The effect of the laser pulse shape on the wakefield generation in field-ionized plasma

In this paper, the effect of the laser pulse shape on the generation and evolution of the wakefield during the interaction of the intense laser pulse with the gas have been studied utilizing the parallel relativistic PIC simulation code. In order to reach this aim, three pulses with length 300 fs and different rise-times 30, 45, and 60 are typically selected. Our results show that, the amplitude of the laser wakefield produced in the gas in comparison with the plasma strongly depends on the laser pulse shape. The simulation results indicate that for the high-slope laser pulse time (here 30 fs), ionization and thus density fluctuations have no significant effect on the wakefield generation because of rapid increase of the laser electric field. While by increasing the laser pulse rise-time to 45 fs, the rapid wave breaking due to the change in the medium refractive index during the gas ionization, prevents from the wakefield amplitude growth, so that the wakefield with larger amplitude is emerged in the plasma. For a slow-sloping pulse (here 60 fs), the ratio of the wakefield generation in the gas to the plasma is altered for the different gas densities and laser intensities. Moreover, it is represented that the longer the laser pulse rise-time, the sooner difference between the wakefield produced in the gas and plasma is observed. In fact, the larger the rise-time, the greater the density fluctuations and, consequently, the larger the initial noise is generated to seed the Raman instability.     

利用等离子体非线性系数实现超强脉冲的压缩

超短脉冲压缩技术在强场物理研究中有非常重要的作用,但由于强场电离现象在惰性气体自相位调制脉冲压缩技术中限制了脉冲的能量。Tempea等人提出可以采用等离子体非线性系数对脉冲进行压缩,本文在考虑毛细管内表面电离的情况下,讨论能量为10mJ左右,脉宽为50fs的脉冲的压缩问题,发现可以将脉冲压缩至5fs左右。计算表明频谱展宽可以在气体密度很低的情况下进行,这样半可以减小电子对脉冲传输的影响。同时,由于毛细管内表面也处于电及状态,从而使脉冲能量不会受到电离阈值的.限制。     

激光与固体靶相互作用中低密度预等离子体对高能电子产生的影响

 对线极化、圆极化的超短超强激光脉冲与靶前有一段低密度预等离子体的固体靶的相互作用进行了理论和粒子模拟研究。激光通过有质动力加速机制加速预等离子体中的电子，研究了电子获得的最大能量随激光强度和预等离子体密度的变化。当激光脉冲与靶直接作用时，靶中的电子由于J×B机制而得到加速，所获得的能量比预等离子体中电子低。研究表明，在超短超强激光脉冲与固体靶相互作用中，预等离子体的存在有利于高能电子的产生。     

Enhanced betatron radiation by a modulating laser pulse in laser wakefield acceleration

We propose a new idea to enhance and control the betatron radiation by using a modulating laser pulse in laser wakefield acceleration. In this scheme, a high-power laser pulse is used for self-trapping and acceleration of the plasma electrons and the accelerated electron beam is modulated by a separately-propagating laser pulse for large amplitude betatron oscillations and microbunching. In this way, the relatively low power modulating laser pulse can enhance the X-ray photon flux and energy significantly. We performed two-dimensional particle-in-cell simulations to demonstrate the idea and the results show that a sub-TW laser pulse is enough for electron beam modulation and it can generate easily-controllable fs X-ray pulses with a wide range of photon energies from soft X-rays to hard X-rays.     

Effects of inverse bremsstrahlung in laser-induced plasmas from a graphite surface

The kinetic energy of electrons emitted due to laser interaction with a graphite surface was studied with a time-of-flight spectrometer. In addition the yields of carbon atomic and molecular ions were measured as a function of laser pulse energy. Pulse energy thresholds for ion emission are observed to correlate with the observed maximum electron energies. Furthermore, the data suggest that ionic carbon clusters can be dissociated by energetic electrons or photons created in the plasma. We believe that initially photoemitted electrons are accelerated by inverse bremsstrahlung to the energies required for electron impact ionization and dissociation     

Few cycle dynamics of multiphoton double ionization

In intense field ionization, an electron removed from the atomic core oscillates in the combined fields of the laser and the parent ion. This oscillation forces repeated revivals of its spatial correlation with the bound electrons. The total probability of double ionization depends on the number of returns and therefore on the number of optical periods in the laser pulse. We observed the yield of Ne(2+) relative to Ne(+) with 12 fs pulses to be clearly less compared to 50 fs pulses in qualitative agreement with our theoretical model.     

Generation of high-density electrons based on plasma grating induced Bragg diffraction in air

Efficient nonlinear Bragg diffraction was observed as an intense infrared femtosecond pulse was focused on a plasma grating induced by interference between two ultraviolet femtosecond laser pulses in air. The preformed electrons inside the plasma grating were accelerated by subsequent intense infrared laser pulses, inducing further collisional ionization and significantly enhancing the local electron density.     

