超重核熔合中的靶核形变效应

利用额外推力模型研究了⁴⁸Ca+²³⁸U俘获和熔合过程中的靶核形变效应.计算表明,在近垒和垒下能区,靶核形变使俘获截面和熔合截面增强,形成的复合核自旋分布展宽.     

Effects of Target Deformation on the Synthesis of Superheavy Nucleus 283^112

We investigate the effects of target deformation on the synthesis of superheavy nucleus 283^112 in the framework of the extra-push model. Our results show that the cross sections of the 3n evaporation residue in the 48^Ca 238^U reaction for the case of β2=0.275 are several times larger than those of β2=0. Meanwhile, the peak position of ER excitation function in the case of the deformed target is shifted to lower energy as compared to that of the spherical target.     

原子核的大质量转移反应和丰中子超重核的产生(英文)

迄今为止,人们合成的超重核都是缺中子的,无论是熔合-裂变反应还是碎化过程都无法使产物达到周期表的“东北区域”。而重核之间(如U核之间) 的近垒大质量转移反应则可能是目前生成丰中子超重核和达到未知丰中子重核区域的唯一途径。在改进的量子分子动力学(ImQMD) 模型结合统计模型框架内,研究了U+U等反应体系的大质量转移反应,计算了反应产生的初生态碎片的质量和电荷分布,并成功再现了产物的终态质量和电荷分布。通过比较3 个反应136Xe+248Cm,48Ca+248Cm和238U+248Cm 产生的106号元素的截面大小,揭示了U+U等重核大质量转移反应对产生丰中子超重核是非常有利的。For elements with Z > 100 only neutron deficient isotopes have been synthesized so far. The “northeast area” of the nuclear map can be reached neither in fusion-fission reactions nor in fragmentation processes.The large mass transfer reactions in near barrier collisions of heavy (U-like) ions seem to be the only reaction mechanism allowing us to produce neutron rich heavy nuclei including those located at the superheavy(SH) island of stability and unexplored area of heavy neutron-rich nuclides. This study is extremely important for nuclear astrophysical investigations and, in particular, for the understanding of the r process. In this paper within the Improved Quantum Molecular Dynamics (ImQMD) model combining with the statistical-evaporation model, the large mass transfer reactions, like 238U+238U have been studied. The charge and mass distributions of transiently formed primary fragments are investigated within the ImQMD model and de-excitation processes of those primary fragments are described by the statistical decay model. The mass distribution of the final products in 238U+238U collisions is obtained and compared with the recent experimental data. Through compared the formation cross sections of transfermium element 106 by three reactions of 136Xe+248Cm, 48Ca+248Cm and 238U+248Cm, it is explored that the large mass transfer reactions, like U+U are very benefit for the production of SH nuclei.     

基于双核模型对Z = 116~ 121 超重核产生截面的研究(英文)

在双核模型的理论框架下系统研究了超重元素Z = 116 ~121 的蒸发剩余截面,计算过程中核子扩散由主方程描述,同时考虑了全熔合与准裂变的竞争。计算基本再现了利用热熔合反应48Ca+245Cm,48Ca+249Cf 和48Ca+249Bk 产生116~118 号同位素的合成截面。同样,分别以249Bk,249Cf 和243Am 为靶,以48Ca,50Ti 和58Fe 为炮弹,计算了Z = 119~ 121 号同位素的生成截面。结果表明,这些超重核的生成截面随着质子数的增大进一步变小。例如,利用58Fe+243Am 反应合成121 号同位素的最大蒸发剩余截面仅在fb 量级。基于对选择的几个反应系统的系统分析,发现双核系统在熔合蒸发过程中偶Z 奇N 和奇Z 偶N 复合核分别有强的3n 和4n 蒸发道。The production cross sections of superheavy elements with Z = 116~121 have been investigated systematically within the dinuclear system (DNS) concept, where the master equation is solved numerically to obtain the fusion probability. The competition between complete fusion and quasifission, which can strongly affect the cross section of the compound nucleus formation, is taken into account. The evaporation residue cross sections ER calculated for the hot fusion actinide-based reactions (48Ca+245Cm, 48Ca+249Cf and 48Ca+249Bk) are basically in agreement with the known experimental data within one order of magnitude. Similar calculations for the synthesis of superheavy elements up to Z = 121 are performed using the available 249Bk, 249Cf and 243Am as targets and 48Ca, 50Ti and 58Fe as projectiles. Their production cross sections are relatively small,especially for the 58Fe+243Am→301121 reaction. A systematic analysis indicates that the 3n and 4n channelsare respectively the most favorable fusion-evaporation channels in the synthesis of even- and odd-Z superheavy elements.     

