Transmission properties of terahertz pulses through subwavelength double split-ring resonators

We present a terahertz time-domain spectroscopy study of the transmission properties of planar composite media made from subwavelength double split-ring resonators (SRRs). The measured amplitude transmission spectra reveal a resonance near 0.5 THz, the central frequency of most ultrafast terahertz systems, for one SRR orientation in normal-incidence geometry. This resonance is attributed to the effect of electric excitation of magnetic resonance of the SRR arrays. In addition, the influences of background substrate, lattice constant, and the shapes of the SRRs on the terahertz resonance are experimentally investigated and agree well with the results of recent numerical studies.     

Experimental observation of true left-handed transmission peaks in metamaterials

We report true left-handed (LH) behavior in a composite metamaterial consisting of a periodically arranged split ring resonator (SRR) and wire structures. We demonstrate the magnetic resonance of the SRR structure by comparing the transmission spectra of SRRs with those of closed SRRs. We have confirmed experimentally that the effective plasma frequency of the LH material composed of SRRs and wires is lower than the plasma frequency of the wires. A well-defined LH transmission band with a peak value of -1.2 dB (-0.3 dB/cm) was obtained. The experimental results agree extremely well with the theoretical calculations.     

Amplitude- and phase-resolved optical near fields of split-ring-resonator-based metamaterials

We investigate the local optical response of split-ring resonator-(SRR)-based metamaterials with an apertureless scanning near-field optical microscope. By mapping the near fields of suitably resonant micrometer-sized SRRs in the near-infrared spectral region with an uncoated silicon tip, we obtain a spatial resolution of better than lambda/50. The experimental results confirm numerical predictions of the near-field excitations of SRRs. Combining experimental near-field optical studies with near- and far-field optical simulations provides a detailed understanding of resonance mechanisms in subwavelength structures and will facilitate an efficient approach to improved designs.     

二维负磁导率材料中的缺陷效应

研究了以金属铜六边形开口谐振环为基元的二维负磁导率材料的缺陷效应.利用电路板刻蚀 技术制备了二维负磁导率材料样品.采用波导法测量了点缺陷和线缺陷对二维负磁导率材料X 波段(8—12GHz)微波透射行为的影响.实验发现，无缺陷的二维负磁导率材料样品存在一个 谐振频率，在稍大于该谐振频率的极窄区域内表现为负磁导率.点缺陷和线缺陷SRR的引入导 致材料主谐振峰的强度下降、谐振频率发生移动，品质因数Q显著下降.缺陷的存在破坏 了材料的周期性结构，从而引起其谐振峰的谐振强度和谐振频率发生变化.缺陷效应的研究 不 关键词： 负磁导率 缺陷效应 开口谐振环     

Identifying magnetic response of split-ring resonators at microwave frequencies

In this study we provide experimental methods to identify the magnetic resonance of split ring resonantors (SRR) at the microwave frequency regime. Transmission measurements were performed on both single SRR unit cell and periodic arrays of SRRs. The magnetic response of the SRR structure was demonstrated by comparing the transmission spectra of SRRs with closed ring resonators (CRR). Effects of the changes in the effective dielectric constant of the SRR medium on the band-gaps of SRR are investigated experimentally. SRRs not only exhibit a magnetic resonance band gap but also a band gap due to the electric resonance. Finally, we present the effect of electric coupling to the magnetic resonance of bianisotropic SRRs by utilizing SRRs with different orientations, and incident electromagnetic wave polarizations.     

Miniband transmission in a photonic crystal coupled-resonator optical waveguide

We demonstrate in the near infrared the coupled-resonator optical waveguide (CROW) concept that was recently proposed by Yariv et al. [Opt. Lett.24, 711 (1999)]. Two-dimensional photonic crystals have been used to define, in a GaAs-based waveguiding heterostructure, an array of micrometer-sized hexagonal cavities coupled through thin walls. With the photoexcitation of InAs quantum dots as an internal source, the transmission spectra of the coupled resonators show marked minibands and minigaps, in agreement with theoretical predictions.     

