共查询到20条相似文献,搜索用时 125 毫秒
1.
本文提出了一种在双色场中使用相干叠加态来提高高次谐波发射效率的方法. 我们首先通过在800nm基本激光脉冲上添加一束控制激光脉冲在理论上得到双色合成激光场;其次,通过求解一维含时薛定谔方程,计算得到了体系处于不同初始态时的高次谐波谱,并结合时频分布图对其微观机理进行分析. 计算结果表明,使用相干叠加态作为体系的初始态,通过调节两束激光的相对相位可以有效实现提高高次谐波的发射效率的目的. 相似文献
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在双色场中使用相干叠加态来提高高次谐波的发射 总被引:1,自引:0,他引:1
本文提出了一种在双色场中使用相干叠加态来提高高次谐波发射效率的方法.我们首先通过在800 nm基本激光脉冲上添加一束控制激光脉冲在理论上得到双色合成激光场;其次,通过求解一维含时薛定谔方程,计算得到了体系处于不同初始态时的高次谐波谱,并结合时频分布图时其微观机理进行分析.计算结果表明,使用相干叠加态作为体系的初始态,通过调节两束激光的相对相位可以有效实现提高高次谐波的发射效率的目的. 相似文献
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本文提出了一种多色合成激光方案用来有效的提高高次谐波谱平台区域的宽度. 我们首先通过在800nm基本激光脉冲上添加一束或者两束控制激光脉冲在理论上得到双色以及三色合成激光场;其次,通过求解一维含时薛定谔方程,计算得到了在多色合成激光场条件下的高次谐波谱,计算结果表明,多色合成激光场方案可以有效的拓展高次谐波谱的平台区域;最后,我们结合电子的经典回碰动能分布以及时频分布,分析了在多色场条件下高次谐波谱平台区域拓宽的机理和微观机制. 相似文献
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本文提出了一种多色合成激光方案用来有效的提高高次谐波谱平台区域的宽度. 我们首先通过在800nm基本激光脉冲上添加一束或者两束控制激光脉冲在理论上得到双色以及三色合成激光场;其次,通过求解一维含时薛定谔方程,计算得到了在多色合成激光场条件下的高次谐波谱,计算结果表明,多色合成激光场方案可以有效的拓展高次谐波谱的平台区域;最后,我们结合电子的经典回碰动能分布以及时频分布,分析了在多色场条件下高次谐波谱平台区域拓宽的机理和微观机制. 相似文献
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通过数值求解双色激光场(基频场和二倍频场)与一维晶体相互作用的含时薛定谔方程,研究了晶体在双色激光脉冲驱动下发射高次谐波的特点.研究结果表明,晶体在双色激光脉冲驱动下发射的高次谐波第二平台强度相对于单色激光脉冲驱动下有显著提高,且随双色激光脉冲的相位差明显变化.进一步的研究发现,在双色激光脉冲其它参数保持不变的情况下,通过调节双色激光脉冲的相位差就能有效提高晶体发射高次谐波第二平台的产额,提高的幅度会随激光脉冲的宽度有所不同. 相似文献
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This paper investigates experimentally high-order harmonic generation(HHG) of neon gas with 5-fs and 25-fs driving laser pulses.It has been demonstrated that the cutoff energy of the harmonic extreme ultraviolet photons is extended to 131 eV and the HHG spectrum near the cutoff region becomes continuum as the driving laser pulse duration is 5 fs;whereas much lower cutoff photon energy and discrete harmonic spectrum near the cutoff region are presented as the laser pulse duration is 25 fs.The results can be explained by the fact that neutral atoms can be exposed to more intense laser field before they are depleted by ionization because of the extremely short rising time of the few-cycle pulse.The 5-fs driving laser pulse paves the way of generation of coherent x-ray in the water window and single attosecond pulse. 相似文献
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D. B. Milo?evi? E. Hasovi? S. Od?ak M. Busulad?i? A. Gazibegovi?-Busulad?i? W. Becker 《Laser Physics》2009,19(2):185-190
Numerical results obtained applying the strong-field approximation to atomic and molecular processes in intense laser fields are presented. In particular, the forward-backward asymmetry in high-order above-threshold ionization (HATI) of Ar atoms by a few-cycle laser pulse is considered. It is shown that the resonantlike enhancements observed in the focal-averaged spectra disappear with the decreasing laser pulse duration. For HATI and high-order harmonic generation (HHG) by molecular systems, we present new results for diatomic molecules. The choice of gauge and the problem of dressing of the initial bound state are discussed. The appearance of the interference minima in molecular HATI and HHG spectra and their role in the characterization of the molecular structure are considered using the example of the Ar2 molecule. 相似文献
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采用多周期的800 nm钛宝石激光组合1600 nm中红外脉 冲辐照氦离子产生高次谐波发射功率谱. 相对于单色场情形, 谐波谱出现明显的双平台结构, 且在第二平台区出现了光滑的连续辐射谱, 其转化效率相对于第一平台低了约两个数量级. 通过附加脉宽为1 fs的27次谐波脉冲到双色激光场的特定时域, 可以控制电子电离在半个光学周期内迅速提升, 获得了由单一短量子路径贡献的连续辐射谱, 使得第二平台区谐波的转化效率相对于组合场情形增强4个数量级, 且连续谱的频谱范围从第二平台区扩展到第一平台区, 叠加该连续谱190次到285次谐波生成了脉宽为29 as的强、短孤立脉冲. 相似文献
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Gang-Tai Zhang 《Molecular physics》2013,111(20):3117-3125
We theoretically demonstrate an efficient method for producing an isolated ultrashort attosecond pulse by high-order harmonic generation in an intense few-cycle chirped laser pulse. Our simulation calculations show that the harmonic spectrum reveals an ultrabroad extreme ultraviolet supercontinuum when the initial state is prepared in a coherent superposition of the ground and first excited states. It is also shown that the method can enhance the short quantum path and eliminate the long one, and then an isolated 23-attosecond pulse is produced. By properly adjusting the chirp parameter, a clean single attosecond pulse as short as 11 attoseconds is directly obtained. 相似文献
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We theoretically propose a three-color laser scheme to enhance the high-order harmonic intensity and generate an isolated attosecond pulse. By adding a 3 fs, 1600 nm laser pulse to a synthesized two-color laser field (5 fs, 800 nm and 10 fs, 1200 nm), the harmonic intensity is effectively enhanced and an isolated attosecond pulse with duration 41 as is generated. In this scheme, the short trajectory is suppressed, the selection of the long quantum path can be achieved. We also investigate emission time of harmonics in terms of the time-frequency analysis and the semi-classical three-step model to illustrate the physical mechanism of high-order harmonic generation. 相似文献
