共查询到19条相似文献,搜索用时 187 毫秒
1.
A four-state model considering the relative velocity distribution function for calculating the cross section of laserinduced collisional energy transfer in a Sr-Li system is presented and profiles of laser-induced collision cross section are obtained.The resulting spectra obtained from different intermediate states are strongly asymmetrical in an opposite asymmetry.Both of the two intermediate states have contributions to the final state,and none of the intermediate states should be neglected.The peak of the laser-induced collisional energy transfer(LICET) profile shifts toward the red and the FWHM becomes narrower obviously with laser field intensity increasing.A cross section of 1.2 × 10-12 cm 2 at a laser field intensity of 2.17 × 10 7 V/m is obtained,which indicates that this collision process can be an effective way to transfer energy selectively from a storage state to a target state.The existence of saturation for cross section with the increase of the laser intensity shows that the high-intensity redistribution of transition probabilities is an important feature of this process,which is not accounted for in a two-state treatment. 相似文献
2.
By considering the relative velocity distribution function and multipole expansion interaction Hamiltonian, a three-state model for calculating the cross section of laser-induced quadrupole-quadrupole collisional energy transfer is presented. Calculated results in Xe-Kr system show that in the present system, the laser-induced collision process occurs for ~4 ps, which is much shorter than the dipole-dipole laser-induced collisional energy transfer (LICET) process. The spectrum of laser-induced quadrupole-quadrupole collisional energy transfer in Xe-Kr system has wider tunable range in an order of magnitude than the dipole-dipole LICET spectra. The peak cross section decreases and moves to the quasi-static wing with increasing temperature and the full width at half peak of the profile becomes larger as the system temperature increases. 相似文献
3.
Entrance Channel Dependence of Production Cross Sections of Superheavy Nuclei in Cold Fusion Reactions 下载免费PDF全文
Production cross sections of superheavy nuclei Rf and Hs for asymmetric and nearly symmetric projectile-target combinations are systematically studied within the framework of the dinuclear system model. The calculated results show that the production cross sections are strongly dependent on the symmetry of reaction systems. The obtained results are in good agreement with the available experimental data for asymmetric reaction systems.For nearly symmetric systems, the model gives opposite results with coupled channel model in which surface vibration and nucleon transfer are included. 相似文献
4.
《中国物理快报》2016,(4)
Influence of the choice of the NN potential model governing the deuteron wave function on the observables for coherent i~0-photoproduction on the deuteron near η-threshold is investigated by using a three-body model for the intermediate ηNN system with separable two-body interactions.Results for unpolarized differential cross section and polarization observables are predicted.It is revealed that the choice of the NN potential model has a visible effect on the differential cross section and most of the polarization observables,especially in the photon energy range of 600-800 MeV and extreme backward pion angles.We find that the deviation among results obtained by using different deuteron wave functions is quite large.The use of the CD-Bonn NN potential for deuteron wave function doubles the differential cross section in this kinematic region.Compared with the experimental data from CLAS collaboration for differential cross section,sizeable discrepancies are found. 相似文献
5.
Differential, elastic integral and moment transfer cross sections for electron scattering from N2 at intermediate- and high-energies 下载免费PDF全文
A complex optical model potential modified by incorporating the concept of bonded atom, with the overlapping effect of electron clouds between two atoms in a molecule taken into consideration, is firstly employed to calculate the differential cross sections, elastic integral cross sections, and moment transfer cross sections for electron scattering from molecular nitrogen over the energy range 300—1000eV by using additivity rule model at Hartree—Fock level. The bonded-atom concept is used in the study of the complex optical model potential composed of static, exchange, correlation polarization and absorption contributions. The calculated quantitative molecular differential cross sections, elastic integral cross sections, and moment transfer cross sections are compared with the experimental and theoretical ones wherever available, and they are found to be in good agreement with each other. It is shown that the additivity rule model together with the complex optical model potential modified by incorporating the concept of bonded atom is completely suitable for the calculations of differential cross section, elastic integral cross section and moment transfer cross section over the intermediate- and high-energy ranges. 相似文献
6.
