阿秒和频相位共轭极化拍频的不对称色锁二阶相干控制

研究了级联三能级系统中孪生色锁随机光场的相位共轭阿秒和频极化拍频(ASPB)不对称新效应。从理论上分析了自关联单光子简并四波混频(DFWM)和双光子非简并四波混频(NDFWM)信号辐射场与物质间不对等效应、混合型太赫兹失谐振荡特性,及双光子非简并共振四波混频信号的延时不对称性;同时也分析了由干涉计两臂不平衡色散效应引起的阿秒和频极化拍频信号的延时不对称性,即阿秒和频极化拍频信号的最大值相对于零延时有一个小偏移,结果表明该不对称性并这不影响阿秒和频极化拍频零差探测两偶极禁戒跃迁能级分裂的总体精度。阿秒和频极化拍频作为一种消除多普勒增宽的超快调制过程,从理论上说它可以扩展到任何两偶极禁戒跃迁能级系统。     

阿秒极化拍的V型三能级对称二阶相干理论

基于两单光子过程的相位共轭二阶极化干涉，从理论上研究了V型三能级系统在阿秒量级的对称和频极化拍频（SFPB），考虑了抽运光束为窄带线宽或宽带线宽的情形，发现测得的信号对任意带宽的马可夫随机光场的统计特征非常敏感，其在测量偶极禁界跃迁两激发态之间的能级和时并不受激光线宽的限制，仅取决于光学跃迁均匀增宽，而且可以得到消除多普勒增宽的测量精度.在窄带情形下，场关联对SFPB信号影响很弱.在宽带情形下，SFPB信号表现出共振 非共振交叉关联.SFPB作为一种阿秒超快调制过程，从理论上说它可以扩展到任何和频能级系统. 关键词： 阿秒 和频 极化拍 二阶相干     

非线性光学 位相共轭、自聚焦等相关效应

O4372006054150阿秒和频相位共轭极化拍频的不对称色锁二阶相干控制=Asymmetric second-order color-locking coherent controlof phase-conjugated attosecond sum-frequency polarizationbeats[刊,中]/余孝军(西安交通大学电子科学与技术系.陕西,西安(710049)),葛浩…//光学学报.—2006,26(6).—953-960研究了级联三能级系统中孪生色锁随机光场的相位共轭阿秒和频极化拍频(ASPB)不对称新效应。从理论上分析了自关联单光子简并四波混频(DFWM)和双光子非简并四波混频(NDFWM)信号辐射场与物质间不对等效应、混合型太赫兹失谐振荡特性,…     

倒V形四能级亚飞秒极化拍的三光子吸收和色散

基于孪生色锁噪声场的互相关效应，从理论上研究了倒V形(RV)四能级飞秒量级差频极化拍与极化拍中五阶非线性极化率，并提出了用一种相位敏感的方法来研究多能级原子相干造成的三光子六波混频过程.在抽泵光束为窄带末端情况下，场关联对信号和极化率的影响都很弱，在非窄带情况下，场关联会使极化强度自相干信号和极化拍信号产生关于零延时的不对称性和时域扫描上的辐射与物质失谐阻尼振荡(RDO)，而极化率会产生频域扫描上的RDO振荡.参考光信号是一路传播方向和六波混频信号稍有区别的双光于非简并四波混频信号.五阶非线性响应则由享生     

倒V形四能级亚飞秒极化拍的三光子吸收和色散

基于孪生色锁噪声场的互相关效应,从理论上研究了倒V形(RV)四能级飞秒量级差频极化拍与极化拍中五阶非线性极化率,并提出了用一种相位敏感的方法来研究多能级原子相干造成的三光子六波混频过程.在抽泵光束为窄带末端情况下,场关联对信号和极化率的影响都很弱,在非窄带情况下,场关联会使极化强度自相干信号和极化拍信号产生关于零延时的不对称性和时域扫描上的辐射与物质失谐阻尼振荡(RDO),而极化率会产生频域扫描上的RDO振荡.参考光信号是一路传播方向和六波混频信号稍有区别的双光于非简并四波混频信号.五阶非线性响应则由享生 关键词： 外差法 吸收 色散 非线性极化     

