Fragmentation of CO in Femtosecond Laser Fields

Fragmentation of CO in a linearly polarized femtosecond laser field within the intensity order of 10^14 W.cm^-2 at 820nm is investigated experimentally by using velocity mapping technique. According to the observed kinetic energy and angular distributions of different charged fragment ions, fragmentation channels of CO are proposed. The angular distributions provide helpful information for assigning the dissociation channels.     

He—Ne激光器粒子数反转径向分布光谱测量

用二维光学多道分析仪考察了He-Ne激光器在632.8nm激光振动和不振荡时氖能级3s_2和2p_k(k=1,2,……8,10)的侧光辐射,进行了Abel反演后,得到了3s_2和2p_k各能级粒子数和3s_2和2p_k间粒子数反转的径向分布,研究了此分布勺放电电流、632.8nm激光辐射强度间的关系,推算了在放电管中心3s_2和2p_k能级间受激辐射的激光增益。     

针一板介质阻挡放电中电子能量空间分布研究

测量了大气压环境下氩气空心针-板放电等离子体中原子与分子谱线强度的空间分布,分析了等离子体中电子能量的空间分布.实验利用空心针-板放电装置,得到了约3 cm长的放电等离子体弧.在300～800 nm范围内采集发射光谱,发现了强度较高的Ar I谱线、N2第二正带系谱线C 3Ⅱu(v=o)→B 3皿(v=0)以及强度较弱的...     

1，2-和1，4-萘醌248 nm激光光解的瞬态吸收光谱研究

利用纳秒级激光光解动态吸收光谱装置,研究１,２－和１,４－萘醌中性水溶液的瞻态吸收光谱,发现１,２－萘醌及,１,４－萘醌被光电离合形成的阳离子自由基在３８０ｎｍ均有最大吸收,但１,４－萘阳离子自由基在衰变过程中又形成了两种新的活性粒子,它们的最大吸收分别位于４１０和５８０ｎｍ,分析表明：４１０ｎｍ属于１,４－蔡醌脱氢自由基的吸收,而５８０ｎｍ很可能归属由于于４１０和５８０ｎｍ,分析表明：４１０ｎｍ     

Octave-spanning visible supercontinuum generation from an aluminum nitride single crystal pumped by a 355 nm nanosecond pulse

Supercontinuum generation(SC) of more than one octave spectrum spanning covering from 400 nm to 820 nm was achieved by pumping a piece of aluminum nitride(AIN) single crystal using a nanosecond 355 nm ultraviolet laser. The AlN with a thickness of ~0.8 mm was grown by an optimized physical vapor transport technique and polished with solidification technology. Compared to previously reported ones, the achieved visible SC exhibited the broadest spectrum spanning from bulk materials pumped by a nanosecond pulse laser. The visible supercontinuum in Al N presents new opportunities for bulk material-based white light SC and may find more potential applications beyond typical applications in integrated semiconductive photoelectronic devices.     

Energy transfer and infrared-to-visible upconversion luminescence of Er/Yb-codoped halide modified tellurite glasses

We report on the energy transfer and frequency upconversion spectroscopic properties of Er³⁺-doped and Er³⁺/Yb³⁺-codoped TeO₂-ZnO-Na₂O-PbCl₂ halide modified tellurite glasses upon excitation with 808 and 978 nm laser diode. Three intense emissions centered at around 529, 546 and 657 nm, alongwith a very weak blue emission at 410 nm have clearly been observed for the Er³⁺/Yb³⁺-codoped halide modified tellurite glasses upon excitation at 978 nm and the involved mechanisms are explained. The quadratic dependence of fluorescence on excitation laser power confirms the fact that the two-photon contribute to the infrared to green-red upconversion emissions. And the blue upconversion at 410 nm involved a sequential three-photon absorption process.     

Continuously tunable external-cavity diode laser with a double-grating arrangement

A new external-cavity diode laser system based on an extended version of the Littman configuration is investigated. In our laser system the tuning mirror is replaced with a second grating mounted at the Littrow angle. This double-grating design provides a smaller passive bandwidth than the grating-mirror configuration, which is used to compensate for the large angle-of-incidence-dependent losses of the grazing-incidence grating. This results in a broader continuous tuning range with an improved mode stability. Because two laser diodes, emitting at 820 and 775 nm, respectively, are used, the external-cavity laser is continuously tunable without mode hops across 35 nm at 820 nm and 27 nm at 775 nm. Such a laser was used to measure the absorption lines of the oxygen A band around 762 nm. The complete R - and P -rotational branches of the b summation operator(g)(1) (+)(nu(??)=0)?X (3) summation operator(g)(-)(nu (?)=0) transition were recorded in a single-wavelength scan.     

