On the treatment of the Δ-contributions in electromagnetic pp-knockout reactions

The treatment of the Δ-current and its contribution in the exclusive ¹⁶O (e, e'pp)¹⁴C and ¹⁶O (γ, pp)¹⁴C knockout reactions are investigated in combination with the effects of correlations. Different parametrizations of the effective Δ-current and different treatments of correlations in the two-nucleon overlap function are considered. The results are presented and discussed for a suitable choice of kinematics. It is found that the investigation of different mutually supplementing kinematics is necessary to resolve the uncertainties in the theoretical ingredients and extract clear and unambiguous information on correlations.     

Electromagnetic proton-neutron knockout off <Superscript>16</Superscript>O : New achievements in theory

Results for the cross-sections of the exclusive ¹⁶O(e, e'pn)¹⁴N and ¹⁶O(γ, pn)¹⁴N knockout reactions are presented and discussed in different kinematics. In comparison with earlier work, a complete treatment of the center-of-mass (CM) effects in the nuclear one-body current is considered in connection with the problem of the lack of orthogonality between initial bound and final scattering states. The effects due to CM and orthogonalization are investigated in combination with different treatments of correlations in the two-nucleon overlap function and for different parametrizations of the two-body currents. The CM effects lead in super-parallel kinematics to a dramatic increase of the ¹⁶O(e, e'pn) cross-section to the 1₂ ⁺ excited state (3.95MeV) of ¹⁴N . In all the situations considered the results are very sensitive to the treatment of correlations. A crucial role is played by tensor correlations, but also the contribution of long-range correlations is important.     

Polarization observables in (γ,NN) reactions

The formalism of ( γ, NN) reactions is given where the incident photon is polarized and the outgoing-nucleon polarization is detected. Sixteen structure functions and fifteen polarization observables are found in the general case, while only eight structure functions and seven polarization observables survive in coplanar kinematics. Numerical examples are presented for the ¹⁶O(γ, np) and ¹⁶O(γ, pp) reactions. The transitions to the ground state of ¹⁴C and ¹⁴N are calculated in a model where realistic short-range and tensor correlations are taken into account for the np pair, while short-range and long-range correlations are included in a consistent way for pp pairs. The effects of the one-body and two-body components of the nuclear current and the role of correlations in cross-sections and polarizations are studied and discussed. Received: 7 June 2001 / Accepted: 26 September 2001     

Study of the isobar configurations in the <Superscript>12</Superscript>C and <Superscript>16</Superscript>O ground states

Experimental research on positive-pion photoproduction on the oxygen nucleus in the ¹⁶O(γ, π⁺p) reaction at high recoil momenta of the residual nuclear system was performed. The yield for the ¹⁶O(γ, π⁺p) reaction was analyzed using a model that takes Δ-isobar configurations in nuclei ground states into account, together with the earlier-measured yield of the¹²C(γ, π⁺p) reaction. The estimated number of isobars per nucleon N _Δ = 0.012 ± 0.005 was obtained for the ¹²C nucleus, and ¹⁶O N _Δ = 0.018 ± 0.004 was obtained for the ¹⁶O nucleus.     

Photon-induced two-nucleon knockout reactions to discrete final states

Cross sections and photon asymmetries of the ¹⁶O(γ, pn)¹⁴N and ¹⁶O(γ, pp)¹⁴C knockout reactions are calculated for transitions to the low-lying discrete final states of the residual nucleus in the photon-energy range between 100 and 400 MeV. Exclusive reactions may represent a test of reaction mechanisms and a promising tool for investigating the dynamics of nucleon pairs in different states. Cross sections and asymmetries for both (γ,pn) and (γ,pp) turn out to be only slightly affected by short-range correlations and dominated by two-body currents. Therefore, two-nucleon knockout reactions induced by real photons appear well suited to investigate the nuclear current and the selectivity of individual transitions to its different components.     

