On the NN final-state interaction in the <Superscript>16</Superscript>O (e,e<Superscript>′</Superscript>pp) reaction

The influence of the mutual interaction between the two outgoing nucleons (NN-FSI) in the ¹⁶O(e, e'pp) reaction has been investigated. Results for various kinematics are discussed. In general, the effect of NN-FSI depends on kinematics and the chosen final state in the excitation spectrum of ¹⁴C. Received: 19 December 2002 / Accepted: 6 February 2003 / Published online: 15 April 2003     

First measurements of the 16O(e, e'pn)14N reaction

This paper reports on the first measurement of the ¹⁶O(e, e'pn)¹⁴N reaction. Data were measured in kinematics centred on a super-parallel geometry at energy and momentum transfers of 215MeV and 316MeV/c. The experimental resolution was sufficient to distinguish groups of states in the residual nucleus but not good enough to separate individual states. The data show a strong dependence on missing momentum and this dependence appears to be different for two groups of states in the residual nucleus. Theoretical calculations of the reaction using the Pavia code do not reproduce the shape or the magnitude of the data. An erratum to this article is available at.     

On the treatment of the Δ-contributions in electromagnetic pp-knockout reactions

The treatment of the Δ-current and its contribution in the exclusive ¹⁶O (e, e'pp)¹⁴C and ¹⁶O (γ, pp)¹⁴C knockout reactions are investigated in combination with the effects of correlations. Different parametrizations of the effective Δ-current and different treatments of correlations in the two-nucleon overlap function are considered. The results are presented and discussed for a suitable choice of kinematics. It is found that the investigation of different mutually supplementing kinematics is necessary to resolve the uncertainties in the theoretical ingredients and extract clear and unambiguous information on correlations.     

A new cluster model interpretation of the anomalous lifetime of <Superscript>14</Superscript>C

A new cluster model solution to the long-standing nuclear structure problem of describing the anomalously long lifetime of ¹⁴C is presented. Related beta-decay data for ¹⁴O to states in ¹⁴N, gamma-decay data between low-lying positive parity states in ¹⁴N and the elastic and inelastic magnetic dipole electron scattering from ¹⁴N data are all shown to be very accurately described by the model. The shapes of the beta spectra for the A = 14 system are also well reproduced by the model. The model invokes four-nucleon tetrahedral symmetric spatial correlations arising from three- and four-nucleon interactions, which yields a high degree of SU(4) singlet structure for the clusters and a tetrahedral intrinsic shape for the doubly magic ¹⁶O ground state. The large quadrupole moment of the ¹⁴N ground state is obtained here for the first time and arises because of the almost 100% d-wave deuteron-like-hole cluster structure inherent in the model.     

Single Folding Optical Potential for Elastic Scattering of Protons from <Superscript>14</Superscript>N and <Superscript>16</Superscript>O in a Wide Range of Energies

Available experimental data for protons elastically scattered from ¹⁴N and ¹⁶O target nuclei are reanalyzed within the framework of single folding optical potential (SFOP) model. In this model, the real part of the potential is derived on the basis of single folding potential. The renormalization factor N _r is extracted for the two aforementioned nuclear systems. Theoretical calculations fairly reproduce the experimental data in the whole angular range. Energy dependence of real and imaginary volume integrals as well as reaction cross sections are discussed.     

Spectroscopy of <Superscript>17</Superscript>C and (sd )<Superscript>3</Superscript> structures in heavy carbon isotopes

The structure of ¹⁷C has been investigated using the three-neutron transfer reaction (¹²C,⁹C) on a ¹⁴C target at 231MeV incident energy, the reaction Q-value is Q ₀ = - 46.930MeV. Eleven new states up to 16.3MeV excitation energy were identified. The same reaction has also been used on a ¹²C target ( Q ₀ = - 38.787MeV), and excited states in ¹⁵C up to 19MeV were observed. In ¹⁷C the three transferred neutrons populate (sd )³ configurations on the ¹⁴C core. The comparison of levels populated by the (¹²C,⁹C) reaction in ¹⁷C, ¹⁶C and ¹⁵C reveals a strong similarity of their properties. This concerns especially nine states in each of the three carbon isotopes, which show practically the same excitation energies except a constant mean shift of +5.82MeV for ¹⁶C and +6.65MeV for ¹⁵C with respect to ¹⁷C. The triples of states from the three isotopes, which correspond to each other, have also similar widths and cross-section ratios. It is concluded that the same (sd )³ structures are populated in the three carbon isotopes. The observed levels of ¹⁷C are also compared to the levels of ¹⁹O with known assignments and to shell model calculations, and their decay properties are discussed.     

