湍流特征光学测试对比

在10℃～230℃温差下,对大气相干长度r0分别采用夏克-哈特曼的到达角起伏法、差分像运动法、波面法三种测量法和四象限探测器进行了测试和对比;对折射率结构常量Cn2及闪烁功率谱分别采用夏克-哈特曼和光电倍增管进行对比.实验结果表明:对于r0,在强湍流时四象限探测器比夏克-哈特曼的稳定性明显降低,且对夏克-哈特曼三种方法,差分像运动法可克服设备抖动等问题,但引入了方向上不一致的问题,波面法可有效避免该问题;对于Cn2,夏克-哈特曼比光电倍增管测量更稳定,拟合相关系数高达0.96;对于闪烁功率谱,由于噪音影响,在200℃时夏克-哈特曼比光电倍增管测得的最大频率高15Hz;最后,通过对夏克-哈特曼子孔径的闪烁功率谱分析得出,若同一子孔径入射光强不在CCD响应的线性区间时无法准确测量闪烁功率谱,否则可通过不同子孔径可完成湍流均匀性的测量.这将为湍流池提供最优的测试方法及理论依据.     

ConCm±(n=1-5; m=1,2)团簇的密度泛函理论研究

本文采用基于自旋极化的密度泛函理论系统研究了Co_nC_m^± (n=1-5; m=1,2)团簇的几何结构和电子结构特性. 将Co_nC^± (n=2-5)团簇中的一个Co替换为C原子, 个体的基态几何结构发生明显变化; 在Co_nC₂^± (n=1-5)团簇的生长序列中, 发现从n=3开始团簇中的两个C原子有彼此分离分布的趋势, 我们分析, 这是Co金属能够维持单壁碳纳米管(SCNTs)保持开口生长, 成为非常有效的一种催化剂的重要原因. 同时, 将Co_nC^± (n=2-5)团簇中添加一个Co原子后系统的总磁矩出现大幅下降的趋势, 但仍保持奇偶交替的规律. 通过比较中性及带电的Co_nC以及Co_nC₂ (n=1-5)团簇的碎裂能, 本工作发现: 由实验获取的SCNTs应均为带正电的体系, 这一结论与已有的实验模型拟合得很好.     

N维各向同性谐振子径向平均值的递推关系和解析表达式

推导出了用于N维各向同性谐振子径向平均值计算的二个递推关系,并在-3≤s≤3的条件下,给出了平均值〈n_rJ_N-2|r^2s|n_rJ_N-2〉的值.二维和三维各向同性谐振子的相关结果均作为特例包含在结论中.     

同步测量大气湍流折射率结构常数和内尺度的光学方法

 基于不同波长的光闪烁，采用修正的大气湍流Hill谱模型，提出了一种同时反演大气湍流内尺度及折射率结构常数的方法。假定内尺度在某一个范围内取值，对于不同波长的闪烁指数，如果当内尺度取某一定值时，由光传输理论计算的C²_n(λ₁,…)和C²n (λ₂,…)相等，反演成功。根据此原理设计了三波长闪烁计并在某地进行了外场测量。近地面大气湍流的内尺度一般在2~10 mm之间，且随折射率结构常数（其量级为10^-16~10^-13）的变化而变化，两者之间存在一定的正相关；任意两波长组合进行反演得到的内尺度(或折射率结构常数)值具有自洽性，其相关系数的最小值为0.81，因此证明了该方法的可行性。     

