排序方式: 共有12条查询结果,搜索用时 15 毫秒
1.
基于孪生色锁噪声场的互相关效应,从理论上研究了倒V形(RV)四能级飞秒量级差频极化拍与极化拍中五阶非线性极化率,并提出了用一种相位敏感的方法来研究多能级原子相干造成的三光子六波混频过程.在抽泵光束为窄带末端情况下,场关联对信号和极化率的影响都很弱,在非窄带情况下,场关联会使极化强度自相干信号和极化拍信号产生关于零延时的不对称性和时域扫描上的辐射与物质失谐阻尼振荡(RDO),而极化率会产生频域扫描上的RDO振荡.参考光信号是一路传播方向和六波混频信号稍有区别的双光于非简并四波混频信号.五阶非线性响应则由享生
关键词:
外差法
吸收
色散
非线性极化 相似文献
2.
研究了级联三能级系统中孪生色锁随机光场的相位共轭阿秒和频极化拍频(ASPB)不对称新效应。从理论上分析了自关联单光子简并四波混频(DFWM)和双光子非简并四波混频(NDFWM)信号辐射场与物质间不对等效应、混合型太赫兹失谐振荡特性,及双光子非简并共振四波混频信号的延时不对称性;同时也分析了由干涉计两臂不平衡色散效应引起的阿秒和频极化拍频信号的延时不对称性,即阿秒和频极化拍频信号的最大值相对于零延时有一个小偏移,结果表明该不对称性并这不影响阿秒和频极化拍频零差探测两偶极禁戒跃迁能级分裂的总体精度。阿秒和频极化拍频作为一种消除多普勒增宽的超快调制过程,从理论上说它可以扩展到任何两偶极禁戒跃迁能级系统。 相似文献
3.
Coherent Phase Control of Ultrafast Polarization Beats in Reverse V-Type Three-Level System 下载免费PDF全文
We investigate the third-order nonlinear absorption and dispersion of femto- and atto-second polarization beats between the one-photon degenerate four-wave mixing process and the two-photon nondegenerate four-wave mixing process in the pure homogeneously-broadened reverse V-three-level using twin noisy fields. The third-order nonlinear response can be controlled and modified by the colour-locked correlation of twin noisy fields. Most importantly, the coherent phase control in optical heterodyne detection for studying the phase dispersion of the third-order susceptibility is demonstrated. The radiation-matter detuning oscillation is also considered in the freauencv domain. 相似文献
4.
Interactions of Three Dual-Dressing Effects of Four-Wave Mixing in a Five-Level Atomic System 下载免费PDF全文
We study the four-wave mixing (FWM) in an opening five-level system with two dressing fields. There axe three kinds of doubly dressing mechanisms (parallel cascade, sequential cascade, and nested cascade) in the system for doubly dressed four-wave mixing. These mechanisms reflect different correlations between two dressing fields and different effects of two dressing fields to the FWM. Investigation of these mechanisms is helpful to understand the generated high-order nonlinear optical signal dressed by multi-fields. 相似文献
5.
The near-threshold highly bound states of all three stable isotopic
variants of molecular hydrogen have been studied. Numerous
perturbations and unexpected transitions are observed as far as
1cm\sj{-1} just below the second dissociation threshold. This
complex structure may arise from a combination of nonadiabatic
coupling between B, B', C electronic states, perturbations due to
fine and hyperfine interactions, and strong shape resonances. The
perturbed near-threshold states and vibrational continuum exhibit
finegrained structure, differing greatly between isotopes because of
varying nonadiabatic coupling. 相似文献
6.
Fifth-order phase-sensitive detection of ultrafast polarization beats in cascade four-level system 下载免费PDF全文
We study the colour-locked twin-noisy-field correlation effects in the fifth-order nonlinear susceptibility of ultrafast polarization beats in a cascade four-level system. More importantly, the fifth-order phase-sensitive heterodyne detection of ultrafast polarization beats has been exploited. The fifth-order nonlinear optical response can be controlled and modified through the colour-locked correlation of twin noisy fields. Thus, this method with the phase dispersion information is a good way to measure the real and imaginary parts of the fifth-order nonlinear susceptibility. 相似文献
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9.
We describe near-threshold high-resolution spectra and continuum resonance dynamical behaviour of all three stable hydrogen isotopic variants, and finally obtain improved values for the dissociation energies of hydrogen molecule and its ion. The second dissociation limit is determined by analysing the onset of the vibrational continuum. 相似文献
10.
基于两双光子过程的相位共轭二阶极化干涉,从理论上研究了四能级系统在阿秒量级的不对称和频极化拍频(FASPB).在抽运光束为窄带情形下,场关联对FASPB信号影响很弱.在宽带情形下,FASPB信号表现出共振-非共振交叉关联,双光子信号展现出混合辐射-物质失谐的THz阻尼振荡,即当激光频率偏离双光子共振跃迁的条件时,信号将呈现阻尼振荡,而且其双光子自相关信号的包络还呈现最大值零延时不对称.还研究了由于两双光子自相关过程零延时的偏差导致的阿秒拍频信号的不对称性,和两个双光子信号的最大值分别向相反的方向偏离零延时点的现象.FASPB作为一种阿秒超快调制过程,从理论上说它可以扩展到任何两偶极禁戒跃迁激发态的能级和系统.
关键词:
阿秒和频
极化拍
四能级
双光子 相似文献