ZnO作为电子传输层的绿光胶体CdSe量子点LED(QD-LED)的制备与表征

通过调节作为发光层的量子点的尺寸,可以制作出覆盖可见光(380～780 nm)以及近红外光谱的量子点LED(QD-LED),其光谱范围很窄且半高宽可达30 nm。然而量子点LED的寿命、亮度以及效率需要进一步提高才能满足商业化的需求。为了研究QD-LED器件的特性,本文采用523 nm波长的CdSe/ZnS核壳型量子点为发光层、poly-TPD为空穴传输层、ZnO为电子传输层,制备了绿光量子点LED,并表征了器件的特性。     

垂直结构多色量子点LED(QD-LED)最新进展

量子点LED以胶体量子点为发光层,通过调节作为发光层量子点的尺寸可以制作出覆盖可见(380-780nm)以及近红外光谱的量子点LED(QD-LED),而且量子点LED器件发出的光谱范围很窄,其光谱半高宽可达30nm。简述了当今国内外关于QD-LED器件结构的研究成果以及器件的制作工艺,介绍了目前课题组最新的一些相关成果。重点阐述了目前已经得到验证的几种量子点器件结构,分析了其存在的优缺点,这些结论对进一步改进QD-LED的结构以及使其可以更有利于商业化提供了参考。     

In组分渐变提高InGaN/GaN多量子阱发光二极管发光性能

利用金属有机物化学气相沉积系统在蓝宝石衬底上通过有源层的变温生长,得到In组分渐变的量子阱结构,从而获得具有三角形能带结构的InGaN/GaN多量子阱发光二极管(LED)(简称三角形量子阱结构LED).变温光致发光谱结果表明,相对于传统具有方形能带结构的量子阱LED(简称方形量子阱结构LED),三角形量子阱结构有效提高了量子阱中电子和空穴波函数的空间交叠,从而增加了LED的内量子效率;电致发光谱结果表明,三角形量子阱结构LED器件与传统结构LED器件相比,明显改善了发光峰值波长随着电流的蓝移现象.通过以上     

利用选择性外延法生长单芯片双波长白光InGaN/GaN多量子阱结构

为了制备单芯片无荧光粉白光InGaN/GaN多量子阱发光结构,利用选择性外延生长法在SiO2条纹掩膜板上生长出具有梯形形貌的GaN微面结构,并在该GaN微面结构上生长InGaN/GaN多量子阱结构,最终在单芯片上获得了双波长发光.结果表明:梯形GaN微面由(0001)和(11-22)面组成,两者的表面能和极性不同,并且在InGaN/GaN多量子阱生长过程中,In原子和Ga原子迁移速率不同,从而使得(0001)和(11-22)面上的多量子阱具有不同的发光波长;该性质可以使(11-22)面的微面量子阱发出蓝光(峰值波长为420nm),而(0001)面的量子阱发出黄光(峰值波长为525nm),最终形成双波长的复合白光外延结构.     

含有量子点的双波长LED的光谱调控

本文通过对含有高In组分量子点的双波长LED进行了模拟计算, 并对器件的能带结构、载流子浓度、复合速率和辐射光谱进行了研究. 通过对器件结构的调整与对比, 发现蓝绿双波长LED的绿光量子阱中加入高In组分量子点后可以拓宽辐射光谱, 使LED光谱具有更高的显色指数, 为实现无荧光粉的白光LED提供指导. 量子点对载流子具有很强的束缚能力, 并且载流子在量子点处具有更短的寿命, 载流子优先在量子点处复合, 量子点处所对应的黄光与量子阱润湿层所对应的绿光的比例随量子点浓度的增大而增大, 载流子浓度较低时以量子点处的黄光辐射为主, 载流子浓度变大后, 量子点复合逐渐达到饱和, 绿光辐射开始占据主导. 对间隔层厚度和间隔层掺杂浓度的调节可以很方便地调控载流子的分布, 从而实现对含有量子点的双波长LED两个活性层辐射速率的调控. 结果表明, 通过对量子点浓度、间隔层厚度、间隔层掺杂浓度的控节可以很好地实现对LED辐射光谱的调控作用. 关键词： GaN 量子点 光谱调控 双波长LED     

渐变型量子阱垒层厚度对GaN基双波长发光二极管发光特性调控的研究

采用软件理论分析的方法对渐变型量子阱垒层厚度的InGaN双波长发光二极(LED)的载流子浓度分布、 能带结构、自发发射谱、内量子效率、发光功率及溢出电子流等进行研究.分析结果表明, 增大量子阱垒层厚度会影响空穴在各量子阱的注入情况, 对双波长LED各量子阱中空穴浓度分布的 均衡性及双波长发光光谱的调控起到一定作用,但会导致内量子效率严重下降; 而当以特定的方式从n电极到p电极方向递减渐变量子阱垒层厚度时, 活性层量子阱的溢出电子流 得到有效的控制, 双发光峰强度达到基本一致, 同时芯片的内量子效率下降得到了有效控制, 且具备大驱动电流下较好的发光特性.     