高分辨率初始光电子能谱由真空紫外激光速度——映射图像的方法

通过采用真空紫外(VUV)激光速度-地图成像-TPE(真空紫外VMI-TPE)方法获得了高分辨率初始光电子(TPE)氯苯(C₆H₅Cl(X¹A₁))的光谱,炔丙基自由基(C₃H₃(X²B₁))和烯丙基(C₃H₅(X²A₁)). 观察到的真空紫外VMI-TPE方法的光电子能量分辨率在1~2 cm^-1,可以和在真空紫外激光脉冲场电离光电子(VUV-PFI-PE)的测量媲美. 类似真空紫外PFI-PE测量,真空紫外VMI-光电子(真空紫外VMI-PE)和真空紫外VMI-TPE测量能量分辨率依赖于直流电场在光电离区加速电子. C₆H₅Cl和C₃H₃的电离初始值的降低为F的函数表示Stark偏移校正为VUV-VMI-TPE测量由-3.1√F管辖,这是半经典预测值-6.1√F的一半. 我们还测量C₆H₅Cl和C₃H₅的真空紫外光能量的真空紫外VMI-PE谱接近其电离初始值. 在VUV-VMI-PE测量中观察到的C₃H₅⁺阳离子振动谱和振动级数,nv₇⁺(n=0~3). 真空紫外VMI-TPE可以实现更高的实验灵敏度和类似真空紫外PFI-PE测量的能量分辨率,使真空紫外VMI-TPE法成为高分辨率真空紫外PFI-PE测量一个很好的替代.     

带有电子-双声子相互作用的一维铁磁性介观环的非经典本征态和非经典本征持续电流

在一维铁磁性织构介观环的基础上, 计及电子-双声子相互作用, 介入了三项非经典效应抑制电子-单声子相互作用引起的量子涨落效应: 1) 跳步电子-单声子相干态关联效应;2) 由压缩相干态引起的声子压缩态-单声子相干态间过程关联效应;3) 声子位移-声子压缩态的表象关联效应．从结果来看, 电子-双声子相互作用明显加强了压缩效应(增大压缩参量), 而跳步电子-单声子相干态关联效应引起本征能量大幅度下降, 持续电流大幅度增加．特别是介入了声子压缩态-单声子相干态间过程关联效应后, 声子压缩参量远大于理想压缩态相应的压缩参量, 有效地抑制了Debye-Waller(D-W)效应．当声子压缩态-单声子相干态间过程关联与声子位移重整化效应结合在一起时, 声子场的压缩将更大幅度地增加, D-W效应(参量w_ph)将更大幅度地减小, w_ph << w_ph⁽⁰⁾, 从而极大幅度地抑制了电子-单声子相互作用导致的量子涨落效应. 这样一来, 非经典态本征能量E_n极大幅度地下降, E_n << E_n⁽⁰⁾, 与此同时, 本征持续电流振幅I_n 则极大幅度地增大, I_n >> I_n⁽⁰⁾.     

态|Ψn(2)>q的广义非线性等阶N次方H压缩效应

构造了一种新型的多模叠加态|Ψ_n⁽²⁾>_q=C_n^(R)|{-iZ_j^*}>_q+C_n⁽⁰⁾|{O_j}>_q;并首次详细地研究了此量子态的等阶N次方H压缩特性.大量的计算和分析表明:态|Ψ_n⁽²⁾>_q是一种多模典型的非经典光场;还发现了"相似压缩"等现象.     

用于DPF装置中子测量的闪烁体探测器

 介绍了一种用于等离子体焦点装置(DPF装置)中子波形测量的塑料闪烁体探测器，该探测器由ST401型塑料闪烁体、XP2262B型光电倍增管构成。利用银活化中子探测器和DPF装置对该塑料闪烁体探测器进行标定，确定其中子灵敏度为0.022 5 pC每中子，，中子产额测量范围达到10⁹～10¹¹每脉冲，可以满足DPF装置中子参数测量的需要。     

杂双子咪唑表面活性剂的合成及其表面性能

合成了一系列以两个亚甲基为联接基的杂双子咪唑表面活性剂([C_m-2-C_nim]Br_{2, m, n}=8, 10, 12, 14, 16; m≠n). 用氢谱和质谱对其结构进行了表征. 探索了物料比、反应温度和时间对反应产率的影响. 对合成的杂双子咪唑表面活性剂的表面活性进行了研究,讨论了分子结构的不对称程度对表面活性的影响.     

