铁磁/有机半导体/铁磁系统的电流自旋极化性质研究

根据有机半导体中的电流自旋极化注入和输运实验现象，理论上研究了铁磁/有机半导体/铁磁系统的电流自旋极化性质.考虑到有机半导体的具体特性，从自旋扩散理论和欧姆定律出发，得到了系统的电流自旋极化率.假设自旋极化子和不带自旋的双极化子为有机半导体中的载流子.通过计算发现，极化子为实现有机半导体中电流极化注入和输运的有效自旋载流子，即使它只占总载流子很少一部分.还进一步研究了自旋相关界面电阻和电导率匹配以及有机半导体长度等因素对系统电流自旋极化的影响. 关键词： 自旋电子学 自旋注入 有机半导体 极化子     

有机自旋阀的磁电阻性质研究

考虑到有机半导体中极化子和双极化子特殊的电荷-自旋关系,从自旋扩散方程和欧姆定律出发,理论研究了"铁磁/有机半导体/铁磁"有机自旋阀结构中的磁电阻性质.计算发现,磁电阻在数值上随有机半导体层中极化子比率的增加而增大,随有机半导体层厚度的增加而迅速减小.同时发现自旋相关界面电阻能在很大程度上提高系统的磁电阻.讨论了铁磁层和有机半导体电导率比率、铁磁层极化率等对系统磁电阻性质的影响. 关键词： 磁电阻 有机自旋电子学 极化子     

肖特基势垒对铁磁/有机半导体结构自旋注入性质的影响

理论研究了铁磁/有机半导体肖特基接触时的电流自旋极化注入,并讨论了电流自旋极化率随界面处肖特基势垒高度、有机半导体层中特殊载流子及其迁移率、界面附近掺杂浓度的变化关系.通过计算发现,寻找在势垒区中载流子迁移率比较大的有机半导体材料对实现有效的自旋注入是必要的;同时还发现,由于铁磁/有机半导体接触而形成的肖特基势垒不利于自旋注入.因此要想实现有效的自旋注入,界面附近必须采用重掺杂来有效减少势垒区的宽度,且势垒的高度要限制在一定的范围内.     

有机器件电流自旋极化放大性质研究

基于自旋扩散漂移方程,考虑到电场的影响及有机半导体中特殊的载流子电荷自旋关系, 对一个简单的T型结构有机自旋器件模型进行了理论研究,得出了此有机器件的电流自旋 极化放大率表达式.研究表明,器件中极化子比率、电场和电流密度都会影响器件的电流 自旋极化放大率,通过调节此有机器件的电场和极化子比率可以获得较大的电流自旋 极化放大率.     

自旋注入有机物的扩散理论

根据自旋注入半导体的相关理论， 考虑到有机体内可能同时含有带自旋的单极化子和不带自旋的双极化子两种载流子，从扩散 理论和欧姆定律出发，建立了自旋注入有机体的唯象模型.通过计算发现，适当选择铁磁层极化率或两层的电导率可以使得有机层内电流具有高的自旋极化.进一步研究了单极化子浓度等因素对注入电流极化的影响. 关键词： 自旋电子学 自旋注入 有机聚合物 极化子     

自旋极化电子从铁磁金属注入半导体时自旋极化的计算

对自旋极化电子从铁磁金属通过绝缘层薄膜注入半导体时的自旋极化率与绝缘层厚度以及所加偏压的关系等作了计算.所得结果与最新实验结果相符，并发现偏压适中、绝缘层较厚时 有较大的电流自旋极化率，偏压很小时电流自旋极化率几乎为零. 关键词： 自旋极化电子注入 Slonczewski模型 隧道磁电阻 非零偏压     

自旋极化有机电致发光器件中单线态与三线态激子的形成及调控

由于有机半导体（OSC）材料自旋弛豫时间长、自旋扩散长度大,OSC自旋器件逐渐成为研究热点.对于有机电致发光器件（OLED）,通过自旋极化电极调控单线态和三线态激子比率是提高其效率的有效方法.本文从漂移扩散方程和载流子浓度连续性方程出发,结合朗之万定律建立了一个自旋注入、输运、复合的理论模型.计算了OSC中的极化电子、空穴浓度,得出了单线态和三线态激子的比率.分析了电场强度、自旋相关界面电导、电极和OSC电导率匹配和电极极化率等因素的影响.计算结果表明：两电极注入反向极化的载流子并提高载流子自旋极化率,有     

影响磁性pn结自旋极化输运特性的因素

利用漂移扩散理论研究了磁性pn结中自旋的输运特性.探讨了外加电压、平衡自旋极化率、外加自旋注入和自旋寿命对磁性pn结电流密度和电阻的影响,讨论了磁性pn结自旋伏特效应与pn结宽度的关系.发现平衡自旋极化率使得不同自旋方向电子具有不同的势垒高度从而能有效调制电流;而外加自旋注入则为磁性pn结提供了非平衡自旋极化电子从而达到对电流的调制作用,同时发现自旋伏特电流随准中性p区宽度减小而增大. 关键词： 磁性pn结 自旋极化率 自旋寿命 自旋伏特效应     

一维铁磁/有机系统的基态与自旋分布研究

文中用一维紧束缚模型描述铁磁金属,用一维非简并的Su-Schrieffer -Heeger (SSH)模型描述共轭聚合物,研究了在一维铁磁/共轭聚合物系统和一维CMR材料/ 聚合物系统中的电子转移和自旋转移.发现在聚合物部分没有自旋的双极化子比有自旋的极化子具有较低的能量而容易产生.然而在铁磁CMR材料/聚合物系统中极化子的产生能低于聚合物中极化子的产生能,增加了有机物中自旋极化输运的可能性.     