低温插入层对绿光LED的发光影响(英文)

利用MOCVD技术在蓝宝石衬底上外延生长了具有低温插入层结构的绿光LED,研究了具有插入层结构的LED的发光特性。插入层的引入增加了In在量子阱中的并入,并且引起了波长红移。经过分析,认为是In的相分离和极化场带来的红移,且恶化了器件的性能。     

GaSb/GaAs复合应力缓冲层上自组装InAs量子点的生长

研究了GaSb/GaAs复合应力缓冲层上自组装生长的InAs量子点.在2ML GaSb/1ML GaAs复合应力缓冲层上获得了高密度的、沿［100］方向择优分布量子点.随着复合应力缓冲层中GaAs层厚度的不同,量子点的密度可以在1.2×10¹⁰cm^-2和8×10¹⁰cm^-2进行调控.适当增加GaAs层的厚度至5ML,量子点的发光波长红移了约25nm,室温下PL光谱波长接近1300nm. 关键词： 自组装量子点 分子束外延 Ⅲ-Ⅴ族化合物半导体     

高Al组分AlGaN多量子阱结构材料发光机制探讨

紫外LED的发光功率和效率还远不能令人们满意,波长短于300 nm的深紫外LED的发光效率普遍较低。厘清高Al组分Al Ga N多量子阱结构的发光机制将有利于探索改善深紫外LED的发光效率的新途径、新方法。为此,本文通过金属有机气相外延技术外延生长了表面平整、界面清晰可辨且陡峭的高Al组分AlGa N多量子阱结构材料,并对其进行变温光致发光谱测试,结合数值计算,深入探讨了Al Ga N量子阱的发光机制。研究表明,量子阱中具有很强的局域化效应,其发光和局域激子的跳跃息息相关,而发光的猝灭则与局域激子的解局域以及位错引起的非辐射复合有关。     

ZnS/CdS/ZnS量子点量子阱的荧光衰减

采用反胶束方法制备了ZnS/CdS/ZnS量子点量子阱，并对其光谱性质进行了研究。结果表明所制得的量子点量子阱尺寸分布均匀，平均粒径为4.5nm，发光峰位于515nm左右，归属于CdS体内的施主－受主对复合。ZnS/CdS/ZnS量子点量子阱中CdS的发光比核－壳结构的ZnS/CdS量子点增强了近四倍，荧光寿命也有所增长。     

Multi-output quantum teleportation of different quantum information with an IBM quantum experience

Multicast-based quantum teleportation(QT) is extensively used in quantum information transmission where a sender sends different information to multiple receivers at the large distance through the quantum entangled channel. In this paper, we introduce the multi-output QT scheme, which deals with the situation that the synchronous transfer of the arbitrary m-and(m+1)-qubit GHZ-class states from one sender to two receivers. Notably, the requirement about synchronous diverse information transmission is satisfied in our scheme with high efficiency. Moreover, we demonstrate the implementation of the special case of above quantum multi-output teleportation scheme on a sixteenqubit quantum computer and a 32-qubit simulator provided by IBM quantum platform, then discuss it in four types of noisy environments, and calculate the fidelities of the output states.     

量子环中量子比特的性质

通过精确求解能量本征方程获得量子环的电子能态,并利用电子的基态和第一激发态构造一个量子比特.对InAs/GaAs量子环的数值计算表明：当环尺寸给定时,量子比特内电子的概率密度分布与坐标位置及时间有关,在环内中心位置处电子出现的概率最大,电子的概率密度随柱坐标内的转角作周期性变化,并且各个空间点处的概率密度均随时间做周期性振荡. 关键词： 量子环 能量本征方程 电子能态 量子比特     