In-beam γ -ray study of the neutron-rich nuclei 240U, 246Pu, and 250Cm produced by the (18O, 16O) reaction

We have measured deexcitation γ rays in the neutron-rich nuclei of ²⁴⁰U, ²⁴⁶Pu, and ²⁵⁰Cm produced by the (¹⁸O, ¹⁶O) two-neutron transfer reactions, in coincidence with the ¹⁶O particles using Si ΔE−E detectors. The γ rays in these nuclei were identified by selecting the kinetic energies of ¹⁶O particles, which correspond to the excitation energies in the residual nuclei below the neutron separation energies. The ground-state bands of ²⁴⁰U, ²⁴⁶Pu, and ²⁵⁰Cm were established up to 12⁺ states and the K ^π = 0⁻ octupole band of ²⁴⁰U was established up to 9⁻ states. The systematics of the moments of inertia of the ground-state bands for actinide nuclei shows that the deformed subshell closure at N = 152 is sustained for ₉₆Cm isotopes and that it disappears for ₉₄Pu isotopes. The text was submitted by the authors in English.     

Isovector deformation and its link to the neutron shell closure

DWBA analysis of the inelastic ^30-40S(p,p') and ^18-22O(p,p') scattering data measured in the inverse kinematics has been performed to determine the isoscalar (δ₀) and isovector (δ₁) deformation lengths of the 2⁺₁ excitations in the Sulfur and Oxygen isotopes using a compact folding approach. A systematic N-dependence of δ₀ and δ₁ has been established which shows a link between δ₁ and the neutron-shell closure. Strong isovector deformations were found in several cases, e.g., the 2⁺₁ state in ²⁰O where δ₁ is nearly three times larger than δ₀. These results confirm the relation δ₁>δ₀ anticipated from the core polarization by the valence neutrons in the open-shell (neutron rich) nuclei. The effect of neutron shell closure at N=14 or 16 has been discussed based on the folding model analysis of the inelastic ²²O+p scattering data at 46.6 MeV/u measured recently at GANIL.     

Antisymmetrized Green’s function approach to (e, e′) reactions with a realistic nuclear density

A completely antisymmetrized Green’s function approach to the inclusive quasielastic (e, e′) scattering, including a realistic one-body density, is presented. The single-particle Green’s function is expanded in terms of the eigenfunctions of the non-hermitian optical potential. This allows one to treat final state interactions consistently in the inclusive and in the exclusive reactions. Nuclear correlations are included in the one-body density. Numerical results for the response functions of ¹⁶O and ⁴⁰Ca are presented and discussed.     

Study of the reaction γp → pπ0η

The reaction γp → pπ⁰η has been studied with the CBELSA detector at the tagged photon beam of the Bonn electron stretcher facility. The reaction shows contributions from Δ⁺(1232)η , N(1535)⁺π⁰ and pa ₀(980) as intermediate states. A partial-wave analysis suggests that the reaction proceeds via formation of six Δ -resonances, Δ(1600)P ₃₃ , Δ(1920)P ₃₃ , Δ(1700)D ₃₃ , Δ(1940)D ₃₃ , Δ(1905)F ₃₅ , Δ(2360)D ₃₃ , and two nucleon resonances N(1880)P ₁₁ and N(2200)P ₁₃ , for which pole positions and decay branching ratios are given.     

Evidence for narrow Δ0(1232) states in the 12 C(e,e'pπ−}11 C Reaction

The reaction ¹²C(e,e'Δ⁰)¹¹C →¹²C(e,e'pπ⁻)¹¹C was investigated at the Mainz Microtron MAMI in a triple coincidence measurement using the three spectrometer setup of the A1 Collaboration. The good missing mass resolution of σ_m= 0.27 MeV/c² allowed to select the events belonging to the ground state of ¹¹C. Cutting on these events the excitation energy spectra of ¹²C_Δ0 show evidence for two peaks of about 4 MeV width (FWHM) at 282 MeV and 296 MeV with a significance of about 4.5 standard deviations. The peaks are interpreted in a simple weak coupling model as bound Δ⁰ states in ¹²C_Δ0. Received: 23 December 1998     

