Double differential cross sections of light charged particle production for the n+~(238)U reaction

Production of light complex particles from the n+~(238) U reaction is analyzed with the exciton model including the improved Iwamoto-Harada pickup mechanism for the preequilibrium process. It is allowed that some of the nucleons forming the complex ejectile come from levels below the Fermi energy, and the intrinsic structure of the emitted particle is taken into account. The equilibrium-state emissions are also considered by using HauserFeshbach theory with the width fluctuation correction and the evaporation model. Moreover, all cross sections,angular distributions, energy spectra and double differential cross sections of neutron, proton, deuteron, triton and alpha emissions for the n+~(238) U reaction are consistently calculated and analyzed with nuclear theoretical models in the energy range En 150 MeV. ENDF-formatted nuclear data including information about the production of light charged particles are obtained.     

The study of the (α, α′ f) reaction at 120 MeV on 232Th and 238U: (II). Fission barrier properties deduced from fission probabilities and angular distributions

The fission probabilities and angular distributions of the fission fragments for the (α, α'f) reaction on ²³²Th and ²³⁸U at a bombarding energy of 120 MeV have been measured from about 4 to 14 MeV excitation energy. Evidence for sub-barrier resonances has been found, the negativeparity ones occurring at the same excitation energy where photofission resonances have been observed. The data are analyzed with the two-humped barrier model. For ²³⁸U the data are reasonably well fitted with barriers similar to those known from the literature. For ²³²Th though, the outer barrier parameters are quite different: the height E_B = 6.6 MeV and the width (khω)_B = 1.2 MeV. Also for ²³²Th, introducing an additional mass symmetric and axially asymmetric outer barrier, as was previously found necessary for ²³⁸U, does not result in a good fit to the data at higher excitation energies.     

贫铀球壳中D-T中子诱发的铀反应率的测量与分析

为校验次临界能源堆的概念设计,在R19.4/30.0 cm的贫铀球壳装置上采用活化法开展14 MeV中子学积分实验.布放6片贫铀活化片于球壳中与入射D离子束90°方向上的不同位置处活化,用HPGe探测器测量238U(n,γ)反应、238U(n,f)及235U(n,f)反应和238U(n,2n)各反应产物发射的特征γ射线,得到了相应的反应率.238U(n,γ)反应率的不确定度为3.6％-3.7％,238U(n,D和235U(n,f)反应率的不确定度为5.1％-5.9％,238U(n,2n)反应率的不确定为4.3％-4.7％.用MCNP5程序在ENDF66c数据库下进行模拟计算,238U(n,γ)反应率的计算值/实验值(C/E)为0.972-1.034,238U(n,f)和235U(n,f)反应率的C/E为0.983-1.058,238U(n,2n)反应率的C/E为0.979-1.019.     

The study of the (α, α'f) reaction at 120 MeV on 232Th and 238U: (I). Fission probabilities and angular distributions in the region of the giant quadrupole resonances

The fission decay channel of ²³²Th and ²³⁸U has been investigated, using the (α, α'f) reaction at 120 MeV bombarding energy. The angular distributions of the fission fragments and the fission probabilities up to around 15 MeV excitation have been measured. No evidence for the fission decay of the giant quadrupole resonance has been found, although for ²³⁸U, a weakly excited structure is seen in the (α, α'f) spectrum at about 9.5 MeV excitation at backward angles with respect to the recoil axis. This effect is similar to what has been found in a (⁶Li, ⁶Li'f) experiment reported recently. The over-all feature of the fission probability for excitation energies above the fission barrier are well reproduced by statistical calculations.     