碱金属Li,Na,K,Rb,Cs,Fr的ns2S1/2,np2P1/2,3/2, nd2D3/2,5/2 和nf2F5/2,7/2 里德伯能级理论研究

本文在多通道量子数亏损理论(MQDT)框架下,利用相对论多通道理论(RMCT),分别在冻结实近似、 考虑Δl=-1的偶极极化效应、Δl=+1的偶极极化效应、Δl=± 1的偶极极化效应、伸缩模效应以及同时考虑偶极极化效应和伸缩模效应等不同层次近似下,系统地计算了碱金属Li, Na, K, Rb, Cs和Fr七个里德伯系列的能级,即ns²S_1/2, np²P_1/2, np²P_3/2, nd²D_3/2, nd²D_5/2, nf²F_5/2 和nf²F_7/2.计算结果表明,电子关联效应对碱金属原子的里德伯能级的影响很大.总的来说,偶极极化效应比伸缩模效应重要,而在偶极极化效应中, Δl = + 1的偶极极化效应比Δl = - 1的偶极极化效应重要.但对于Na的ns²S_1/2,(nd²D_3/2,nd²D_5/2)里德伯系列的能级,和Li的(np²P_1/2,np²P_3/2)里德伯系列的能级,是伸缩模效应比较重要.     

Analysis of Inner-Scale Effect on Atmosphere Scintillation for Infrared Laser Beam Propagating on Earth-Space Paths

On Earth-space paths, based on ITU-R C_n² (h) model, by means of a modification of the Rytov method that incorporates an amplitude spatial frequency filter function under strong fluctuation conditions, considering atmospheric turbulence inner-scale, an expression is developed for the scintillation index of a visible or a near and middle infrared laser beam wave that is valid under moderate to strong irradiance fluctuations. The quantitative analyses of scintillation index are done by this analytic model for laser Gaussian collimated beam wave at visible or near and middle infrared wave band. The results agree with theoretic analysis scintillation. This scintillation model can be converted into a Gaussian beam wave model with finite inner-scale on horizontal sight paths of invariable C_n².     

Study of Scintillation for Infrared Laser Beam Propagating in Atmospheric Turbulence on Earth-Space Paths

On earth-space paths, by applying a modification of the Rytov method that incorporates spatial frequency filter function under strong atmosphere fluctuation conditions, a tractable model is developed for the scintillation index of infrared laser Gaussian beam wave that is valid under moderate-to-strong irradiance fluctuations. At Infrared band, based on ITU-R C ² _n model, the scintillation indexes for collimation laser beam are predicted by this analytic model. The results agree with theoretic expected scintillation. This scintillation model can be converted into a plane or a sphere wave scintillation index model on earth-space paths, and also reduced to a Gaussian beam wave model on horizontal sight paths of invariable C ² _n.     

Persistence of the Feigenbaum Attractor in One-Parameter Families

Consider a map ψ₀ of class C ^r for large r of a manifold of dimension n greater than or equal to 2 having a Feigenbaum attractor. We prove that any such ψ₀ is a point of a local codimension-one manifold of C ^r transformations also exhibiting Feigenbaum attractors. In particular, the attractor persists when perturbing a one-parameter family transversal to that manifold at ψ₀. We also construct such a transversal family for any given ψ₀, and apply this construction to prove a conjecture by J. Palis stating that a map exhibiting a Feigenbaum attractor can be perturbed to obtain homoclinic tangencies. Received: 4 August 1998 / Accepted: 11 May 1999     

Viscoelastic behaviour of fluids with steeply repulsive potentials

We analyse the shear stress, C _s(t) and pressure or ‘bulk’, C _b(t) time-correlation functions for steeply repulsive inverse power fluids (SRP) in which the particles interact via a pair potential with the analytic form, φ(r) = ε(σ/r) ⁿ , in a new approach to the understanding of their viscoelastic properties. We show analytically, and confirm by molecular dynamics simulations, that close to the hard-sphere limit both these time-correlation functions have the analytic form, C _s(t)/C _s(0) and C _b(t)/C _b(0) = 1 – T*(nt*)²+ O((nt*)⁴), where T* = k _B T/ε, is the reduced temperature, k _B is Boltzmann's constant and t* = (ε/mσ²)^½ t is the reduced time. This leads to an alternative and much simpler derivation of formulae for the shear and bulk viscosities which for the limiting case of hard spheres are numerically very close to the traditional Enskog relations. These simple relations for the finite and continuous SRP interaction are in satisfactory agreement with the essentially exact molecular dynamics simulation results for ca. n ≥ 18.     

