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Capillary electrophoretic studies on quantum dots and histidine appended peptides self‐assembly 下载免费PDF全文
Jianhao Wang Jingyan Li Yao Chen Yiwan Teng Cheli Wang Jinchen Li Li Liu Bingyu Dong Lin Qiu Pengju Jiang 《Electrophoresis》2015,36(19):2419-2424
Herein, we designed four peptides appended with different numbers of histidine (Hisn‐peptide). We launched a systematic investigation on quantum dots (QDs) and Hisn‐peptide self‐assembly in solution using fluorescence coupled CE (CE‐FL). The results indicated that CE‐FL was a powerful method to probe how ligands interaction on the surface of nanoparticles. The self‐assembly of QDs and peptide was determined by the numbers of histidine. We also observed that longer polyhistidine tags (n ≤ 6) could improve the self‐assembly efficiency. Furthermore, the formation and separation of QD‐peptide assembly were also studied by CE‐FL inside a capillary. The total time for the mixing, self‐assembly, separation, and detection was less than 10 min. Our method greatly expands the application of CE‐FL in QDs‐based biolabeling and bioanalysis. 相似文献
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Nonlinear Dynamics - Mathematical models and analyses can assist in designing the control strategies to prevent the spread of infectious disease. The present paper investigates the bifurcations and... 相似文献
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Wenjie Li Lihong Huang Jinchen Ji 《Mathematical Methods in the Applied Sciences》2019,42(13):4498-4515
This paper investigates the periodic solution of a delayed Beddington‐DeAngelis (BD) type predator‐prey model with discontinuous control strategy. Firstly, the regularity and visibility analysis of the delayed predator‐prey model is carried out by using the principle of differential inclusion. Secondly, the positiveness and boundeness of the solution is discussed by employing the comparison theorem. Based on the boundary conditions of the model and the Mawhin‐like coincidence theorem, it is shown that the solution of the delayed BD system is asymptotically stable in finite time. Furthermore, it is found that there exists at least one periodic solution of the nonautonomous delayed predator‐prey model by using the principle of topological degree and set value mapping. Specially, when the nonautonomous delayed BD system degenerates into an autonomous system, some criteria are obtained to guarantee the convergence behavior of the harvesting solutions for the corresponding autonomous delayed BD system. Finally, numerical examples are given to demonstrate the applicability and effectiveness of main results. It is worthy to point out that the discontinuous control strategy is superior to the continuous harvesting policies adopted in existing literature. 相似文献
4.
Zhao Feng Ji Jinchen Luo Quantian Cao Shuqian Chen Lumin Du Wenliao 《Nonlinear dynamics》2021,104(1):349-365
Nonlinear Dynamics - Quasi-zero stiffness (QZS) isolators can achieve superior performance in vibration isolation; however, this superiority is often effective only for an excitation with the small... 相似文献
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Xin?Qin Penghui?ShiEmail author Haolin?Liu Jinchen?Fan Yulin?Min Qunjie?XuEmail author Weifeng?Yao 《Journal of nanoparticle research》2017,19(6):225
Metal nanoparticles have been combined with magnet metal–organic frameworks (MOFs) to afford new materials that demonstrate an efficient catalytic degradation, high stability, and excellent reusability in areas of catalysis because of their exceptionally high surface areas and structural diversity. Magnetic M x O y @N-C (M = Fe, Co, Mn) nanocrystals were formed on nitrogen-doped carbon surface by using 8-hydroxyquinoline as a C/N precursor. The Co@N-C, MnO@N-C, and Fe/Fe2O3@N-C catalysts were characterized by X-ray diffraction (XRD), Raman, scanning electron microscopy (SEM), high-resolution transmission electron microscopy (HRTEM), N2 adsorption/desorption, and X-ray photoelectron spectroscopy (XPS). The catalytic performances of catalysts were thoroughly investigated in the oxidation of aniline solution based on sulfate radicals (SO4 ?.) toward Fenton-like reaction. Magnetic M x O y @N-C exhibits an unexpectedly high catalytic activity in the degradation of aniline in water. A high magnetic M x O y @N-C catalytic activity was observed after the evaluation by aniline degradation in water. Aniline degradation was found to follow the first-order kinetics, and as a result, various metals significantly affected the structures and performances of the catalysts, and their catalytic activity followed the order of Co > Mn > Fe. The nanoparticles displayed good magnetic separation under the magnetic field. 相似文献
6.
