二维X射线衍射及其应用研究进展

介绍了三维、一维和二维X射线衍射的有关概念,给出二维X射线衍射的定义:在X射线衍射实验中使用二维探测器,并对由二维探测器记录的二维象、二维衍射花样的数据进行处理分析和解释的X射线衍射方法称为二维X射线衍射术。之后,分四部分综述二维X射线衍射(2D-XRD)和散射及其应用的进展。1)单晶样品的二维衍射包括经典的劳厄法定向和用二维探测器(带衰减底片组件、CCD和IP等)的劳厄法测定晶体结构的单晶样品现代二维衍射术;2)随后,评述多晶样品二维衍射的衍射几何、实验装置,以及在物相鉴定、应力测定和织构测定方面应用的方法和基本公式;3)二维小角散射(2D-SAXS)也作了简介。4)把一维和二维衍射术作了较全面的比较和综合评论。     

二维X射线衍射及其应用研究进展

介绍了三维、一维和二维X射线衍射的有关概念,给出二维X射线衍射的定义:在X射线衍射实验中使用二维探测器,并对由二维探测器记录的二维象、二维衍射花样的数据进行处理分析和解释的X射线衍射方法称为二维X射线衍射术。之后,分四部分综述二维X射线衍射(2D-XRD)和散射及其应用的进展。1)单晶样品的二维衍射包括经典的劳厄法定向和用二维探测器(带衰减底片组件、CCD和IP等)的劳厄法测定晶体结构的单晶样品现代二维衍射术;2)随后,评述多晶样品二维衍射的衍射几何、实验装置,以及在物相鉴定、应力测定和织构测定方面应用的方法和基本公式;3)二维小角散射(2D-SAXS)也作了简介。4)把一维和二维衍射术作了较全面的比较和综合评论。     

多丝正比室阴极感应电荷重心读出定位性能的研究

制作了一个带有阴极条的有效面积为100×100mm²的多丝正比室模型,测量了⁵⁵Fe的X射线(5.9keV)在阴极面上产生的感应电荷分布和多丝室沿阳极丝方向的位置分辨,研究了阴极条取样数对位置分辨的影响,最后和理论计算的结果进行了比较.     

多丝正比室W–S阴极条两维读出方法研究

对一种简便的多丝室楔形一条形(W–S)阴极的感应电荷分布进行了详细的计算,制作了100×100mm²的丝室模型,用55FeX射线测量丝室的定位精度,并获得入射X射线的二维图像.     

气体探测器的最新应用

本文讨论了气体探测器在下述领域的最新应用:放射性痕量元素的二维图像;用X 射线衍射研究晶体结构;工业射线照相法;用核扩散的射线照相;契伦柯夫环探测器;流光管量热计;渡越辐射测量;用作电磁量热计的高密度显像室;用作探测契伦柯夫环的显像室。     

倾斜多丝正比室辐射状阴极条感应电荷重心读出的定位性能研究

本文针对倾斜多丝室辐射状阴极条的具体结构,研究了阴极面上感应电荷密度分布,给出了四或五根条取样时重心读出定位修正函数和相应的定位精度,用⁵⁵Fe X射线进行了定位测量,实验和理论符合得较好.     

NaCl单晶非切割晶面X射线衍射的实验研究

现有的德国莱宝教具公司生产的X射线实验仪采用多道脉冲幅度分析器测量衍射能谱,默认的COUPLED模式仅能得到NaCl单晶的(100)切割晶面的衍射能谱.通过旋转靶台,重新设置测角零点,再利用COUPLED模式测量,即可得到其他非切割晶面的衍射能谱.由于此X射线实验仪无角度自动校正功能,故通过二维扫描的方式对靶台和探测器转角进行修正,可以减少误差.     

基于读出条读出的二维位置灵敏气体电子倍增器的研制

为研发能够满足北京同步辐射(BSRF)实验要求的二维探测器,研制了基于读出条读出的二维位置灵敏X射线气体电子倍增器(GEM).实验过程中通过改进读出条的周期,并基于中科院高能所实验物理中心电子学组研制的多路电荷放大器系统与VME存储-ADC系统,对软X射线源的位置分辨率进行了精密测量且得到了优异的二维位置分辨:X方向约为84μm,Y方向约为75μm.研究了三级GEM压差之和对位置分辨的影响,并测试了探测器的位置准确度与线性.对基于阳极读出的GEM用于模拟读出测试系统得到了一定的理论认识,侧重研究了GEM探测器基于模拟读出的系统特性,给出了相关的分析与讨论.     