Study of the isobar configurations in the <Superscript>12</Superscript>C and <Superscript>16</Superscript>O ground states

Experimental research on positive-pion photoproduction on the oxygen nucleus in the ¹⁶O(γ, π⁺p) reaction at high recoil momenta of the residual nuclear system was performed. The yield for the ¹⁶O(γ, π⁺p) reaction was analyzed using a model that takes Δ-isobar configurations in nuclei ground states into account, together with the earlier-measured yield of the¹²C(γ, π⁺p) reaction. The estimated number of isobars per nucleon N _Δ = 0.012 ± 0.005 was obtained for the ¹²C nucleus, and ¹⁶O N _Δ = 0.018 ± 0.004 was obtained for the ¹⁶O nucleus.     

Description of elastic scattering in the <Superscript>16</Superscript>O + <Superscript>16</Superscript>O and <Superscript>16</Superscript>O + <Superscript>12</Superscript>C systems

The objective of the present study was to describe more precisely experimental data on elastic scattering in the ¹⁶O + ¹⁶O system at E _lab = 124, 145, 250, 350, and 480 MeV and in the ¹⁶O + ¹²C system at E _lab = 132, 170, 181, 200, 230, 260, and 281 MeV. The role of exchange interaction in the region of backward angles is investigated. The coefficient of incompressibility of nuclear matter is estimated at K = 205 MeV ± 15%.     

Nuclear rainbow in the elastic scattering of <Superscript>16</Superscript>O nuclei on carbon isotopes

An investigation of refractive effects in heavy-ion scattering is continued. For the elastic scattering of ¹⁶O nuclei on a ¹³C target at E(¹⁶O) = 132 MeV, the differential cross sections are measured for the first time in addition to previous measurements for targets from the carbon isotopes ¹²C and ¹⁴C. Airy structures that are similar for all isotopes and which have close cross sections are observed and are found to be consistent with the energy systematics of Airy minima that were obtained previously. The volume integrals of the real and imaginary parts of the optical potentials found in the present study are nearly identical for all of the isotopes considered here and are also in good agreement with the systematics obtained previously.     

Studies of multi-nucleon transfer reactions in <Superscript>90</Superscript>Zr(<Superscript>18</Superscript>O,X) and <Superscript>90</Superscript>Zr(<Superscript>16</Superscript>O,X)

Multi-nucleon transfer reactions in ¹⁸O + ⁹⁰Zr and ¹⁶O + ⁹⁰Zr have been studied at an incident energy of 90 MeV. The energy spectra and angular distributions are measured. The data have been analyzed to obtain cross-section dependence on the number of nucleons transferred and on the ground-state Q-values. In the ⁹⁰Zr(¹⁸O, X); X = ¹⁶O, ^17,16,15,14N, ^14,13,12C, ^12,11,10B, ^10,9,7Be and ^7,6Li reactions, 2n and 2n-correlated transfer cross-sections are observed to be enhanced as compared to the ¹⁶O + ⁹⁰Zr reaction. A detailed comparison in the multi-particle stripping and elastic-scattering cross-section between these two systems are made in order to investigate the possible influence of the two valence neutrons in ¹⁸O nucleus. Diffractional model DWBA calculations, based on the direct surface transfer model, have been performed to understand the reaction mechanism of multi-nucleon transfer to continuum.Received: 12 September 2002, Revised: 24 September 2003, Published online: 27 January 2004PACS: 25.70.Hi Transfer reactions - 25.70.Bc Elastic and quasielastic scattering     