超重核合成的同位素依赖探讨

利用二参量Smoluchowski方程计算了54Fe+204Pb,56Fe+206Pb,58Fe+208Pb冷熔合和32,34,36S+238U热熔合的复合核形成截面和蒸发残余截面, 结果清楚地显示出超重核合成截面随同位素的变化。 由于较低的入射道库仑位垒、 较低的不对称裂变谷中的条件鞍点和较小的中子分离能, 一般地说, 丰中子同位素的超重核形成截面明显增强。 The cross sections of the compound nucleus formation and e vaporation residue for the 54Fe+204Pb, 56Fe+206Pb, 58Fe+208Pb cold fusion and 32,34, 36S+238U hot fusion have been calculated by using a two parameter Smoluchowski equation. Our results clearly show the isotope dependence of superheavy nucleus production. The formation cross sections of the neutron rich isotope are, generally speaking, obviously enhanced due to the lower Coloumb barrier , lower height of the conditional saddle point, and smaller neutron separation energy.     

Theoretical study of fusion reactions 32S + 94,96Zr and 40Ca + 94,96Zr and quadrupole deformation of 94Zr

The dynamic coupling effects on fusion cross sections for reactions~(32)S + ~(94,96)Zr and ~(40)Ca + ~(94,96)Zr are studied with the universal fusion function formalism and an empirical coupled channel(ECC) model. An examination of the reduced fusion functions shows that the total effect of couplings to inelastic excitations and neutron transfer channels on fusion in ~(32)S +~(94)Zr(~(40)Ca +~(94)Zr) is almost the same as that in ~(32)S +~(96)Zr(~(40)Ca +~(96)Zr). The enhancements of the fusion cross section at sub-barrier energies due to inelastic channel coupling and neutron transfer channel coupling are evaluated separately by using the ECC model. The results show that effect of couplings to inelastic excitations channels in the reactions with94 Zr as target should be similar as that in the reactions with ~(96) Zr as target. This implies that the quadrupole deformation parameters β_2of ~(94)Zr and~(96) Zr should be similar to each other.However, β_2 's predicted from the finite-range droplet model, which are used in the ECC model, are quite different. Experiments on~(48) Ca +~(94)Zr or~(36) S +~(94)Zr are suggested to solve the puzzling issue concerning β_2for~(94)Zr.     

高能核-核碰撞中蒸发碎片的研究

在高能核－核碰撞中,基于简单的模型计算,描述了来自弹核和靶核旁观体的蒸发碎片的多重数分布与角分布． Based on the simple modelling calculation,the multiplicity and angular distribution of evaporated fragments from both projectile and target spectators in high energy nucleus-nucleus collisions are described.     

重离子碰撞中超重核的形成机制(英文)

在双核模型框架下,用数值解主方程方法计算了超重核的熔合几率。 明确描述了包含能量、角动量和碎片形变弛豫的相对运动,并与核子扩散过程相耦合。因此,用微观方法推导出的核子跃迁几率是与时间相关的。所计算的以Pb为靶的冷熔合超重核形成截面和以48Ca为弹核的热熔合超重核形成激发函数与已知的实验值在合理的范围内符合。In the dinuclear system conception, the master equation is solved numerically to calculate the fusion probabilities of super heavy nuclei. The relative motion concerning the energy, the angular momentum and the fragment deformation relaxations is explicitly treated to couple with the diffusion process. The nucleon transition probabilities, which are derived microscopically, are related with the energy dissipation of the relative motion, thus they are time dependent. The formation cross sections of the super heavy nuclei from Pb based cold fusion and excitation functions from 48Ca induced hot fusion are reasonably consistent with known experimental data.     