Fe-site assignments in Y1Ba2Cu3O7 revisited

A new symmetric Fe³⁺ site (labelled E) (δ=0.28(2) mm/s and Δ=0.15 mm/s) is observed in the R₁Ba₂Cu₃O₇ family of superconductors for R=Y and Eu. The decay and growth of site E are established in two seemingly unrelated experiments, one as a function of room temperature aging for R=Y, and the other as a function of oxygen loading at elevated temperatures and pressures for R=Eu. In each experiment, the results show that site E is genetically related to the well documented chainsites A(Δ=1.9 mm/s), C(Δ=1.1 mm/s) and D(Δ=1.6 mm/s). We propose that site E represents a quasi-octahedral chain-site having pairs of O(1), O(4) and O(5) nearestneighbor oxygen sites. The two remaining doublets, B(Δ≈0.4 mm/s) and B′(Δ=0.78 mm/s) represent Fe³⁺ dopant sites present in the all-important CuO₂ planes, possessing coordination numbers of 6 and 5, respectively.     

Excited states in neutron-rich 188W produced by an 18O-induced 2-neutron transfer reaction

Excited states in neutron-rich ¹⁸⁸W have been populated using a ¹⁸⁶W(¹⁸O,¹⁶O) reaction. In-beam γ-rays were measured in coincidence with scattered particles detected by a high-resolution ΔE-E Si telescope. In this experiment, the ground-state band has been identified up to I ^π = 8⁺. The γ band, the K ^π = 2^- octupole band, and a 2-quasiparticle state were also observed. The results are compared with predictions of self-consistent HFB cranking calculations and blocked-BCS multi-quasiparticle calculations.     

16O-8Be break-up states and cluster structure of 24Mg

High-spin states of ²⁴Mg produced in the ¹⁶O + ¹²C interaction and decaying into the ¹⁶O_g.s. + ⁸Be_g.s. channel have been observed in the excitation region between 35 and 52 MeV. Spins have been assigned on the basis of the analysis of the measured angular correlations. Some of these states with positive parity correspond to the known resonances of the ¹²C( ¹²C, ⁸Be_g.s.) ¹⁶O reaction belonging to the ¹⁶O-2α rotational band of ²⁴Mg. Moreover other resonances show up at higher excitation energy with an energy-spin relationship again suggesting a ¹⁶O-2α cluster structure for the associated configuration. Received: 6 July 2001 / Accepted: 16 October 2001     

Covalently bound molecular structures in the α + 16O system

Using the concept of covalent molecular orbitals for neutrons and the known properties of the local α + ¹⁶O potential the formation of asymmetric molecular structures in neon isotopes is discussed. Experimental evidence for parity doublets in ²¹Ne is reviewed and a corresponding band structure for the states in ²¹Ne at moderate excitation energy of E _x = 0-8 MeV is proposed. The structure of some bands can be interpreted as consisting of an instrinsic asymmetric ( ⁴He + ¹⁶O) structure bound by a covalent neutron in σ and π orbitals. An extension of the observed structures to symmetric molecular structures in isotopes of Mg and heavier nuclei is suggested. In particular shape isomers in isotopes of magnesium, namely (He)₂O molecules, can be predicted and an extended Ikeda diagram is proposed. Received: 11 July 2001 / Accepted: 22 August 2001     

Sensitive detection of methane and nitrous oxide isotopomers using a continuous wave quantum cascade laser

A continuous wave quantum cascade laser (QCL), operating near 8.1 μm, was used for wavelength modulation spectroscopy of methane (CH₄) and nitrous oxide (N₂O) stable isotopes. Several rotational transitions of ¹⁴N₂ ¹⁶O, ¹⁵N¹⁴N¹⁶O, ¹⁴N₂ ¹⁸O, ¹⁴N₂ ¹⁷O, ¹³CH₄ and ¹²CH₄ fundamental bands were detected. The noise-equivalent absorbance was measured to be less than 10^-5 in a 1-Hz bandwidth. A characterization of the laser source was also performed. The use of a QCL spectrometer for high-precision isotope ratio measurements is discussed. Received 14 March 2002     

Role of charge-transfer complexes in oxygen quenching of excited states of anthracene derivatives in the gas phase

