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1.
S=1/2 One‐Dimensional Random‐Exchange Ferromagnetic Zigzag Ladder,Which Exhibits Competing Interactions in a Critical Regime 下载免费PDF全文
Susan N. Herringer Dr. Mercè Deumal Dr. Jordi Ribas‐Arino Prof. Juan J. Novoa Prof. Christopher P. Landee Prof. Jan L. Wikaira Prof. Mark M. Turnbull 《Chemistry (Weinheim an der Bergstrasse, Germany)》2014,20(27):8355-8362
The synthesis, crystal structure, and magnetic properties (from a combined experimental and First‐Principles Bottom‐Up theoretical study) of the new compound catena‐dichloro(2‐Cl‐3Mpy)copper(II), 1 , [2‐Cl‐3Mpy=2‐chloro‐3‐methylpyridine] are described and rationalized. Crystals of 1 present well isolated magnetic 1D chains (no 3D order was experimentally observed down to 1.8 K) and magnetic frustration stemming from competing ferromagnetic nearest‐neighbor (JNN) interactions and antiferromagnetic next‐nearest neighbor (JNNN) interactions, in which α=JNNN/JNN <?0.25. These magnetic interactions give rise to a unique magnetic topology: a two‐leg zigzag ladder composed of edge‐sharing up‐down triangles with antiferromagnetic interactions along the rails and ferromagnetic interactions along the zigzag chain that connects the rails. Crystals of 1 also present a random distribution of the 2‐Cl‐3Mpy groups, which are arranged in two different orientations, each with a 50 % occupancy. This translates into a random static structural disorder within each chain by virtue of which the value of the JNN magnetic interactions can randomly take one of the following three values: 53, 36, and 16 cm?1. The structural disorder does not affect the JNNN value, which in all cases is approximately ?9 cm?1. A proper statistical treatment of this disorder provides a computed magnetic susceptibility curve that reproduces the main features of the experimental data. 相似文献
2.
本文利用KDV方程所对应的线性方程解所具有的光滑效应及压缩映像原理,得到了Hirota-Satsuma系统初值问题的局部和整体适定性结果. 相似文献
3.
The vibronic vapour phase photoacoustic spectrum of Br2 in the wavelength region 505–541 nm (19796–18480 cm−1) has been recorded using microphone as well as pump-probe method. Discrete vibronic bands superimposed on a monotonically
increasing continuum background towards the dissociation limit results from the overlapping B
3Π
0u
/+
← X
1Σ
g
/+
and 1Π1u
← X
1Σ
g
/+
electronic transitions. Vibronic bands originating from υ″=0 have been used to estimate the relative rate of non-radiative relaxation as a function of the excited state B
3Π0u
vibrational quantum number υ′. A comparison with the optical absorption spectroscopy of Br2 leads to the identification of three broad spectral regions between 505 and 541 nm (19796 and 18480 cm−1) on the basis of different non-radiative relaxation processes. 相似文献
4.
Ninios K Hong T Manabe T Hotta C Herringer SN Turnbull MM Landee CP Takano Y Chan HB 《Physical review letters》2012,108(9):097201
Using micromechanical force magnetometry, we have measured the magnetization of the strong-leg spin-1/2 ladder compound (C(7)H(10)N)(2)CuBr(2) at temperatures down to 45 mK. Low-temperature magnetic susceptibility as a function of field exhibits a maximum near the critical field H(c) at which the magnon gap vanishes, as expected for a gapped one-dimensional antiferromagnet. Above H(c) a clear minimum appears in the magnetization as a function of temperature, as predicted by theory. In this field region, the susceptibility in conjunction with our specific-heat data yields the Wilson ratio R(W). The result supports the relation R(W)=4K, where K is the Tomonaga-Luttinger-liquid parameter. 相似文献
5.
Herringer SN Turnbull MM Landee CP Wikaira JL 《Dalton transactions (Cambridge, England : 2003)》2011,40(16):4242-4252
An isocoordinate family of compounds has been generated with the general formula (2-X-3-methylpyridine)(2)CuX'(2), where X, X' = Cl or Br. While each forms trans-ligand compounds, they vary in copper coordination geometry, canting of the pyridine rings and magnetic behavior. The copper bromide analogues exhibit weak ferromagnetic interactions whereas the copper chloride analogues exhibit antiferromagnetic interactions. Each compound has been characterized by IR, powder X-ray diffraction, single-crystal X-ray diffraction, and temperature dependent magnetic susceptibility. 相似文献
6.
Ki Hwan Bae 《中国化学快报》2009,20(11):1321-1323
Phytochemical study on the BuOH-soluble fraction of the stem bark of Populus davidiana resulted in the isolation of a new salicin derivative(1),named davidianoside.The structure was elucidated on the basis of extensive physicochemical and spectroscopic analyses. 相似文献
7.
8.
From the transport studies in the bilayer manganites LaSr2−x
Ca
x
Mn2O7, we have found the variable-range hopping model proposed by Viret et al to be inadequate to describe the transport of charge in these materials. The polarons appear to hop to their nearest neighbors
with an activation energy, which in part is dependent on the magnetic interactions in the lattice. 相似文献
9.
S Chanda Sarmishtha Bhattacharyya Tumpa Bhattacharjee SS Ghugre Swapan Kumar Basu S Muralithar RP Singh B Mukherjee RK Bhowmik SN Ray 《Pramana》2001,57(1):175-179
The high spin states in N=80 139Pr have been investigated by in-beam γ-spectroscopic techniques following the reaction 130Te (14N, 5n) reaction at E=75 MeV, using a gamma detector array, consisting of seven 23% compton-suppressed high purity germanium detectors and a multiplicity
ball of fourteen bismuth germanate elements. Based on γ-γ coincidence data, the level scheme of 139Pr has been considerably extended up to 7.2 MeV excitation. Tentative spin-parity assignments are done for the newly proposed
levels on the basis of the DCO ratios corresponding to strong gates and the available information from the earlier light ion
experiments. 相似文献
10.
MVN Murthy Urjit A Yajnik KRS Balaji G Bhattacharyya Amol Dighe Shashikant Dugad ND Hari Dass PK Kabir Kamales Kar D Indumathi John G Learned Debasish Majumdar NK Mondal MVN Murthy SN Nayak Sandip Pakvasa Amitava Raychaudhuri RS Raghavan G Rajasekaran R Ramachandran Alak K Ray Asim K Ray Saurabh Rindani HS Sharatchandra Rahul Sinha Nita Sinha S Umasankar Urjit A Yajnik 《Pramana》2000,55(1-2):347-355
We have identified some important and worthwhile physics opportunities with a possible neutrino detector located in India.
Particular emphasis is placed on the geographical advantage with a stress on the complimentary aspects with respect to other
neutrino detectors already in operation. 相似文献