热熔合反应合成超重核产生截面的同位素依赖性

通过在形成超重核的重离子俘获和熔合过程中引入位垒分布函数的方法对双核模型做了进一步发展. 超重核形成过程中的俘获、熔合和蒸发3个阶段分别采用了半经验的耦合道模型、数值求解主方程和统计蒸发模型的方法来描述. 计算了近年来Dubna小组利用热熔合反应⁴⁸Ca(²⁴³Am, 3n—5n)^288—286115和⁴⁸Ca(²⁴⁸Cm, 3n—5n)^293—291116合成超重新核素的蒸发余核激发函数. 系统分析了⁴⁸Ca轰击锕系元素U,Np,Pu,Am,Cm合成超重核Z=112—116产生截面的同位素依赖性. 给出了合成超重新核素最佳的弹靶组合和入射能量, 即有最大的超重核产生截面. 计算说明, 壳修正能和中子分离能是影响超重核生成截面产生同位素依赖性的主要因素.     

Measurements of effective delayed neutron fraction in a fast neutron reactor using the perturbation method

A perturbation method is proposed to obtain the effective delayed neutron fraction β_(eff) of a cylindrical highly enriched uranium reactor.Based on reactivity measurements with and without a sample at a specified position using the positive period technique,the reactor reactivity perturbation △ρ of the sample in β_(eff) units is measured.Simulations of the perturbation experiments are performed using the MCNP program.The PERT card is used to provide the difference dκ of effective neutron multiplication factors with and without the sample inside the reactor.Based on the relationship between the effective multiplication factor and the reactivity,the equation β~(eff)=dκ/△ρ is derived.In this paper,the reactivity perturbations of 13 metal samples at the designable position of the reactor are measured and calculated.The average β_(eff) value of the reactor is given as 0.00645,and the standard uncertainty is 3.0%.Additionally,the perturbation experiments for β_(eff) can be used to evaluate the reliabilities of the delayed neutron parameters.This work shows that the delayed neutron data of ~(235)U and ~(238)U from G.R.Keepin's publication are more reliable than those from ENDF-B6.0.ENDF-B7.0,JENDL3.3 and CENDL2.2.     

The N~* physics program at Jefferson Lab

Recent measurements of nucleon resonance transition form factors with CLAS at Jefferson Lab are discussed. The new data confirm the assertion of the symmetric constituent quark model of the Roper as the first radial excitation of the nucleon. The data on high Q~2 nπ~+ production better constrain the branching ratios β_(Nπ) and β_(Nη). For the first time, the longitudinal transition amplitude to the S_(11)(1535) was extracted from the nπ~+ data. Also, new results on the transition amplitudes for the D_(13)(1520) resonance are presented showing a rapid transition from helicity 3/2 dominance seen at the real photon point to helicty 1/2 dominance at higher Q~2. I also discuss the status of the search for new excited nucleon states.     

Statistical properties of a single-mode laser driven by additive and multiplicative coloured noises with a coloured cross-correlation for different correlation times

We study a system for a single-mode laser driven by additive and multiplicative coloured noises with a coloured cross-correlation. The analytical expression of the stationary intensity distribution (SID) for the laser is derived in the case of three different correlation times. The influences of each stochastic parameter on the SID are discussed, the effects of the noise "colour" and the cross-correlation of noises on the mean intensity , the variance, λ_2(0), and the skewness,λ_3(0) of the single-mode laser are investigated. We find that there are colourful phase transitions for the SID above a threshold, and re-entrant transitions induced by the "colour" of the additive noises. Further research of the curves of -τ_i, λ_2(0)-τ_i, and λ_3(0)-τ_i (i=1,2,3) (where τ_i is the correlation time) shows that the output intensity not only increases with the additive noise correlation time τ_2 and the cross-correlation time τ_3, but also the quality of the output of laser beams is optimized.     

