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We propose a new mechanism/scheme to explain the ultrafast population inversion of molecular ions which takes place in a time scale comparable to the femtosecond laser pulse. The nonlinear pumping process including the pump photons and the self-generated harmonic photons of the pump laser would be responsible for building up population inversion to realize remote molecule lasers in femtosecond laser filaments in gases. It is shown that the remote laser emissions in molecular ions of gases may be a universal process in the femtosecond laser filament. 相似文献
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<正>With the evolution of a laser pulse in water,the formation of a nonlinear X wave during femtosecond filamentation is investigated based on numerical simulations.In particular,we analyze the far-field angularly resolved spectra obtained for different temporal portions of the ultrashort pulse during its propagation. Our result shows that the refocusing of ultrashort pulse leads to the formation of dynamic X wave which essentially manifests itself as conical emission. 相似文献
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Recent progress in filament-induced atmospheric sensing is reviewed.Self-guided propagation of ultrashort laser pulses in air induces laser filamentation.All molecules in the path of a filament can be dissociated into highly excited fragments,resulting in emission of characteristic fluorescence spectra.The fluorescence spectra provide information about the various molecules in the filaments.By using a filament-induced"fingerprinting"fluorescence technique,molecules in the atmosphere can be identified. 相似文献
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We report on a systematic study of the laser polarization effect on a femtosecond laser filamentation in air.By changing the laser's ellipticity from linear polarization to circular polarization, the onset position of laser filament formation becomes farther from the focusing optics, the filament length is shorter, and less laser energy is deposited. The laser polarization effect on air filaments is supported by a simulation and analysis of the polarization-dependent critical power and ionization rates in air. 相似文献
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非线性荧光光谱的神经网络分析及其应用 总被引:8,自引:4,他引:4
大功率超快脉冲激光和气体相互作用可产生非线性荧光光谱,不同的气体分子具有不同的非线性荧光光谱。因而这种光谱可以作为物质的指纹模式加以识别分类,进而获知气体的成分。由于不同气体分子的光谱在同一波段上有很大的交叉重叠,用传统的光谱分析方法分析存在困难,采用神经网络方法分析上述非线性荧光光谱,利用经过预处理的荧光光谱数据作为模式样本,其中一部分样本作为学习样本对级联神经网络进行训练,用训练好的网络对所有样本进行实时识别,学习样本和测试样本的的正确识别率均可达100%,结果表明此方法可实时判断混合气体的组分。 相似文献
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