Possible α decay chains from isotopes of superheavy element 120

We investigate the α decay half-lives of even-Z superheavy nuclei up to Z = 120 by the modified two-potential approach. Based on the density-dependent cluster model, the α daughter potential is obtained from the double folding integral, taking into account the effect of nuclear deformation. A reasonable formula related with the fissility parameter and the fission barrier height, is applied to evaluate the spontaneous fission half-lives of the studied nuclei. After the performance of the competition between α decay and spontaneous fission, possible α decay chains are proposed in pursuit of being useful for the future experiment.     

Research on some superheavy nuclei

Studies on some superheavy nuclei are performed. The α decay energies are calculated by an improved local binding energy formula, and the α decay half-lives are calculated by the Viola-Seaborg formula. Good agreements between theoretical and experimental results are reached.     

超重核294118和291116及其α衰变链上各核素半衰期的研究

运用推广的液滴模型（GLDM）确定了超重核294118和291116及其α衰变链上各核素的衰变势垒, 采用量子力学中的WKB方法计算α衰变中的势垒穿透几率, 对该链上各原子核的α衰变半衰期进行了研究。 此外, 还利用Royer公式对该链上各原子核的α衰变半衰期进行了计算。 结果表明, GLDM 考虑亲和能与Royer公式给出的α衰变半衰期与超重核区的实验值符合很好, 验证了GLDM和Royer公式在超重核区的适用性,可以用来预测超重核的半衰期。 最后, 预言了Z=118 和116 同位素链上各核素的半衰期, 结果表明, 在Z=118和116中存在α衰变长寿命同位素, 这需要实验上的检验。The α decay potential barrier of the newly synthesized superheavy nuclei starting from 294118 and 291116 have been determined and their half lives have been studied with the Generalized Liquid Drop Model(GLDM) connected with WKB approximation and Royer’s formulae．The α decay half lives of the nuclei belonging to the superheavy nuclei starting from 294118 and 291116 have been calculated．The calculated results are in agreement with the experimental data, which show that the α decay half lives of superheavy nuclei with the GLDM and Royer’s formulae can be applied in the studying on superheavy nuclei successfully．Finally, the half lives of Z=118 and 116 isotopes have been predicted, and the results suggest there may be some long lived superheavy nuclei for α decay in those isotopes.     

可能合成的超重核的alpha衰变能和半衰期

本文考察和研究了将来可能在实验上合成的超重新元素和新核素的基态性质。研究的重点主要放在原子核的alpha衰变能和半衰期。详细比较和讨论了不同理论模型计算的alpha衰变能和半衰期。通过这些计算和比较,从理论上提出了将来在实验上比较容易合成的超重新元素和新核素的性质。理论计算结果可为将来的超重核实验提供理论参考。     

Alpha decay energies and half-lives for possibly synthesized superheavy elements

We investigate the ground state properties of some superheavy nuclei, which may be synthesized in future experiments. Special emphases are placed on the alpha decay energies and half-lives. The alpha decay energies and half-lives from different theoretical models are compared and discussed comprehensively. Through these calculations and comparisons, the optimal superheavy elements to be synthesized in future experiments are proposed theoretically.     

Half-Lives for Alpha Radioactivity of Elements with 104 ≤ Z ≤ 120 within Unified Fission Model

α decay half-lives are calculated using the Qα values obtained by Semi-empirical Shell Model in the framework of the Unified Fission Model (UFM) with the Coulomb repulsion, nuclear attraction due to proximity potential, and rotational energy due to angular momentum transfer of α particle. In addition, the calculated and experimental half-lives of 425 nuclei are compared to check the validity of the model applied on α decay. The calculated half-lives of α decay are in good agreement with the experimental data. Finally, some usefulpredications on the α decay half-lives are provided for future experiments.     

Heavy-particle radioactivity of superheavy nuclei

The concept of heavy-particle radioactivity (HPR) is changed to allow emitted particles with Z(e) > 28 from parents with Z > 110 and daughter around (208)Pb. Calculations for superheavy (SH) nuclei with Z = 104-124 are showing a trend toward shorter half-lives and larger branching ratio relative to α decay for heavier SHs. It is possible to find regions in which HPR is stronger than alpha decay. The new mass table AME11 and the theoretical KTUY05 and FRDM95 masses are used to determine the released energy. For 124 we found isotopes with half-lives in the range of ns to ps.     

Alpha decay half-lives of heavy nuclei within a generalized liquid drop model

Theoretical α-decay half-lives of the heaviest nuclei are calculated using the experimental Qα value. The barriers in the quasi-molecular shape path is determined within a Generalized Liquid Drop Model (GLDM) and the WKB approximation is used. The results are compared with calculations using the DensityDependent M3Y (DDM3Y) effective interaction and the Viola-Seaborg-Sobiczewski (VSS) formulae. The calculations provide consistent estimates for the half-lives of the α decay chains of these superheavy elements. The experimental data stand between the GLDM calculations and VSS ones in the most time.     

