Coherent population trapping spectra in presence of ac magnetic fields

Experimental and theoretical investigations are reported on the effects induced by an alternating magnetic field on coherent population trapping resonances. We show that the ac magnetic field produces sidebands of these resonances in such a way that the spectrum observed is similar to those observed via the FM spectroscopic technique. Because of the very narrow linewidth of the resonances, sidebands are resolved even for ac field frequencies as low as a fraction of a kHz. The theoretical model developed, which takes into account a very simple atomic structure, fits the experimental data quite well.     

基于磁悬浮大体积交叉光学偶极阱的Dimple光阱装载研究

三维拉曼边带冷却后的铯原子样品装载于一个磁悬浮的大体积交叉光学偶极阱中, 继续加载一个小体积的光学偶极阱后, 实现了Dimple光学偶极阱对铯原子的高效装载. 对不同磁场下磁悬浮大体积光阱的有效装载势能进行理论分析与实验测量, 得出最优化的梯度磁场和均匀偏置磁场, 获得了基于磁悬浮大体积光阱的Dimple光学偶极阱的装载势能曲线, 实现了Dimple光学偶极阱对经拉曼边带冷却后俘获在磁悬浮的大体积光阱中的铯原子样品的有效装载. 比较了Dimple光学偶极阱分别从拉曼边带冷却、大体积的交叉光阱和消除反俘获势后的磁悬浮大体积光阱装载的结果, 将俘获在磁悬浮大体积光阱中的铯原子样品装载到Dimple光学偶极阱, 铯原子样品的密度提高了约15倍.     

Measuring the complete force field of an optical trap

The use of optical traps to measure or apply forces on the molecular level requires a precise knowledge of the trapping force field. Close to the trap center, this field is typically approximated as linear in the displacement of the trapped microsphere. However, applications demanding high forces at low laser intensities can probe the light-microsphere interaction beyond the linear regime. Here, we measured the full nonlinear force and displacement response of an optical trap in two dimensions using a dual-beam optical trap setup with back-focal-plane photodetection. We observed a substantial stiffening of the trap beyond the linear regime that depends on microsphere size, in agreement with Mie theory calculations. Surprisingly, we found that the linear detection range for forces exceeds the one for displacement by far. Our approach allows for a complete calibration of an optical trap.     

Effect of a stray magnetic field on nonlinear magneto-optical resonances observed in the geometry of counter-propagating light waves

Magneto-optical resonances of electromagnetically induced absorption (EIA) in a cell filled with the vapor of alkali atoms and buffer gas are considered. The atoms are excited using a configuration of electromagnetic fields composed of two counter-propagating linearly polarized light waves and a static magnetic field. We focus on the influence of the residual magnetic field on the parameters of nonlinear resonances. In real experiments, a residual field is always present in the cell due to imperfect magnetic-field shielding. On the basis of calculations, we formulate practical recommendations for controlling the residual magnetic field in the experiments aimed at observation of high-quality EIA resonances. The results from this work can find application in quantum magnetometry and nonlinear optics.     

Microtrap on a concave grating reflector for atom trapping

We propose a novel scheme of optical confinement for atoms by using a concave grating reflector.The two-dimension grating structure with a concave surface shape exhibits strong focusing ability under radially polarized illumination.Especially,the light intensity at the focal point is about 100 times higher than that of the incident light.Such a focusing optical field reflected from the curved grating structure can provide a deep potential to trap cold atoms.We discuss the feasibility of the structure serving as an optical dipole trap.Our results are as follows.(i) Van der Waals attraction potential to the surface of the structure has a low effect on trapped atoms,(ⅱ) The maximum trapping potential is ~1.14 mK in the optical trap,which is high enough to trap cold ~(87)Rb atoms from a standard magneto-optical trap with a temperature of 120 μK,and the maximum photon scattering rate is lower than 1/s.(ⅲ) Such a microtrap array can also manipulate and control cold molecules,or microscopic particles.     

