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识别和解析石墨烯中缺陷的精确原子结构是研究不同类型缺陷的物化特性, 实现石墨烯物性调控的前提, 可以为在原子尺度研究石墨烯缺陷的构效关系提供重要的实验依据. 本文结合扫描隧道显微镜(STM)和原子力显微镜(AFM)确认了在Ir(111)表面生长的石墨烯中自发形成的缺陷, 以及通过离子轰击方法在石墨烯中引入的多种缺陷结构, 包括单空位缺陷、 非六元环拓扑结构以及石墨烯层下的基底缺陷. 相似文献
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Determinations of plasma density and decay time in the hollow cathode discharge by microwave transmission 下载免费PDF全文
The microwave (MW) transmission method is employed to measure both the plasma density and the plasma decay time in the hollow cathode discharge (HCD) in argon at low pressure. The plasma density in DC-driven or pulsed HCD is on the order of 1012 cm-3, which can block the X-band MW effectively. In the case of pulsed HCD, the MW transmittance shows the same waveform as the pulsed current during the rising edge if the driving frequency is low, but with a longer delay during the falling edge. The MW transmittance reaches a constant low level when the driving frequency is high enough. The plasma decay time in the HCD system is measured to be about 100 μs around a pressure of 120 Pa. The ambipolar diffusion is considered to be the major mechanism in the decay process. 相似文献
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由于在水下爆炸冲击波的数值仿真研究中,水的状态方程、人工黏性系数和网格尺寸对数值计算结果影响很大,采用常规TNT炸药的水下爆炸为例,以冲击波的峰值压力和比冲量为衡量指标,研究了这3个主要影响因素对数值仿真结果的影响。首先,通过采用常用的5种水的状态方程进行系列仿真,给出了各种状态方程的适用范围;其次,讨论了人工黏性系数对计算结果的影响,并给出了一次与二次人工黏性系数的建议取值范围;最后,通过对不同炸药当量及不同网格尺寸开展系列运算,从而得到不同炸药当量在满足工程计算精度要求下所对应的建议网格尺寸,并得到了不同炸药当量所对应的建议网格尺寸的表达式。 相似文献
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Quantum spin liquids(QSLs) represent a novel state of matter in which quantum fluctuations prevent the conventional magnetic order from being established, and the spins remain disordered even at zero temperature. There have been many theoretical developments proposing various QSL states. On the other hand, experimental movement was relatively slow largely due to limitations on the candidate materials and difficulties in the measurements. In recent years, the experimental progress has been accelerated. In this topical review, we give a brief summary of experiments on the QSL candidates under magnetic fields. We arrange our discussions by two categories: i) Geometrically-frustrated systems, including triangularlattice compounds YbMgGaO_4 and YbZnGaO_4, κ-(BEDT-TTF)_2 Cu_2(CN)_3, and EtMe_3 Sb[Pd(dmit)_2]_2, and the kagom′e system ZnCu_3(OH)_6 Cl_2; ii) the Kitaev material α-RuCl_3. Among these, we will pay special attention to α-RuCl_3, which has been intensively studied by ours and other groups recently. We will present evidence that both supports and rejects the QSL ground state for these materials, based on which we give several perspectives to stimulate further research activities. 相似文献
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本文对本研究组主要的研究领域——利用中子散射研究铁基超导体系Fe1+yTe1-xSex中磁性与超导的相互作用进行简要综述. Fe1+yTe1-xSex具有和其他铁基、铜基超导体相似的相图——母相Fe1+yTe是反铁磁体, 随着Se掺杂的增加, 母相的反铁磁序受到抑制, 随后在x~30%处体超导出现, 在x~50%处达到最佳掺杂, 此时超导转变温度Tc~ 15 K, 达到整个体系在常压下的Tc最大值. 它们的相图又存在着差别: 在相图末端, 即当Se掺杂达100%时, Fe1+ySe 仍然超导, Tc~8 K. 该体系母相磁有序的面内波矢大致为(0.5,0) (采用每个原胞含2个铁原子的四方结构), 随着Se含量的增加, 在超导逐渐发展的同时, 磁激发谱的谱重被逐渐转移到波矢为(0.5,0.5) 处. (0.5,0.5) 处在温度低于Tc 时出现中子-自旋共振峰. 施加外磁场后, 超导受到抑制, 该共振峰也被压制. 从这些实验结果我们得到以下的结论: 在这个体系中磁性和超导紧密耦合在一起——(0.5,0) 处的静态磁有序与超导互相竞争, (0.5,0.5) 附近的自旋激发则可能对超导电性的形成具有重要的促进作用. 本文还将简要讨论磁性的来源和3d 过渡金属的替代效应. 相似文献
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设计合成了具有光热和NO释放性的抗菌、抗氧化水凝胶。利用Fe3+和戊二醛将聚赖氨酸、单宁酸(TA)交联形成水凝胶,并负载NO供体分子S-亚硝基-N-乙酰基-DL-青霉胺(SNAP)获得兼具光热和NO控释功能的水凝胶(NO-Fex-TA20, x=5, 7, 9)。所合成的Fe9-TA20水凝胶具有良好的光热性能,在1 W/cm2近红外光照射下10 min内温度可达到43.8℃。在可见光和37℃恒温下,NO-Fe9-TA20水凝胶3 h累计释放的NO达到36.48μmol/L。抗菌实验表明,水凝胶对金黄色葡萄球菌具有优异的杀菌活性,杀菌活性大于99.9%;同时,其能够高效清除2,2-联苯基-1-苦基胼基(DPPH)自由基,清除率大于84.3%,抗氧化效果显著。 相似文献
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