压缩真空态光场中二能级原子的简并双光子荧光谱

利用原子约化密度算符主方程的方法研究了多模压缩真空态光场中二能级原子的双光子荧光谱，我们发现存在一种Ｒａｂｉ振荡阈值，在阈值之下原子的简并双光子荧光谱呈现洛仑兹线型单峰结构，在阈值之上具有三峰结构，其三峰的线宽和峰高均呈现很强的相敏性，中峰线宽可小于热光场中的线宽，但大于真空场中双光子的自然线宽，两边峰的线宽随压缩光的强度增大而增宽，边峰到中峰的距离也依赖于压缩真空态光场的压缩特征。     

压缩真空态光场中两能级原子的双光子荧光的反聚束效应

利用已得到的原子约化密度算符主方程，研究了两能级原子与宽带压缩真空态光场的双光子相互作用．通过求解双光子Bloch方程，利用量子回归定理，得到双光子荧光的二阶关联函数．在此基础上讨论了原子的双光子荧光的反聚束效应． 关键词：     

缀饰原子系统中双光子共振非简并四波混频

本文研究了缀饰原子系统中的双光子共振非简并四波混频.理论上我们研究了多普勒增宽的四能级系统中耦合光场对双光子共振非简并四波混频的影响,发现加入强耦合场后,非简并四波混频频谱出现Autler-Townes分裂;在不同双光子共振失谐时,由于量子干涉双光子共振非简并四波混频的信号能够被抑制或增强.实验上我们在Ba原子蒸汽中,通过引入基态6s2和自电离里德堡态6pnd之间的原子相干证实了该现象.本方法提供了一种不仅可以测得共振频率和横向弛豫,而且可以测得两个高激发原子态之间的跃迁的偶极矩阵元的新的光谱学工具.     

压缩真空场中非简并双光子过程中系统约化密度主方程

在本文中我们利用投影算符技巧通过刘维方程推导了系统约化密度主方程。这种方法特别适合于赝非马尔可夫的库场情况。所得结果和改进的路易塞尔方法的结果一致，这种方法能正确地在各种库的情况下给出单光子过程和双光子过程的系统的主方程，我们首次求得压缩真空库场中非简并双光子过程的系统约化密度主方程。     

非简并拉曼过程中交流斯塔克位移对腔场谱的影响

研究了原子与双模光场非简并拉曼耦合过程中交流斯塔克位移对腔场谱的影响.给出了原子处于基态且双模初始场为光子数态、相干态和压缩真空态时光谱结构的数值结果.发现数态光场在弱场条件下每模腔场谱都是三峰结构，在强场条件下则为双峰或单峰结构，相干态和压缩真空态光场的腔场谱在弱场或强场条件下都是双峰结构.随着斯塔克位移参数的变化,双峰的高度此长彼消. 关键词： 交流斯塔克位移 非简并拉曼过程 腔场谱     

纠缠相干态光场驱动下∧-型三能级原子的辐射谱

采用时间演化算符方法,研究∧-型=三能级原子与纠缠相干态光场共振相互作用的辐射谱.给出了辐射谱一般公式,并讨论在纠缠相干态光场驱动下的辐射频谱结构.结果表明,无论下能级简并与否纠缠相干态光场平均光子数很小时均出现拉比分裂,且强度随双模光场纠缠程度的增加而增加.当两下能级简并时,若两模场的平均光子数较小,辐射谱呈现对称多峰结构,若两模场的平均光子数较大,辐射谱呈现对称五峰结构.当两下能级非简并时,若两模场的平均光子数较小,辐射谱呈现对称多峰结构.若两模场的平均光子数较大,辐射谱呈现对称十峰结构.纠缠相干光与非纠缠相干光辐射谱的本质差别有两点:一是双模光场强量子关联导致纠缠度越强拉比峰强度越高;二是存在纠缠时由于两模场相干性导致辐射谱呈现对称多峰结构.     

偏振调制双光子光谱理论计算

本文从密度矩阵运动方程出发,推导出当各种不同偏振调制激光场与三能级粒子系统相互作用时,同核双原子分(具近共振中间能波)单重电子态之间的双光子跃迁所产生的荧光信号强度和线型.对比偏振调制的与光子强调制的信号强度和线型时,表明:偏振调制双光子光谱(PMTPS)不仅能消除由吸收同一光束的同向双光子所产生的多普勒加宽背景,极大地提高光谱分辨率;而且不同电子态之间跃迁的O、P、Q、R、S支谱线强度与激光偏振状态有关,可借以标识分子的高激发电子终态和转动能级,有选择地简化复杂的分子光谱.可以预期,PMTPS是研究分子光谱和高分辨率激光光谱极有用的一种技术.     

