腔内倾斜标准具法压缩KrF激光线宽的研究

我们对采用腔内倾斜标准具法压缩激光线宽进行了研究，较详细地讨论了影响线宽压缩效果的各种因素。并在一台长脉冲放电泵浦ＫｒＦ准分子激光器上，采用三个标准具作为线宽压缩元件，获得了线宽小于３ＧＨｚ，发散角近似衍射极限的高质ＫｒＦ激光输出。实验中研究了不同光阑孔径及输出耦合率对输出线宽和输出能量的影响。     

放电型高增益KrF激光器非稳腔的研究

给出了放电型高增益非稳腔KrF激光器具有衍射极限的激光模式建立的时间与非稳腔放大率和腔长之间的关系。实验对放大率M=8,腔长L=1.75m和放大率M=13.3,腔长L=1.85m的正支共焦非稳腔在不同增益下输出光的发散角进行了测量。充电电压为30kV,发散角分别是39倍衍射极限和33倍衍射极限。当充电电压降至26kV,即降低腔内介质的增益时,它们的发散角分别是20倍和5倍衍射极限。表明了具有衍射极限的模式建立时间受放大率、腔长以及饱和效应的影响。要得到衍射极限光,其衍射极限光的建立时间必须小于饱和时间。     

惰性气体化学的新进展

汇集了惰性气体化学30年来尤其是近10年(1982—1992)所取得的进展和研究成果。10年来,人们对惰气氟化物的氧化和氟化性质进行了广泛的研究;合成了许多惰气加成物,并详细研究了它们的结构和性质;发展了xe—O、Xe—N、Kr—O、Kr—N键化合物的合成方法,并对它们的性质和结构进行了表征。     

Investigation of stimulated Brillouin scattering for broadband KrF laser

Stimulated Brillouin scattering (SBS) numerical mode for broadband multimode KrF laser pump with optical breakdown has been built up in this paper. The basic premises of the model are that KrF spectrum is composed of an umber of lines and SBS arises from these lines with coupling to some extent. The broadband SBS threshold strongly depends on pump bandwidth. SBS and optical breakdown occur nearly simultaneously when broadband SBS and breakdown have the same threshold. The decrease of saturation reflectivity for broadband pump radiation is explained with this model. Experimental results agree well with the model.     

Electron impact ionization of large krypton clusters

We show that the detection of ionization of very large van der Waals clusters in a pulsed jet or a beam can be realized by using a fast ion gauge. Rapid positive feedback electron impact ionization and fragmentation processes, which are initially ignited by electron impact ionization of the krypton clusters with the electron current of the ion gauge, result in the appearance of a progressional oscillation-like ion spectrum, or just of a single fast event under critical conditions. Each line in the spectrum represents a correlated explosion or avalanche ionization of the clusters. The phenomena have been analysed qualitatively along with a Rayleigh scattering experiment of the corresponding cluster jet.     

激光气体靶产生的类氖氪离子4d-2p共振跃迁其类Na 3l4l′双电子伴线的研究

用相对论多组态(HXR)方法,详细计算了类Ne氪离子4d-2p类Na3l4l′双电子伴线波长和强度因子,并模拟了实验光谱,解释了最新利用激光气体靶产生的0.525～0.555nm范围的氪X-Ray光谱,计算结果与实验符合得相当好。此外,还讨论了组态相互作用对双电子伴线结构的影响。     

电子束泵浦百焦耳级准分子激光实验研究

利用“闪光二号”相对论电子束加速器研制了百焦耳级ＸｅＣｌ和ＫｒＦ准分子激光器，激光器激活体积２４ｌ，输出口径２０×２０ｃｍ２，泵浦功率密度１．５～２．０ＭＷ／ｃｍ３。ＸｅＣｌ激光器最大能量１３６Ｊ，波长３０８ｎｍ，脉宽５０～１００ｎｓ，峰值功率１．５ＧＷ，采用虚共焦非稳腔技术，束散角达１．３ｍｒａｄ；ＫｒＦ激光最大能量１５７Ｊ，波长２４８ｎｍ，脉宽８０～１００ｎｓ，峰值功率２ＧＷ。     

直接进样气相色谱-质谱法分析大气中的氪和氙

大气中氪和氙体积比浓度的测量对于氪-85和放射性氙同位素监测具有重要意义。本实验设计了一套集成定量稀释功能的可调样量进样装置,对质谱检测器的工作参数进行了实验优化,确定了灯丝电离能量70 eV、灯丝发射电流40 mA、推斥极电压27 mV、离子聚焦电压85 mV和透镜补偿电压20 V等最佳工作条件。建立了空气样品直接进样条件下氪和氙的气质联用分析方法,氪和氙的最低可检测浓度分别为3.3×10-8(V/V)和2.6×10-9(V/V)。同时应用本方法测量了实验室所处开放空间大气中氪和氙的体积比浓度,分别为1.1×10-6(V/V)和9.3×10-8(V/V),相对合成标准不确定度分别为2.38%和3.15%。     

Interaction Study of Guest with Host in Clathrate Hydrate

Lattice dynamical simulations of noble gas hydrate structuresⅠandⅡhave been performed. Potential energies were investigated to study the influence of guest species on the stability of the hydrate structure.Results show that when the diameter of inclusion molecules is between 3(?)and 4.2(?),such as Ar and Kr,the critical role of the 5~(12)cage in the stabilization of hydrates becomes effective.For Xe hydrates SⅠand SⅡ,with the help of lattice dynamical calcnlations,the modes attributions are identified directly.We proposed the resonant effect of the fingerprint frequency at about 7 meV and 10 meV which arise from the coupling of Xe molecules in the 5~(12)cage with the host lattice.     

慢电子与Kr,Xe和Rn原子弹性散射截面的计算

根据文献〔1〕中提出的慢电子散射的等效势模型,本文采用Slater波函数来描述原子核外电子的形为,导出了入射电子与Kr、Xe和Rn原子之间较为简单的等效势。对慢电子与Kr、Xe和Rn的弹性散射总截面、动量转移截面和微分散射截面进行了计算。对e-Kr和e-Xe的散射,我们的计算结果与其他理论和实验数据符合的较好。对于e-Rn散射,我们发现也存在着Ramsauer-Townsend效应。研究表明,本方法特别适用于慢电子与复杂原子之间的散射。