Jialu Gao Yu Ma Jianbo Li Jinchen Fan Penghui Shi Qunjie Xu Yulin Min 《Journal of nanoparticle research》2018,20(11):298
As two-dimensional layered nanomaterials, the tungsten disulfide (WS2) nanosheets can be used as building blocks of paper-like electrodes for high-performance FSs. However, poor conductivity and mechanical property of WS2 nanosheets (NSs) paper greatly hinders their capacitance and/or rate performance. To solve these problems, we fabricated the WS2-multiwalled carbon nanotubes (MWCNTs)/polyaniline (PANI) composite papers based on liquid exfoliation and electrochemical deposition for high-performance flexible supercapacitors. The WS2-MWCNTs/PANI with conductive PANI chains linked WS2 NSs and MWCNTs takes the advantages of high-electronic double-layer capacitance originated from the internal surface areas of MWCNTs and effective pseudocapacitance generated by exfoliated WS2 NSs and PANI. Electrochemical studies showed that the gravimetric-specific capacitance of WS2-MWCNTs/PANI can reach ~760.1 F/g at a current density of 1 A/g. A symmetric flexible solid-state supercapacitor was also assembled and studied. The WS2-MWCNTs/PANI-assembled FS device also has an excellent area specific capacitance of 1158.7 mF/cm2 at a current density of 0.5 mA/cm2 together with a high-capacity retention of ~82.5% after 2000 cycles. 相似文献
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非线性振动系统动力学行为的实验研究 总被引:5,自引:0,他引:5
本文综述了非线性振动系统动力学行为的实验研究,详细叙述了机械模型实验,实验数据的分析与处理,并对今后发展趋势作了述评. 相似文献
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Simultaneous monitoring of quantum dots and their assembly and disassembly with PreScission protease using capillary electrophoresis with fluorescence detection 下载免费PDF全文
Jianhao Wang Jinchen Li Jianpeng Wang Li Liu Jinping Li Haifang Qin Shumin Ding Minli Fu Junling Ji Pengju Jiang Lin Qiu 《Journal of separation science》2016,39(9):1785-1791
A novel assay was developed for the simultaneous monitoring of quantum dots and their assembly and disassembly with PreScission protease using capillary electrophoresis with fluorescence detection. Quantum dots and PreScission protease were injected into a capillary sequentially, then mixed and assembled via a thioether bond upon coupling to glutathione S‐transferase tag inside the capillary. The in‐capillary assembly was influenced by the molar ratio and the time interval of injection. Furthermore, the simultaneous monitoring of quantum dots and their assembly with PreScission protease and glutathione induced disassembly was achieved by adjusting the sampling sequence and the time interval of injection. More importantly, the in‐capillary assay could be also applied to the online detection of glutathione. 相似文献
10.
Wang Jianhao Li Jingyan Teng Yiwan Hu Wei Chai Hong Li Jinchen Wang Cheli Qiu Lin Jiang Pengju 《Journal of nanoparticle research》2014,16(7):1-7
A method is presented for using a single laser pulse to transform polymorphic polycrystalline gold nanoparticles (Au NPs) into crystalline nanospheres. Transmission electron microscope analysis of the nominally 60-nm-diameter Au NP starting material and the product suspension confirms the production of slightly smaller particles that exhibit greater crystallinity and feature reduced caliper diameter aspect ratios and anisotropy. Centrifugation followed by ultrasonic resuspension into citrate solution separates the nanospheres from the <15 nm ablation fragments, providing a route to monodisperse spherical crystalline Au NPs. 相似文献