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71.
R6G单分子表面增强共振拉曼散射光谱探测研究 总被引:3,自引:1,他引:2
以共焦显微系统为平台,研究了不同浓度的R6G银溶胶的表面增强共振拉曼散射(SERRS)光谱, 结果表明不同浓度溶液中的R6G分子表现出了不同的光谱特性。在浓度为10-13mol·L-1的R6G银溶胶中 得到了R6G单分子的表面增强共振拉曼散射光谱,观察到了一些光谱非均匀变化现象,如谱色散、谱线的 强度起伏、拉曼谱的偏振化以及分子的闪烁等,并对这些现象进行了分析,证明得到的是R6G单分子的 SERRS光谱。文章还对单分子检测中的一些关键问题进行了分析与讨论,确定了单分子SERRS光谱检测的 适当条件。 相似文献
72.
A compact two-stage optical parametric chirped pulse amplifier based on photonic crystal fibre is demonstrated.A 1064-nm soliton pulse is obtained in a home-made photonic crystal fibre (PCF) with femtosecond pulse pumping and then amplified to 2 mJ in an Nd:YAG regenerative amplifier.After the amplified pulses pass through the LBO crystal,the 532-nm double-frequency light with an energy of 0.8 mJ and a duration of over 100 ps at 10-Hz repetition rate is generated as a pump source in the following two-stage optical parametric amplification (OPA).The 850-nm chirped signal light gain from the stretcher is 1.5×10 4 in the first-stage OPA while it is 120 in the second-stage OPA.The total signal gain of optical parametric chirped pulse amplification (OPCPA) can reach 1.8×10 6. 相似文献
73.
Coulomb expansion of deuterated methane clusters irradiated by an ultrashort intense laser pulse 下载免费PDF全文
The simulations of three-dimensional particle dynamics show that when irradiated by an ultrashort intense laser pulse, the deuterated methane cluster expands and the majority of deuterons overrun the more slowly expanding carbon ions, resulting in the creation of two separated subelusters. The enhanced deuteron kinetic energy and a narrow peak around the energy maximum in the deuteron energy distribution make a considerable contribution to the efficiency of nuclear fusion compared with the ease of homonuelear deuterium clusters. With the intense laser irradiation, the nuclear fusion yield increases with the increase of the cluster size, so that deuterated heteronuelear clusters with larger sizes are required to achieve a greater neutron yield. 相似文献
74.
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76.
Characteristics of ultrafast K line hard x—ray source from femtosecond terawatt laser—produced plasma 下载免费PDF全文
Theoretical studies and analytical scalings were carried out to find the optimized laser parameters and target conditions so that ultrashort hard x-ray pulses and high x-ray power could be achieved.The dependence of laser intensity and wavelength on the yield of K-shell x-ray emission was studied.We propose an optimal design for a foil target for producing high-yield hard x-ray pulses of customizing duration. 相似文献
77.
Study on the interaction of intense femtosecond laser pulses with nanometre-sized hydrogen clusters 下载免费PDF全文
The interaction of intense femtosecond laser pulses with hydrogen clusters
has been experimentally studied. The hydrogen clusters were produced from
expansion of high-pressure hydrogen gas (backed up to 8\tm106Pa) into vacuum
through a conical nozzle cryogenically cooled by liquid nitrogen. The
average size of hydrogen clusters was estimated by Rayleigh scattering
measurement and the maximum proton energy of up to 4.2keV has been obtained
from the Coulomb explosion of hydrogen clusters under 2×1016 W/cm2 laser irradiation. Dependence of the maximum proton energy on cluster size and laser intensity was
investigated, indicating the correlation between the laser intensity and the
cluster size. The maximum proton energy is found to be directly proportional
to the laser intensity, which is consistent with the theoretical prediction. 相似文献
78.
Surface-enhanced resonance Raman scattering (SERRS) of
Rhodamine 6G (R6G) adsorbed on colloidal silver clusters has been studied.
Based on the great enhancement of the Raman signal and the quench of the
fluorescence, the SERRS spectra of R6G were recorded for the samples of dye
colloidal solution with different concentrations. Spectral inhomogeneity
behaviours from single molecules in the dried sample films were observed with
complementary evidences, such as spectral polarization, spectral diffusion,
intensity fluctuation of vibrational lines and even ``breathing' of the
molecules. Sequential spectra observed from a liquid sample with an average of
0.3 dye molecules in the probed volume exhibited the expected Poisson
distribution for actually measuring 0, 1 or 2 molecules. Difference between
the SERRS spectra of R6G excited by linearly and circularly polarized light
were experimentally measured. 相似文献
79.
Accurate determination of the absolute phase and temporal-pulse phase of few-cycle laser pulses 下载免费PDF全文
A Fourier analysis method is used to accurately determine not
only the absolute phase but also the temporal-pulse phase of an
isolated few-cycle (chirped) laser pulse. This method is
independent of the pulse shape and can fully characterize the
light wave even though only a few samples per optical cycle are
available. It paves the way for investigating the absolute
phase-dependent extreme nonlinear optics, and the evolutions of
the absolute phase and the temporal-pulse phase of few-cycle
laser pulses. 相似文献
80.