用激光增益获取弱增益拉曼模式的受激拉曼散射光谱

当酒精的弱增益拉曼模式处于罗丹明640染料分子的激光增益范围时，在由悬垂液滴构成的圆形谐振腔中，观察到乙醇分子C—H伸缩系列模中多个弱增益拉曼模式的受激拉曼散射（SRS）光谱.随着抽运光的增强，迅速增长的强增益拉曼模式的受激辐射抑制了其他弱增益模式的SRS，并导致染料激光的完全淬灭.通过分析圆形腔腔模的光子速率方程和激光染料分子的三能级粒子数速率方程，解释了观察到的实验现象. 关键词： 受激拉曼散射 悬垂液滴 弱拉曼增益模式 激光增益     

用染料荧光增益增强弱增益拉曼模式的受激拉曼散射的经典理论

建立了用染料荧光增益增强弱拉曼模式的受激拉曼散射(SRS)的经典理论,详细给出了拉曼增益gR,染料荧光增益gD和总损耗α的表达式,并在其推导过程中对经典理论作了修正,最后得到了荧光增益和受激拉曼增益可以共同使SRS强度的指数部分快速增长的结果,可以很好地解释观察到的实验现象,并为其提供理论依据。     

KDP晶体受激拉曼散射特性

详细比较了磷酸二氢钾(KDP)晶体的自发拉曼散射和受激拉曼散射光谱,在受激拉曼散射(SRS)中观察到了自发拉曼散射中最强的振动模的三阶Stokes光(559.43,589.74,623.50nm),由于其他振动模的受激拉曼散射增益系数较小,其SRS光谱未观察到。另外,比较了传统生长的未退火和退火后的KDP晶体及快速生长的锥区和柱区KDP晶体的受激拉曼散射增益系数,结果表明生长方法和热退火对KDP晶体的受激拉曼散射增益系数无明显影响。     

DCM荧光增强C3H6O 受激拉曼散射（SRS）的增益特性研究

报道荧光染料DCM对丙酮SRS的高效放大, 研究了DCM中Stokes波的增益特性. 改变DCM乙醇溶 液浓度，变化进入DCM的Stokes光强度以及抽运激光功率，测量并分析了Stokes波增益与上 述条件的关系. 研究结果发现，当DCM浓度为 2×10^-4mol/L时，Stokes波 获得最大功 率增益达到57；抽运激光功率增加或进入DCM的Stokes信号增强时Stokes波输出增强，但 过强的Stokes 信号将导致增益饱和. 关键词： 受激拉曼散射 荧光增强Stokes波 丙酮 DCM     

非线性拉曼激光雷达测量CO2气体的研究

提出了利用气体的受激拉曼散射(SRS)效应激光雷达光源来探测大气中的CO2气体的新方法,设计出探测大气中CO2气体含量的非线性拉曼增益激光雷达,用Nd:YAG激光器(1064 nm)的三倍频光(354.7 nm)通过分别装有CO2气体和N2气体的拉曼管,分别得到CO2气体和N2气体的受激拉曼散射的一阶斯托克斯线(S1),并用S1线作为雷达的种子发射光源.通过实验得到拉曼管中的气压与S1能量的变化关系,对其优化条件和物理机制进行了分析.该实验方法已经成功测出了大气中CO2气体的回波电压信号.     

Au纳米粒子增强丙酮受激拉曼散射研究

受激拉曼散射(stimulated Raman scattering,SRS)具有激光的特性,并且容易获取不同波长的激光,从而成为调谐激光频率的重要途径之一。然而,由于其转化效率低,限制了它的实际应用。金属纳米粒子具有很强的表面增强效应,曾被广泛地用于增强拉曼散射而获得良好的效果。本文提出将金属纳米粒子的这种性质用于增强SRS。把Au纳米粒子混合于拉曼介质丙酮中,以532nm的纳秒脉冲激光作为激发光,研究了Au纳米粒子在丙酮中的浓度对丙酮SRS一阶Stokes光强的影响,并通过仿真计算对实验结果进行了解释和分析。     

非线性拉曼激光雷达系统检测CO2气体的受激拉曼过程

 利用气体的受激拉曼散射增益效应的非线性雷达技术是探测大气中的CO₂气体的重要方法，用Nd:YAG固体激光器（1 064 nm）的三倍频光（354.7 nm）注入装有CO₂和N₂高压气体的拉曼管中，气体的受激拉曼散射（SRS）过程产生两种气体的一阶斯托克斯光，用来作为拉曼雷达的发射种子光源。介绍了产生光源的实验装置，论述了SRS中气体气压变化与一阶斯托克斯光能量输出变化的定量关系，得到最佳能量输出的优化条件，并对SRS中一阶斯托克斯光产生过程的物理机制进行了讨论。并根据光源的试验结果，设计了非线性受激拉曼雷达系统，对前期的普通拉曼雷达进行了实验，得到了初步的实验结果。     