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Generation of an isolated sub-30 attosecond pulse in a two-color laser field and a static electric field 下载免费PDF全文
We theoretically investigate high-order harmonic generation(HHG) from a helium ion model in a two-color laser field,which is synthesized by a fundamental pulse and its second harmonic pulse.It is shown that a supercontinuum spectrum can be generated in the two-color field.However,the spectral intensity is very low,limiting the application of the generated attosecond(as) pulse.By adding a static electric field to the synthesized two-color field,not only is the ionization yield of electrons contributing to the harmonic emission remarkably increased,but also the quantum paths of the HHG can be significantly modulated.As a result,the extension and enhancement of the supercontinuum spectrum are achieved,producing an intense isolated 26-as pulse with a bandwidth of about 170.5 eV.In particular,we also analyse the influence of the laser parameters on the ultrabroad supercontinuum spectrum and isolated sub-30-as pulse generation. 相似文献
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We theoretically study the high-order harmonic generation (HHG) from a hydrogen atom in an intense few-cycle chirped fundamental laser in combination with an ultraviolet (uv) controlling pulse.The high-order harmonic spectrum is calculated by solving the time-dependent Schr¨odinger equation using the split-operator method.In our calculation,we present the difference of the high-order harmonic spectrum from one-dimensional (1D) model hydrogen atom and three-dimensional (3D) real hydrogen atom.We found that the plateau of the high-order harmonic generation from the 1D case and 3D case are all extended effectively to I p + 35U p due to the presence of the chirped laser pulse and the HHG supercontinuum spectrum is generated by adding an ultraviolet controlling pulse at a proper time,but the efficiency of the HHG for 3D case is more higher at the near cut-off region than the 1D case.Therefore,the generation of the attosecond pulse by synthesizing the harmonics near cut-off region have some slight differences between 1D and 3D simulations.As a real 3D case study,we show that an isolated 18 as pulse with a bandwidth of 232.5 eV is generated directly by optmizing the combination laser fields. 相似文献
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The isotopic effect on the generation of the molecular high-order harmonics is studied by numerically solving the one-dimensional time-dependent Schrödinger equation when the model hydrogen molecule ions/hydrogen deuterium molecule ions are exposed to an intense laser pulse. To explain the effect more clearly, not only the ionization probabilities but also the electron–nuclear probability density distributions and time-frequency profiles are calculated. The results show that more intense harmonics are generated in the asymmetric diatomic molecule ions/hydrogen deuterium molecule ions than those of hydrogen molecule ions. Moreover, the interference minimum in the harmonic spectra is investigated by adjusting the laser intensity and the initial vibrational state. It is shown that the interference minimum is sensitive to the laser intensity and the initial vibrational level for hydrogen molecule ions; in contrast, it is only dependent on the initial vibrational level for hydrogen deuterium molecule ions. 相似文献
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High-order harmonic generation of CO_2 with different vibrational modes in an intense laser field 下载免费PDF全文
We apply the strong-field Lewenstein model to demonstrate the high-order harmonic generation of CO_2 with three vibrational modes(balance vibration,bending vibration,and stretching vibration) driven by an intense laser field.The results show that the intensity of harmonic spectra is sensitive to molecular vibrational modes,and the high harmonic efficiency with stretching vibrational mode is the strongest.The underlying physical mechanism of the harmonic emission can be well explained by the corresponding ionization yield and the time-frequency analysis.Finally,we demonstrate the attosecond pulse generation with different vibrational modes and an isolated attosecond pulse with a duration of about 112 as is generated. 相似文献
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Harmonic Enhancement Mechanism of a Superposition State Atom Irradiated by Short Pulses 总被引:1,自引:0,他引:1 下载免费PDF全文
We investigate the high-order harmonic generation (HHG) of a model atom whose initial state is prepared in a superposition of its ground state and an excited state irradiated by different duration laser pulses. Compared to the HHG generated from an atom whose initial state is in its ground state, its conversion efficiency obtains some enhancement. The enhancement originates from the higher ionization rate (rather than the ionization yield) of the atom with superposition initial state. 相似文献