Field—Correlation Effects on Rayleigh—Enhanced Nondegenerate Four—Wave Mixing

We study Rayleigh-enhanced nondegenerate four-wave mixing (NFWM) with time-delayed,correlated fluctuating fields.The importance of the field correlation is revealed in the Rayleigh-enhanced NFWM spectrum when the time delay is varied.The Rayleigh-enhanced NFWM is employed to study the ultrafast processes in the frequency domain.A relaxation time as short as 220 fs was deduced in the Rayleigh-enhanced NFWM experiments in carbon disulphide.     

激光感生双光栅中频谱分辨率的研究

研究了用于测量两束光频差的时间延迟激光感生双光栅的频谱分辨率，确定了当泵浦光具有高斯线型时四波混频信号的产生条件，此条件通过在可调谐的窄带激光和宽带激光间的拍频实验得到证实。     

缀饰原子系统中双光子共振非简并四波混频

本文研究了缀饰原子系统中的双光子共振非简并四波混频.理论上我们研究了多普勒增宽的四能级系统中耦合光场对双光子共振非简并四波混频的影响,发现加入强耦合场后,非简并四波混频频谱出现Autler-Townes分裂;在不同双光子共振失谐时,由于量子干涉双光子共振非简并四波混频的信号能够被抑制或增强.实验上我们在Ba原子蒸汽中,通过引入基态6s2和自电离里德堡态6pnd之间的原子相干证实了该现象.本方法提供了一种不仅可以测得共振频率和横向弛豫,而且可以测得两个高激发原子态之间的跃迁的偶极矩阵元的新的光谱学工具.     

Atomic coherence in nondegenerate four-wave mixing

Two-photon resonant nondegenerate four-wave mixing (NFWM) with the addition of a coupling field in Ba atomic vapour has been studied. We find that coherence of the atomic level transitions leads to suppression of the NFWM signal, giving rise to a dip with a linewidth that is linearly proportional to the intensity of the coupling field.     

Three-Photon Resonant Six-Wave Mixing with Phase-Conjugation Geometry in Na Atomic Vapour

We report a three-photon resonant six-wave mixing (SWM) with phase- conjugation geometry. It has advantages that phase matching condition is not critical and the generation of SWM signal is efficient. This technique provides a new spectroscopic tool for studying the highly excited atomic or molecular states with high resolution. The feasibility of this technique is demonstrated in sodium vapour.     

染料分子电子激发态振动失相过程的非相干光时延四波混频研究

本文对噁嗪(Oxagine)、甲酚紫(cresyl violet)染料分子的吸收带和吸收边进行了非相干光时延四波混频(TDFWM-IL)的详细研究,得到了有关失相参量的数据,并利用非相干光时延四渡混频的多能理论解释了实验结果和失相参量的物理意义。     

Suppression and Enhancement in Parametric Two-Photon Resonant Nondegenerate Four-Wave Mixing via Quantum Interference

Quantum interference may lead to suppression and enhancement of the two-photon resonant nondegenerate fourwave mixing signal in a cascade four-level system.Such phenomena are demonstrated in Ba through inducing atomic coherence between the ground state 6s^2 and the doubly excited autoionizing Rydberg state 6trod.This method can be used as a new spectroscopic tool for measuring the transition dipole moment between two highly excited atomic states.     

THIRD ORDER NONLINEAR OPTICAL PROPERTIES OF PERNIGRANILINE SOLUTION IN CONCENTRATED SULFURIC ACID

The fully oxidized state of polyaniline (PANI), pernigraniline (PN), was synthesizedby oxidation of the emeraldine base form of PANI dissolved in NMP solvent with m-chloroperoxybenzoic acid. The resulted PN was characterized by FTIR and UV-Visiblespectra. The third-order nonlinear optical properties of PN in concentrated sulfuric acid(PN/H_2SO_4) were measured by a degenerated four wave mixing (DFWM) method. The re-sults obtained suggest that the soliton-pair intermediate state associated with thedegenerated state does not play a major role in the third order nonlinear optical prop-erties of PANI.     

用时间延迟激光感生双光栅方法测量两束光的相对相位变化

用时间延迟激光感生双光栅研究光路中的相位变化.实验结果表明,通过拍频信号峰值的位移,可以测量两束频率与偏振均不相同的光经过介质后相对相位的变化.     

非相干光时延四波混频的多能级理论——非均匀加宽情形

本文将我们建立的非相干光时延四波混频(TDFWM-IL)的多能级理论由均匀加宽情形发展到非均匀加宽情形,得到吸收带同时存在均匀和非均匀加宽时,TDFWM-IL多能级理论给出的信号强度随两束泵光相对延时的一般关系式,讨论非均匀加宽占绝对优势时,非相干光光子回波的多能级理论结果,及其与二能级理论结果的差异,论证等效二能级模型同样适用于近似分析存在非均匀加宽影响时,吸收带TDFWM-IL的实验结果,报道在红宝石零声子线和甲酚紫固体膜吸收边上的实验结果,并与上述理论做了比较。