α decay energies and half-lives from a macroscopic-microscopic model

α decay energies of 323 heavy nuclei with Z≥82 are evaluated with a macroscopic-microscopic model.In this model,the macroscopic part is treated by the continuous medium model and the microscopic part consists of shell and pairing corrections based on the Nilsson potential.α decay half-lives are calculated by Viola-Seaborg formula.The results of α decay energies and half-lives are compared with experimental values and satisfactory agreement is found.The recoiling effect of the daughter nucleus on α decay half-life is also discussed.     

Systematic studies on α-decay half-lives for super heavy nuclei

Radioactive decay of super heavy nuclei via the emission of α-particles has been studied theoretically in the preformed cluster model (PCM). The nucleus-nucleus (NN) potential is obtained by double folding the density distributions of the α-particle and the daughter nucleus with a realistic effective interaction. The M3Y effective interaction, supplemented by a zero-range pseudo-potential for exchange term, is used to calculate the NN potential. The α decay half-lives for 317 nuclei at Z=102–120 are performed in the PCM framework with the theoretical Q values extracted from the Mller-Nix-Kratz and Liran-Marinov-Zeldes mass tables and are compared with the experimental data. The calculated results are also compared with those obtained by using Q values from the Muntian-Hofmann-Patyk-Sobiczewski and Myers-Swiatecki mass estimates.     

Proton radioactivity with a Yukawa effective interaction

The half-lives of proton radioactivity of proton emitters are investigated theoretically. Proton-nucleus interaction potentials are obtained by folding the densities of the daughter nuclei with a finite-range effective nucleon-nucleon interaction having Yukawa form. The Wood-Saxon density distributions for the nuclei used in calculating the nuclear as well as the Coulomb interaction potentials are predictions of the interaction. The quantum mechanical tunneling probability is calculated within the WKB framework. These calculations provide reasonable estimates for the observed proton radioactivity lifetimes. The effects of neutron-proton effective mass splitting in neutron-rich asymmetric matter as well as the nuclear matter incompressibility on the decay probability are investigated.     

Effect of properties of superheavy nuclei on their production and decay

Properties and stability of superheavy nuclei resulting from hot fusion are discussed. It is shown that the microscopic–macroscopic approach allows obtaining the closed proton shell at Z ≥ 120. Isotopic trends of K-isomeric states in superheavy nuclei are predicted. Evaporation residue cross sections in hot fusion reactions are calculated using the predicted properties of superheavy nuclei. Interruption of α decay chains by spontaneous fission is analyzed. Alpha decay chains through isomeric states are considered. Internal level densities in superheavy nuclei are microscopically calculated.     

New approach for alpha decay half-lives of superheavy nuclei and applicability of WKB approximation

The α decay half-lives of recently synthesized superheavy nuclei (SHN) are calculated by applying a new approach which estimates them with the help of their neighbors based on some simple formulas. The estimated half-life values are in very good agreement with the experimental ones, indicating the reliability of the experimental observations and measurements to a large extent as well as the predictive power of our approach. The second part of this work is to test the applicability of the Wentzel-Kramers-Brillouin (WKB) approximation for the quantum mechanical tunneling probability. We calculated the accurate barrier penetrability for alpha decay along with proton and cluster radioactivity by numerically solving Schrödinger equation. The calculated results are compared with those of the WKB method to find that WKB approximation works well for the three physically analogical decay modes.     

α Decay Properties of Even-Even Nuclei~(296-308)120 Within the Two-Potential Approach

In the present work,we predict the α decay half-lives of unknown even-even nuclei ~(296-308)120 within the two-potential approach,whose α decay energy Qa is calculated using WS3+mass model.To reduce the deviations between the predictions and experimental data due to nuclear shell effect,the analytic formula of α decay hindrance factor is introduced to the two-potential approach,whose parameters had been extracted from even-even nuclei in the region of 82 Z 126 and 152 N 184 in our previous work [Deng et al.,Chin.Phys.C 42(2018) 044102].In addition,for comparing,we use a type of α decay general formula Universal Decay Law(UDL) and a semi-empirical formula in the superheavy nucleus(SEMFLS) to calculate the half-lives of even-even nuclei ~(296-308)120.The results indicate that our predicted values and the calculated values of the above two empirical formulas are mutually confirmed.Meanwhile,we systematically study α decay chains of ~(296-308)120 and predict the decay modes for superheavy nuclei to help to identify new superheavy isotopes.     