掺铒矾酸钇晶体上转换荧光研究

使用波长为808和658nm的半导体激光器和染料激光器作为激发源，测量了Er³⁺：YVO₄晶体的波长在553和410nm附近的上转换荧光.对激发过程的分析表明，贡献于上转换荧光的主要激发机制为激发态吸收.在不同浓度下对上转换荧光的寿命测量结果显示，随Er³⁺浓度的提高，553nm绿光的荧光寿命随浓度的增加而减小，但410nm的荧光寿命随Er³⁺浓度无明显变化.结合绿光强度随掺杂浓度增加而减小的结果，认为在所测浓度范围内 关键词：     

碳纳米管的热解法制备、电子显微镜观察及拉曼光谱研究

以二茂铁和二甲苯为原料在Ar和H2 气氛中不同温度下热解制备出了不同直径分布的碳纳米管。在 740℃、780℃、82 0℃和 880℃下制备出的碳纳米管的外径分布分别为 1 7-80nm、2 0 - 73nm、40 - 70nm、1 7- 2 7nm。拉曼光谱和透射电子显微镜 (TEM )观察表明 ,在82 0℃下制备的碳纳米管晶形最完整     

Experimental Study on Optical Limiting and Transient All-optical Switching Properties of a Cubanelike Transition-metal Cluster Compound (n-Bu4N)3[MoAg3BrI3S4]

１ＩｎｔｒｏｄｕｃｔｉｏｎＩｎｒｅｃｅｎｔｙｅａｒｓ,ｔｈｅｐｏｔｅｎｔｉａｌｏｆｒｅｖｅｒｓｅｓａｔｕｒａｂｌｅａｂｓｏｒｐｔｉｏｎ（ＲＳＡ）ｍａｔｅｒｉａｌｓｉｎｏｐｔｉｃａｌｌｉｍｉｔｉｎｇａｎｄｏｐｔｉｃａｌｓｗｉｔｃｈｉｎｇｈａｖｅｇｒａｄ...     

Measurements of nanoparticle size distribution produced by laser ablation of tungsten and boron-carbide in N2 ambient

Nanoparticles (NPs) were produced by ablating tungsten and boron-carbide (B₄C) target materials in atmospheric pressure nitrogen ambient using ArF excimer laser pulses. The size distributions of the NPs formed during the ablation were monitored—within a 7-133 nm size window—by a condensation particle counter connected to a differential mobility analyzer. The laser repetition rate was varied between 1-50 Hz, and the fluence was systematically changed in the range of 0.5-15 J/cm², for both materials, allowing a comparative study in an extended laser parameter regime. The multishot ablation threshold (Φ_th) of B₄C was determined to be ∼1.9 J/cm² for the laser used (ArF excimer, λ = 193 nm). Similarly to earlier studies, it was shown that the size distributions consist of mainly small nanoparticles (<∼20 nm) attributed to a non-thermal ablation mechanism below Φ_th. An additional broad peak appears (between 20 and 40 nm) above Φ_th as a consequence of the thermally induced macroscopic ablation. Chemical composition of deposited polydisperse nanoparticles was studied by X-ray photoelectron spectroscopy showing nitrogen incorporation into the boron-carbide.     

正交双色场中氢分子非次序双电离的研究

利用经典系综模型,研究了正交双色场作用下氢分子非次序双电离中双电离电子的相关特性.结果表明,双电离电子相关动量谱强烈地依赖于正交双色场的相对相位.通过改变正交双色场的相对相位,相关动量可以从反相关模式转变为相关模式.向后分析表明,相关电子动量谱对双色场相对相位的依赖关系起源于碰撞过程中碰撞电子碰撞角和碰撞动量对相对相位...     

Tuning ranges of 355 nm pumped dyes from 410 to 715 nm

Wavelength tuning ranges and optimal concentrations are reported for 16 commercially available laser dyes pumped with the third harmonic of a Nd-YAG laser at 355 nm. The laser dye outputs cover the visible range from 410 to 715 nm.     