"两原子-双模腔场"系统的腔场谱

研究了存在偶极相互作用的两等同原子与双模腔场共振相互作用双光子过程的腔场谱,研究发现,当两模初态都为光子数态或相干态时,两模腔场谱之间有很强的相互影响,在两模场强相同时,两划的光谱结构也相同,且在强场下呈现三峰结构;当两模初态场强不同时,较强的一模出现简单的单峰结构,而较弱模光谱中三峰的距离随另一模光子数的增加而增大。当两模均为压缩真空态时,在强场下得到经典共振荧光谱,且两模腔场谱之间的相互影响很弱。     

薄原子蒸汽膜的双光子光谱及Dicke窄化

薄原子蒸汽膜的单光子Dcike窄化吸收光谱可以拓展到双光子情形，以级联三能级系统为例,从理论上得到了亚多普勒结构的双光子吸收光谱，其线型表现出和单光子过程相似的与膜厚和探测光波长的比值(L/λ)相关的周期性.当L/λ=(2n+1)/2(膜厚为半波长的奇数倍)时，吸收谱线窄化现象明显.当L/λ=2n/2(膜厚为半波长的偶数倍)时，单光子情形的谱线窄化现象消失，而双光子情形的谱线仍表现为亚多普勒结构，尤其在异侧入射的情形下，可以获得极窄的双光子谱线结构. 这种结构来自原子与腔壁碰撞的消激发效应和双光子过程的抽运-探测机制的贡献. 关键词： 薄原子蒸汽膜 双光子光谱 Dicke窄化     

消除简并双光子过程中二能级原子的消相干性

研究了置于外部环境(热库)中的二能级原子在外加驱动场时原子的消相干问题.得到简并双光子过程中原子约化密度算符非对角元.在二能级原子的消相干被消除的情况下,讨论外加驱动场的特性. 关键词： 简并双光子过程 二能级原子 消相干性     

劣腔情况失谐双光子光学双稳系统的原子压缩效应

本文采用广义Wigner分布函数的Fokker-Planck方程的方法,讨论了劣腔极限下失谐双光子光学双稳系统的原子压缩效应,得到压缩区在失谐参数△-θ平面的分布,发现在足够大的原子失谐条件下,原子算符R₂也可能出现压缩效应。 关键词：     

One- and two-photon resonance fluorescence of a three-level atom at high photon densities

We consider the possible physical processes that may arise in a three-level atom when only two of its levels interact with a strong electromagnetic field and when the atomic transition frequency is nearly equal to once and twice the frequency of the laser field, respectively. There have been found pronounced cooperative effects in the spectrum of the two-level system, which is in resonance with the laser field, arising from the presence of the third level. The excitation spectra describing the transitions from the first excited state into the second excited state and from that to the ground state consist, apart from the two central peaks, of two pairs of sidebands which are induced by the laser field of the neighbouring system. Detailed expressions of the spectral functions for the physical processes of one- and two-photon resonance fluorescence have been derived and discussed in the limit of high photon densities. The excitation spectrum of the low frequency modes has been considered and discussed in detail. It is found that quantum beats in spontaneous emission may appear in the spectra of the one- and two-photon resonance fluorescence arising from the interference between the two atomic transition frequencies and the frequency of the laser field. The importance of the low frequency modes that occur in the processes in question has been pointed out.     

Spontaneous emission of a three-level lambda-type atom coupled to separate reservoirs

Considering the anisotropic dispersion model, the upper state population and spontaneous emission spectrum of three-level lambda-type atom with two transitions coupled to separate reservoirs are investigated using the resolvent operator. The upper state population reaches to a steady state value after a weak oscillation when the decay rate is zero and one transition frequency is inside the bandgap. The spectrum associated with each transition was given. Compared with results that were obtained by using isotropic dispersion model, the shape of spectrum changes significantly, and no dark line appears in the spectra.     

