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排序方式: 共有115条查询结果,搜索用时 31 毫秒
81.
Bai Z Blaylock GT Bolton T Browder TE Brown JS Bunnell KO Burnett TH Cassell RE Coffman D Cook V DeJongh F Dorfan DE Drinkard J Dubois GP Eigen G Einsweiler KF Eisenstein BI Freese T Gatto C Gladding G Hauser J Heusch CA Hitlin DG Izen JM Kim PC Labs J Li A Lockman WS Mallik U Matthews CG Mincer AI Mir R Mockett PM Mozley RF Nemati B Odian A Parrish L Partridge R Pitman D Plaetzer SA Richman JD Sadrozinski HF Scarlatella M Schalk TL Schindler RH Seiden A Simopoulos C Stockdale IE Toki W 《Physical review letters》1990,65(11):1309-1312
82.
Coffman D DeJongh F Dubois G Eigen G Hauser J Hitlin DG Matthews CG Mincer A Richman JD Wisniewski WJ Zhu Y Burchell M Dorfan DE Drinkard J Gatto C Hamilton RP Heusch CA Köpke L Lockman WS Partridge R Sadrozinski HF Scarlatella M Schalk TL Seiden A Weinstein AJ Weseler S Xu R Becker JJ Blaylock GT Eisenstein BI Freese T Gladding G Izen JM Plaetzer SA Simopoulos C Spadafora AL Stockdale IE Tripsas B Mallik U Roco M Wang MZ Adler J Bolton T Brient JC Bunnell KO Cassell RE Coward DH Einsweiler KF 《Physical review D: Particles and fields》1990,41(5):1410-1413
83.
Baltrusaitis RM Becker JJ Blaylock GT Brown JS Bunnell KO Burnett TH Cassell RE Coffman D Cook V Coward DH Dado S Del Papa C Dorfan DE Dubois GP Duncan AL Einsweiler KF Eisenstein BI Fabrizio R Gladding G Grancagnolo F Hamilton RP Hauser J Heusch CA Hitlin DG Koepke L Lockman WS Mockett PM Moss L Mozley RF Nappi A Odian A Partridge R Perrier J Plaetzer SA Richman JD Roehrig JR Russell JJ Sadrozinski HF Scarlatella M Schalk TL Schindler RH Seiden A Sleeman JC Spadafora AL Thaler JJ Toki W 《Physical review letters》1985,54(18):1976-1979
84.
采用含时密度泛函理论方法(TDDFT)计算了IB族过渡金属及第5周期的金属杂化偶氮苯生色团的二阶非线性光学极化率。研究了金属杂化偶氮苯生色团的电子激发跃迁。结果表明, 与金属离子络合后的杂化偶氮苯生色团, 二阶非线性光学极化率明显改变, 是金属的推拉电子效应的结果。IB族金属的在原有机偶氮苯共轭体系的电荷转移方向的强拉电子效应, 增大了电荷转移范围, 使二阶非线性光学极化率增大。与Nb络合的杂化生色团, 沿原电荷转移相反的方向拉动电荷, 电荷转移跃迁局限于金属离子附近, 未能产生大的激发跃迁偶极矩, 体系的二阶非线性光学响应因而降低。激发跃迁能量是另一个主要影响因素, 同一类跃迁中, 金属杂化生色团的跃迁能量越低, 其二阶非线性光学响应就越大。络合Rh的生色团与Nb杂化生色团类似, 电荷转移跃迁范围都比较小, 同时由于Rh与羧基结合时几乎垂直羧基平面, 电荷同时沿X, Y方向转移跃迁, 属于二维电荷转移类型。 相似文献
85.
研究了具有欠完整立方烷构型的过渡金属原子簇分子的二阶非线性光学性质。利用TDDFT方法计算了选取的簇分子及相应模拟构造分子的静态和动态的一阶非线性光学超级化率(ijk);并计算了不同金属、桥原子和配体以及簇芯对该类化合物一阶超级化率的影响。选取其中的一个簇分子为基本模型,分析了该分子的电子结构和分子轨道,在微观水平上阐述了其非线性光学性质的可能起源。认为由过渡金属和硫原子组成的簇芯和与桥原子相连的配体对该类簇合物的二阶非线性光学性质的起决定性的作用。 相似文献
86.