有机自旋器件磁性渗透层中双极化子对自旋极化输运的影响

根据实验发现的有机器件如Co/有机半导体/La_0.7Sr_0.3MnO₃中磁性原子渗透现象, 利用自旋漂移-扩散方程, 理论研究了磁性渗透层中极化子-双极化子的转化对自旋极化输运的影响. 研究发现: 磁性渗透层具有不同于纯净有机层的迁移率和自旋反转时间, 都将影响极化子-双极化子的转化, 进而影响自旋极化的输运; 在磁性渗透层中极化子自旋反转时间的劈裂是引起自旋弛豫的主要因素, 而极化子和双极化子之间的转化是重要因素.     

Effects of electric field and magnetic induction on spin injection into organic semiconductors

Spin-polarized injection and transport into ferromagnetic/organic semiconductor structure are studied theoretically in the presence of the external electric field and magnetic induction. Based on the spin-drift-diffusion theory and Ohm's law, we obtain the charge current polarization, which takes into account the special carriers of organic semiconductors. From the calculation, it is found that the current spin polarization is enhanced by several orders of magnitude by tuning the magnetic induction and electric fields. To get an apparent current spin polarization, the effects of spin-depended interfacial resistances and the special carriers in the organic semiconductor, which are polarons and bipolarons, are also discussed.     

The effects of electric and magnetic fields on the current spin polarization and magnetoresistance in a ferromagnetic/organic semiconductor/ferromagnetic（FM/OSC/FM） system

From experimental results of spin polarized injection and transport in organic semiconductors(OSCs),we theoretically study the current spin polarization and magnetoresistance under an electric and a magnetic field in a ferromagnetic/organic semiconductor/ferromagnetic(FM/OSC/FM) sandwich structure according to the spin drift-diffusion theory and Ohm’s law.From the calculations,it is found that the interfacial current spin polarization is enhanced by several orders of magnitude through tuning the magnetic and electric fields by taking into account the specific characteristics of OSC.Furthermore,the effects of the electric and magnetic fields on the magnetoresistance are also discussed in the sandwich structure.     

Effect of Carrier Differences on Spin Polarized Injection into Organic and Inorganic Semiconductors

Spin polarized injection into organic and inorganic semiconductors are studied theoretically from the spin diffusion theory and Ohm＇s law, and the emphases are placed on the effect of the carrier differences on the current spin polarization. The mobility and the spin-flip time of carriers in organic and inorganic semiconductors are different. From the calculation, it is found that current spin polarization at a ferromagnetic/organic interface is higher than that at a ferromagnetic/inorganic interface because of different carriers in them. Effects of the conductivity matching, the spin dependent interracial resistances, and the bulk spin polarization of the ferromagnetic layer on the spin polarized injection are also discussed.     

Theoretical study on spin-polarized injection of electrical currents into polymer semiconductors

Different from electrons and holes in traditional inorganic semiconductors, the charge carriers in polymer semiconductors are spin polarons and spinless bipolarons. In this paper, a theoretical model is presented to describe the spin-polarized injection of electrical currents from a ferromagnetic contact into a nonmagnetic polymer semiconductor. In this model, a new relation of conductivity to concentration polarization for polymer semiconductors is introduced based on a three-channel model to describe the spin-polarized injection of electrical currents under large electrical current densities. The calculated results of the model reveal the effects of the polaron ratio, the carrier concentration polarization, the interfacial conductance, the bulk conductivity of materials, and the electrical current density, etc. on the spin polarization of electrical currents. As conclusions, the large and matched bulk conductivity of materials, the small spin-dependent interfacial conductance, the thin polymer thickness and the large enough electrical current are critical factors for upgrading the spin polarization of electrical currents in polymer semiconductors. Particularly, when the polaron ratio in polymer semiconductors approaches the concentration polarization of the ferromagnetic contact, a modest concentration polarization is sufficient for achieving a nearly complete spin-polarized injection of electrical currents.     

Effect of Electric Field on Spin Polarized Current in Ferromagnetic/Organic Semiconductor Systems

Considering the special carriers in organic semiconductors, the spin polarized current under electric field in a ferromagnetic/organic semiconductor system is theoretically studied. Based on the spin-diffusion theory, the current spin polarization under the electric field is obtained. It is found that electric field can enhance the current spin polarization.