AlF<Subscript>3</Subscript> coating of LiNi<Subscript>0.5</Subscript>Mn<Subscript>1.5</Subscript>O<Subscript>4</Subscript> for high-performance Li-ion batteries

AlF₃-coating is attempted to improve the performance of LiNi_0.5Mn_1.5O₄ cathode materials for Li-ion batteries. The prepared powders are characterized by scanning electron microscope, powder X-ray diffraction, charge/discharge, and impedance. The coated LiNi_0.5Mn_1.5O₄ samples show higher discharge capacity, better rate capability, and higher capacity retention than the uncoated samples. Among the coated samples, 1.0 mol% AlF₃-coated sample shows highest capacity after charge–discharged at 30 mA/g for 3 cycles, but 4.0 mol% coated sample exhibits the highest capacity and cycling stability when cycled at high rate of 150 and 300 mA/g. The 40th cycle discharge capacity at 300 mA/g current still remains 114.8 mAh/g for 4.0 mol% AlF₃-coated LiNi_0.5Mn_1.5O₄, while only 84.3 mAh/g for the uncoated sample.     

柴油机轴系扭振系统的强非线性主共振

研究柴油机轴系扭振系统强非线性问题.根据拉格朗日方程建立柴油机轴系扭振系统的动力学模型,通过参数变换,应用Modified Lindstedt-Poincaré方法得到柴油机轴系扭振系统强非线性主共振的幅频响应方程,分析系统不同参数对主共振幅频响应的影响.结果表明,系统的幅频响应曲线存在跳跃,随着简谐力矩的减小和阻尼的增大,系统的非线性跳跃减弱,系统的振幅减小,系统主共振的区域也随之减小;随着调谐参数的变化,系统的主共振力幅响应曲线存在两种拓扑结构.MLP方法得出的近似解析解与龙格库塔法得出的数值解吻合.     

Minimum Hellinger distance estimation for a two-sample semiparametric cure rate model with censored survival data

Efficiency and robustness are two essential concerns on statistical estimation. Unfortunately, it was widely accepted that there existed a contradiction between achieving efficiency and robustness simultaneously. For parametric models with complete data, the minimum Hellinger distance estimation introduced by Beran (Ann Stat 5:445–463, 1977) has been shown that it can reconcile this contradiction. Because data in biostatistics, actuarial science or economics are often subject to censoring and even involve a fraction of long-term survivors, our study aims to extend the minimum Hellinger distance estimation to a two-sample semiparametric cure rate model with right-censored survival data. The asymptotic properties such as consistency, efficiency, normality, and robustness of the proposed estimator have been considered and its performances are examined via simulation studies in comparison with those of the maximum semiparametric conditional likelihood estimator introduced by Shen et al. (J Am Stat Assoc 102:1235–1244, 2007). Finally, our method is illustrated by analyzing a real data set: Bone Marrow Transplant Data.     

Flexible Broad‐Range Pressure Sensors Enabled by Deformation‐Induced Conductive Channels in 3D Graphene Foam@Polydimethylsiloxane Composite for Precise Vibrational Signal Detection

Here we report the design and fabrication of high‐performance pressure sensors based on three‐ dimensional (3D) graphene foam filled polydimethylsiloxane (GF@PDMS) composite with a broad sensing range spaning from 0.05 kPa to 130 kPa. The interpretation of device functioning mechanism can be classified into low and high pressure sensing regions. In the low pressure region (<15 kPa), the pressure loading leads to the temporal connection of micro‐cracks in GF scaffold and forming conductive channels. In the high pressure region (15 kPa to 130 kPa), the pressure induced deformation of GF results in the better connections among micro‐cracks and the shortening of conductive pathway to further decrease the electrical resistance. The GF@PDMS sensors exhibited accuracy, sensibility and reproducibility to detect pressure signals with remarkable stability for over 16000 loading‐unloading cycles, indicating its great potential for practical applications. Moreover, the GF@PDMS sensors also showed high performances in the detection of dynamic pressures, such as subtle mechanical vibration signals, as well as physiology vibrational signals generated by human throats. We expect this technology could be integrated into different sensing systems for the applications in wearable smart electronics and human‐machine communications.     

对超重、失重实验的改进

本文介绍了利用发光显示超重、失重演示器的直观性效果好的特点。     

带粗糙核的Carleson测度

证明了如果b∈BMO(Rn),对于Fefferman C.的一个经典结果(ψ∈S(Rn)∫ψ(x)dx=0,那么│ψt*6(x)│2dxdt/t为R+n+1上的Carleson测度当且仅当b∈BMO(Rn)).确定的Carleson 测度,ψ的光滑性条件是不必要的.作为此结果的应用,还给出了带粗糙核的仿积的L2有界性以及带粗糙核的Littlewood-Paley算子在BLO(Rn)上的有界性,它们分别改进了某些已知结果.     

Hierarchical Nanotubes Constructed by Co9S8/MoS2 Ultrathin Nanosheets Wrapped with Reduced Graphene Oxide for Advanced Lithium Storage

Nanostructured hybrid metal sulfides have attracted intensive attention due to their fascinating properties that are unattainable by the single‐phased counterpart. Herein, we report an efficient approach to construct cobalt sulfide/molybdenum disulfide (Co₉S₈/MoS₂) wrapped with reduced graphene oxide (rGO). The unique structures constructed by ultrathin nanosheets and synergetic effects benefitting from bimetallic sulfides provide improved lithium ions reaction kinetics, and they retain good structural integrity. Interestingly, the conductive rGO can facilitate electron transfer, increase the electronic conductivity and accommodate the strain during cycling. When evaluated as anode materials for lithium‐ion batteries (LIBs), the resultant reduced graphene oxide‐coated cobalt sulfide/molybdenum disulfide (Co₉S₈/MoS₂@rGO) nanotubes deliver high specific capacities of 1140, 948, 897, 852, 820, 798 and 784 mAh g^?1 at the various discharging current densities of 0.2, 0.5, 1, 2, 3, 4 and 5 A g^?1, respectively. In addition, they can maintain an excellent cycle stability with a discharge capacity of 807 mAh g^?1 at 0.2 A g^?1 after 70 cycles, 787 mAh g^?1 at 1 A g^?1 after 180 cycles and 541 mAh g^?1 at 2 A g^?1 after 200 cycles. The proposed method may offer fundamental understanding for the rational design of other hybrid functional composites with high Li‐storage properties.     

Lp-gradient estimates for the commutators of the Kato square roots of second-order elliptic operators on ℝn

Let L=-div(A▽) be a second-order divergent-form elliptic operator,where A is an accretive n×n matrix with bounded and measurable complex coefficients on Herein,we prove that the commutator [b,L1/2]of the Kato square root L1/2 and b with ▽b∈Ln(Rn)(n> 2),is bounded from the homogenous Sobolev space L1p(Rn) to Lp(Rn)(p-(L)     

A new adaptive nonuniformity correction algorithm for infrared line scanner based on neural networks

The striping pattern nonuniformity of the infrared line scanner (IRLS) severely limits the system performance. An adaptive nonuniformity correction (NUC) algorithm for IRLS using neural network is proposed.It uses a one-dimensional median filter to generate ideal output of network and can complete NUC by a single frame with a high correction level. Applications to both simulated and real infrared images show that the algorithm can obtain a satisfactory result with low complexity, no need of scene diversity or global motion between consecutive frames. It has the potential to realize real-time hardware-based applications.