Glucose is required to maintain high ATP-levels for the energy-utilizing steps during PDT-induced apoptosis 总被引:1,自引:0,他引:1
Photodynamic therapy (PDT) may trigger apoptosis or necrosis in cancer cells. Several steps in the induction and execution of apoptosis require high amounts of adenosine-5'-triphosphate (ATP). Because the mitochondrial membrane potential (delta psi) decreases early in apoptosis, we raised the question about the mechanisms of maintaining a sufficiently high ATP level. We therefore monitored delta psi and the intracellular ATP level of apoptotic human epidermoid carcinoma cells (A431) after photodynamic treatment with aluminum (III) phthalocyanine tetrasulfonate. A maximum of caspase-3-like activity and nuclear fragmentation was found at fluences of about 4 J cm(-2). Under these conditions apoptotic cells reduced delta psi rapidly, while the ATP level remained high for 4-6 h after treatment for cells supplied with glucose. To analyze the contribution of glycolysis to the energy supply during apoptosis, experiments were carried out with cells deprived of glucose. These cells showed a rapid drop of ATP content and neither caspase activation nor nuclear fragmentation could be detected. We conclude that the use of glucose as a source of ATP is obligatory for the execution of PDT-induced apoptosis. 相似文献
87.
LIAO Rong-Baoa b LIU Cai-Pinga b SA Rong-Jiana LI Fu-Juna b HE Jian-Ganga b WU Ke-Chena② a 《结构化学》2008,27(6):724-732
The ground-state dipole moments and second-order nonlinear optical (NLO) properties of a series of one-dimensional (1D) chromophores with donor-bridge-acceptor (D-B-A) structures have been investigated by using the second-order MФller-Plesset (MP2) and density functional theory (DFT) methods with the basis set of 6-31+G(d). According to the calculated results, the relationship between the molecular static first hyperpolarizability (βμ) and the directions of electron transition has been summarized. In terms of the sign of βμ, these 1D organic chromophores were classified into two categories: type Ⅰ with negative βμ and type Ⅱ bearing positive βμ. The analyses show that the remarkable difference of the first hyperpolarizabilities between Ⅰ and Ⅱ chromophores is associated mainly with the electrostatic interaction between terminal groups and the transport electrons in excited states. Moreover, different from the popular viewpoint, the obtained results also show that most of this series of 1D D-B-A molecules are more charge-separated in the ground states than in the excited states. As a whole, this theoretical investigation, to some extent, can be considered as a useful reference in designing the NLO chromophores with large first hyperpolarizabilities. 相似文献
88.
用描写相对论性核 核碰撞的LUCIAE模型及相应的MonteCarlo事例产生器分析了WA97最近发表的 1 5 8AGeVp Pb和Pb Pb碰撞中单奇异粒子 (Λ ,Λ)和多奇异粒子 (Ξ-,Ξ-,Ω-,Ω-)的多重数和横质量分布 .由于LUCIAE模型包含了弦碎裂微观过程中奇异夸克压低因子随碰撞体系的能量、中心度和质量的增大而增大 ,以及由它导致的相对论性核 核碰撞宏观过程中奇异粒子产额随上述三因素之增而增的物理机制 ;LUCIAE模型计算结果能较好描写WA97实验所揭示的相对论性核 核碰撞中奇异粒子产额随中心度之增而增和奇异粒子增强随奇异夸克数之增而增的实验事实 ,以及单奇异和多奇异粒子的横质量分布 . 相似文献
89.
Ben-Hao SA 《理论物理通讯》1997,27(4):507-510
We use the event generator LUClAE to analyze the WA85 data of ratio of Ω- to Ω- in reaction (200A GeV/c)S + W. The result indicates that the reproduction of WA85 data might be achieved in hadronic rescattering regime of LUCIAE and might need not to rely on the formation of QGP. 相似文献
90.
The dependence of phase transition,associated with the disassembly of hot nuclei,on the mass number of hot nuclei is investigated.By studying six hot nuclei ranging from 56Ni* to 238U*,we find that in the curves of excitation energy of hot nuclei vs.Thermodynamic temperature T(E*) of 63Cu* and heavier ones there are always two temperature plateaus,but in T(E*) of 56Ni the first temperature plateau (at lower excitation energy) shrinks into a kink. 相似文献