Mesoporous silicas with covalently immobilized β-cyclodextrin moieties: synthesis,structure, and sorption properties

Mesoporous silicas with chemically attached macrocyclic moieties were successfully prepared by sol-gel condensation of tetraethyl orthosilicate and β-cyclodextrin-silane in the presence of a structure-directing agent. Introduction of β-cyclodextrin groups into the silica framework was confirmed by the results of IR spectral, thermogravimetric, and quantitative chemical analysis of surface compounds. The porous structure of the obtained materials was characterized by nitrogen adsorption-desorption measurements, powder X-ray diffraction, transmission electron microscopy, and dynamic light scattering. It was found that the composition of the reaction mixture used in β-cyclodextrin-silane synthesis significantly affects the structural parameters of the resulting silicas. The increase in (3-aminopropyl)triethoxysilane as well as the coupling agent content in relation to β-cyclodextrin leads ultimately to the lowering or complete loss of hexagonal arrangement of pore channels in the synthesized materials. Formation of hexagonally ordered mesoporous structure was observed at molar composition of the mixture 0.049 TEOS:0.001 β-CD-silane:0.007 CTMAB:0.27 NH₄OH:7.2 H₂O and equimolar ratio of components in β-CD-silane synthesis. The sorption of alizarin yellow on starting silica and synthesized materials with chemically attached β-cyclodextrin moieties was studied in phosphate buffer solutions with pH 7.0. Experimental results of the dye equilibrium sorption were analyzed using Langmuir, Freundlich, and Redlich-Peterson isotherm models. It was proved that the Redlich-Peterson isotherm model is the most appropriate for fitting the equilibrium sorption of alizarin yellow on parent silica with hexagonally arranged mesoporous structure as well as on modified one with chemically immobilized β-cyclodextrin groups.

Open image in new window

Graphical abstract

     

A theoretical study on electron transfer in low-energy collisions of a collinear meta-stable with a $ {\rm{Na}}_3^ - $ {\rm{Na}}_3^ - " border="0"> Na

Electron transfer in the collisions of a with a Na is theoretically studied. It is assumed that the target is collinear (D _h ) and that its electronic state is meta-stable triplet state. Adiabatic potential energy surfaces and non-adiabatic couplings of the system are calculated by using a semi-empirical diatomics-in-molecules (DIM) method. The positions of (avoided)-crossings of potential surfaces are investigated and the non-adiabatic couplings between two different electronic states are calculated. An avoided crossing is found in the region where the separation between the target and projectile is relatively large (10–15 bohr). A dynamical calculation demonstrates that this crossing causes charge transfer between the target and projectile. Another intersection at a smaller separation changes the targets spin state (from triplet state to singlet state or vice versa). The cross-sections for charge and spin transfer reaction are estimated at the collision energy of 6.8 keV. It is found that the charge transfer cross-section is extremely enhanced when the target cluster ion is in its meta-stable triplet state comared to the case where the cluster is the ground singlet state.     

ASYMMETRY PARAMETERS AND DIFFERENTIAL CROSS SECTIONS FOR PHOTOIONIZATION-EXCITATION OF HELIUM

Asymmetry parameter β₂ for photoionization of helium leaving the He⁺ ion in the n=2 level and differential cross sections(DCSs) in the n=2,3,4 levels with photon emission angle θ=90⁰ are provided at photon energies 69-76.8 eV employing the R-matrix method with a 20-term target representation, in which five polarization orbitals \bar{6}l are included. The asymmetry parameter β₂ and the DCS, in the n=2 level in the region of 69-73 eV, are in good agreement with available experimental and theoretical results. Above the n=3 threshold, we present new theoretical results along with measurements. No theoretical and experimental results can be used to compare with the present calculations of the DCSs for photoionization into the He⁺ ion in the n=3,4 levels.     