与双单色场作用的三能级原子的荧光光谱及双光子过程

本文应用修饰(Dress)变换理论研究了与一强单色激光场和一弱单色激光场相互作用的三能级原子系统,分析了系统的双光子过程特性,得出了原子的荧光光谱分布,并证明了它们与驱动激光场的强度以及频差的依赖关系。 关键词：     

Kerr效应对二项式腔场谱量子干涉的影响

研究了含Kerr介质高Q腔内单个二能级原子与双模二项式光场发生双光子共振相互作用系统的腔场谱,给出了Kerr效应与量子干涉项ΔS(ω)关系的数值计算结果,讨论了Kerr效应对二项式腔场谱量子干涉的影响.结果表明:若初始时刻原子处于激发态而双模光场处于二项式态,随Kerr效应的增强,致使量子干涉项引起谱线强度的改变量呈现出"不规则的周期性衰减振荡"特性,震荡幅度与两模光场的频差密切相关.在Kerr系数χg(g为光场与原子的耦合常数)时,Kerr效应对干涉项的影响比较强烈;在χg时,趋于平稳.随着Kerr效应的增强,系统腔场谱由对称结构逐渐演化为不对称的多谱线结构.     

非共振耗散腔耦合系统的发射光谱

研究了非共振耗散二能级双原子与双单模腔耦合系统发射光谱的性质。探讨了原子和腔场之间的失谐、腔场衰减率及原子失相对该系统发射光谱的影响。结果表明,体系的腔场谱呈现出三重峰结构,原子发射谱呈现出二重峰结构。非共振情况时,腔场谱和原子发射谱的图像皆为非对称图像。在原子与腔场失谐时,与共振情况相比,峰位发生了明显的漂移,且中峰明显增大。增大腔场与原子的失谐,会引起边峰向低频段漂移,并改变其光谱强度;增大原子与腔场的失谐,可以使光谱整体向低频段漂移,并改变其所有峰的光谱强度。随着腔场衰减率的增大,共振情况下,会导致边峰的强度减小;失谐情况下,会导致所有峰的强度均减小。随着原子失相的增大,共振或失谐情况下,会使光谱所有峰的强度均减小。     

Engineering transient spectrum for a two-level system interacting with two-mode intelligent states

The problem of a single two-level atom in its excited state, placed in a bimodal cavity in which an arbitrary form of the intensity-dependent atom–field coupling is present, is solved exactly. Expressions for the energy eigenvalues and eigenvectors are derived, and an exact representation for the time-dependent unitary evolution operator of the system is given, by means of which we analyze the analytic form of the fluorescence spectrum using the transitions among the dressed states of the system. The influence of parameter misfits on the quantum system is discussed. An interesting relation between the fluorescence spectrum and the dynamical evolution is found when the initial field states are prepared in properly intelligent states. By comparison with exact numerical results, we demonstrate that features of the fluorescence spectrum are influenced significantly by the different kinds of the nonlinearity of the intensity-dependent atom–field coupling. We provide numerous examples to illustrate this correspondence, and provide evidence of its usefulness. The present work considerably extends earlier results for two-level systems.     

The influence of quantum interference effects on the resonance fluorescence spectra of a degenerate three-level atom

The resonance fluorescence spectra of a degenerate three-level atom of the V-type in the field of an intense monochromatic wave with an arbitrary polarization composition are investigated. Analytical expressions are derived for the resonance fluorescence spectra, and the angular distribution of spontaneous fluorescence of atoms is analyzed for the D-line emitted by vapors of alkali atoms. It is shown that the number of lines in the spectrum may decrease in the case of the linear polarization of spontaneous radiation. The radiation relaxation operator is obtained for the D-line of alkali metals in the case when an atom is near the metal surface. Interference effects for such systems are analyzed.     

Resonant Fluorescence of a Λ-type Three-level Atom Driven by Microwave Field

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邻-吡啶苯并噻二唑衍生物的合成与双光子荧光传感性能

以吡啶苯并噻二唑基元为荧光传感"接受体(齿)",将其与咔唑"核"键合获得单齿和双齿两个化合物:2,8-(2-吡啶苯并噻二唑)-N-乙基氮杂笏(CPTZ1)和2,8-双(2-吡啶苯并噻二唑)-N-乙基氮杂芴(CPTZ2),并通过红外光谱、核磁共振谱、质谱表征.通过稳态/瞬态单光子荧光测试和飞秒钛宝石激光器泵浦探测,探讨了CPTZ1和CPTZ2化合物对质子[H+]的敏感性.Stern-Volmer方程给出CPTZ1的单、双光子荧光的猝灭常数分别为:k1PSV=0.04 L·mol-1,k2PSV=0.20 L·moL-1;而CPTZ2的猝灭常数则分别为k1PSV=0.10 L·moL-1,k2PSV(CPTZ2)=0.22 L·moL-1.研究结果表明,双光子荧光(TPF)检测表现出对质子更高的敏感性,其灵敏度是相应的单光子荧光(OPF)的2～5倍.