表面等离激元量子信息应用研究进展

近年来表面等离激元得到了越来越多的关注和研究,得益于其能把电磁场束缚在金属-介质界面附近的亚波长尺度范围内.本文回顾了近年来表面等离激元在量子信息领域中的理论和实验研究,包括表面等离激元的基本量子性质、表面等离激元量子回路、在量子尺度下与物质的相互作用及其潜在应用.量子表面等离激元开辟了对表面等离激元基本物理性质研究的新方向,可以应用于高度集成化的量子集成光学回路,同时也可以用来增强光与量子发光体的相互作用.     

金属-电介质微盘阵列红外吸收器的光学特性分析

根据亚波长微结构的异常光谱特性,提出了一种"圆形铝盘-圆形SiO_2盘-铝衬底"的二维周期性微结构可调谐红外吸波器.利用有限元算法对其红外光谱反射性质进行了数值模拟,发现该结构对入射的TE或TM光偏振态、在0°~60°大入射角范围内具有良好的吸波效果,共振波长调谐范围4~11μm.用局域等离子体激元共振理论解释了红外吸波机理,证明了所提出的多层微盘结构具有更宽的调谐特性和更好的吸收效率.     

Deep‐UV tip‐enhanced Raman scattering

We report for the first time the tip‐enhancement of resonance Raman scattering using deep ultraviolet (DUV) excitation wavelength. The tip‐enhancement was successfully demonstrated with an aluminum‐coated silicon tip that acts as a plasmonic material in DUV wavelengths. Both the crystal violet and adenine molecules, which were used as test samples, show electronic resonance at the 266‐nm excitation used in the experiments. With results demonstrated here, molecular analysis and imaging with nanoscale spatial resolution in DUV resonance Raman spectroscopy can be realized using the tip‐enhancement effect. Copyright © 2009 John Wiley & Sons, Ltd.     

飞秒激光烧蚀硅材料表面形成周期波纹形貌研究

基于Sipe-Drude模型和表面等离子体激元(SPP)的干涉理论分别对单脉冲飞秒激光诱导硅表面形成低频率周期性波纹进行分析研究.探究了波长800 nm、脉宽150 fs的单个飞秒激光烧蚀硅造成不同激发水平下波纹形貌的变化,考虑到材料的光学性质变化(由Drude模型得到的介电常数变化),引入包含双温方程的电子数密度模型.计算结果表明,Sipe-Drude和SPP理论都适用于分析和解释高激发态下周期性波纹,但Sipe-Drude理论更适合分析更为广泛的周期性波纹结构.同时,波纹延伸方向总是垂直于入射激光偏振方向,其空间周期略小于激光波长,并受到入射激光通量的影响.在激光通量为0.38 J/cm~2时,波纹周期达到最小值.另外,还得到了不同入射角度的波纹周期变化情况,并在不同偏振态下随入射角度增大时波纹周期呈现相反的变化趋势.该研究对于理解飞秒激光造成硅表面形成周期结构及其在加工硅材料领域具有重要参考意义.     

The subwavelength tuned magneto-optical Kerr effect in L1_0-FePt films with perpendicular magnetic anisotropy

For L10-FePt films with strong perpendicular anisotropy covered by arrays of hexagonal close-packed polystyrene spheres(PSSs),fine structures are observed in magneto-optical Kerr rotation spectra in the visible spectral range.The reflection minima are found to be located at the same wavelengths as the Kerr rotation peaks.The Kerr rotation enhancement is attributed to the excitation of both the surface plasmon polariton in the dielectric PSS/metal interface and the guide waves(guide mode)in the PSS array.The two-dimensional PSSs/SiO2/FePt system exhibiting a tunable magneto-optical Kerr effect and a high perpendicular magnetic anisotropy will be helpful for designing and fabricating magneto-optics devices.     

The surface plasmon polariton dispersion relations in a nonlinear-metal-nonlinear dielectric structure of arbitrary nonlinearity

The analytic surface plasmon polaritons(SPPs) dispersion relation is studied in a system consisting of a thin metallic film bounded by two sides media of nonlinear dielectric of arbitrary nonlinearity is studied by applying a generalised first integral approach.We consider both asymmetric and symmetric structures.Especially,in the symmetric system,two possible modes can exist:the odd mode and the even mode.The dispersion relations of the two modes are obtained.Due to the nonlinear dielectric,the magnitude of the electric field at the interface appears and alters the dispersion relations.The changes in SPPs dispersion relations depending on film thicknesses and nonlinearity are studied.     

Optical Tamm state polaritons in a quantum well microcavity with gold layers

A new type of cavity polariton,the optical Tamm state(OTS) polariton,is proposed to be realized by sandwiching a quantum well(QW) between a gold layer and a distributed Bragg reflector(DBR).It is shown that OTS polaritons can be generated from the strong couplings between the QW excitons and the free OTSs.In addition,if a second gold layer is introduced into the bottom of the DBR,two independent free OTSs can interact strongly with the QW excitons to produce extra OTS polaritons.     

Surface Plasmon Polariton Fizeaus Dragging: via Relative Rotational Sensing

A new scheme focusing on the surface plasmon polariton interferometry between the metal and dielectric interface is introduced. The phase shift is measured by using surface plasmon polariton wave, generated at the interface of metallic and dielectric media. The phase shift of SPPs is modi?ed under phase and amplitude control of complex conductivity for interferometry. The control ?elds strongly in?uence the phase shift of SPPs for detection of molecular motion. The phase shift of SPPs is further modi?ed by Plasmon polariton Fizeaus dragging effect. We measure 20%–25%fractional change in delay and their phases shift between two left and right SPPs modes. Our results may have signi?cant applications in sensor interferometer technology.     

在具有强非线性效应的离子晶体中光脉冲传播的孤立子特性

从理论上研究了原胞内存在强离子间非线性相互作用的离子晶体,得出光脉冲在其中的传播具有孤立子特性,并分析了当非线性系数g分别为大于0与小于0时形成的亮孤立子与暗孤立子的具体特征.研究表明,不论非线性系数g取正值还是负值,在纵光学模声子频率ωLO以上频区,光脉冲可形成亮孤立子,在g>0时,在横光学模频率ωTO以下频区可形成暗孤立子;值得注意的是在ωTO—ωLO区间,光脉冲可形成超前型暗孤立子;在g<0时,从ωTO往下临近ωTO有一个由超前型亮孤立子向推迟型暗孤立子的转变区 关键词： 孤立子 极化激元 光脉冲     

采用飞秒激光诱导制备彩色金属

采用脉宽为35～65fs,中心波长为800nm的飞秒脉冲激光对经抛光的镍片进行表面扫描处理,并在金属表面上制备了彩色镍图案;设置不同的激光扫描速度和能量密度扫描处理不锈钢表面,亦制备了彩色图案。介绍了实验过程,分析了实验结果,扫描电子显微镜（SEM）形貌分析显示,经过飞秒激光扫描处理的金属表面出现了纳米量级的激光诱导周期表面结构（NC—LIPSS）,在镍上形成的结构周期约为480—510nm,在不锈钢上形成的结构周期约为480～540nm。