A special class of stationary flows for two-dimensional Euler equations: A statistical mechanics description

We consider the canonical Gibbs measure associated to aN-vortex system in a bounded domain Λ, at inverse temperature \(\widetilde\beta \) and prove that, in the limitN→∞, \(\widetilde\beta \) /N→β, αN→1, where β∈(?8π, + ∞) (here α denotes the vorticity intensity of each vortex), the one particle distribution function ?^N = ? ^N x,x∈Λ converges to a superposition of solutions ? _α of the following Mean Field Equation: $$\left\{ {\begin{array}{*{20}c} {\varrho _{\beta (x) = } \frac{{e^{ - \beta \psi } }}{{\mathop \smallint \limits_\Lambda e^{ - \beta \psi } }}; - \Delta \psi = \varrho _\beta in\Lambda } \\ {\psi |_{\partial \Lambda } = 0.} \\ \end{array} } \right.$$ Moreover, we study the variational principles associated to Eq. (A.1) and prove thai, when β→?8π⁺, either ?_β → δ _{x 0} (weakly in the sense of measures) wherex ₀ denotes and equilibrium point of a single point vortex in Λ, or ?_β converges to a smooth solution of (A.1) for β=?8π. Examples of both possibilities are given, although we are not able to solve the alternative for a given Λ. Finally, we discuss a possible connection of the present analysis with the 2-D turbulence.     

Chains of twists and induced deformations

Chains of extended twists are composed of factors . The set of Jordanian twists { } can be applied to the initial Hopf algebra . In this case the remaining (transformed) factors of the chain can serve as extensions for such a multijordanian twist. We study the properties of these generalized extensions and the spectra of deformations of the corresponding Heisenberg-like algebras. The results are explicitly demonstrated for the case when .     

Statistics of impedance,local density of states,and reflection in quantum chaotic systems with absorption

We are interested in finding the joint distribution function of the real and imaginary parts of the local Green’s function for a system with chaotic internal wave scattering and a uniform energy loss (absorption). For a microwave cavity attached to a single-mode antenna, the same quantity has a meaning of the complex cavity impedance. Using the random matrix approach, we relate its statistics to that of the reflection coefficient and scattering phase and provide exact distributions for systems with the β=2 and β=4 symmetry class. In the case of β=1, we provide an interpolation formula that incorporates all the known limiting cases and excellently fits the available experimental data as well as diverse numeric tests.     

Quantum interference effects in a multidriven transition Fg=3←→Fe=2

We have theoretically and experimentally studied the quantum coherence effects of a degenerate transition Fg =3←→Fe=2 system interacting with a weak linearly polarized （with σ＋ components） probe light and a strong linearly polarized （with σ＋ components） coupling field. Due to the competition between the drive Rabi frequency and the Zeeman splitting, electromagnetically induced transparency （EIT） and electromagnetically induced absorption （EIA） are present at the different values of applied magnetic field in the case where the Zeeman splitting of excited state Δe is larger than the Zeeman splitting of ground state Δg （i.e.Δe 〉 Δg）.     

On aC*-algebra approach to phase transition in the two-dimensional Ising model. II

We investigate the statesφ _β on theC*-algebra of Pauli spins on a one-dimensional lattice (infinitely extended in both directions) which give rise to the thermodynamic limit of the Gibbs ensemble in the two-dimensional Ising model (with nearest neighbour interaction) at inverse temperature β. We show that if β _c is the known inverse critical temperature, then there exists a family {v _β :β≠β _c } of automorphisms of the Pauli algebra such that $$\phi _\beta = \left\{ {_{\phi _\infty \circ v_\beta ,}^{\phi _0 \circ v_\beta ,} } \right. _{\beta > \beta _c .}^{0 \leqslant \beta< \beta _c } $$ .