Low-energy neutron-deuteron reactions with N 3 LO chiral forces

Based on the preformed cluster model (PCM), we have extended our earlier study on cluster decays of heavy parent nuclei to analyze the effects of different nuclear proximity potentials in the ground-state clusterization of superheavy nuclei with Z = 113, 115 and 117. In order to look for the possible role of deformations, calculations are performed for spherical as well as β ₂-deformed choices of fragmentation. The relevance of “hot compact” over “cold elongated” configurations due to orientations is also explored, in addition to the role of Q value and angular momentum ℓ effects. As the PCM is based on collective clusterization picture, the preformation and penetration probabilities get modified considerably, and hence do so the decay constants and half-lives of the clusters, with the use of different nuclear proximity potentials. The comparative importance of nuclear proximity potentials Prox-1977 and Prox-2000 is analyzed and the calculated decay half-lives in the framework of PCM are compared with the recent predictions of the analytical super-asymmetric fission model (ASAFM). The possible role of shell corrections is also investigated for understanding the dynamics of heavy particle radioactivity. Finally, the potential energy surfaces are compared for different proton and neutron magic numbers in superheavy mass region.

     

Search for decay modes of heavy and superheavy nuclei

Spontaneous fission(SF) with a new formula based on a liquid drop model is proposed and used in the calculation of the SF half-lives of heavy and superheavy nuclei(Z = 90–120). The predicted half-lives are in agreement with the experimental SF half-lives. The half-lives of decay(AD) for the same nuclei are obtained by using the Wentzel-Kramers-Brillouin(WKB) method together with Bohr-Sommerfeld(BS) quantization condition considering the isospin-dependent effects for the cosh potential. The decay modes and branching ratios of superheavy nuclei(Z =104-118) with experimental decay modes are obtained, and the modes are compared with the experimental ones and with the predictions found in the literature. Although some nuclei have predicted decay modes that are different from their experimental decay modes, decay modes same as the experimental ones are predicted for many nuclei. The SF and AD half-lives, branching ratios, and decay modes are obtained for superheavy nuclei(Z = 119–120) with unknown decay modes and compared with the predictions obtained in a previous study. The present results provide useful information for future experimental studies performed on both the AD and SF of superheavy nuclei.     

超重核α衰变寿命的理论研究

建立了计算球形核α衰变寿命的新模型——密度依赖的结团模型(DDCM)。在此基础上,通过引入子核的形变自由度,发展了形变的密度依赖的结团模型, 编写了形变的DDCM程序。并系统计算了Z=106—110的超重核α衰变寿命。通过与已有的实验数据的对比分析, 发现理论结果和实验数据符合得很好,验证了DDCM在超重核区域的适用性。We proposed a deformed version of density dependent cluster model (DDCM) by including nuclear deformation of the daughter nucleus. A systematic calculation of α decay half lives of superheavy nuclei (Z=106—110) is carried out by the deformed DDCM. The good agreement between theory and data is obtained. It is shown that the deformed DDCM works well in the superheavy mass region.     

Systematic study of α decay half-lives for even–even nuclei within a deformed two-potential approach

In this work, we systematically study the α decay half-lives of 196 even–even nuclei using a two-potential approach improved by considering nuclear deformation. The results show that the accuracy of this model has been improved after considering nuclear deformation. In addition, we extend this model to predict the α decay half-lives of Z = 118 and 120 isotopes by inputting the α decay energies extracted from the Weizsacker–Skyrme-type (WS-type) mass model, a simple nuclear mass formula, relativistic continuum Hartree–Bogoliubov theory and Duflo-Zuker-19 (DZ19) mass model. It is useful for identifying the new superheavy elements or isotopes for future experiments. Finally, the predicted α decay energies and half-lives of Z = 118 and 120 isotopes are analyzed, and the shell structure of superheavy nuclei is discussed. It shows that the shell effect is obvious at N = 184, while the shell effect at N = 178 depends on the nuclear mass model.     

超重核的生成和衰变

简单介绍了近年来在超重核研究方面所取得的成就和理论方面所面临的挑战.着重介绍推广的液滴模型和准分子形状机制,它们的优点是考虑了精确的核半经、质量和电荷的不对称性、形变、亲和力和温度等.推广的液滴模型和准分子形状机制能很好地描述重核和超重核的裂变、衰变及完全熔合反应.The progress and challenge on studies of superheavy elements both experiments and theories has been briefly introduced. It is emphasis to introduce a generalized liquid drop model, including the proximity effects, the asymmetry, an accurate nuclear radius, and quasi molecular shapes. The α decay half lives of 373 nuclei and superheavy elements have been calculated in the generalized liquid drop model and compared with the available experimental data. The deformed energies have also been obtained ...     

The relative stability of superheavy elements

The relative stability of superheavy elements against beta-decay and spontaneous fission has been investigated. A simple criterion of beta-stability using the Fermi gas model has been developed, tested in the range of stable nuclei and extended to the superheavy region. Spontaneous fission half-lives have been calculated using the statistical model in the expected region of relative beta-stability for superheavy nuclei. Our results have been compared with previous calculations.