍频晶体,十分不方便.因此,提出了一种改进型的瞬态光栅频率分辨光学开关(TG-FROG)方法用于测量飞秒脉冲.该方法结合四波混频和频率分辨光学开关方法,其基本过程是将待测脉冲分为三束,其中两束脉冲经过精密的延时控制并聚焦在光学介质上达到时空重合,利用三阶非线性效应产生稳定的瞬态光栅作为开关光;另一束脉冲作为探测光与产生的瞬态光栅进行相互作用产生一个信号光,使用光谱仪对该信号光的光谱与延迟时间进行测量,并通过反演迭代算法处理而获取待测飞秒脉冲的光谱与电场信息.该方法只需要待测光的功率密度达到三阶非线性效应就可以实现测量,因此可以应用于任意中心波长的飞秒脉冲测量.利用该方法对中心波长分别为800 nm, 400 nm的飞秒脉冲,以及超连续亚10 fs的周期量级超宽光谱飞秒脉冲进行了测量,并与常规的干涉自相关仪器测量结果进行了比较,所得测量结果基本一致.实验结果表明,建立的基于TG-FROG方法对不同中心波长,不同脉冲宽度的飞秒脉冲测量是十分有效的.     

铁磁薄膜中圆偏振光感应的瞬态磁光Kerr峰的物理起源

使用飞秒时间分辨抽运-探测磁光Kerr光谱技术,实验研究了圆偏振光抽运面内磁化FePt和垂直磁化GdFeCo薄膜的磁化演化动力学,发现在时间延迟零点处均出现瞬态Kerr峰.分析了此Kerr峰的起源,指出此瞬态Kerr峰与铁磁性无关,可能起源于自由电子的顺磁磁化,而顺磁磁化的外磁场来自圆偏振抽运光的逆Faraday效应.基于顺磁磁化模型的计算结果支持此观点.基于此观点,逆Faraday效应感应的磁场脉冲宽度应该与激光脉冲宽度一致.     

Micromagnetic investigation of all-optical switching

This Letter investigates all-optical magnetization switching from micromagnetic perspective. The influence of circularly polarized light on a magnetic sample was considered to be both directly through the inverse Faraday effect and indirectly aided by thermal induced effects by the laser beam. Dependence of all-optical switching on pulse duration, laser intensity and the magneto-optical susceptibility strength is studied. An important aspect of this investigation is the analysis of how the cooling process influences the successive switches, especially through limiting the successive writing time.     

The study of ultrafast magnetization dynamics induced by femtosecond laser pulses in GdFeCo amorphous film

The time-resolved magneto-optical Kerr spectroscopy technique is used to study the ultrafast magnetization dynamics induced by femtosecond laser pulses in GdFeCo amorphous film. We study concretely the influence of the different pump fluence and the different external magnetic field on magnetization dynamics of ultrafast demagnetization, magnetization reversal and magnetization recovery. The pump fluence dependence magnetization dynamics shows that the degree of demagnetization, the degree of magnetization reversal and the time of magnetization recovery increase with pump fluence, which can be interpreted by the “three-temperature” model. The external magnetic field dependence magnetization dynamics shows that the rate of magnetization reversal increases with the external field, which accord with the magnetization reversal mechanism based on the reversed magnetic domain nucleation and domain-wall motion.     

High-density all-optical magnetic recording using a high-NA lens illuminated by circularly polarized pulse lights

We propose a method for high-density all-optical magnetic recording. Our analyses, based on the vector diffraction theory, show that owing to the inverse Faraday effect, circularly polarized laser pulses focused by a high numerical aperture (NA) lens can induce a small magnetization domain. For an example, the FWHM of the effective magnetization domain is 0.4646λ when NA=0.85. The magnetization direction is basically perpendicular to the surface of the optic-magneto film within the effective magnetization domain and the switching direction of magnetization can be controlled by the helicity of the incident circularly polarized light. These characteristics are useful to next-generation high-density all-optical magnetic storage.     