三能级系统电子分布转移的数值模拟

原子能级中的分布可以人为的加以控制,受激拉曼迁移过程为我们提供了一种有效转移电子分布的方法,特别是可以有选择地实现分子高振动能级的分布转移.要对该过程有一个全面的了解,就必须对偏离共振和激光强度对电子分布转移所产生的影响有深刻的认识.使用数值模拟的方法系统地分析了三能级系统在受激拉曼迁移过程中电子分布的转移情况,计算了系统处于双光子共振时和偏离共振时的转移率,分析了偏离双光子共振、偏离单光子共振以及两束激光相对强度对转移率的影响.计算结果表明在双光子共振时可以完全转移;当偏离双光子共振很小的时候,基本可以达到完全转移;转移率对两束激光的相对强度不是很敏感.     

差频瑞利增强极化拍的零差探测研究

基于马尔可夫随机场模型的理论给出了差频瑞利增强极化拍（REPB）的解析解，并且研究了三种马尔可夫随机场模型下场关联效应和瑞利型共振增强效应对拍频信号的影响，指出了振幅涨落和位相涨落在时域和频域的不同作用.差频REPB信号展现出了时域对称特性，信号在三种马尔可夫随机场模型下的差别随着带宽的增大逐渐消失.     

级联三能级系统中极化拍频的不对称特性

在泵浦光为窄带或宽带的情形下,我们对级联三能级系统中极化拍频的不对称特性进行了研究,发现这种不对称特性是由于光学元件色散所导致的零延时的漂移引起的.     

四能级系统极化拍频的不对称特性

在泵光为窄带或宽带的情形下,对四能级系统中极化拍频的不对称特性进行了研究,发现这种不对称特性是由于光学元件色散所导致的零延时的漂移引起的. 关键词：     

对氟甲苯分子四光子电离过程的分析

根据量子力学微扰理论给出了相干扰激发电离情形下双光子共振三光子近共振和双光子近共振三光子共振这两种两光子电离过程的电离截面表达式，表明这两种过程的离子强度与它们的起始能级有关，根据这一结论分析了实验测得的对氟甲苯分子的多光子电离谱，结果表明获得该电离谱的过程为三光子共振四光子电离过程。     

Fifth-order attosecond polarization beats using twin color-locked noisy lights in cascade three-level system with Doppler-free approach

Fifth-order attosecond sum-frequency polarization beat (FASPB) is studied in a cascade three level system with the phase-conjugation fourth-order coherence function theory. An improved schematic diagram of geometry, which is different from that inducing fifth-order femtosecond different-frequency polarization beat(FFDPB), is used to obtain FASPB. By analyzing the cases that pump beams have either narrow or broad bandwidth, it is found that the temporal behavior of the sum-frequency polarization beat signal depends on the properties of the lasers and transverse relaxation rate of the atomic energy-level system. Finally,the cascaded four-wave mixing (FWM) processes and the difference between attosecond and femtosecond polarization beats have been discussed, it is found that cascaded or sequential lower processes can often obscure the direct fifth-order polarization beat processes.     

用光电子能谱相位确定法同时测量阿秒超紫外线XUV脉冲的频率和强度时间分布

介绍阿秒超紫外线(XUV)激发惰性气体原子产生光电子并在强激光电场中运动的半经典近似 方法，以及同时、直接、全面地测量阿秒XUV脉冲频率和强度时间分布的光电子能谱相位确定法. 采用飞秒超短脉冲激光和XUV间的交叉关联技术，从不同激光强度下、与激光线性极化方向成0°或180°方向上测得的光电子能量积分谱，可以重建XUV的频率和强度时间分布. XUV脉冲时间宽度的测量范围从1／4到1／2激光振荡周期，时间分辨率取决于激光束和XUV脉冲之间的相对延时控制精度和光路抖动时间. 所述方法可用于在阿秒尺度上的超快速测量，以及有关电子在原子和分子中运动的超快速动力学过程研究. 关键词： 阿秒测量 光电子能谱 相位确定法 超紫外线 频率和强度时间分布     

Use of a single-mode fiber coupler for second-harmonic-generation microscopy

We present a compact second-harmonic-generation (SHG) microscope based on a three-port single-mode fiber coupler. The fiber coupler is used to deliver a near-infrared ultrashort-pulsed laser beam as well as to collect the SHG signal in the visible wavelength range. The SHG microscope exhibits an axial resolution of 1.8 microm, which shows a slight enhancement of the optical sectioning effect compared with that for two-photon excitation at the same excitation wavelength. It is also demonstrated that SHG and two-photon fluorescence images under parallel and perpendicular laser excitation polarization can be simultaneously obtained.     

