二阶级联声光双稳态超浑沌的周期驱动控制

本文提出了对二阶级联声光双稳态超浑沌进行外周期激励,从而实现了对其进行有效控制.     

Spectral deep learning for prediction and prospective validation of functional groups

State-of-the-art identification of the functional groups present in an unknown chemical entity requires the expertise of a skilled spectroscopist to analyse and interpret Fourier transform infra-red (FTIR), mass spectroscopy (MS) and/or nuclear magnetic resonance (NMR) data. This process can be time-consuming and error-prone, especially for complex chemical entities that are poorly characterised in the literature, or inefficient to use with synthetic robots producing molecules at an accelerated rate. Herein, we introduce a fast, multi-label deep neural network for accurately identifying all the functional groups of unknown compounds using a combination of FTIR and MS spectra. We do not use any database, pre-established rules, procedures, or peak-matching methods. Our trained neural network reveals patterns typically used by human chemists to identify standard groups. Finally, we experimentally validated our neural network, trained on single compounds, to predict functional groups in compound mixtures. Our methodology showcases practical utility for future use in autonomous analytical detection.

A new multi-label deep neural network architecture is used to combine Infrared and mass spectra, trained on single compounds to predict functional groups, and experimentally validated on complex mixtures.     

Mo/Si multilayers used for the EUV normal incidence solar telescope

This paper first reviews an EUV normal incidence solar telescope that we have developed in our lab. The telescope is composed of four EUV telescopes and the operation wavelengths are 13.0 nm, 17.1 nm, 19.5 nm, and 30.4 nm. These four wavelengths, fundamental to the research of the solar activity and the atmosphere dynamics, are always chosen by the EUV normal incidence solar telescope. In the EUV region, almost all materials have strong absorption, so optics used in this region must be coated by the multila...     

海洋大气气溶胶光学模型参数的相关性研究

气溶胶光学模型参数在气溶胶遥感和气候强迫研究中都具有重要的作用.通过对全球近90个气溶胶自动观测网(AERONET)的海洋站点数据进行筛选、分类和分析,发现了气溶胶模型的中值半径及其标准偏差间的负相关性,并给出了经验关系.利用该关系对现行中分辩率成像光谱仪(MODIS)海洋气溶胶模型进行了评估,并指出了该模型存在的不足...     

A 2‐Tyr‐1‐carboxylate Mononuclear Iron Center Forms the Active Site of a Paracoccus Dimethylformamidase

N,N‐dimethyl formamide (DMF) is an extensively used organic solvent but is also a potent pollutant. Certain bacterial species from genera such as Paracoccus, Pseudomonas, and Alcaligenes have evolved to use DMF as a sole carbon and nitrogen source for growth via degradation by a dimethylformamidase (DMFase). We show that DMFase from Paracoccus sp. strain DMF is a halophilic and thermostable enzyme comprising a multimeric complex of the α₂β₂ or (α₂β₂)₂ type. One of the three domains of the large subunit and the small subunit are hitherto undescribed protein folds of unknown evolutionary origin. The active site consists of a mononuclear iron coordinated by two Tyr side‐chain phenolates and one carboxylate from Glu. The Fe³⁺ ion in the active site catalyzes the hydrolytic cleavage of the amide bond in DMF. Kinetic characterization reveals that the enzyme shows cooperativity between subunits, and mutagenesis and structural data provide clues to the catalytic mechanism.     

Acid-base cooperativity of heterogeneous catalyst containing acidic framework and sterically hindered base for aldol condensation

A bifunctional heterogeneous catalyst containing two mutually incompatible acidic and basic sites,which exhibits cooperative catalytic behavior in the aldol condensation of acetone and various aldehydes,was synthesized by postgrafting of 1,5,7- triazabicyclo[4.4.0]dec-5-ene(TBD,a sterically hindered organic base) onto Al-MCM-41 molecular sieve.     

光线量子理论研究薄膜介质光场能量分布

因为光线量子力学方程的光线哈密顿算符不表示能量,而是具有可变折射率的物理意义,因此应用光线量子论讨论波导中光场能量分布是一个有待研究的问题.本文借鉴量子力学几率密度和几率密度矢量概念推导出光场能量分布的普遍性公式,并证明流线结构的光场中守恒定律的成立.     

HpD肿瘤定位组份的时间分辨荧光光谱研究

采用微微秒激光作激发源的时间相关单光子计数系统测量了血卟啉衍生物的肿瘤定位组分(TLF)在缓冲液中不同阳离子表面活性剂浓度下的荧光衰减波形I(t)和时间分辨光谱I(λ,t).     

半导体微碟激光器设计原理与工艺制作

用经典量子电动力学理论初步研究了半导体碟型微腔激光器的设计原理，采用光刻、反应离子刻蚀和选择化学腐蚀等现代微加工技术制备出抽运阈值功率很低用品质因数很高的低温光抽运InGaAs/InGaAsP多量子阱微碟激光器。这种激光器制作工艺简单，对有效光子状态密度调制较大，是比较理想的半导体微腔激光器。     

温度涨落和波长偏离对衍射透镜性能的影响

根据菲涅耳衍射透镜的特点,阐明了温度色散和波长色散的概念,并建立了相应的数学表达式,给出了衍射效率与温度和波长的关系式,在此基础上做了较为全面系统的理论和数值分析,评估了温度场发生变化以及使用波长和设计波长发生偏离对衍射透镜性能的影响程度.结果表明:波长偏离对衍射透镜性能的影响要比温度涨落明显得多,其中,波长色散具有非线性特征.