罗丹明B荧光增强苯受激拉曼散射研究

将液芯光纤技术与荧光增强受激拉曼散射技术相结合,能够大大增强受激拉曼散射光谱强度,降低受激拉曼散射阈值。通过对罗丹明B苯溶液在液芯光纤中的受激拉曼散射进行研究,结果表明:荧光染料Rhodamine B可以降低苯溶液的各阶受激拉曼散射阈值近一个数量级;在一定浓度范围内(10-6mol/L~10-8mol/L)各阶Stokes阈值随浓度降低而降低,并在理论上给出了解释。并且理论推导了在荧光种子作用下的四阶耦合波方程。液芯光纤中的受激拉曼光谱技术在对实现宽带受激辐射激光器、种子激光,以及生物大分子结构研究、生物分子的非生物过程研究等领域等有光明应用前景。     

利用一维Vlasov和Maxwell方程模拟激光等离子体相互作用

应用一维Vlasov和Maxwell耦合程序详细研究了激光等离子体相互作用中的基本问题——受激拉曼散射(SRS). 通过研究发现, SRS的产生与电子速度分布函数在相空间中的结构密切相关, 当电子速度分布函数形成相空间涡旋时,背向SRS光大幅增加,而当电子等离子体波相速度附近的电子速度分布函数曲线变平坦后, 背向SRS光基本停止发生. 在模拟中观测到了SRS的爆发、电子速度分布函数形成相空间涡旋、电子俘获等清晰的物理图像. 关键词： Vlasov-Maxwell模拟 受激拉曼散射     

激光等离子体相互作用的受激拉曼散射饱和效应

在激光等离子体相互作用过程中,受激拉曼散射（SRS）会通过Langmuir波衰减不稳定性（LDI）和电子俘获两种机理饱和.文章给出均匀一维等离子体和低强度非相对论激光作用中,LDI和电子俘获两种机理下的SRS饱和时间的解析表达式.SRS饱和时间与入射激光强度,电子密度,电子温度,初始电子密度微扰等参数有关.解析理论计算得到了与模拟和实验相符的结果. 关键词： 受激拉曼散射 饱和 Langmuir波衰变不稳定性（LDI） 电子俘获     

Stimulated Raman scattering in three-dimensional photonic crystals

The results of experimental studies of stimulated Raman scattering of light (SRS) excited in three-dimensional photonic crystals — synthetic opal matrices infiltrated with Raman active media are presented. It is shown that the SRS threshold in such structures decreases with respect to the SRS threshold in Raman active bulk materials. The influence of the photonic-band structure of the active materials used on the SRS properties is estimated.     

Observation of Raman conversion for 70-fs pulses in KGd(WO4)2 crystal in the regime of impulsive stimulated Raman scattering

Raman conversion of femtosecond pulses in a solid-state medium is reported. Stimulated Raman scattering (SRS) was observed in an impulsive SRS regime when the pump pulse's duration was comparable with the period of Raman-active vibration. The generation of super broadband radiation, which is a distinguishing feature of impulsive SRS, is shown.     

Picosecond stimulated Raman scattering in crystals

The comparative values of the peak and integral cross sections of spontaneous Raman scattering and the optical dephasing time of molecular vibrations were determined for several oxide crystals by spontaneous Raman spectroscopy. The spectral, time, and energy parameters of stimulated Raman scattering (SRS) were measured for ten crystals using picosecond YLF: Nd laser pumping with a radiation wavelength of 1047 nm. An analysis of the experimental dependence of the threshold energy of pumping SRS on the integral and peak cross sections of spontaneous Raman scattering showed that the SRS gain increment explicitly depended on the integral cross section and was independent of the peak cross section of spontaneous Raman scattering as the ratio between the pumping pulse width (11 ps) and the time of optical dephasing of molecular vibrations changed from 0.42 to 9.3. The gain coefficients of steady-state stimulated Raman scattering under threshold stimulated Raman scattering conditions were determined for all the crystals studied on the basis of the measured threshold SRS pumping energies, the duration and width of the spectrum of pulses, the nonlinear interaction length, the intensity of pumping, and the theoretical dependences that relate the steady-state and transient SRS gain increments. The steady-state SRS gain coefficients obtained in this work fitted well a linear dependence on the peak cross sections of spontaneous Raman scattering, which substantiated the correctness of our analysis and measurements.     