Manipulation of Nanoparticles Using Dark-Field-Illumination Optical Tweezers with Compensating Spherical Aberration

Based on our previous investigation of optical tweezers with dark field illumination [Chin. Phys. Left. 25（2008）329] nanoparticles at large trap depth are better viewed in wide field and real time for a long time, but with poor forces. Here we present the mismatched tube length to compensate for spherical aberration of an oil-immersion objective in a glass-water interface in an optical tweezers system for manipulating nanoparticles. In this way, the critical power of stable trapping particles is measured at different trap depths. It is found that trap depth is enlarged for trapping nanoparticles and trapping forces are enhanced at large trap depth. According to the measurement, 70-nm particles are manipulated in three dimensions and observed clearly at large appropriate depth. This will expand applications of optical tweezers in a nanometre-scale colloidal system.     

通过圆孔衍射实现冷分子(或冷原子)囚禁的光学偶极阱

以单色标量波衍射理论为基础,研究单色平面波由圆孔衍射产生实现冷分子(或冷原子)光学囚禁的光阱。运用圆孔衍射理论分析讨论了光学偶极阱的光强分布、光学势及偶极力,并导出了有关光阱的几何参量、光强分布、强度梯度及其曲率与光学系统参量(如照明光波的波长、小孔的孔径)间的解析关系。研究表明,当激光功率与波长分别为P=500 W和λ=1.08μm,小孔半径a=20μm时,产生囚禁甲烷CH4分子的光阱光学势约为57.9μK。通过圆孔衍射可实现冷分子或冷原子囚禁,该方案不仅简单可行、操作方便,而且在冷分子物理、原子光学、分子光学和量子光学等领域中有着广阔的应用前景。     

Collisions in a cesium hybrid optical and magnetic trap

A new scheme for trapping Cs atoms in a non dissipative trap has been developed. The trap involves both optical dipole forces and magnetic forces. This device is suitable for Cs atoms in the lowest energy Zeeman sublevel, thus avoiding the two-body inelastic collisions which prevented reaching Bose-Einstein condensation of Cs in purely magnetic traps. Furthermore, an additional magnetic field can be applied, allowing a fine tuning of the two-body elastic collision cross-section. We report on the experimental realization of such a trap and describe the characteristics of the trapped atomic sample. An analysis of the collisional regime is performed using measurements of the damping of the oscillatory modes of the trapped atom cloud.     

激光捕获技术及其发展

激光捕获技术是利用光辐射力来捕捉、移动和操纵微粒的先进技术。光镊即单光束梯度力光阱是通过在高度会聚的激光束束腰附近所产生的极高的场强梯度来形成皮牛顿量级的力,可以三维地捕获和操纵微小粒子。阐述了激光捕获技术的模型和原理以及系统的基本结构;追踪了激光捕获技术的最新研究进展;介绍了非高斯型光阱、光纤光阱和全息光镊等几种特殊形式,并分析了每种形式的特点。展望了激光捕获技术的发展前景。     

Determination of the structure of hyperfine sublevels of Rb in strong magnetic fields by means of the coherent population trapping technique

The splitting of hyperfine sublevels of the ⁸⁵Rb atom in strong magnetic fields has been studied by means of the coherent population trapping technique. Narrow resonances with a high signal-to-noise ratio have been detected in a 30-μm-thick spectroscopic cell. The magnetic field in the direction transverse to the laser beams has been created by permanent magnets and has reached 1600 G. Owing to the exclusive narrowness of the cell, the field in it is almost uniform. The break of the coupling between the electronic and nuclear moments, as well as the transition to the Paschen-Back regime in magnetic fields above 600 G, has been observed. The derivatives of the frequency shifts of the observed resonances and their asymptotic values in strong magnetic fields have been determined in terms of the magnetic field strength. The experimental results have been interpreted within a theoretical model based on the known constants of the hyperfine structure of the Rb atom.     

