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以NH3为还原剂的选择性催化还原(SCR)技术可实现工业烟气中氮氧化物(NOx)的超低排放,现有钒钛系脱硝催化剂具有生物毒性,且报废后为危险废物。稀土元素(REEs)具有独特的4f电子轨道,表现出优异的储释氧性能,在催化反应中可发挥重要作用,是当前新型脱硝催化剂的重要研究对象,也是国家鼓励的现有钒钛系催化剂的替代品。本文主要总结了铈、钐、镧等12种REEs在新型脱硝催化剂中的近5年研究进展,另有钪、镥等5种REEs的相关研究较少,重点阐述了REEs改善催化剂脱硝活性与稳定性的作用机制及耦合过渡金属的协同催化机理,初步提出了脱硝催化剂的设计原则,并展望了稀土脱硝催化剂的发展前景。 相似文献
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Current-voltage characteristics of lead zirconate titanate/nickel bilayered hollow cylindrical magnetoelectric composites 下载免费PDF全文
Current--voltage measurements obtained from lead zirconate
titanate/nickel bilayered hollow cylindrical magnetoelectric
composite showed that a sinusoidal current applied to the copper
coil wrapped around the hollow cylinder circumference induces
voltage across the lead zirconate titanate layer thickness. The
current--voltage coefficient and the maximum induced voltage in lead
zirconate titanate at 1~kHz and resonance (60.1~kHz) frequencies
increased linearly with the number of the coil turns and the applied
current. The resonance frequency corresponds to the
electromechanical resonance frequency. The current--voltage
coefficient can be significantly improved by optimizing the
magnetoelectric structure geometry and/or increasing the number of
coil turns. Hollow cylindrical lead zirconate titanate/nickel
structures can be potentially used as current sensors. 相似文献
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