基于飞秒激光的一维速度场测量方法

飞秒激光诱导氰基化学发光利用飞秒光丝标记流场中的气体分子,通过观测被标记分子在固定时间内的位移可获得流场的速度信息。一维的光丝在实验结果中包含了一维的速度场信息,但由于无法将光丝移动前后的位置信息精确关联,因此只能给出中心一点的速度。针对此问题,我们提出了一种一维速度场反演算法,可根据移动后光丝的位置及其线型反演出整条光丝位置处的速度,得到光丝上1D-2C的速度场信息。利用多条发光线的移动轨迹,还可获得二维速度场信息。     

二维位置灵敏探测器输出图像畸变的修正

高分辨(e,2e)谱仪采用二维位置灵敏探测器同时对能量和角度进行多道测量.二维位置灵敏探测器由级联使用的微通道板和电阻阳极板组成,由于电阻阳极板的边缘效应和制造工艺的缺陷,测量得到的位置图像与实际图像总会有一定的形变,存在一定的非线性.本文针对高分辨(e,2e)谱仪二维位置灵敏探测器输出图像的“桶形”畸变及位置非线性,采用一种简易的冷刻法(用脉冲信号来模拟真实电子束团),检验了二维位置灵敏探测器的Gear型电阻阳极板的线性好坏,并用分割成小三角形的方法找出测量得到的畸变图像与原始真实图像的映射关系,再用此关系对其它测量得到的畸变图像进行修正,并对修正的结果进行了评估.通过修正,由“桶形”畸变所造成的图像扭曲得到明显改善.修正后的x方向非线性由修正前的2.1%变为0.59%.这种检验和修正方法对其它领域类似探测器输出图像的修正也有一定的指导意义.     

Design and experimental study of a two-dimensional position sensitive X-ray detector

A prototype of a two-dimensional position sensitive X-ray detector was designed and constructed for small angle X-ray scattering experiments at BSFR (Beijing Synchrotron Radiation Facility). The detector is based on MWPC with cathode strip readout, and has a sensitive area of 200 mmx200 mm. The spatial resolution (FWHM) of about 210 μm along the anode wire direction was obtained from the 55Fe X-ray test of the detector.     

CCD detector for high time resolution experiments with SR beams

A detector for fast diagnostics of particle beams in storage rings using an optical component of synchrotron radiation (SR) is developed. The detector records a limited series of one-dimensional or small two-dimensional images at a rate of (1?10) × 10⁶ frames/s. It can also be used for investigating fast processes in X-ray SR beams. In particular, matched with a structured scintillation screen (with low deexcitation time), this detector provides a recording with an SR flash rate of shadowgraph images (for axially symmetric objects, initial data for tomograms) or a record of the distribution of small-angle X-ray scattering. It is also possible to apply this detector as a dispersion-free image spectrometer; this would make it possible to perform pulsed X-ray diffraction studies with ??white?? SR beams. In the single-flash mode this would provide a record of the formation and behavior of crystalline phases in shock and detonation waves with a time resolution of up to 1 ns.     

Design and performance of a 2-D multi-wire position sensitive X-ray detector

A 2-D multi-wire position sensitive detector for X-ray diffraction and small angle X-ray scattering studies is described. The detector has an active area of 100 mm × 100 mm and consists of an anode plane with 10 μm SS wires at 3 mm spacing and a pair of orthogonal cathode readout planes with 25 μm SS wires placed at 1.5 mm spacing. The position information is obtained using charge division method and recorded using a laboratory built data acquisition system. The resolution and gas gain was measured for 5.9 keV X-rays (⁵⁵Fe-source) as a function of the anode wire voltage and gas pressure. It was observed that the proportional region of the PSD at 100 kPa pressure extended up to a high voltage value of around 1.5 kV and it shifted to high values up to 2 kV for gas pressure of 300 kPa. The energy resolution improved from 18% (FWHM) to 12% with increase in pressure. The spatial resolution of the PSD also showed improvement, with a value of 1.2 mm × 1.4 mm at 300 kPa gas pressure. A maximum gain of 5 × 10⁴ is obtained.     