State-to-state dynamics of F(~2P) + HO(~2Π) → O(~3P) + HF(~1Σ~+)reaction on 1~3A〞 potential energy surface 下载免费PDF全文
State-to-state time-dependent quantum dynamics calculations are carried out to study F(~2P) + HO(~2Π) → O(~3P) +HF(~1Σ~+) reaction on 1~3A〞 ground potential energy surface(PES). The vibrationally resolved reaction probabilities and the total integral cross section agree well with the previous results. Due to the heavy–light–heavy(HLH) system and the large exoergicity, the obvious vibrational inversion is found in a state-resolved integral cross section. The total differential cross section is found to be forward–backward scattering biased with strong oscillations at energy lower than a threshold of 0.10 eV, which is the indication of the indirect complex-forming mechanism. When the collision energy increases to greater than 0.10 eV, the angular distribution of the product becomes a strong forward scattering, and almost all the products are distributed at θ_t = 0°. This forward-peaked distribution can be attributed to the larger J partial waves and the property of the F atom itself, which make this reaction a direct abstraction process. The state-resolved differential cross sections are basically forward-backward symmetric for v' = 0, 1, and 2 at a collision energy of 0.07 eV; for a collision energy of 0.30 eV,it changes from backward/sideward scattering to forward peaked as v increasing from 0 to 3. These results indicate that the contribution of differential cross sections with more highly vibrational excited states to the total differential cross sections is principal, which further verifies the vibrational inversion in the products. 相似文献
7.
《中国物理 B》2015,(10)
The resonant charge transfer process for Li+–Li(2s) collision is investigated by the quantum-mechanical molecular orbital close-coupling(QMOCC) method and the two-center atomic-orbital close-coupling(AOCC) method in an energy range of 1.0 e V/u–104e V/u. Accurate molecular structure data and charge transfer cross sections are given. Both the allelectron model(AEM) and one-electron model(OEM) are used in the QMOCC calculations, and the discrepancies between the two models are analyzed. The OEM calculation can also give a reliable prediction of the cross sections for energies below 1 ke V/u. 相似文献
8.
The interaction potential for spherical-deformed reaction partners is calculated. The shape, separation and orientation dependence of the interaction potential and fusion cross section of the system ^32S+^154Sm are investigated within the double-folding model of the deformed nuclei. The effective nucleon-nucleon interaction is taken to be the M3Y-Reid potential. The density is considered for three terms of the expansion using the truncated multipole expansion method, which is a deformed Fermi shape With quadrupole and hexadecapole for the density distribution of ^154Sm. It is found for the interaction potential that the height and the position of barrier strongly depend on the deformations, the orientation angle of the deformed nucleus, and hence produce great effects on fusion cross section. The integrated fusion cross section is in good agreement with the experimental data. 相似文献
9.
The differential interference angle in collisional quantum interference on rotational energy transfer 下载免费PDF全文
Collisional quantum interference (CQI) in the intramolecular rotational energy transfer was observed in experiment by Sha and co-workers. The interference angle, which measuring the degree of the coherence, were measured in the experiment of the static cell. Based on the first Born approximation of time dependent perturbation theory, taking into accounts the anisotropic Lennard-Jones interaction potentials, this paper describes the theoretical model of CQI in intramolecular rotational energy transfer in an atom-diatom collision system. In the model, the differential interference angle for the experiment of the molecular beam is calculated, the changing tendencies of the differential interference angle with the impact parameter and collision partners are obtained. This theoretical model is important for understanding or performing this kind of experiments. 相似文献
10.
