Superconductivity of the FeSe/SrTiO_3 Interface in View of BCS–BEC Crossover

In paired Fermi systems,strong many-body effects exhibit in the crossover regime between the Bardeen-CooperSchrieffer(BCS)and the Bose-Einstein condensation(BEC)limits.The concept of the BCS-BEC crossover,which is studied intensively in the research field of cold atoms,has been extended to condensed matters.Here by anal.yzing the typical superconductors within the BCS-BEC phase diagram,we find that FeSe-based superconductors are prone to shift their positions in the BCS-BEC crossover regime by charge doping or substrate substitution,since their Fermi energies and the superconducting gap sizes are comparable.Especiall.y at the interface of single-layer FeSe on SrTiO_3 substrate,the superconductivity is relocated closer to the crossover unitary than other doped FeSe-based materials,indicating that the pairing interaction is effectively modulated.We further show that hole-doping can drive the interfacial system into the phase with possible pre-paired electrons,demonstrating its flexible tunability within the BCS-BEC crossover regime.     

能量与空间分辨的单分子显微术--透过碳笼"看"富勒烯包合物内的金属原子

文章作者用探测扫描隧道电流微分谱的方法，对金属富勒烯包合物分子进行了研究，得到了Dy@C82同分异构体Ⅰ的金属-碳笼杂化态在实空间的能量分布图，通过将实验与理论模拟的结果进行比较，推断出Dy原子在碳笼中的位置以及金属富勒烯包合物分子在衬底表面的吸附取向．这项技术为单分子纳米器件的表征和诊断提供了新的途径．     

扫描隧道显微术中的微分谱学及其应用

文章介绍了扫描隧道显微术中微分谱学的原理及其在实验中的诸多应用。微分谱（dI／dV谱）和dI／dV成像可用来研究电子局域态密度在能量和空间的分布，即微分谱固定空间一点，反映电子态密度以能量为变量的分布；而dI／dV图像则反映某给定能量的电子局域态密度以空间为变量的分布，二次微分谱（d^2I／dV^2谱）和二次微分成像可以用来反映分子的非弹性隧穿过程，从而研究分子的振动态。     

LaTiO3(110)薄膜分子束外延生长的精确控制和表面截止层的研究

LaTiO₃ 是一种典型的强关联电子材料, 其(110) 薄膜为通过晶格对称性、应变等的设计调控外延结构的物理性质提供了新的机会. 本文研究了SrTiO₃(110) 衬底表面金属La 和Ti 沉积所引起的微观结构变化, 进而利用电子衍射信号对分子束外延薄膜生长表面阳离子浓度的灵敏响应, 发展了原位、实时、精确控制金属蒸发源沉积速率的方法, 实现了高质量LaTiO₃(110) 薄膜的生长和对阳离子化学配比的精确控制. 由于LaTiO₃中Ti³⁺ 3d 电子的库仑排斥作用, 氧原子层截止的(110) 表面更容易实现极性补偿, 因此生长得到的薄膜表面暴露出单一类型的氧截止面.