In situ observation of a Au (1 1 1) electrode surface using the X-ray reciprocal-lattice space imaging method

A rapid X-ray diffraction method was proposed for in situ observation of a surface-intermediate structure on a liquid-solid interface. It used a combination of higher-energy monochromatic synchrotron X-rays in grazing incidence and an X-ray two-dimensional detector. Overall patterns were in situ taken, with one-time exposure, of the reciprocal-lattice space of a Au (1 1 1) electrode surface which was fixed at an angular position. We deduced change in crystal domain shapes of surface intermediates as well as its smaller lattice distortion by observing images of reconstructed surface rods during a surface-structural phase transition from the reconstructed surface to the bulk terminated surface. An anisotropic shape of surface-crystal domains was also observed.     

Characterization of a triple-GEM position sensitive detector for X-ray fluorescence imaging

In this work, we characterized an X-ray position sensitive gaseous detector based in a triple stack of gas electron multipliers. The readout circuit is divided in 256 strips for each dimension and using a resistive chain interconnecting the strips, we are able to reconstruct the radiation interaction points by resistive charge division. The detector achieved gains above 10⁴, energy resolution of 15.28% (full width at half maximum) for 5.9 keV X-rays, and position resolution of 1.2 mm, while operating in Ar/CO₂(90/10) at atmospheric pressure.     

CCD探测器在测量金属丝线膨胀系数中的应用

利用CCD探测器分别测出常温和高温下金属丝衍射花样相邻暗纹的间距，用光学高温计测出加热时的温度值，从而求出线膨胀系数。     

New method for measuring beam profiles using a parametric X-ray pinhole camera

We propose a new method for measuring electron beam profiles using parametric X-ray radiation. In this method, a pinhole is placed between the source of parametric X-ray radiation and a two-dimensional X-ray detector, and the beam profile can be reconstructed on the detector, i.e., based on the principle of a pinhole camera. The profiles are in good agreement with the results obtained using a standard method with optical transition radiation. This method may prove useful to measure profiles of electron beams with short bunch lengths in recent advanced linear accelerators.     

二维多丝室探测器读出方法的优化

中国散裂中子源将建设一台基于~3He气体的二维多丝室,作为多功能反射谱仪束线的中子探测器.基于已有的研究,为优化选择二维多丝室探测器的丝结构,本文研究了三种不同的丝结构,并采用重心读出方法和数字读出方法进行了探测器的性能测量,得到了满足多功能反射谱仪探测器需求的读出方法.实验结果表明:对同种丝结构的二维多丝室探测器,重心读出方法的位置分辨和成像性能都好于数字读出方法;基于重心法读出的多丝室探测器位置分辨率可以达到约160μm,基于数字读出方法的多丝室探测器位置分辨率可以达到约400μm.优化设计的丝结构为:基于重心读出法的阳极丝间距1.5 mm、读出通道间距4 mm,基于数字读出法的阳极丝间距1.5 mm、读出通道间距2 mm.优化设计的丝结构均能满足谱仪的位置分辨要求.     

Ring artifacts correction based on the projection-field in neutron CT

Ring artifacts will happen mostly when the detector has inconsistent response among the detector channels, and the characteristic produced rings centered in the iso-center in the reconstructed slices inevitably affect the recognition and analysis of the corresponding sample structures in neutron computed tomography(CT). In this work, a ring correction method based on the projection-field(RCP) is proposed, it is a pre-processing method and provides the corrected projection data directly, which is also conducive to efficient data storage and other algorithmic researches. Simulation and physical experiments are performed for verifying the effect of the method, and one of the correction methods based on the imagefield is used for comparison. The results demonstrate that the RCP can correct the ring artifacts well without reducing the image resolution or over-correction.     

基于成像板-X射线条纹相机的精密耦合技术

为实现惯性约束聚变(ICF)实验中同时获取靶点的X射线1维动态和2维静态积分图像,提出了一种全新的X射线图像采集方法。结合成像板与X射线条纹相机的工作特性,通过在阴极狭缝前精密耦合成像板,实现X射线图像到达狭缝的同时采集其外围区域的静态积分图像。该方法具有对靶点X射线图像的1维动态与2维静态图像对比分析、成像系统像面位置精密空间定位的功能。利用该方法在神光Ⅱ装置上实现搭载Kirkpatrick-Baez(KB)显微镜获得内爆靶球压缩流线图,并应用于流体不稳定性实验中。