Oxygen quenching of excited triplet and singlet states of gas-phase anthracene and its derivatives that have similar energies of the lower triplet levels but widely different oxidation potentials (0.44 < E_ox < 1.89 V) was studied. Quenching rate constants for singlet (k_S^O2) and triplet (k_T^O2) states in addition to the fraction of oxygen-quenched singlet and triplet states q_{S 1}(T₁^O2 were determined from the decay rates, fluorescence intensities, and delayed fluorescence as functions of oxygen pressure. It was found that k_S^O2 values vary from 2·10⁴ (9,10-dicyanoanthracene) to 1.2·10⁷ sec⁻¹·torr⁻¹ (anthracene, 9-methylanthracene, 2-aminoanthracene) and k_S^O2 values from 5·10² to 1·10⁵ sec⁻¹·torr⁻¹. The k_S^O2 values for anthracene, 9-methylanthracene, and 2-aminoanthracene, which have fast rates of interconversion from S₁ to T₁, are close to the rate constants for gas-kinetic collisions and are independent of the oxidation potentials (E_ox). The quenching rate constants k_S^O2 for the other anthracene derivatives and k_T^O2 for all studied compounds decrease with increasing free energy of electron transfer ΔG_ET, which indicates the important role of charge-transfer interactions in the oxygen quenching of singlet S_1- and triplet T₁ states. __________ Translated from Zhurnal Prikladnoi Spektroskopii, Vol. 75, No. 1, pp. 36–42, January–February, 2008.     

Shape co-existence and structural evolution of the yrast band in 157Yb

The high-spin states of ¹⁵⁷Yb have been studied via the ¹⁴⁴Sm(¹⁶O, 3n) reaction at ¹⁶O energy of 90 MeV using techniques of in-beam γ-ray spectroscopy. Measurement of γ-γ-t coincidences was performed with 11 BGO(AC)HPGe detectors. Based on the measured results of γ-γ coincidences, γ-ray anisotropies and DCO ratios, the level scheme for ¹⁵⁷Yb was established. The shape co-existence and structural evolution of the νi _13/2 band with increasing angular momentum in ¹⁵⁷Yb have been discussed. The systematics of the νi _13/2 bands in the N = 87 odd-A isotones have been compared. Received: 7 January 2002 / Accepted: 10 April 2002     

Mode selectivity in ion–molecule reactions of NH3+

Ammonia ions (NH₃ ⁺) are prepared in two internal states of nearly the same energy, a state with five quanta in the umbrella bending mode (E_int=0.60 eV) and another state with one quantum in the all-symmetric stretch and two quanta in the umbrella bending mode (E_int=0.63 eV). These ions are allowed to react with different neutral reagents, and the product ions are mass analyzed and detected. For each reaction, the product branching ratios are measured as a function of center-of-mass collision energy. Whereas reactions with D₂O, D₂, and CD₄ are found to be uninfluenced by the state preparation of the NH₃ ⁺ reagent, reactions with ND₃, partially deuterated methylamine (CD₃NH₂), and tetrahydrofuran (c-(CH₂)₄O)show varying degrees of mode selectivity, the reaction with tetrahydrofuran to the least extent. We suggest that mode selectivity in these ion–molecule reactions should be a general feature when the charge transfer channel is energetically open, the geometry of the reagent ion differs markedly from the corresponding neutral, and different reaction pathways compete for product production. Received: 14 December 1999 / Published online: 16 August 2000     

Kinetics of formation of O2(1Σ) molecules in reactions involving excited O2(1Δ) oxygen molecules and I(2P1/2) iodine atoms

The results of our experimental study of the kinetics of formation of O₂(¹Σ) molecules in energy-exchange reactions O₂(¹Δ) + I(⁵ p,² P _1/2) and O₂(a,¹Δ) + O₂(a,¹Δ) are presented. The ratio of rate constants was obtained for these reactions (4800 ± 300). Setting the rate constant of the deactivation of O₂(¹Σ) molecules on CO₂ molecules at 4.1 · 10^–13 cm³/s, we evaluated the rate constants for these reactions at a temperature of approximately 330 K: (1.7 ± 0.2) · 10⁻¹³ and (3.6 ± 0.5) · 10⁻¹⁷ cm³/s, respectively.