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Magnetic,electrical transport and electron spin resonance studies of Fe-doped manganite LaMn0.7Fe0.3O3+δ
Authors:XJ Liu  ZQ Li  A Yu  ML Liu  WR Li  BL Li  P Wu  HL Bai  EY Jiang
Institution:1. Faculty of Science, Institute of Advanced Materials Physics, Tianjin University, Tianjin 300072, China;2. Tianjin Key Laboratory of Low Dimensional Materials Physics and Preparing Technology, Tianjin University, Tianjin 300072, China;3. Central Laboratory, Nankai University, Tianjin 300071, China;4. Analysis Test Center, Jilin University, Changchun 130023, China
Abstract:We have investigated the magnetic, electrical transport and electron spin resonance (ESR) properties of polycrystalline Fe-doped manganite LaMn0.7Fe0.3O3+δ prepared by sol–gel method. A typical cluster-glass feature is presented by DC magnetization and AC susceptibility measurements and a sharp but shallow memory effect was observed. Symmetrical Lorentzian lines of the Mn/Fe spectra were detected above 120 K, where the sample is a paramagnetic (PM) insulator. When the temperature decreases from 120 K, magnetic clusters contributed from ferromagnetic (FM) interaction between Mn3+ and Mn3+/Fe3+ ions develop and coexist with PM phase. At lower temperature, these FM clusters compete with antiferromagnetic (AFM) ones between Fe3+ ions, which are associated with a distinct field-cooled (FC) effect in characteristic of cluster-glass state.
Keywords:75  47  Lx  75  50  Lk  75  40  Gb  76  30  -v
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