Investigations into the alpha-decay of <Superscript>195</Superscript>At

The low-energy nuclear structure and decay properties of the neutron-deficient isotopes ¹⁹⁵At and ¹⁹¹Bi have been studied. ¹⁹⁵At was produced in the reaction ¹⁴²Nd(⁵⁶Fe,p2n)¹⁹⁵At and ¹⁹¹Bi as the daughter activity of ¹⁹⁵At. The activities were implanted in a position-sensitive silicon detector after being separated from the primary beam by a gas-filled recoil separator. The 1/2⁺ intruder state was determined to be the ground state in ¹⁹⁵At with an alpha-decay energy of E _α = 6953(3) keV and a half-life T _1/2 = 328(20) ms. Another state with an alpha-decay energy E _α = 7075(4) keV and a half-life T _1/2 = 147(5) ms was found to decay to a 148.7(5) keV excited state in ¹⁹¹Bi for which a spin and parity of 7/2^- were deduced. Consequently, the same 7/2^- character was assigned to the initial state at 32(7) keV in ¹⁹⁵At on the basis of unhindered alpha-decay. The 9/2^- state, being the ground state in heavier odd-mass astatine isotopes, was not observed. Received: 16 September 2002 / Accepted: 19 December 2002 / Published online: 25 March 2003 RID="a" ID="a"e-mail: heikki.kettunen@phys.jyu.fi RID="b" ID="b"Present address: Laboratory of Radiochemistry, P.O. Box 55, FIN-00014, University of Helsinki, Finland. RID="c" ID="c"Present address: Radiation and Nuclear Safety Authority, P.O. Box 14, FIN-00881 Helsinki, Finland. Communicated by W. Henning     

EPR and Optical Studies of Mo<Superscript>5+</Superscript> Ions in Lithium Molybdoborate Glasses

Electron paramagnetic resonance (EPR) and optical absorption studies of Li₂O–MoO₃–B₂O₃ with varying concentrations of Li₂O, MoO₃ and B₂O₃ have been carried out at room temperature. Two series of glasses, one with constant MoO₃ (CM) and another with constant borate (CB), have been investigated. Characteristic EPR spectra of Mo⁵⁺ have been observed centered around g ≅ 2.00, which are attributed to Mo⁵⁺ ion in an octahedral coordination sphere with an axial distortion. The spectra also show strong dependence on the concentration of Li₂O and B₂O₃. Spin concentrations (N) and magnetic susceptibilities (χ) have been calculated. In the CM series, the N values decrease with increasing Li₂O content up to 30 mol%, while in the CB series variation of N is found to increase initially up to 20 mol%, and with further increase in the Li₂O content the N values tend to decrease. The variation of magnetic susceptibilities is almost similar to that observed with the variation of N. From the optical absorption spectra, an absorption edge (α) has been evaluated. In the CM series, the values of α show a blueshift. On the other hand, in the CB series a redshift is observed. The observed variations in spectral parameters are explained by considering the molybdoborate network. Addition of Li₂O to the CM and CB series results in modification of [MoO_6/2]⁰ → [MoOO_5/2]⁻ and [BO_3/2]⁰ → [BO_4/2]⁻ → [BOO_2/2]⁻ groups, respectively, leading to creation of nonbridging oxygens. The optical basicity of the glasses has been evaluated in both the CM and the CB glasses. The optical basicity can be used to classify the covalent-to-ionic ratios of the glass, since an increasing optical basicity indicates decreasing covalency. It is observed that the covalency between Mo⁵⁺ ions and oxygen ligands increases in the CB series, whereas in the CM series the covalency between Mo⁵⁺ ions and oxygen ligands decreases. Authors' address: R. P. Sreekanth Chakradhar, Glass Technology Laboratory, Central Glass and Ceramic Research Institute, Kolkata 700032, India     

Density-constrained time-dependent Hartree-Fock calculation of <Superscript>16</Superscript>O + <Superscript>208</Superscript>Pb fusion cross-sections

We present a fully microscopic study of the ¹⁶O + ²⁰⁸Pb fusion using the density-constrained time-dependent Hartree-Fock theory. The calculated fusion cross-sections are in good agreement with the experimental data for the entire energy range indicating that the incorporation of dynamical effects is crucial in describing heavy-ion fusion.     