Effective medium theory of left-handed materials

We analyze the transmission and reflection data obtained through transfer matrix calculations on metamaterials of finite lengths, to determine their effective permittivity epsilon and permeability micro. Our study concerns metamaterial structures composed of periodic arrangements of wires, cut wires, split ring resonators (SRRs), closed SRRs, and both wires and SRRs. We find that the SRRs have a strong electric response, equivalent to that of cut wires, which dominates the behavior of left-handed materials (LHM). Analytical expressions for the effective parameters of the different structures are given, which can be used to explain the transmission characteristics of LHMs. Of particular relevance is the criterion introduced by our studies to identify if an experimental transmission peak is left or right handed.     

Simulation and micro-fabrication of optically switchable split ring resonators

The effect of conductivity variation as a proposed method for the investigation of photoconductive switching properties of split ring resonators (SRRs) is simulated. Three different systems that are applicable under certain fabrication and/or optical excitation conditions are described. The simulated transmission spectrum indicates that for a large range of dark conductivity values, complete switching of the SRR resonance is possible. One of the simulated systems, involving split ring resonators on Si substrate, was fabricated and characterized. The transmission spectrum of that system was measured, with the Si in its high-resistivity state, and a −60 dB dip between 108 and 115 GHz, due to SRRs magnetic resonance, was observed.     

非均匀缺陷环对微波左手材料的影响

以金属铜六边形开口谐振环(SRRs)与金属铜线的组合为结构单元，研究了三维左手材料中的 缺陷效应. 利用电路板刻蚀技术制备了左手材料样品，采用波导法测量了SRRs构成的点缺陷 和线缺陷对左手材料X波段（8—12 GHz）微波透射行为的影响. 实验结果表明，引入不同尺 寸SRRs构成的点缺陷，材料谐振峰强度下降，最多达6 dB，相当于原来的186%，谐振频率 移动，通频带宽在630—720 MHz范围变化；引入不同尺寸SRRs构成三种取向的线缺陷时，材 料谐振峰强度下降，最多达11 dB，相当于原来的34 关键词： 左手材料 缺陷效应     

Improved TL-RLC model for terahertz circular split-ring resonators

Three geometries of split-ring resonators (SRRs) including circular geometry and two elliptical geometries were fabricated by modern photolithography process. The samples were measured by terahertz time-domain transmission spectroscopy. These spectra clearly revealed the lower-frequency LC resonances and the higher-frequency dipole resonances; meanwhile, the coupling effect between the LC and dipole resonance had played an important role in the overall response. Comparing the results shows that the LC resonance, dipole resonance, and the coupling effect can be designed. A simple transmission-line (TL) RLC circuit model was used to help us understand this coupling behavior and the extent of its effects. But the simple model has some disadvantage. For better matching TL-RLC model results with measured data, an improved model was introduced for the circular and y-direction stretched elliptical geometry SRRs. Other resonances and modes existing at higher frequencies except the typical LC and dipole resonances were revealed by the improved model.     

非对称开口六边形谐振单环的微波透射特性

受自然界树型结构的启发，设计了分叉树型微结构单元，用电路板刻蚀技术制作了非对称开口六边形谐振单环及其组合结构.采用计算机模拟和实验研究了单个和多个谐振环在微波段(7—12 GHz)的电磁响应行为.研究结果表明：该结构具有负磁导率特性，开口谐振环几何尺寸影响环的磁谐振频率；两环环间距较小时出现二次谐振；带高级分支的辐射状环列相对于不带分支环列透射峰向低频移动.实验和模拟结果相符. 关键词： 负磁导率 开口谐振环 透射率     