非线性晶体产生的空心光束中大尺寸粒子囚禁与导引

提出了一种基于非线性ZnSe晶体产生的空心光束与光泳力的大尺寸粒子二维囚禁与一维导引、三维囚禁方案.理论上分析并计算了单个非线性ZnSe晶体产生的空心光束内粒子受到的横向与纵向光泳力,纵向光泳力的大小同粒子尺寸与光束尺寸比例的四次方成正比,与空心光束功率成正比,方向与光束传播方向一致.粒子尺寸与空心光束尺寸越接近时,横向光泳力的大小越大.结果表明该光泳力可以实现对大尺寸粒子的二维囚禁,同时可对粒子进行长距离(米量级)一维定向导引;理论上分析并计算了基于双非线性ZnSe晶体产生的局域空心光束内粒子所受横向与纵向光泳力情况,光泳力与系统参数的依赖关系与单个非线性晶体产生的空心光束中的粒子受力情况类似,不同的是该条件下纵向光泳力指向光束中心.结果表明该局域空心光束可以实现大尺寸粒子的三维有效囚禁.基于非线性ZnSe晶体产生的空心光束或者局域空心光束可以作为大尺寸粒子非接触式有效操控的工具,在现代光学以及生物医学中有潜在的应用.     

The effect of experimental geometry and initial conditions on the shape of coherent population trapping resonances on the fine structure levels of thallium atoms

Specific features of the coherent population trapping effect are considered in the generalized Λ system whose lower levels are the magnetic sublevels of the fine structure levels of the thallium atom. Numerical experiments were performed aimed at examination of the coherent population trapping for the case of nontrivial, but feasible, initial populations of the upper metastable fine structure level. Such populations may be obtained, for example, due to the photodissociation of TlBr molecules. The possibility of reducing the number of resonances of the coherent population trapping in a multilevel system, which may be useful for high-resolution spectroscopy, is demonstrated. It is shown that the magnitude and shape of the resonances can be controlled by varying the orientation of the polarization vectors of the light field components with respect to each other and to a magnetic field. In addition, studying the shape of the coherent population trapping resonances for the atoms obtained by photodissociation of molecules may provide information about these molecules.     

一种新颖的实现冷原子或冷分子囚禁的可控制光学四阱及其二维光学晶格

原子光学晶格为精确操控中性原子和研究某些基本物理问题提供了一种方法。提出了一种利用单光束照明余弦型振幅光栅与透镜组合系统实现冷原子或冷分子囚禁的可控制光学四阱新方案,计算了四阱的光强分布,讨论了从光学四阱到双阱或单阱的演化过程,并导出了光学四阱的几何参量、光强分布、强度梯度及其曲率与光学透镜系统参量间的解析关系,获得了四阱间距与光栅空间频率的关系。研究表明通过改变余弦光栅的空间频率即可实现从光学四阱到双阱或单阱的连续双向演化。     

Optical trapping of single fluorescent molecules at the detection spots of nanoprobes

We propose a scheme of optical trapping of fluorescent molecules, based on the strongly enhanced optical field due to surface plasmon resonances at laser illuminated metal tips or particles. A semiclassical approach is compared to a quantum-mechanical one. Attractive as well as repulsive forces are possible depending on the wavelength of the optical field. The trapping potential is shown to be strong enough to overcome the Brownian motion in water solution for common optical tweezer light inten-sities. Single molecule resonance Raman spectroscopy probes are particularly well suited for the trap-ping scheme. Finally we propose intracellular probing of the function of biomolecules as an application.     

Laser cooling and trapping of ytterbium atoms

The experiments on the laser cooling and trapping of ytterbium atoms are reported, including the two-dimensional transversal cooling, longitudinal velocity Zeeman deceleration, and a magneto-optical trap with a broadband transition at a wavelength of 399 nm. The magnetic field distributions along the axis of a Zeeman slower were measured and in a good agreement with the calculated results. Cold ytterbium atoms were produced with a number of about 10⁷ and a temperature of a few milli-Kelvin. In addition, using a 556-nm laser, the excitations of cold ytterbium atoms at ¹S₀-³P₁ transition were observed. The ytterbium atoms will be further cooled in a 556-nm magneto-optical trap and loaded into a three-dimensional optical lattice to make an ytterbium optical clock.      