Quasi-classical trajectory study of H+LiH(v=0,1,2,j=0)→Li+H_2 reaction on a new global potential energy surface 下载免费PDF全文
《中国物理 B》2019,(8)
Quasi-classical trajectory(QCT) calculations are reported for the H+LiH(v = 0–2, j = 0)→Li+H_2 reaction on a new ground electronic state global potential energy surface(PES) of the LiH_2 system. Reaction probability and integral cross sections(ICSs) are calculated for collision energies in the range of 0 eV–0.5 eV. Reasonable agreement is found in the comparison between present results and previous available theoretical results. We carried out statistical analyses with all the trajectories and found two main distinct reaction mechanisms in the collision process, in which the stripping mechanism(i.e., without roaming process) is dominated over the collision energy range. The polarization dependent differential cross sections(PDDCSs) indicate that forward scattering dominates the reaction due to the dominated mechanism. Furthermore,the reactant vibration leads to a reduction of the reactivity because of the barrierless and attractive features of PES and mass combination of the system. 相似文献
11.
激光感生碰撞能量转移的四能级理论模型 总被引:6,自引:2,他引:4
首次考虑了两个中间态对激光感生碰撞能量转移的影响,发展了激光感生碰撞能量转移的四能级理论模型,推导出态振幅的运动方程,并给出碰撞截面的近似表达式,通过对Eu-Sr和Cs-Sr系统的数值计算表明,当频率差│ω21│大小和│ω43│可以相比时,利用三能级近似理论就难以获得令人满意的计算结果,而四能级理论模型则适合于任何情况下的激光感生碰能量转移。 相似文献
12.
By considering the relative velocity distribution function and multipole expansion interaction Hamiltonian, a three-state model for calculating the cross section of laser-induced quadrupole-quadrupole collisional energy transfer is presented. Calculated results in Xe-Kr system show that in the present system, the laser-induced collision process occurs for ~4 ps, which is much shorter than the dipole-dipole laser-induced collisional energy transfer (LICET) process. The spectrum of laser-induced quadrupole-quadrupole collisional energy transfer in Xe-Kr system has wider tunable range in an order of magnitude than the dipole-dipole LICET spectra. The peak cross section decreases and moves to the quasi-static wing with increasing temperature and the full width at half peak of the profile becomes larger as the system temperature increases. 相似文献
13.
LU ZhenZhong CHEN DeYing FAN RongWei & XIA YuanQin National Key Laboratory of Science Technology on Tunable Laser Harbin Institute of Technology Harbin China 《中国科学:物理学 力学 天文学(英文版)》2011,(2)
Based on the four-state model of laser-induced collisional energy transfer,the cross section of the collisional energy transfer in the Sr-Ca system is obtained.Various factors,including field intensity,relative speed,and temperature,which influence the collisional cross section,are discussed for illustrating the features of the Sr-Ca laser-induced collisional energy transfer(LICET) process.The calculated results show that the LICET spectral profiles obviously become narrower when the laser field intensity i... 相似文献
14.
This paper studies the process of mutual neutralization of Si^+ and H^- ions in slow collisions within the multichannel Landau-Zener model. All important ionic-covalent couplings in this collision system are included in the collision dynamics. The cross sections for population of specific final states of product Si atom are calculated in the CM energy range 0.05 e∨/u-5 ke∨/u. Both singlet and triplet states are considered. At collision energies below -10 e∨/u, the most populated singlet state is Si(3p4p, ^1S0), while for energies above -150e∨/u it is the Si(3p, 4p, ^1P1) state. In the case of triplet states, the mixed 3p4p(^3S1 +^3P0) states are the most populated in the entire collision energy range investigated. The total cross section exhibits a broad maximum around 200 300e∨/u and for ECM ≤ 10e∨/u it monotonically increases with decreasing the collision energy, reaching a value of 8 × 10^-13 cm^2 at ECM = 0.05 e∨/u. The ion-pair formation process in Si(3p^2 ^3PJ)+H(1s) collisions has also been considered and its cross section in the considered energy range is very small (smaller than 10^-20 cm^2 in the energy region below 1 ke∨/u). 相似文献
15.