Double nanohole apex-enhanced transmission in metal films

We first present experimental results of enhanced transmission through nanofabricated double-hole arrays in a gold film. An increase in the transmission is observed when the holes are overlapping to produce two apexes, with the transmission more than doubling when the apexes are nearly touching. When the holes are non-overlapping, the transmission maximum drops. The measured spectra through these arrays showed a red-shift in the peak transmission wavelength around 770 nm of nearly 30 nm. These experimental results agree well with our finite-difference time-domain simulations of the double-hole arrays. PACS 78.66.Bz; 42.79.Ag; 42.79.Dj     

谐振频率可调的环状开口谐振器结构及其效应

理论和实验研究表明，开口谐振环(SRRs)中可以激励磁谐振从而实现负磁导率.通过在SRRs结构中引入与其开口边平行的金属短杆设计并制备了新的磁谐振单元，采用波导法系统研究了短杆对SRRs和左手材料的微波透射特性以及左手效应的影响.实验和数值模拟表明：金属短杆和SRRs开口边形成附加电容，导致SRRs开口电容增大从而引起谐振频率降低.随短杆长度l和短杆与SRRs间距d的增大，SRRs谐振频率也随之减小和增加.短杆的加入不影响SRRs的负磁导率特性，改变短杆与SRRs间距d< 关键词： 开口谐振环 金属短杆 调控 左手材料     

Formation of metallic nanophases in silica by ion beam mixing. Part II: cluster formation

2 matrix by ion-beam mixing of SiO₂/Ag multilayers is studied via Rutherford backscattering spectrometry, optical absorption, and transmission electron microscopy experiments. In a first step, irradiation with MeV heavy ions transforms the continuous Ag layers into a string of micrometer-sized Ag inclusions. This mechanism can be attributed to lateral segregation of metallic atoms induced by irradiation. In a second step, the Ag inclusions are broken up by incoming ions and Ag nanoclusters are formed by agglomeration of mobile Ag atoms. The latter mechanism is likely due to a combination of ballistic mixing and radiation-induced segregation or radiation-enhanced diffusion processes. The size of the metallic nanoclusters formed depends also on the irradiation temperature. Received: 27 October 1997/Accepted: 3 February 1998     

Surface-enhanced Raman scattering (SERS) spectra of Methyl Orange in Ag colloids prepared by electrolysis method

Polyvinyl alcohol (PVA)-protected Ag colloids were prepared by an electrolysis method. The surface-enhanced Raman scattering (SERS) spectra of Methyl Orange (MO), one of the Azo-dye molecules, in Ag colloids were successfully recorded with good concordance comparing to the theoretical results calculated by the Gaussian’98 program. The MO was adsorbed on the surface of Ag nanoparticles by trans-form which plays an important role for the SERS effect. However, the SERS spectra of MO in Ag colloids prepared by chemical reduction method did not appear which may be because of the competition of the borate or citrate ions with the MO. In order to test the applicability of these colloids, the SERS spectra of Sudan red (III) (SR), another of Azo-dye molecules, were measured and the result was good.     

水体细菌微生物多波长透射光谱快速准确获取方法研究

为实现水体细菌微生物快速在线监测,搭建了多波长透射光谱快速测量实验系统,利用该系统分别测量了重铬酸钾标准溶液紫外波段及中性滤光片可见波段的透射光谱,并与紫外-可见分光光度计测得的透射光谱进行对比分析,验证了实验系统测量透射光谱的准确性;以水体中常见的金黄色葡萄球菌作为研究对象,利用搭建的实验系统获取金黄色葡萄球菌溶液在220～900 nm波段的前向小角度透射光谱,进一步验证了实验系统测量细菌微生物透射光谱的准确性和快速性。结果表明,由实验系统和紫外-可见分光光度计测得的重铬酸钾标准溶液,与中性滤光片紫外波段及可见波段透射光谱的线性拟合相关系数分别为0.999 7和0.999 5,光密度误差分别在5.00%和4.58%以内,说明两个系统测量光谱的一致性较好,所搭建的实验系统测量标准样品紫外-可见透射光谱准确度较高;对于金黄色葡萄球菌,实验系统测得的透射光谱经过校正后,与紫外-可见分光光度计测得的透射光谱线性拟合的相关系数为0.999 97,两者相比的光密度误差在0.74%以内;系统重复30次细菌光谱信号采集获得平均透射光谱单次测量时间为15 s,说明该实验系统相对于紫外-可见分光光度计能够快速准确获取水体细菌微生物多波长透射光谱,在保证测量结果准确的同时缩短了光谱测量时间,为水体细菌微生物快速检测提供技术支持。     