Probing electron-electron correlation with attosecond pulses

We study two-photon double ionization of helium in its ground state at sufficiently low laser intensities so that three and more photon absorptions are negligible. In the regime where sequential ionization dominates, the two-photon double ionization one-electron energy spectrum exhibits a well defined double peak structure directly related to the electron-electron correlation in the ground state. We demonstrate that when helium is exposed to subfemtosecond or attosecond pulses, both peaks move and their displacement is a signature of the time needed by the He⁺ orbital to relax after the ejection of the first electron. This result rests on the numerical solution of the corresponding non-relativistic time-dependent Schrödinger equation.Received: 17 January 2003, Published online: 18 March 2003PACS: 32.80.Rm Multiphoton ionization and excitation to highly excited states (e.g., Rydberg states) - 32.80.Dz Autoionization     

The statistical fluctuation of a single-mode laser system driven by coloured pump noise with signal modulation and the quantum noise with cross-correlation between its real and imaginary parts

Using the linear approximation method, this paper studies the statistical property of a single-mode laser driven by both coloured pump noise with signal modulation and the quantum noise with cross-correlation between its real and imaginary parts, and calculates the steady-state mean normalized intensity fluctuation and intensity correlation time. It analyses the influences of the modulation signal, the net gain coefficient, the noise and its correlation form on the statistical fluctuation of the laser system respectively. It is found that the coloured pump noise modulated by the signal has a great suppressing action on the statistical fluctuation of the laser system; the pump noise self-correlation time and the specific frequency of modulation signal have the result that the statistical fluctuation tends to zero. Furthermore, the `colour' correlation of pump noise has much influences on the statistical fluctuation of the laser system. Increasing the intensity of pump noise will augment the statistical fluctuation of the laser system, but the intensity of quantum noise and the coefficient of cross-correlation between its real and imaginary parts have less influence on the statistical fluctuation of the laser system. Therefore, from the conclusions of this paper the statistical property can be known and a theoretical basis for steady operation and output of the laser system can be provided.     

Time evolution of the intensity correlation function in a single-mode laser driven by both the coloured pump noise with signal modulation and the quantum noise with cross-correlation between the real and imaginary parts

Using the linear approximation, we have studied the time evolution of intensity correlation function C（t） in a single-mode laser driven by both the colored pump noise with signal modulation and the quantum noise with cross-correlation between its real and imaginary parts. In the case of the pump noise self-correlation time, we find that the time evolution of C（t） varies with modulation signal frequency Ω, amplitude B, and net gain ɑ0. (i) As the Ω increases, the time evolution of C（t） experiences a process changing from the monotonous descension to the descension with a flat appearing initially, and finally to the a form of damping oscillation; (ii) As the B increases, it experiences from monotonous descension to the appearance of a maximum; (iii) As the net gain ɑ0 increases, it experiences a process repeatedly changing from the monotonous descension to monotonous ascension, and to the appearance of a maximum, finally to monotonous descension again. However, in the case of, the time evolution of C（t） only exhibits a form of damping oscillation .     

偏置信号调制下噪声关联的周期调制对单模激光随机共振的影响

在噪声受偏置信号调制的情况下,讨论色噪声之间的关联受时间周期调制所驱动的单模激光系统中的随机共振.用线性化近似的方法计算了输出信噪比.具体讨论输出信噪比随噪声自关联时间、噪声强度和偏置信号的变化关系.发现输出信噪比随抽运噪声强度和自关联时间的变化出现随机共振,而偏置信号会降低随机共振的峰值.实际应用中应控制优选偏置信号强度. 关键词： 偏置信号 色噪声 时间周期调制 噪声间关联程度