以现有的激光感生碰撞能量转移的四能级理论模型为基础,通过直接积分态振幅的运动方程,对弱场、强场两种情况下Ba-Sr系统的激光感生碰撞能量转移过程进行了数值计算,得到了两种情况下的激光感生碰撞跃迁概率和碰撞截面的谱线线型.在弱场情况下的数值计算结果与近似解析解的计算结果符合很好.对强场情况下的数值积分计算结果表明:激光感生碰撞作用随转换激光强度的增大而增强;强场时激光感生碰撞截面谱线的峰值位置明显偏离了共振频率并向紫端移动,且碰撞截面谱线的半宽度(即调谐范围)较之弱场明显变小.
关键词:
激光感生碰撞能量转移
碰撞截面
Ba-Sr系统
强场 相似文献
16.
Ho^3+ : GdVO4 is a new laser material suitable for high-power laser systems. In this paper we measure the absorption spectra of Ho^3+ in the sample Ho^3+: GdVO4. The intensity parameters are calculated by using the Judd-Ofelt theory. Some predicted spectroscopic parameters, such as the spontaneous radiative transition rate, branching ratio and integrated emission cross section are dealt with. And we also compare the optical parameters with those of other materials. From these results, it is found that there are many transitions which have large oscillator strengths and large integrated emission cross sections. Especially the transitions such as ^5 F4 → ^5 I 8, ^5 S2→^5 I8, ^5 F5 → ^5 I8 and ^5 I7 →^ 5 I8 are useful in solid-state lasers and other fields. Finally, we discuss the splitting of the energy levels of Ho^3+ in the crystal GdVO4 based on the group theory. 相似文献
17.
18.
An interaction potential for an N2(X1σg+) molecule is constructed by using the highly accurate
valence internally contracted multireference configuration
interaction method and the largest basis set, aug-cc-pV6Z, in the
valence range. The potential is used to investigate the elastic
scattering of two N atoms at energies from 1.0× 10-11
to 1.0× 10-4 a.u. The derived total elastic cross
sections are very large and almost constant at ultralow
temperatures, and the shape of total elastic cross section curve is
mainly dominated by the s-partial wave at very low collision
energies. Three shape resonances are found in the total elastic
cross sections. Concretely, the first one is very sharp and strong.
It results from the g-partial-wave contribution and the resonant
energy is 3.645× 10-6 a.u. The second one is contributed
by the h-partial wave and the resonant energy is 1.752× 10-5 a.u. This resonance is broadened by those from the d- and
f-partial waves. The third one comes from the l = 6 partial wave
contribution and the resonant energy is 3.522× 10-5 a.u.
This resonance is broadened by those from the g- and h-partial
waves. The N2(X1σg+) molecular
parameters, which are determined at the current theoretical level,
achieve very high accuracy due to the employment of the largest
correlation-consistent basis set in the valence range. 相似文献
19.
Elastic scattering of two H(^2Sg) and N(^4Su) atoms at low temperatures and accurate spectroscopic parameters of NH (X^3∑^-) radical 下载免费PDF全文
This paper reports that the interaction potential for the X3Z- state of NH radical is constructed at the CCSD(T)/ cc-PV6Z level of theory. Using this potential, this paper calculates the spectroscopic parameters (De, Re, ωe, ωeχe, αe and Be) and their values are of 3.578eV, 0.10368nm, 3286.833cm^-1, 78.433cm^-1, 0.6469cm^-1 and 16.6735cm^-1 respectively, which are in excellent agreement with the experiments. Then the total of 14 vibrational states has been found when J=0 by solving the radial Schrodinger equation of nuclear motion. For each vibrational state, the vibrational manifolds are reported for the first time. And last, the total cross sections, s-wave, p-wave and d-wave cross sections are computed for the elastic collisions between two ground-state atoms (hydrogen and nitrogen) at low temperatures. It finds that the total elastic cross sections are dominated by s-wave scattering when the collision energy is below 10^-6a.u. The pronounced shape resonance is found at energy of 6.1 × 10^-6a.u. Calculations have shown that the shape resonance comes from the p-wave contributions. 相似文献