基于双核模型对超重元素合成机制的研究

在双核模型基础上，考虑了熔合与准裂变的竞争，通过数值法求解主方程，计算了⁵⁰Ti，⁵⁸Fe+²⁰⁸Pb，²⁰⁹Bi这4个反应系统通过冷熔合反应合成超重元素的激发函数，得到了与实验比较符合的结果.计算了不同入射能量时各角动量分波对熔合概率和超重核存活概率的影响以及对蒸发剩余截面的贡献.这些结果对进一步理解超重核的合成机制有重要意义. 关键词： 超重元素 双核模型 熔合反应 蒸发剩余截面     

基于RMF理论对超重核结构和合成以及滴线外核的研究

总结和回顾了超重核结构和反应研究的历史和现状,利用形变约束的相对论平均场理论系统计算了实验观测到的Z=102—112号元素的能量随形变的变化,得到了这些核素的基态和鞍点性质,利用Strutinsky壳修正方法研究了壳效应对这些核素的影响.利用所得到的结构信息,计算了相应的冷熔合反应的截面,给出了与实验相仿的结果,得到Z=118号元素的合成截面为23pb,比宏观模型的结果小20倍.讨论了相关物理量对反应截面的影响.同时,还给出了相对论连续谱Hartree Bogoliubov(RCHB)理论对滴线外核1800Sn的描述. The studieson structure and reaction for superheavy elements are reviewed. Based on constrained relativistic mean field(CRMF) theory, binding energiesof elements from Z=102 to Z=112, which can be measured experimentally, as a function of deformation arecalculated, and the properties of equilibrium and saddle point of these nuclides are obtained. Using the single particle levels based on CRMF, the shell effects are obtained with Structinsky method. The cross sections of the cold fusion are est...     

通过48Ca+249Bk 合成Z=117的可能性研究

利用两步模型对可能合成 Z=117 的核反应48Ca+249Bk 进行了研究。模型将熔合过程分为弹靶接触前的粘连过程和从弹靶接触到形成复合核的形成过程。结合统计蒸发模型,计算了297117 蒸发数个中子的剩余截面。结果表明,在激发能 E* = 31 MeV且复合核蒸发3中子时的剩余截面最大为 0.34 pb ,已经可以用实验方法进行探测。     

超重核性质与合成机制的理论研究

探索原子核的电荷与质量极限,合成长寿命超重核是当前原子核物理研究的重要前沿问题之一。本文综述了我们近几年在超重原子核结构性质与合成机制方面取得的理论研究进展。在结构性质方面,利用处理对关联的粒子数守恒方法,基于推转壳模型,系统研究了锕系核与超镄核低激发谱,发展了多维形状约束的协变密度泛函理论并用于研究锕系核势能面和裂变位垒以及N=150同中子素中的非轴对称八极关联等。在超重核合成机制方面,系统研究了利用重离子熔合反应合成超重核的三步过程,包括俘获过程——提出了一个位垒穿透概率新公式、熔合过程——提出了一个基于动力学形变势能面的双核模型、存活过程——系统研究了激发态超重复合核存活概率等。系统研究了合成超重核的热熔合反应,得到的熔合蒸发截面与实验符合,并预言了合成119和120号超重元素的生成截面。     

重离子熔合反应形成超重核的截面研究

在双核系统框架下,通过数值法解主方程计算了双核间的核子跃迁全熔合几率.两碰撞核内部激发能由相对运动能损提供,因此能够将核子转移过程与相对运动耦合起来.对一些以Pb为靶的形成超重核的冷熔合反应,计算了最佳激发能、形成双核系统的俘获截面、复合核形成几率及存活几率等,所得到的形成超重核蒸发剩余截面与已知实验值符合较好. In the concept of Dinuclear system (DNS) the complete fusion probability of two touch nuclei via nucleon transfer is described by numerically solving the Master equation. The excitation energy of two colliding nuclei is supplied by the energy dissipation of their relative motion, thus the nucleon transfer process and the relative motion are coupled. For Pb based cold fusion reactions to form super heavy nuclei, the optimal excitation energy, the capture cross section to form a DNS ...     

离线γ技术测量重离子熔合复合核平均角动量

使用离线γ测量技术在质心系25.0—40.5MeV的能区测量了¹²C+⁹³Nb熔合反应产生的二中子和三中子蒸发道的激发函数。由于在相同的激发能下,蒸发道的相对截面比与复合核的角动量有很强的依赖关系,应用统计蒸发程序(CASCADE),从二中子和三中子蒸发道的截面中提取不同能量下的复合核平均角动量和熔合截面。同时从能很好地拟合熔合激发函数的简单耦合道模型(CCFUS)计算中提取复合核的平均角动量。两种方法得到的复合核平均角动量随入射能量的变化相自洽,表明耦合道模型 关键词：     

重离子碰撞中熔合位垒的研究

熔合位垒的研究对熔合反应以及超重核合成有重要的意义。在改进的同位旋相关的量子分子动力学(ImIQMD)模型框架下,提取了熔合反应体系40Ca+40Ca,48Ca+208Pb,48Ca+204Pb和16O+154Sm的熔合位垒。研究了壳修正能对熔合位垒的影响、动力学位垒的能量依赖性、同位旋效应以及形变核的方向效应。计算发现壳修正能降低了熔合反应的位垒。在研究动力学位垒的能量依赖性时,发现位垒高度和位垒半径表现出相反的能量依赖行为。在动力学反应中,当两个核距离接近时,缺中子体系的库仑势同样表现出一定的能量依赖性。对于丰中子体系,由于中子屏蔽作用,库仑势基本没有能量依赖性。     

