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31.
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Abstract: The cross sections of ee-→π+π-hc at center-of-mass energies from 3.90 to 4.42 GeV were measured by the BESIII and the CLEO-c experiments. Resonant structures are evident in the ee-→π+π-hc line shape. The fit to the line shape results in a narrow structure at a mass of (4216±18) MeV/c2 and a width of (39±2) MeV, and a possible wide structure of mass (4293±9) MeV/c2 and width (222=k67) MeV. Here, the errors are combined statistical and systematic errors. This may indicate that the Y(4260) state observed in ee-→π+π-J/ψ has a fine structure in it.  相似文献   
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Extra-large-pore zeolites for processing large molecules have long been sought after by both the academia and industry. However, the synthesis of these materials, particularly extra-large-pore pure silica zeolites, remains a big challenge. Herein we report the synthesis of a new extra-large-pore silica zeolite, designated NUD-6, by using an easily synthesized aromatic organic cation as structure-directing agent. NUD-6 possesses an intersecting 16×8×8-membered ring pore channel system constructed by four-connected (Q4) and unusual three-connected (Q3) silicon species. The organic cations in NUD-6 can be removed in nitric acid to yield a porous material with high surface area and pore volume. The synthesis of NUD-6 presents a feasible means to prepare extra-large pore silica zeolites by using assembled aromatic organic cations as structure-directing agents.  相似文献   
35.
Hot carriers (HCs) and thermal effects, stemming from plasmon decays, are crucial for most plasmonic applications. However, quantifying these two effects remains extremely challenging due to the experimental difficulty in accurately measuring the temperature at reaction sites. Herein, we provide a novel strategy to disentangle HCs from photothermal effects based on the different traits of heat dissipation (long range) and HCs transport (short range), and quantitatively uncover the dominant and potential-dependent role of photothermal effect by investigating the rapid- and slow-response currents in plasmon-mediated electrochemistry at nanostructured Ag electrode. Furthermore, the plasmoelectric surface potential is found to contribute to the rapid-response currents, which is absent in the previous studies.  相似文献   
36.
《Comptes Rendus Chimie》2014,17(7-8):687-700
The influence of the presence of H2O on the contact between carbon, used as model soot, and a model four-way catalyst (1% Pt–10% BaO/Al2O3) was investigated. NO<em>xem> adsorption/TPD cycles at 300 °C together with XRD, XPS and DRIFTS characterizations showed that only surface nitrate species are destabilized by the carbon present in the catalytic bed, leading to a decrease of the NO<em>xem> storage capacity and carbonate species formation. In another way, injection of water in the reactive gas flow decreases also the NO<em>xem> storage capacity of the catalyst, but promotes the formation of stable nitrate species. A non-cumulative effect of carbon and water was observed. It was proposed that a competition between the destabilization, by carbon, of weakly bonded surface nitrate species and the enhancement of bulk nitrate species formation in the presence of water occurs.  相似文献   
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In this paper, the qualitative properties of general nonautonomous Lotka-Volterra n-species competitive systems with impulsive effects are studied. Some new criteria on the permanence, extinction and global attractivity of partial species are established by used the methods of inequalities estimate and Liapunov functions. As applications, nonautonomous two species Lotka-Volterra systems with impulses are discussed.  相似文献   
39.
In this paper, the problem of controller design for Lur’e systems guaranteeing dichotomy is investigated. On the basis of Kalman-Yakubovich-Popov (KYP) lemma and two frequency equalities, a new methodology for the dichotomy analysis of the Lur’e systems is proposed. A linear matrix inequality (LMI) based criterion is derived, which is equivalent to the Leonov’s frequency-domain one, while for the dichotomy analysis and synthesis which is more straightforward than the frequency-domain one. In virtue of this result, a dynamic output feedback controller ensuring the dichotomy property for Lur’e systems is designed. Finally a numerical example is included to demonstrate the validity and the applicability of the proposed approach.  相似文献   
40.
It has been conjectured that the relative phase between strong and electromagnetic amplitudes is universally -90° in charmonium decays. ψ′ decaying into a pseudoscalar pair provides a possibility to test this conjecture. However, the experimentally observed cross section for such a process is depicted by the two-fold integral, which takes into account the initial state radiative (ISR) correction and energy spread effect. Using the generalized linear regression approach, a complex energy-dependent factor is ...  相似文献   
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