N2O+离子A2Σ+电子态的光解动力学研究

用一束波长为360.55nm的激光，通过N2O分子的（3+1）共振多光子电离（REMPI）过程制备纯净且布居完全处于X2Π(000)态的母体离子N2O+，然后用另一束波长在275—328nm范围内的可调谐激光将制备的N2O+离子激发至预解离电子态A2Σ+.实验发现，由于解离碎片NO+所具有的一定的反冲速度，其TOF质谱峰明显比N2O+母体宽.通过分析NO+碎片TOF质谱峰形状，得到了解离产物的总平均平动能〈ET〉；通过考察〈ET〉随光解能量的变化，发现光解能量在32000cm-1附近约250cm-1的变化 关键词： N2O+离子A2Σ+态 TOF质谱峰 预解离机理     

描述激光二极管远场光强分布的理论模型

 介绍了描述激光二极管远场光强分布的几种典型理论模型,并与实验结果作了详细比较。结果表明：激光二极管的传输和远场特性应当用非傍轴理论描述,并且远场光强分布一般与输出功率大小有关。在不同功率水平下,异质结激光二极管快轴与慢轴方向的远场行为应选用不同的模型模拟。此外,还对厄米-高斯模型做了修正,考虑了奇数阶厄米-高斯模的贡献,并用厄米-高斯模的非相干叠加代替厄米-高斯模的相干叠加。改进的厄米-高斯模型能更好描述100 mW双异质结GaAlAs LD慢轴方向的远场光强分布。     

Correlated two-electron momentum spectra for strong-field nonsequential double ionization of He at 800 nm

We report on a kinematically complete experiment on nonsequential double ionization of He by 25 fs 800 nm laser pulses at 1.5 PW/cm;{2}. The suppression of the recollision-induced excitation at this high intensity allows us to address in a clean way direct (e,2e) ionization by the recolliding electron. In contrast with earlier experimental results, but in agreement with various theoretical predictions, the two-electron momentum distributions along the laser polarization axis exhibit a pronounced V-shaped structure, which can be explained by the role of Coulomb repulsion and typical (e,2e) kinematics.     

Study on optical characteristics of Nd:YVO4/YVO4 composite crystal laser

Thermal effect in crystals is the main obstacle blocking diode-pumped solid state laser to get high and stable output power. Diffusion bonding crystal has been demonstrated to be an effective method to relieve the thermal lensing theoretically based on the numerical heat analysis to the end-pumped anisotropic laser crystal. The temperature distributions in Nd:YVO4/YVO4 composite crystal and conventional crystal were analyzed and compared. The end-pumped Nd:YVO4/YVO4 composite crystal laser was designed and set up with z-cavity. The maximum output powers of 9.87 W at 1064 nm and 6.14 W at 532 nm were obtained at the incident pump power of 16.5 W. The highest optical-optical conversion efficiencies were up to 59.8% at 1064 nm and 37.2% at 532 nm respectively.     

HN3分子在190-248 nm的紫外光分解动力学

利用氢原子里德堡态飞行时间谱技术研究HN3分子在紫外光(190?248 nm)光照射下的H+N3通道的光解动力学结果．通过测量H+N3通道的产物平动能分布以及产物的角分布，得到了在不同波长光解下N3产物分子的振动态分布． 实验结果表明， 在大于225 nm时，HN3分子主要是通过一个排斥态解离的．而在低于225 nm时，有一个慢的通道从220 nm 开始出现．这一新的解离通道是一个闭环产生环状N3产物的通道．当光解能量增加时，这一新通道相对的变得越来越重要．     

Laser induced fluorescence of CdHg excimer

The fluorescence of CdHg excimer has been observed over the spectral range 220-320 nm for temperature between 660-820K. The spectra were excited in a Cd-Hg mixture contained in a quartz vapor cell by laser pulses at 326.1nm. The peaks of these bands are at about 232, 256 and 286 nm respectively. An interpretation has been given out according to the potential-energy curves.     

射频超导腔加速性能的改进

为提高超导加速腔的加速梯度和Q值，改进了薄膜型超导腔的加速性能。研究证明，对于铜铌溅射腔，在无氧铜衬底和铌膜之间加入NbN 层可以提高铌膜的超导转变温度，改善晶格结构；对纯铌超导腔提出了改进方法，在传统的纯铌超导腔表面制备多层的超导-绝缘-超导复合膜可以屏蔽Nb腔表面的界面场，提高超导腔的临界磁场，从而提高了铌腔的加速梯度。