热熔合反应合成超重核产生截面的同位素依赖性

通过在形成超重核的重离子俘获和熔合过程中引入位垒分布函数的方法对双核模型做了进一步发展. 超重核形成过程中的俘获、熔合和蒸发3个阶段分别采用了半经验的耦合道模型、数值求解主方程和统计蒸发模型的方法来描述. 计算了近年来Dubna小组利用热熔合反应⁴⁸Ca(²⁴³Am, 3n—5n)^288—286115和⁴⁸Ca(²⁴⁸Cm, 3n—5n)^293—291116合成超重新核素的蒸发余核激发函数. 系统分析了⁴⁸Ca轰击锕系元素U,Np,Pu,Am,Cm合成超重核Z=112—116产生截面的同位素依赖性. 给出了合成超重新核素最佳的弹靶组合和入射能量, 即有最大的超重核产生截面. 计算说明, 壳修正能和中子分离能是影响超重核生成截面产生同位素依赖性的主要因素.     

16O+65Cu反应的全熔合与非完全熔合

在45—96MeV ¹⁶O和⁶⁵Cu反应中,用放射化学技术测量了反应余核的激发函数、角分布和微分射程分布.将实验数据和基于复合核统计蒸发模型的Monte-Carlo模拟计算进行了比较,指出重余核来自全熔合形成的复合核的衰变.提取了该系统的全熔合截面,得到的激发函数与理论计算结果相符合.非完全熔合或大质量转移是生成质量数接近靶质量余核的主要生成机制.     

Fusion cross sections for superheavy nuclei in the dinuclear system concept

Using the dinuclear system concept we present calculations of production cross sections for the heaviest nuclei. The obtained results are in a good agreement with the experimental data. The experimentally observed rapid fall-off of the cross sections of the cold fusion with increasing charge number Z of the compound nucleus is explained. Optimal reactions for the synthesis of the superheavy nuclei are suggested.     

Origin of Unexpected Isotopic Trends in Synthesis of Superheavy Nuclei

We investigate the dependence of the yield of superheavy nuclei with Z = 110, 112, 114 on the neutron excess of the projectile nucleus with a two-parameter Smoluchowski equation. It is confirmed that in some cases, the cold fusion reactions with less neutron excess are more favourable than those with more neutron excess. In order to probe the origin of these unexpected isotopic trends, we also investigate the probabilities of capture, fusion and survival in the cold fusion reactions in detail It is found that the maximal ER cross sections of the superheavy nuclei exponentially increase as a function of Bf - Sn with Bf being the fission barrier and Sn being the neutron separation energy. Although the probabilities of capture and fusion have some influences, the unexpected isotopic trends mainly due to the dependence of the ER cross sections on the Bf - Sn value. Therefore, the reactions with larger Bf - Sn values should be more favourable for synthesis of superheavy nuclei.     

Synthesis of superheavy nuclei with <Superscript>238</Superscript>U target

The production of superheavy nuclei with Z=108-116 via hot fusion reactions of the neutron-rich projectiles with 238U target is systematically studied.The results show that the production cross sections of superheavy nuclei do not decrease monotonously as the atomic number Z increasing.The cross sections of the superheavy nuclei at Z = 112 and 115 are enhanced as compared with the whole Z-trend in synthesis of the superheavy nuclei,which clearly illustrates that the reactions with large negative Q-value and...     

基于双核模型对Z = 116~ 121 超重核产生截面的研究(英文)

在双核模型的理论框架下系统研究了超重元素Z = 116 ~121 的蒸发剩余截面,计算过程中核子扩散由主方程描述,同时考虑了全熔合与准裂变的竞争。计算基本再现了利用热熔合反应48Ca+245Cm,48Ca+249Cf 和48Ca+249Bk 产生116~118 号同位素的合成截面。同样,分别以249Bk,249Cf 和243Am 为靶,以48Ca,50Ti 和58Fe 为炮弹,计算了Z = 119~ 121 号同位素的生成截面。结果表明,这些超重核的生成截面随着质子数的增大进一步变小。例如,利用58Fe+243Am 反应合成121 号同位素的最大蒸发剩余截面仅在fb 量级。基于对选择的几个反应系统的系统分析,发现双核系统在熔合蒸发过程中偶Z 奇N 和奇Z 偶N 复合核分别有强的3n 和4n 蒸发道。The production cross sections of superheavy elements with Z = 116~121 have been investigated systematically within the dinuclear system (DNS) concept, where the master equation is solved numerically to obtain the fusion probability. The competition between complete fusion and quasifission, which can strongly affect the cross section of the compound nucleus formation, is taken into account. The evaporation residue cross sections ER calculated for the hot fusion actinide-based reactions (48Ca+245Cm, 48Ca+249Cf and 48Ca+249Bk) are basically in agreement with the known experimental data within one order of magnitude. Similar calculations for the synthesis of superheavy elements up to Z = 121 are performed using the available 249Bk, 249Cf and 243Am as targets and 48Ca, 50Ti and 58Fe as projectiles. Their production cross sections are relatively small,especially for the 58Fe+243Am→301121 reaction. A systematic analysis indicates that the 3n and 4n channelsare respectively the most favorable fusion-evaporation channels in the synthesis of even- and odd-Z superheavy elements.     

The analysis of reactions leading to synthesis of super heavy elements within the dinuclear system concept

The dinuclear system concept of complete fusion of nuclei has been applied to the analysis of superheavy elements synthesis. The optimal excitation energy of compound nuclei and production cross sections in the cold synthesis of heavy elements with charge Z=102–112 have been calculated. The possibility of synthesizing the element with magic number Z=114 in cold and hot fusion reactions has been considered.