Fusion reactions around the barrier for Be+~(238)U

Fusion-evaporation cross sections of ~(238)U (~9Be,5n)~(242)Cm are measured over a wide energy range around the Coulomb barrier.These measured cross sections are compared with model calculations using two codes,namely HIVAP2 and KEWPIE2.HIVAP2 calculations overestimate the measured fusion-evaporation cross sections by a factor of approximately 3.In KEWPIE2 calculations,two approaches,namely the Wentzel-Kramers-Brillouin(WKB) approximation and the empirical barrier-distribution (EBD) method,are used for the capture probability;both of them properly describe the measured cross sections.Additionally,fusion cross sections of ~(7,9)Be+~(238)U measured in two experiments are applied to constrain model calculations further through three codes,i.e.,HIVAP2,KEWPIE2,and CCFULL.Parameters in these codes are also examined by comparison with measured fusion cross sections.All the comparisons indicate that the KEWPIE2 calculations using the WKB approximation agree well with the measured cross sections of both fusion reactions ~(7,9)Be+~(238)U and the fusion-evaporation reaction ~(238)U (~9Be,5n)~(242)Cm.Calculations using the fusion code CCFULL are also in good agreement with the measured fusion cross sections of ~(7,9)Be+~(238)U.     

Monte Carlo simulation of fast neutron-induced fission of ~(237)Np

The potential-driving model is used to describe the driving potential distribution and to calculate the preneutron emission mass distributions for different incident energies in the ~(237) Np(n, f)reaction. The potential-driving model is implemented in Geant4 and used to calculate the fission-fragment yield distributions, kinetic energy distributions, fission neutron spectrum and the total nubar for the ~(237) Np(n, f)reaction. Compared with the built-in G4 ParaFissionModel, the calculated results from the potential-driving model are in better agreement with the experimental data and evaluated data. Given the good agreement with the experimental data, the potential-driving model in Geant4 can describe well the neutron-induced fission of actinide nuclei, which is very important for the study of neutron transmutation physics and the design of a transmutation system.     

Direct observation of a rho decay of the D13(1520) baryon resonance

The reaction gammap-->pi(+)pi(0)n has been measured at MAMI for photon energies up to 820 MeV. Invariant mass spectra of the particles in the final state (pi(+)n), (pi(0)n), (pi(+)pi(0)) have been determined for several bins of incident photon energy. Differences in pi(+)pi(0) and simultaneously measured pi(0)pi(0) invariant mass distributions are assigned to a rho branch of the D13(1520) nucleon resonance.     

Large contribution of deep inelastic processes to reactions of40Ar and48Ca with238U

Differential recoil range distributions have been measured for heavy-reaction products ranging from Te(Z=52) to quasielastic transfer products near the charge and mass of the targets for the reactions of 276 MeV⁴⁸Ca+²³⁸U, 237MeV and 250 MeV⁴⁰Ar+²³⁸U, and 259 MeV⁴⁰Ar+¹⁹⁷Au. The measured recoil range distributions for the⁴⁰Ar+¹⁹⁷Au reaction agree with range distributions calculated from the known projectile-like fragment angular distributions for this reaction. The angular distributions of recoil products formed in the uranium target reactions are deduced and show that the products in the₇₅Re to₈₃Bi region have backward peaked angular distributions characteristic of deep inelastic reactions. The heavy product angular distributions smoothly vary from a (1/sinθ) shape to an exponential shaped backward peak as the atomic number of the product increases from 52 to 83. The trend in the deduced angular distributions for those elements for which recoil range distributions were determined in the⁴⁰Ar+¹⁹⁷Au reaction and the 250 MeV⁴⁰Ar+²³⁸U reaction is similar, suggesting that just as for the Ar+Au system the composite system for the uranium target reaction is also not fully equilibrated along the mass asymmetry coordinate. These conclusions show that the fraction of the total reaction cross section resulting in complete fusion must be re-evaluated for the⁴⁰Ar+²³⁸U reaction and similar heavy-target reactions.     

Study of the heavy products from84Kr+238U collisions at 522 MeV

Angular distributions and integral cross sections for heavy reaction products from⁸⁴Kr +²³⁸U collisions at 522 MeV were measured using catcher foil techniques and off-line X-ray identification of individual reaction product isotopes. There is no evidence for a fission-fusion mechanism being responsible for the formation of the “gold finger”. The data show that usual deep inelastic collisions account for the formation of all products with 70≦Z≦86. Compared to existing data atE≦605 MeV, the deduced mass distribution indicates reduced fission probabilities forZ≧80 fragments at 522 MeV. This is consistent with the expected dependence of fission probability on excitation energy and especially on angular momentum.     