Dynamical electric and magnetic metamaterial response at terahertz frequencies

Utilizing terahertz time domain spectroscopy, we have characterized the electromagnetic response of a planar array of split ring resonators (SRRs) fabricated upon a high resistivity GaAs substrate. The measured frequency dependent magnetic and electric resonances are in excellent agreement with theory and simulation. For two polarizations, the SRRs yield a negative electric response (epsilon < 0). We demonstrate, for the first time, dynamical control of the electrical response of the SRRs through photoexcitation of free carriers in the substrate. An excited carrier density of approximately 4 x 10(16) cm(-3) is sufficient to short the gap of the SRRs, thereby turning off the electric resonance, demonstrating the potential of such structures as terahertz switches. Because of the universality of metamaterial response over many decades of frequency, these results have implications for other regions of the electromagnetic spectrum.     

Fabrication of terahertz metamaterials by laser printing

A laser printing technique was used to fabricate split-ring resonators (SRRs) on Si substrates for terahertz (THz) metamaterials and their resonance behavior evaluated by THz time-domain spectroscopy. The laser-printed Ag SRRs exhibited sharp edge definition and excellent thickness uniformity, which resulted in an electromagnetic response similar to that from identical Au SRR structures prepared by conventional photolithography. These results demonstrate that laser printing is a practical alternative to conventional photolithography for fabricating metamaterial structures at terahertz frequencies, since it allows their design to be easily modified and optimized.     

杂质银对氧化锌薄膜气敏光学特性的影响

用反应式射频磁控溅射方法制备了纯氧化锌（ＺｎＯ）薄膜和掺Ａｇ的ＺｎＯ气敏光学传感薄膜。测量了这些薄膜在ＮＯｘ气体中的透射光谱，然后由透射光谱获得了灵敏度的变化规律，发现掺Ａｇ后的ＺｎＯ薄膜对ＮＯｘ气体的灵敏度高于纯ＺｎＯ薄膜，用俄歇电子能谱（ＡＥＳ）测试了这些薄膜的组分，发现当掺Ａｇ量为５％时灵敏度最高，并结合朗缪尔（Ｌａｎｇｍｕｉｒ）型吸附平衡关系式解释了这些现象，理论和实验结果能很好的相符。     

Investigation of the thickness of Ag, AgI films in the capillary for hollow waveguides

A metallic (Ag)–dielectric (AgI) hollow glass waveguide is a promising and flexible fiber for the delivery of high-power CO₂ laser radiation. The thickness of metallic (Ag) films and dielectric (AgI) films is a critical factor which greatly influences the attenuation of the waveguides. In this paper, metallic (Ag)–dielectric (AgI) films were successfully prepared in the capillary whose inner diameter is 0.53 mm, and firstly investigated with theoretical analysis and measured by means of AES and SEM. There is good agreement between theoretical thickness and experimental results, which confirms the validity of the theoretical analysis, which makes the estimate of the thickness of both the metallic and dielectric films possible with high accuracy prior to the preparation of hollow glass waveguides. The attenuation spectra of Ag/AgI hollow waveguides shows the loss increases with the thickness of Ag, AgI films and indicates that the Ag/AgI hollow waveguide is suitable for the transmission of IR radiation.