Excitation of low-lying nuclear states by the ion line emission in femtosecond laser plasma

A scheme of nuclear excitation by the ionic X-ray lines in laser plasma using two femtosecond laser pulses is proposed. The first pulse produces plasma with a given degree of ionization, allowing the X-ray line energies of the target ions to be tuned to resonance with the nuclear transition, while the second pulse generates hot electrons that are necessary for X-ray generation.     

500 fs超短脉冲激光对CCD探测器的破坏效应

 采用脉宽500 fs，脉冲能量250 μJ的超短脉冲激光辐照线阵CCD探测器，观察到了CCD从线性响应到像元饱和、饱和串音直至硬损伤的整个过程，并着重对两种辐照能量密度下的硬损伤机理进行了理论分析。结果表明：激光能量密度为0.45 μJ/cm²时，达到像元饱和；能量密度为0.14 J/cm²时，辐照6个脉冲后实现了CCD器件的硬损伤，硬损伤源于晶格被加热并汽化形成等离子体；能量密度为1.41 J/cm²时，单个脉冲就使CCD器件的输出波形无法辨认，2个脉冲后CCD器件没有任何信号输出，硬破坏源于电荷分离形成的电场库仑力。     

150fs～10ps脉宽下熔石英激光损伤的仿真与分析

基于约化电子数密度增长速率方程,建立了熔石英导带电子数密度随脉冲持续时间变化的模型。利用电子数临界密度这一概念,得到了150fs~10ps脉宽下,熔石英激光损伤阈值范围。分析表明,5~10ps,雪崩电离仍然起主要作用,而光致电离提供的初始电子使雪崩电离不再依赖材料原有的初始电子;当脉宽减小到约为4ps时,光致电离与雪崩电离作用相等;之后,光致电离起主要作用。通过仿真出的损伤阈值拟合,得到了该脉宽区间下新的脉宽定律:熔石英的损伤阈值正比于脉宽的0.38次方;考虑温度对熔石英损伤阈值的影响,熔石英的损伤阈值正比于脉宽的0.34次方。     

Combination of high-intensity femtosecond laser pulses for generation of time-dependent polarization pulses and ionization of atomic gas

Time-dependent polarization pulses are generated by combining two perpendicularly polarized, high-intensity laser pulses. The time evolution of the polarization state of the combined laser pulse is measured by the POLLIWOG technique. We observed changes in the polarization state while varying the relative delay. In order to investigate the effect of pulse combination on the ionization of atoms, the electron signals and the ion signals are measured by irradiating combinations of two perpendicularly polarized pulses or two parallel polarized pulses. With the two parallel polarized pulses, high-order fringe-resolved autocorrelations are obtained by measuring the time-integrated ion signals as a function of the time delay. When two perpendicularly polarized pulses are combined, the fringe period of the time-integrated electron signal as a function of the time delay is different from that of the time-integrated ion signal. This is due to the fact that the electron signal depends on the direction of the field vibration and the number of generated electrons. We also measured the electron energy distributions at different relative delays and confirmed that these depend on the polarization state of generated pulses.     

Pulse shape and molecular orientation determine the attosecond charge migration in Caffeine

The recent reduction of laser pulse duration down to the attosecond regime offers unprecedented opportunities to investigate ultrafast changes in the electron density before nuclear motion sets in. Here, we investigate the hole dynamics in the Caffeine molecule that is induced by an ionizing XUV pulse of 6 fs duration using the approximate time-dependent density functional theory method TD-DFTB. In order to account for ionization in a localized atomic orbital basis we apply a complex absorbing potential to model the continuum. Propagation of the time-dependent Kohn–Sham equations allows us to extract the time-dependent hole density taking the pulse shape explicitly into account. Results show that the sudden ionization picture, which is often used to motivate an uncorrelated initial state, fails for realistic pulses. We further find a strong dependence of the hole dynamics on the polarization of the laser field. Notwithstanding, we observe fs charge migration between two distant functional groups in Caffeine even after averaging over the molecular orientation.     

紧聚焦飞秒脉冲与石英玻璃相互作用过程中的电子动量弛豫时间研究

本文通过数值模拟(3+1)维扩展的广义非线性薛定谔方程,研究了紧聚焦飞秒激光脉冲在诱导石英玻璃的非线性电离过程中电子动量弛豫时间对于该电离过程的影响.计算结果证明电子动量弛豫时间会直接影响入射脉冲在焦点区域所形成的峰值场强、自由电子态密度和能流等参量的分布态势,因此在与实验结果相比较后发现适合于相互作用过程的电子动量弛豫时间的理论值约为1.27 fs.进一步的研究表明,电子动量弛豫时间与逆韧致吸收效应、雪崩电离的概率、等离子体密度、等离子体的自散焦效果以及间接引起的焦平面位置的移动都有着密切的联系.当前的研究结果表明电子动量弛豫时间在飞秒激光脉冲与物质相互作用的过程中发挥着重要作用.     