Interband optical excitation of space-charge waves in high-resistance semiconductors

A fairly complete theory is proposed for trap recharging waves upon their optical excitation under conditions of dominant interband transitions. It is demonstrated that the occurrence of interband transitions reduces the role of trapping centers existing in the crystal and the carrier lifetime. This leads to a decrease in the lifetime of trap recharging waves and can result in their complete disappearance as eigenmodes of electron oscillations in the semiconductor crystal. It is shown that a large number of specific cases can occur depending on the illumination intensity and the ratio of recombination parameters. The physical meaning of the effective trap concentration and its relation to the screening length of the internal electric field are discussed.     

Plasmonic coherent drive of an optical trap

We demonstrate that optical trapping can be driven by delocalized surface plasmon modes resonantly excited within a standing wave trap. Dynamical modifications are shown to be determined by the near-field symmetry of the plasmonic modes with negligible thermal effect. With low trapping powers and polarization control, remarkable stiffness enhancements are recorded, the larger the smaller the particle. The results can be simply modeled accounting for a coherent interaction between the plasmon field and the Gaussian standing wave of the trap.     

Extending the trapping lifetime of single atom in a microscopic far-off-resonance optical dipole trap

In our experiment, a single cesium atom prepared in a large-magnetic-gradient magneto–optical trap (MOT) can be efficiently transferred into a 1064-nm far-off-resonance microscopic optical dipole trap (FORT). The efficient transfer of the single atom between the two traps is used to determine the trapping lifetime and the effective temperature of the single atom in FORT. The typical trapping lifetime has been improved from ～ 6.9 s to ～ 130 s by decreasing the background pressure from ～ 1 × 10^–10 Torr to ～ 2 × 10^–11Torr and applying one-shot 10-ms laser cooling phase. We also theoretically investigate the dependence of trapping lifetimes of a single atom in a FORT on trap parameters based on the FORT beam’s intensity noise induced heating. Numerical simulations show that the heating depends on the FORT beam’s waist size and the trap depth. The trapping time can be predicted based on effective temperature measurement of a single atom in the FORT and the intensity noise spectra of the FORT beam. These experimental results are found to be in agreement with the predictions of the heating model.     

Accumulation of cold cesium molecules via photoassociation in a mixed atomic and molecular trap

We have realized a mixed atomic and molecular trap, constituted by a Cs vapor-cell magneto-optical trap and a quadrupolar magnetic C s(2) trap, using the same magnetic field gradient. We observed the trapping of 2x 10(5) molecules, formed and accumulated in the metastable a (3)Sigma(+ )(u) state at a temperature of 30+/-10 microK through a approximately 150 ms photoassociation process. The lifetime of the trapped molecular cloud limited by the Cs background gas pressure is on the order of 1 s.     

轴向多光阱微粒捕获与实时直接观测技术

传统的光镊技术使用单个物镜同时进行光学捕获与显微成像,使得捕获与成像区域被限制在物镜焦平面附近,无法同时观察到沿光轴方向(即Z向)捕获的多个微粒.本文提出一种轴平面(XZ平面)GerchbergSaxton迭代算法来产生沿轴向分布的多光阱阵列,将轴平面成像技术与光镊结合,实现了沿轴向对二氧化硅微球的多光阱同时捕获与实时观测.通过视频分析法测量了多个二氧化硅微球在轴向光镊阵列中的布朗运动,并标定了光阱刚度.本文提出的轴向多光阱微粒捕获与实时观测技术为光学微操纵提供了一个新的观测视角和操纵方法,为生物医学、物理学等相关领域研究提供了一种新的技术手段.