Propagation of the off-axis superposition of partially coherent beams through atmospheric turbulence

The propagation properties of the off-axis superposition of partially coherent beams through atmospheric turbulence and their beam quality in terms of the mean-squared beam width w(z) and the power in the bucket (PIB) are studied in detail, where the effects of partial coherence, off-axis beam superposition and atmospheric turbulence are considered. The analytical expressions for the intensity, the beam width and the PIB are derived, and illustrative examples are given numerically. It is shown that the maximum intensity I_max and the PIB decrease and w(z) increases as the refraction index structure constant C_n² increases. Therefore, the turbulence results in a degradation of the beam quality. However, the resulting partially coherent beam with a smaller value of spatial correlation parameter γ and larger values of separate distance x_d and beam number M is less affected by the turbulence than that with a larger value of γ and smaller values of x_d and M. The main results obtained in this paper are explained physically.     

Kinetic energy distributions of the fragment ions from multiply ionized C2H6 as functions of the charge state of the intermediate states

Here, we report the kinetic energy distributions (KEDs) of the fragment ions produced from multiply ionized ethane (C₂H₆) molecules in single electron capture collisions with 1.2 MeV C²⁺. To systematically investigate the fragmentation dynamics, the KEDs were obtained as functions of the charge state of the intermediate C₂H₆^r+* ions r transiently generated prior to fragmentation. r was determined from coincidence measurement of the fragment ions and the number of emitted electrons. The KEDs are drastically different depending on the number of broken C–H bonds. The underlying causes are explained by the variation of the relative contributions of the multiply ionized states and preferential fragmentation pathways. For instance, CH_n⁺ fragment ions with smaller n exhibit lower KEs because they are likely to be correlated with H⁺ emission, which carries away a large portion of the KE release. In addition, we report the KEDs of H₃⁺ produced from doubly and triply charged states.     

Statistical properties of freely decaying two-dimensional hydrodynamic turbulence

Statistical characteristics of freely decaying two-dimensional hydrodynamic turbulence at high Reynolds numbers are numerically studied. In particular, numerical experiments (with resolution up to 8192 × 8192) provide a Kraichnan-type turbulence spectrum E _k ～ k ^?3. By means of spatial filtration, it is found that the main contribution to the spectrum comes from sharp vorticity gradients in the form of quasi-shocks. Such quasi-singularities are responsible for a strong angular dependence of the spectrum owing to well-localized (in terms of the angle) jets with minor and/or large overlapping. In each jet, the spectrum decreases as k ^?3. The behavior of the third-order structure function accurately agrees with the Kraichnan direct cascade concept corresponding to a constant enstrophy flux. It is shown that the power law exponents ξ _n for higher structure functions grow with n more slowly than the linear dependence, thus indicating turbulence intermittency.     

部分相干厄米-双曲正弦-高斯光束通过湍流大气传输的平均光强分布演化和角扩展

推导出部分相干厄米-双曲正弦-高斯(H-ShG)光束通过湍流大气的平均光强和角扩展的解析表示式,并用以研究了部分相干H-ShG光束在湍流中的平均光强分布演化和角扩展. 结果表明,折射率结构常数C²_n的增加和空间相关长度σ₀的减小都会加速演化过程. 引入相对角扩展来定量描述光束抗拒湍流的能力. 空间相关长度σ₀,束腰宽度w₀和双曲 关键词： 平均光强分布演化 角扩展 湍流大气 部分相干厄米-双曲正弦-高斯(H-ShG)光束     

Express analysis of turbulence parameters

A method utilizing a Hartmann sensor for obtaining estimates of the external scale L ₀ of turbulent fluctuations and the structural constant C _n ² during the variation of the parameters of the wavefront of a light beam that has passed through turbulence is suggested. The method is based on Zernike polynomial decomposition of phase fluctuations at the given aperture and on analysis of this expansion coefficient’s statistics. Application of the method for making an estimate of the turbulence characteristics in a water cell yielded results that are in good agreement with the estimates obtained by other methods.