新型金属团簇(Et_4N)_3WOS_3Cu_3I_4的皮秒光限幅特性研究

应用波长为532nm,脉冲宽度为40ps的激光脉冲研究了新型金属团簇(Et4N)3WOS3Cu3I4的光限幅性能。实验结果表明,该金属团簇在皮秒激光脉冲的作用下,具有很强的光限幅特性。利用非线性吸收的唯象理论对实验结果进行了分析。     

Wavelength-dependent nonlinear absorption of gold nanocages

The dipole resonances of gold nanocages were investigated theoretically using finite difference time domain method.The results show that field enhancement is obtained at the walls of the gold nanocages.It is believed that the effect can cause a strong optical nonlinear property.To test the hypothesis,nonlinear absorption was investigated using a broadband 5 ns Z scan.It was found that at low intensities the sample shows saturable absorption(SA),while at higher intensities a switch from SA to reverse SA occurs.Moreover,the nonlinear absorption of the sample is sensitively wavelength-dependent,and,in the resonant region,saturation intensity is the largest.