Probabilistic quantum teleportation of shared quantum secret

Very recently, Lee et al. proposed a secure quantum teleportation protocol to transfer shared quantum secret between multiple parties in a network[Phys. Rev. Lett. 124 060501 (2020)]. This quantum network is encoded with a maximally entangled GHZ state. In this paper, we consider a partially entangled GHZ state as the entanglement channel, where it can achieve, probabilistically, unity fidelity transfer of the state. Two kinds of strategies are given. One arises when an auxiliary particle is introduced and a general evolution at any receiver's location is then adopted. The other one involves performing a single generalized Bell-state measurement at the location of any sender. This could allow the receivers to recover the transmitted state with a certain probability, in which only the local Pauli operators are performed, instead of introducing an auxiliary particle. In addition, the successful probability is provided, which is determined by the degree of entanglement of the partially multipartite entangled state. Moreover, the proposed protocol is robust against the bit and phase flip noise.     

Experimental quantum teleportation of arbitrary quantum states

Received: 1 July 1998/Revised version: 2 October 1998     

Synthesis of quantum superpositions by quantum computation

The quantum search algorithm can be looked at as a technique for synthesizing a particular kind of superposition-one whose amplitude is concentrated in a single basis state. This basis state is defined by a binary function f(&xmacr;) that is nonzero in this desired basis state and zero everywhere else. This paper extends the quantum search algorithm to an algorithm that can create an arbitrarily specified superposition on a space of size N in O(sqrt[N] ) steps. The superposition is specified by a complex valued function f(&xmacr;) that specifies the desired amplitude of the system in basis state &xmacr;.     

Electronic structure of quantum spheres and quantum wires

The electronic structures of quantum spheres and quantum wires are studied in the framework of the effective-mass theory. The spin-orbital coupling (SOC) effect is taken into account. On the basis of the zero SOC limit and strong SOC limit the hole quantum energy levels as functions of SOC parameter λ are obtained. There is a fan region in which the ground and low-lying excited states approach those in the strong SOC limit as λ increases. Besides, some theoretical results on the corrugated superlattices (CSL) are given.     

On quantum operations as quantum states

We formalize Jamiolkowski’s correspondence between quantum states and quantum operations isometrically, and harness its consequences. This correspondence was already implicit in Choi’s proof of the operator sum representation of Completely Positive-preserving linear maps; we go further and show that all of the important theorems concerning quantum operations can be derived directly from those concerning quantum states. As we do so the discussion first provides an elegant and original review of the main features of quantum operations. Next (in the second half of the paper) we find more results stemming from our formulation of the correspondence. Thus, we provide a factorizability condition for quantum operations, and give two novel Schmidt-type decompositions of bipartite pure states. By translating the composition law of quantum operations, we define a group structure upon the set of totally entangled states. The question whether the correspondence is merely mathematical or can be given a physical interpretation is addressed throughout the text: we provide formulae which suggest quantum states inherently define a quantum operation between two of their subsystems, and which turn out to have applications in quantum cryptography.     

Two-way quantum communication: Generalization of secure quantum information exchange to quantum network

The idea of secure quantum information exchange (SQIE) [J. Phys. B: At. Mol. Opt. Phys.44, 115504 (2011)] is introduced for the secure exchange of single qubit information states between two legitimate users, Alice and Bob. In the present paper, we extend this original SQIE protocol by presenting a scheme, which enables the secure exchange of n-single qubit information states among the n nodes of a quantum network, with the aid of a special kind of 4n-qubit entangled state and the classical assistance of an extra participant Charlie. For experimental realization of our extended SQIE protocol, we suggest an efficient scheme for the generation of a special kind of 4n-qubit entangled state using the interaction between highly detuned Λ-type three-level atoms and optical coherent field. Further, by discussing the various experimental parameters, we show that the special kind 4n-qubit entangled state can be generated with the presently available technology.     

Quantifying quantum correlation via quantum coherence

Resource theory is applied to quantify the quantum correlation of a bipartite state and a computable measure is proposed. Since this measure is based on quantum coherence, we present another possible physical meaning for quantum correlation, i.e., the minimum quantum coherence achieved under local unitary transformations. This measure satisfies the basic requirements for quantifying quantum correlation and coincides with concurrence for pure states. Since no optimization is involved in the final definition, this measure is easy to compute irrespective of the Hilbert space dimension of the bipartite state.     

From quantum optics to quantum communications

We review the possible roles of quantum optics and quantum information methods for future developments of optical telecommunications. To cite this article: I. Abram, P. Grangier, C. R. Physique 4 (2003).