非自治拉曼多色孤子的管理和传输

以变系数的非自治非线性薛定谔方程为模型,考虑了一种色散、非线性和自发拉曼散射效应管理下的非自治系统,通过简单变换显式给出了该系统的精确非自治拉曼多色孤子解。基于精确孤子解,解析研究了该拉曼多色孤子在非自治管理系统中的演化特性,发现孤子的中心位置、波数与色散和非线性以及拉曼效应有关,而孤子频移仅与拉曼效应的参数决定,拉曼效应主导了非自治孤子的自频移,引起了孤子的频移在传输过程中不断的发生变化,导致了孤子的多色性。另外,我们数值讨论了该非自治孤子的传输稳定性,结果表明:该非自治拉曼多色孤子在有限的扰动下具有较好的稳定性。     

一维动理学数值模拟激光与等离子体的相互作用

利用一维(1D3V)、显式、全电磁、相对论粒子模拟代码研究动理学范畴内激光与等离子体相互作用中的受激拉曼散射,给出了粒子代码的控制方程及其数值离散的详细方案,研究表明:动理学效应在受激拉曼散射不稳定性中十分重要;时问平均的反射率在阈值强度处跃升,在更高的激光强度处达到饱和;受激拉曼背向散射周期性地在次皮秒内爆发,离子效应延迟背向拉曼散射的发生;电子俘获导致了背向拉曼散射出现爆发;Langmuir波的非线性频移使得背向散射达到饱和。     

碰撞对受激Raman散射的影响

从动力学方程出发，引入有效碰撞，讨论了碰撞对受激Raman散射线性增长率的影响.结果表 明，碰撞阻尼和Landau阻尼使得受激Raman散射线性增长率有了实质性的下降，受激Raman散 射只能发生在电子温度和电子密度平面的一个有限区域.现在的理论模型能够解释受激Raman 散射光谱上存在的“缝”(gap)现象. 关键词： 受激Raman散射 碰撞阻尼 线性增长率     

New crystals for Raman lasers

Steady-state and transient stimulated Raman scattering (SRS) in crystals is analyzed. The basic laws of an increase in the SRS gain in crystals are revealed, and methods for searching and creating new SRS laser materials are developed. New crystals for picosecond and nanosecond SRS lasers are proposed, fabricated, and characterized. These materials have the highest SRS cross section, a low SRS threshold, and a wide spectral range of operation.     

单模石英光纤受激拉曼散射温度特性研究

研究了在不同温度下单模石英光纤的受激拉曼散射光谱,从实验和理论上分析了温度对拉曼散射光谱特性的影响,在脉冲调Q倍频YAG激光的泵浦作用下,获得了石英光纤一级斯托克斯光的拉曼频移、带宽及光强随温度的变化规律。实验表明随着温度的升高,拉曼频移逐渐增大,在一定的温度范围内拉曼频移和温度成线性关系。在相同的泵浦功率作用下,当温度较低时,拉曼光谱的级次较低, 低温对高阶斯托克斯光有抑制作用; 温度越低其阈值越高;而拉曼光谱的谱线宽度随温度的变化不是线性的,存在一个谱线宽度极大值点。理论和实验表明温度对光纤受激拉曼散射的光谱特性有直接的影响。     

Numerical simulations of pulsed and quasi-cw regimes of synchronously pumped Raman oscillators

Synchronously pumped Raman oscillators allow for an efficient frequency conversion of pump pulses whose power is well below the threshold for extracavity stimulated Raman scattering (SRS). Numerical simulations show that the cavity mismatch of pump laser and Raman oscillator is critical for maximum conversion efficiency and minimum pulse duration for transient and stationary SRS. At a certain mismatch the simulations predict a quasi-cw Raman oscillator output even at moderate cavity quality factors. Optimum operation conditions are discussed for pump pulse trains of finite lengths. The results of the numerical calculations are in qualitative agreement with a simple phenomenological model. PACS 42.55.Ye; 42.65.Dr; 42.55.Lt     

Nonlinear-laser effects in χ(<Superscript>3</Superscript>)-and χ(<Superscript>2</Superscript>)-active organic single crystals

The process of stimulated Raman scattering (SRS) allows one to convert laser emission wavelength of crystals, providing suitable molecular or lattice modes which contribute to third-order nonlinear optical susceptibility. Renewed interest in this field emerged because of the discovery of SRS in crystals that contain molecular units exhibiting Raman active modes. Particularly, organic nonlinear optical crystals used so far for frequency doubling and third harmonic generation seem to have a great potential for SRS application. This review paper reported same results on efficient SRS lasing effects that were discovered recently in organic crystals.