中子与裂变核238U反应双微分截面的理论分析

根据中子与原子核U及其同位素反应的总截面,去弹性散射截面和弹性散射角分布的实验数据,获得了入射中子能量0.1—20MeV的一组普适中子与U及其同位素反应的光学模型势参数.应用光学模型,核裂变理论,耦合道理论,扭曲波玻恩近似理论,宽度涨落修正的Hauser-Feshbach理论和预平衡反应的激子模型,计算和分析了中子与²³⁸U反应的所有截面、角分布、能谱和双微分截面.理论计算与实验数据进行了分析比较     

Energy levels in even actinide isotopes from (t,p) reactions

Energy levels in^{232, 234}Th,^{236, 238, 240}U and in²⁵⁰Cm have been measured using the (t, p) reaction. Angular distributions were obtained for the^{234, 238}U targets and evidence for second order effects in the direct reaction mechanism was found.     

Theoretical Analysis of Double Differential Cross Sections for n+ 238U Reaction

Based on the new measurements of total, nonelastic, elastic cross section and elastic scattering angular distributions for n+U reactions, a set of neutron optical model potential parameters is obtained in the region of incident neutron energy from 0.1 to 20 MeV. The cross sections, angular distributions, energy spectra and double differential cross sections are calculated and analyzed by optical model, nuclear fission theory, distorted wave Born approximation theory, coupled channel theory, the unified Hauser-Feshbach theory, as well as exciton model. The results indicate that our theoretical model can reasonably analysis n+ ²³⁸U reaction data with neutron energy lower than 20 MeV.     

The study of prompt and delayed muon induced fission

Mass yield and total kinetic energy release (TKE) distributions of fragments from prompt and delayed muon induced fission, separately, have been measured for the isotopes²³⁵U,²³⁸U,²³⁷Np and²⁴²Pu. The distributions from prompt muon induced fission are compared with the corresponding distributions from hadronic reactions and from spontaneous fission (s.f.). The distributions from the delayed muonic fission processes are compared to the distributions for neutron and proton-induced fission. No mass distributions measured in the prompt muonic fission process show any signature, which can be attributed to the presence of the muon. Differences observed between the TKE distributions of prompt muon induced and hadron induced fission can be explained by the screening effect of the negative charge of the muon bound in the orbit of one of the fission fragments. The observed yield of symmetric muon induced fission was found to be defined merely by the value of the excitation energy.     

238U photofission in the energy region of the giant dipole resonance

²³⁸U photofission is studied in the region of nuclear excitation energies that extends up to 20 MeV. Independent photofission-fragment yields and cumulative photofission-fragment yields after the emission of fast neutrons are measured by gamma-spectroscopy methods. The mass distributions of photofission fragments are obtained at the endpoint bremsstrahlung energies of 19.5, 29.1, 48.3, and 67.7 MeV. A comparative analysis of the behavior of the symmetric and asymmetric modes of photoninduced fission as a function of the average excitation energy of the fissioning nucleus is performed. The integrated yield of ²³⁸U photofission is calculated, and the evaluated cross sections for photofission and for photoneutron reactions are discussed.     

149Sm(n,α)146Nd cross sections in the MeV region

We have measured the (149)Sm(n,α)(146)Nd cross section at 4.5, 5.0, 5.5, 6.0, and 6.5 MeV. Measurements were performed at the 4.5 MV Van de Graaff accelerator of Peking University with monoenergetic neutrons produced via the (2)H(d,n)(3)He reaction using a deuterium gas target. Alpha particles were detected with a double-section gridded ionization chamber having two back-to-back (149)Sm(2)O(3) samples attached to the common cathode. Absolute neutron flux was measured using a small (238)U fission chamber and monitored by a BF(3) long counter. These are the first reported cross sections for this reaction at these energies, except at 6.0 eV, where our new data are in good agreement with our earlier result. The present results help to much better constrain the (149)Sm(n,α)(146)Nd cross section in a region where its energy dependence is changing fairly rapidly and there are large differences between evaluated nuclear data libraries.     