Experimental investigation of ablation efficiency and plasma expansion during femtosecond and nanosecond laser ablation of silicon

Femtosecond laser (Ti:sapphire, 100 fs pulse duration) ablation of silicon in air was compared with nanosecond laser (Nd:YAG, 3 ns pulse duration) ablation at ultraviolet wavelength (266 nm). Laser ablation efficiency was studied by measuring crater depth as a function of pulse number. For the same number of laser pulses, the fs-ablated crater was about two times deeper than the ns-crater. The temperature and electron number density of the laser-induced plasma were determined from spectroscopic measurements. The electron number density and temperature of fs-induced plasmas decreased faster than ns-induced plasmas due to different energy deposition mechanisms. Images of the laser-induced plasma were obtained with femtosecond time-resolved laser shadowgraph imaging. Plasma expansion in both the perpendicular and the lateral directions were compared. PACS 52.38.Mf; 52.30.-q     

Plasma channel formed by ultraviolet laser pulses at 193 nm in air

The propagation of picosecond deep ultraviolet laser pulse at wavelength of 193 nm in air is numerically investigated. Long plasma channel can be formed due to the competition between Kerr self-focusing and ionization induced defocusing. The plasma channel with electron density of above 10^13/cm^3 can be formed over 70 m by 50-ps, 20-mJ laser pulses. The fluctuation of laser intensity and electron density inside ultraviolet （UV） plasma channel is significantly lower UV laser by air is considered in the simulation and it the limit of the length of plasma channel. than that of infrared pulse. The linear absorption of is shown that the linear absorption is important for the limit of the length of plasma channel.     

Near-GeV-energy laser-wakefield acceleration of self-injected electrons in a centimeter-scale plasma channel

The first three-dimensional, particle-in-cell (PIC) simulations of laser-wakefield acceleration of self-injected electrons in a 0.84 cm long plasma channel are reported. The frequency evolution of the initially 50 fs (FWHM) long laser pulse by photon interaction with the wake followed by plasma dispersion enhances the wake which eventually leads to self-injection of electrons from the channel wall. This first bunch of electrons remains spatially highly localized. Its phase space rotation due to slippage with respect to the wake leads to a monoenergetic bunch of electrons with a central energy of 0.26 GeV after 0.55 cm propagation. At later times, spatial bunching of the laser enhances the acceleration of a second bunch of electrons to energies up to 0.84 GeV before the laser pulse intensity is significantly reduced.     

Stable laser-pulse propagation in plasma channels for GeV electron acceleration

To achieve multi-GeV electron energies in the laser wakefield accelerator (LWFA) it is necessary to propagate an intense laser pulse long distances in plasma without disruption. A 3D envelope equation for a laser pulse in a tapered plasma channel is derived, which includes wakefields and relativistic and nonparaxial effects, such as finite pulse length and group velocity dispersion. It is shown that electron energies of approximately GeV in a plasma-channel LWFA can be achieved by using short pulses where the forward Raman and modulation nonlinearities tend to cancel. Further energy gain can be achieved by tapering the plasma density to reduce electron dephasing.     

Particle simulation on electron acceleration process by the laser ponderomotive force in inhomogeneous underdense plasma layers

The mechanism of electron ponderomotive acceleration due to increasing group velocity of laser pulse in inhomogeneous underdense plasma layers is studied by two-dimensional relativistic parallel particle-in-cell code. The electrons within the laser pulse move with it and can be strongly accelerated ponderomotively when the duration of laser pulse is much shorter than the duration of optimum condition for acceleration in the wake. The extra energy gain can be attributed to the change of laser group velocity. More high energy electrons are generated in the plasma layer with descending density profile than that with ascending density profile. The process and character of electron acceleration in three kinds of underdense plasma layers are presented and compared.     

Laser-energy transfer and enhancement of plasma waves and electron beams by interfering high-intensity laser pulses

The effects of interference due to crossed laser beams were studied experimentally in the high-intensity regime. Two ultrashort (400 fs), high-intensity (4 x 10(17) and 1.6 x 10(18) W/cm(2)) and 1 microm wavelength laser pulses were crossed in a plasma of density 4 x 10(19) cm(3). Energy was observed to be transferred from the higher-power to the lower-power pulse, increasing the amplitude of the plasma wave propagating in the direction of the latter. This results in increased electron self-trapping and plasma-wave acceleration gradient, which led to an increased number of hot electrons (by 300%) and hot-electron temperature (by 70%) and a decreased electron-beam divergence angle (by 45%), as compared with single-pulse illumination. Simulations reveal that increased stochastic heating of electrons may have also contributed to the electron-beam enhancement.     

Spectral and temporal analysis of ultrashort ultraviolet pulses generated by high-intensity laser radiation in the atmosphere

We report direct spectral and temporal characterization of ultrashort ultraviolet (UV) pulses resulting from third-harmonic generation by high-intensity Ti: sapphire laser radiation in the atmosphere. The experimental technique implemented in this work enables the measurement of the pulse width and the chirp of the UV field, as well as the electron density of the plasma produced by laser pulses. The bandwidth of the third harmonic generated in our experiments by laser pulses with an initial pulse width of 45 fs supports transform-limited UV pulses as short as 30 fs.