Magnetohydrodynamic Kelvin-Helmholtz instability for finite-thickness fluid layers

We have derived the analytical formulas for the Kelvin-Helmholtz instability (KHI) of two superposed finite-thickness fluid layers with the magnetic field effect into consideration. The linear growth rate of KHI will be reduced when the thickness of the fluid with large density is decreased or the thickness of fluid with small density is increased. When the thickness and the magnetic field act together on the KHI, the effect of thickness is more obvious when the magnetic field intensity is weak. The magnetic field transition layer destabilizes (enforces) the KHI, especially in the case of small thickness of the magnetic field transition layer. When considering the effect of magnetic field, the linear growth rate of KHI always decreases after reaching the maximum with the increase of total thickness. The stronger the magnetic field intensity is, the more obvious the growth rate decreases with the total thickness. Thus, it should be included in applications where the effect of fluid thickness on the KHI cannot be ignored, such as in double-cone ignition scheme for inertial confinement fusion.     

Rayleigh-Taylor instability of multi-fluid layers in cylindrical geometry

Rayleigh-Taylor instability of three fluid layers with two interfaces in cylindrical geometry is investigated analytically.The growth rates and the amplitudes of perturbation on the two interfaces are obtained. The feedback factor from outer to inner interface is larger than that from inner to outer interface under the same conditions. The growth rate on the initially unstable interface is larger than the corresponding result in planar geometry for low mode perturbation. The two interfaces are decoupled for a larger mode number perturbation. The dependencies of the amplitudes of perturbation on different initial conditions are analyzed. The negative feedback effect from initially stable interface to another unstable interface is observed. In the limit of infinity inner radius and finite shell thickness, the results in planar geometry are recovered.     

可见光促进有机硅化合物参与的化学转化

有机硅化合物具有重要用途,被广泛应用于材料科学与药物化学等领域.因此,有机硅试剂参与的化学转化一直倍受关注.近年来,可见光催化迅速发展,为有机合成化学提供了新的机遇.在光氧化还原体系下,有机硅试剂可以经由氢原子转移(Hydrogen atom transfer,HAT)或单电子转移(Single electron transfer,SET)过程转化为硅自由基或碳自由基进行反应,具有条件温和、选择性好和原子经济性高等优势.根据反应类型不同,主要综述了有机硅试剂作为硅自由基前体参与的烯(炔)烃硅氢化反应、烯(炔)烃双官能化反应、氮杂芳烃的硅基化反应,以及有机硅化合物作为碳自由基前体参与的亲核加成反应、Minisci反应、均裂取代反应和过渡金属介导的交叉偶联反应.     

激光聚变内爆流体不稳定性基础问题研究进展

激光聚变有望一劳永逸地解决人类的能源问题,因而受到国际社会的普遍重视,一直是国际研究的前沿热点。目前实现激光惯性约束聚变所面临的最大科学障碍（属于内禀困难）是对内爆过程中高能量密度流体力学不稳定性引起的非线性流动的有效控制,对其研究涵盖高能量密度物理、等离子体物理、流体力学、计算科学、强冲击物理和高压原子物理等多个学科,同时还要具备大规模多物理多尺度多介质流动的数值模拟能力和高功率大型激光装置等研究条件。作为新兴研究课题,高能量密度非线性流动问题充满了各种新奇的现象亟待探索。此外,流体力学不稳定性及其引起的湍流混合,还是天体物理现象（如星系碰撞与合并、恒星演化、原始恒星的形成以及超新星爆炸）中的重要过程,涉及天体物理的一些核心研究内容。本文首先综述了高能量密度非线性流动研究的现状和进展,梳理了其中的挑战和机遇。然后介绍了传统中心点火激光聚变内爆过程发生的主要流体力学不稳定性,在大量分解和综合物理研究基础上,凝练出了目前制约美国国家点火装置（NIF）内爆性能的主要流体不稳定性问题。接下来,总结了国外激光聚变流体不稳定性实验物理的研究概况。最后,展示了内爆物理团队近些年在激光聚变内爆流体不稳定性基础性问题方面的主要研究进展。该团队一直从事激光聚变内爆非线性流动研究与控制,以及聚变靶物理研究与设计,注重理论探索和实验研究相结合,近年来在内爆重要流体力学不稳定性问题的解析理论、数值模拟和激光装置实验设计与数据分析等方面取得了一系列重要成果,有力地推动了该研究方向在国内的发展。     

Coupling between velocity and interface perturbations in cylindrical Rayleigh–Taylor instability

Rayleigh–Taylor instability(RTI) in cylindrical geometry initiated by velocity and interface perturbations is investigated analytically through a third-order weakly nonlinear(WN) model. When the initial velocity perturbation is comparable to the interface perturbation, the coupling between them plays a significant role. The difference between the RTI growth initiated only by a velocity perturbation and that only by an interface perturbation in the WN stage is negligibly small. The effects of the mode number on the first three harmonics are discussed respectively. The low-mode number perturbation leads to large amplitudes of RTI growth. The Atwood number and initial perturbation dependencies of the nonlinear saturation amplitude of the fundamental mode are analyzed clearly. When the mode number of the perturbation is large enough,the WN results in planar geometry are recovered.     

Weakly Nonlinear Rayleigh–Taylor Instability in Cylindrically Convergent Geometry

The Rayleigh–Taylor instability(RTI) in cylindrical geometry is investigated analytically through a second-order weakly nonlinear(WN) theory considering the Bell–Plesset(BP) effect. The governing equations for the combined perturbation growth are derived. The WN solutions for an exponentially convergent cylinder are obtained. It is found that the BP and RTI growths are strongly coupled, which results in the bubble-spike asymmetric structure in the WN stage. The large Atwood number leads to the large deformation of the convergent interface. The amplitude of the spike grows faster than that of the bubble especially for large mode number m and large Atwood number A. The averaged interface radius is small for large mode number perturbation due to the mode-coupling effect.     

Effect of initial phase on the Rayleigh—Taylor instability of a finite-thickness fluid shell

Rayleigh—Taylor instability (RTI) of finite-thickness shell plays an important role in deep understanding the characteristics of shell deformation and material mixing. The RTI of a finite-thickness fluid layer is studied analytically considering an arbitrary perturbation phase difference on the two interfaces of the shell. The third-order weakly nonlinear (WN) solutions for RTI are derived. It is found the main feature (bubble-spike structure) of the interface is not affected by phase difference. However, the positions of bubble and spike are sensitive to the initial phase difference, especially for a thin shell (kd<1), which will be detrimental to the integrity of the shell. Furthermore, the larger phase difference results in much more serious RTI growth, significant shell deformation can be obtained in the WN stage for perturbations with large phase difference. Therefore, it should be considered in applications where the interface coupling and perturbation phase effects are important, such as inertial confinement fusion.     

Rayleigh–Taylor instability at spherical interfaces of incompressible fluids

Rayleigh–Taylor instability(RTI) of three incompressible fluids with two interfaces in spherical geometry is derived analytically. The growth rate on the two interfaces and the perturbation feedthrough coefficients between two spherical interfaces are derived. For low-mode perturbation, the feedthrough effect from outer interface to inner interface is much more severe than the corresponding planar case, while the feedback from inner interface to the outer interface is smaller than that in planar geometry. The low-mode perturbations lead to the pronounced RTI growth on the inner interface of a spherical shell that are larger than the cylindrical and planar results. It is the low-mode perturbation that results in the difference between the RTI growth in spherical and cylindrical geometry. When the mode number of the perturbation is large enough, the results in cylindrical geometry are recovered.