Correlation between fragment mass-distribution fine structure,charge distribution and nuclear structure for thermal-neutron-induced fission of 233U and 235U

Masses corresponding to observed fine-structure peaks in the fragment mass distributions for thermal-neutron-induced fission of ²³³U and ²³⁵U are shown to correspond to average measured masses for even-even nuclear charge splits. Evidence is presented that the yield enhancement for even-Z fragments is not restricted just to fission events with higher-than-average total kinetic energy. The anomalously high yield of fragments with mass 134 in ²³⁵U(n, f) as opposed to ²³³(n, f) is tentatively correlated with rapidly changing nuclear structure properties as a function of the mass of the complementary light (Z = 40) fragments.     

原子核的大质量转移反应和丰中子超重核的产生(英文)

迄今为止,人们合成的超重核都是缺中子的,无论是熔合-裂变反应还是碎化过程都无法使产物达到周期表的“东北区域”。而重核之间(如U核之间) 的近垒大质量转移反应则可能是目前生成丰中子超重核和达到未知丰中子重核区域的唯一途径。在改进的量子分子动力学(ImQMD) 模型结合统计模型框架内,研究了U+U等反应体系的大质量转移反应,计算了反应产生的初生态碎片的质量和电荷分布,并成功再现了产物的终态质量和电荷分布。通过比较3 个反应136Xe+248Cm,48Ca+248Cm和238U+248Cm 产生的106号元素的截面大小,揭示了U+U等重核大质量转移反应对产生丰中子超重核是非常有利的。For elements with Z > 100 only neutron deficient isotopes have been synthesized so far. The “northeast area” of the nuclear map can be reached neither in fusion-fission reactions nor in fragmentation processes.The large mass transfer reactions in near barrier collisions of heavy (U-like) ions seem to be the only reaction mechanism allowing us to produce neutron rich heavy nuclei including those located at the superheavy(SH) island of stability and unexplored area of heavy neutron-rich nuclides. This study is extremely important for nuclear astrophysical investigations and, in particular, for the understanding of the r process. In this paper within the Improved Quantum Molecular Dynamics (ImQMD) model combining with the statistical-evaporation model, the large mass transfer reactions, like 238U+238U have been studied. The charge and mass distributions of transiently formed primary fragments are investigated within the ImQMD model and de-excitation processes of those primary fragments are described by the statistical decay model. The mass distribution of the final products in 238U+238U collisions is obtained and compared with the recent experimental data. Through compared the formation cross sections of transfermium element 106 by three reactions of 136Xe+248Cm, 48Ca+248Cm and 238U+248Cm, it is explored that the large mass transfer reactions, like U+U are very benefit for the production of SH nuclei.     

The interaction of 538 MeV 56Fe with 238U

Binary coincident fragments from the ⁵⁶Fe+²³⁸U reaction at 538 MeV have been studied. Fragment energies were measured and fragment masses determined by a kinematic method. Three types of event are defined by suitable adjacent limits in the mass versus energy event space. The angular distributions of cross section, energy and mass have determined for each event region and particular attention paid to that part containing possible fissions following complete fusion. The total reaction cross section consists of about 50 % of binary fragmentation channels. The remaining channels correspond to a ternary process of heavy recoil fission.     

Peculiarities in fragment mass distribution in the 238U + 40Ar (243 MeV) reaction

A pronounced fine structure (FS) in the form of distinct peaks was observed in neutron gated mass spectra from the decay of the ²⁷⁸110 composite system produced in the reaction ²³⁸U + ⁴⁰Ar (243 MeV) at an initial excitation energy E ^* > 70 MeV. The FS peaks are located in the vicinity of mass numbers 70-80, 100, and 130, which correspond to those of magic nuclei (clusters). In the data there is also evidence for a new type of decay -- collinear cluster tripartition of an excited nucleus. Received: 8 August 2000 / Accepted: 2 February 2001