Quantum field theory of optical birefringence phenomena

The inverse Faraday effect, in which a magnetization is induced in a solution through which is passed a polarized light beam of arbitrary ellipticity, is discussed on the basis of the S-matrix formulation of optical birefringence. It is shown that the Faraday effect and the inverse Faraday effect are topologically identical problems of diagrammatic perturbation theory and so it follows automatically that the magnetization should be proportional to the Verdet constant. The optical Faraday effect is the circular birefringence induced by an intense circularly polarized beam of light propagated colinearly with the weak measuring beam: the electric vector of the circularly polarized beam interacts with the molecule in a way that resembles the interaction of a static magnetic field. The interrelations of these two effects and the normal Faraday effect the self-rotation of the polarization ellipse of an intense beam are discussed.     

磁光光纤Bragg光栅中圆偏振光的非线性传输特性

提出了磁光光纤Bragg光栅的理论模型,给出了圆偏振光在磁光光纤光栅中传播的非线性耦合模方程. 研究表明,在磁光光纤Bragg光栅中,光栅引起正反传播方向的导波光发生耦合,法拉第效应引起磁圆双折射效应,而非线性效应则将左旋和右旋圆偏振光耦合在一起,它们的共同作用可使双稳态状态发生反转、非线性光控光开关阈值功率降低. 与传统光纤光栅相比,利用左旋和右旋磁圆偏振光之间的交叉相位调制实现的脉冲整形具有磁光偏置可调特性,为基于磁光光纤光栅的动态灵活全光3R再生器的研制提供了理论基础. 关键词： 磁光光纤Bragg光栅 圆偏振光 脉冲整形     

Symmetry properties of three-dimensional magnetization distributions induced by focused circularly polarized lights

We analyze symmetry properties of the three-dimensional magnetization distribution in the optic-magneto film induced by focused circularly polarized lights. The magnetization distributions are derived and evaluated based on the vector diffraction theory and the inverse Faraday effect of the isotropic and nonmagnetically ordered material. It is shown that for any radial symmetrical amplitude, phase, or hybrid amplitude-phase pupil filter, the magnetization distribution of the axial component is circular symmetric but those of the radial and azimuthal components are annular symmetric with regard to the optical axis. All of the three components have a symmetric distribution with regard to the focal plane. The direction of both axial and radial components can be inversed with the helicity of incident circularly polarized light but the direction of azimuthal component is independent of helicity. The axial component has a decisive effect to all-optical magnetic recording, and within the effective axial range, the size of its magnetization domain hardly expands in the transverse direction.     

Dependence of femtosecond time-resolved magneto-optical Kerr rotation on the direction of polarization of the probe beam

We demonstrate that the femtosecond time-resolved magneto-optical Kerr rotation oscillates with the direction of polarization of the probe beam when a sample of Al0.25Ga0.75As/GaAs multi-quantum wells is excited by a circularly polarized pump and detected by a linearly polarized probe at wavelengths from 800 to 830 nm. Analytical expressions are derived to explain the mechanism, which is in good agreement with the numerical computation and the experimental data. The results suggest that the Kerr signal can ...     

Femtosecond magneto-optical Kerr microscopy

We have developed a magneto-optical Kerr microscope that allows us to measure the ultrafast magnetization dynamics of ferromagnetic nanostructures. The magneto-optical signal can be recorded in a confocal reflection geometry with an accurate selection of the polarization. The magnetization dynamics is obtained from pump-probe measurements using frequency nondegenerate collinear pump and probe beams with a temporal resolution of 180 fs. Both probe and pump beams are focused to their diffraction limit, leading to an overall spatial resolution of 600 nm. The efficiency of the apparatus is tested by investigating the magnetization dynamics of individual CoPt(3) disks with a submicrometer diameter and a thickness of 15 nm.