Decay of quasimolecular states in <Superscript>26</Superscript>Mg

A resonance-like structure in the excitation function for elastic and inelastic ¹⁴C + ¹²C interactions is investigated. Angular distributions for the ¹⁴C(¹²C,¹⁰Be)¹⁶O reaction at center-of-mass energies of 21.1, 23.5, and 24.6 MeV are obtained. It is shown that the angular distribution at the maximum cross section corresponds to the 12⁺ resonance and the ¹⁰Be + ¹⁶O structure. The position of the level with an angular momentum of 10⁺ is predicted.     

New insight in the level structure of <Superscript>153</Superscript>Er

The high-spin level structure of the ¹⁵³Er nucleus has been reinvestigated by in-beam γ-ray and electron spectroscopy with (¹⁴N,pxn) reaction. Excitation energies, spin and parity assignments are unambiguously established for the two lowest isomers T _1/2≃ 380 ns and T_1/2\simeq 10 ns. The characteristics of the third one (T _1/2≃ 250 ns) at 5.2 MeV are still questionable but its main decay modes are better known. An extension of the level scheme is proposed up to 8.4 MeV.Experimental results have been discussed in terms of shell model multiplets and compared with the other structures observed in N=85 neighbouring nuclei. Received: 8 November 1999 / Revised version: 13 December 1999     

Observation of complete- and incomplete-fusion components in <Superscript>159</Superscript>Tb , <Superscript>169</Superscript>Tm ( <Superscript>16</Superscript>O,x) reactions: Measurement and analysis of forward recoil ranges at E/A ≈ 5-6 MeV

With a view to study complete- and incomplete-fusion components in ¹⁵⁹Tb , ¹⁶⁹Tm ( ¹⁶O , x reactions, experiments have been carried out at the Inter-University Accelerator Center, New Delhi, India using the 15UD Pelletron accelerator facilities. The forward mean recoil ranges for some radio-nuclides; ^168m Lu , ¹⁶⁷Lu , ¹⁶⁷Yb , ¹⁶⁶Tm produced in the ¹⁶O$ + $¹⁵⁹Tb system at ≈ 90 MeV, and ¹⁷⁹Re , ¹⁷⁷Re , ¹⁷⁷W , ¹⁷⁸Ta and ¹⁷⁷Hf produced in the ¹⁶O$ + $¹⁶⁹Tm system at ≈ 87 MeV have been measured. The recoil-catcher activation technique followed by off-line γ -spectrometry has been employed in the present work. The analysis of forward mean ranges for different radio-nuclides has been done in the framework of the degree of linear momentum transfer from projectile to target nucleus by adopting break-up fusion model considerations. Different complete- and incomplete-fusion components, which may be attributed to the fusion of ¹⁶O and/or ¹²C and ⁸Be transfer from the ¹⁶O projectile to the target nucleus have been observed. An attempt has also been made to separate out the relative percentage contributions of complete- and incomplete-fusion components using experimentally measured forward recoil ranges. The complete-fusion contributions deduced from recoil range distribution are found to be consistent with the prediction of the theoretical model code PACE. The analysis of data indicates the complete- and incomplete-fusion competition for both the systems at the given energies.     

Nuclear quadrupole moments of 5/2<Superscript>-</Superscript> and 9/2<Superscript>-</Superscript> states in <Superscript>169</Superscript>Ta

The nuclear spectroscopic quadrupole moments for the πh_9/25/2^-, 1/2^-[541] and the πh_11/29/2^-, 9/2^-[514] isomeric states in ¹⁶⁹Ta have been measured employing the time differential perturbed angular-distribution technique following the nuclear reaction ¹⁵⁹Tb(¹⁶O, 6nγ)¹⁶⁹Ta at beam energy 104 MeV. The ratio of the intrinsic quadrupole moments has been derived as 1.87(13) from the measured quadrupole precession frequencies of the corresponding states. The model-independent analysis of the equilibrium deformation indicates strong prolate- and oblate-driving nature of the 1/2^-[541] and 9/2^-[514] orbitals in ^169,171Ta isotopes, respectively.