非线性光学 非线性光学概论

O437 2006054144高斯光束在克尔型非线性介质中的演化特性=Evolutionfeature of Gaussian beam propagating in absorptive Kerrmedium[刊,中]/刘雅洁(嘉兴学院物理教研室.浙江,嘉兴(314001))//光散射学报.—2006,18(2).—183-187由光束在克尔型吸收介质中传输的非线性薛定谔方程,推导了高斯光束注入介质后满足的耦合方程,并分别在不考虑吸收和高阶展开项的情况下,对脉冲的腰斑半径的演化进行了理论分析。发现当注入脉冲满足一定的条件时,脉冲可以以“孤波”的形式传播。当考虑吸收和高阶展开项时,脉冲不存在“孤波”形式,而是存在一个阈…     

金属Fe薄膜的PLD制备及其非线性光学性质研究

采用脉冲激光沉积（PLD）技术在MgO基片上制备了金属Fe薄膜.利用原子力显微镜研究了不同制备温度对薄膜表面形貌的影响.x射线衍射分析表明沉积温度大于500℃时，Fe薄膜在MgO基片上有很好的结晶性，并有单一取向.通过z扫描方法测量了超薄Fe膜的光学非线性，得到了Fe薄膜的非线性折射率n₂＝709×10^-5cm²/ kW，非线性吸收系数 β＝-552×10^-3cm/W. 关键词： Fe薄膜 非线性 脉冲激光沉积     

非线性光学 非线性光学概论

O437 2007054311三阶色散和自频移效应对孤子压缩的影响=Influence of third -dispersion and Raman self-scattering on optical pulse compression[刊,中]/曹冬梅(延安大学物理与电子信息学院.陕西,延安(716000)) ,曾祥梅//常熟理工学院学报(自然科学版) .? 2007 ,21(4) .? 38-41通过数值求解高阶非线性Schr dinger方程,发现三阶色散和喇曼自频移效应对孤子脉冲的压缩会产生影响。正的三阶色散( TOD)和喇曼( RSS)效应使得孤子脉冲的压缩比减小;负的TOD和RSS效应使得孤子脉冲的压缩比增大。其中对于负的TOD和RSS效应,存在一个最佳…     

五阶非线性光纤中连续谱相位扰动下的光传输与脉冲串产生

根据包含五阶非线性的扩展非线性薛定谔方程,数值研究了高斯型连续谱相位扰动而不是传统单色扰动下基于调制不稳定性的高重复率脉冲串产生.结果表明:脉冲串也能像传统情形那样形成,但却呈现出不同的特性.如脉冲数目有限,且各脉冲的高度、强度及间距不等.脉冲数目随传输距离增加而增加.而五阶非线性能使脉冲宽度和间距变小因而有利于高重复率脉冲串产生,负五阶非线性则相反.对脉冲串形成过程中演变啁啾的数值计算表明,啁啾及其随距离的变化都是高度非单调的,五阶非线性将改变啁啾的范围和量值.     

基于交叉相位调制的堆积脉冲非线性传输

基于子脉冲交叉相位调制的非线性相互作用,利用耦合非线性传输模型,对堆积脉冲的非线性传输和峰均比进行了研究.研究发现,当堆积脉冲的子脉冲间存在重叠时,在传输过程中时间相干会导致子脉冲间发生相互作用从而改变其脉冲质量.在不同的子脉冲延迟情况下,堆积脉冲的强度和峰均比随传输距离的变化而改变,且变化幅度均随子脉冲延迟的增大而减小.对于高斯型堆积脉冲,当归一化子脉冲延迟大约为3时其在非线性传输过程中保持脉冲形状基本不变;而对于超高斯型的堆积脉冲,归一化子脉冲延迟则约为2.2.     

五阶非线性光纤中连续谱相位扰动下的光传输与脉冲串产生

根据包含五阶非线性的扩展非线性薛定谔方程,数值研究了高斯型连续谱相位扰动而不是传统单色扰动下基于调制不稳定性的高重复率脉冲串产生.结果表明:脉冲串也能像传统情形那样形成,但却呈现出不同的特性.如脉冲数目有限,且各脉冲的高度、强度及间距不等.脉冲数目随传输距离增加而增加.而五阶非线性能使脉冲宽度和间距变小因而有利于高重复...     

共振增强的光学参变下转换

多光子纠缠态是量子通讯网络中的重要资源,光与二阶非线性介质相互作用的自发参变下转换过程是目前制备多光子态较成熟的方案之一.尽管脉冲光可以提高非线性转换效率并简化通信协议,但是进一步增强光与介质间的相互作用对提高多光子的产生效率依然必要.设计了飞秒脉冲激光谐振腔系统,在不改变脉冲重复频率和频率梳结构的情况下,提高了下转换...     

高非线性光纤产生自相似抛物线脉冲的特性研究

基于脉冲在光纤中传输所满足的非线性薛定谔方程,采用数值计算的方法对脉冲在高非线性光纤中演化成自相似抛物线脉冲的传输特性进行了研究。结果表明,脉冲在不同初始能量和啁啾参量的情况下,高非线性光纤产生自相似抛物线脉冲,且随着归一化长度的增大,脉冲的自相似指数从0.0796减小到0.0720。进一步的研究表明:啁啾高斯脉冲在光纤传输过程中,脉冲逐渐展宽,同时正啁啾越大,其自相似演化结果越差;参数N=8的正负啁啾脉冲分别演化成平顶自相似抛物线脉冲以及三角形脉冲。     

非线性传输线高功率实验北大核心CSCD

设计了基于交叉耦合铁氧体非线性传输线高功率射频微波产生系统,系统由脉冲形成线、非线性传输线以及高功率匹配负载(或组合振子辐射天线)组成。由100kV高压电源和高压微波电缆构成单传输线高功率脉冲形成线,形成线输出脉冲幅度35kV,脉冲半宽60ns。高压脉冲经过非线性传输线的脉冲压缩和调制,与高功率匹配负载相连时,实验得到了峰峰值31kV、中心频率308 MHz、3dB带宽为13%的射频振荡脉冲;与组合振子天线相连时,实验得到了中心频率380MHz、3dB带宽为12%的宽谱辐射。实验结果与数值模拟基本吻合。     

富勒烯有机-无机杂化材料的非共珍三阶非线性光学特性

采用中心波长800 nm、脉宽30 fs的超短激光脉冲,通过飞秒光开关技术（Optical Kerr Shutter,OKS）对富勒烯有机-无机杂化材料的飞秒超快非线性特性进行了实验研究.获得270 fs的开关时间,所得的富勒烯有机-无机杂化材料的三阶非线性系数χ(3)约为4.5×10－14 esu,比C60分子的三阶非线性系数χ(3)高一个数量级.通过实验测定的光克尔信号强度与激发光和探测光偏振方向夹角的依赖关系表明：30 fs的超短激光脉冲激发富勒烯有机-无机杂化材料的克尔信号主要是源于光诱导双折射效应,而非用200 fs的超短激光脉冲时来自瞬态栅的自衍射效应.     

周期量级长波长光源，极端非线性光学以及阿秒科学

介绍了长波长光源的发展以及其在非线性光学以及强场物理方面的应用。长波长光源的产生以各种方式推动了强场和阿秒物理学的发展：在隧穿机制下光电离的研究,用于X射线成像的飞秒量级KeV辐射源的产生。考虑到这些前景,何如产生高能量、长波长以及周期量级的光源是一件非常有挑战性的工作。在过去几年,一直致力于产生和发展波长在2～3μm、载波相位稳定,周期量级的强光源,其重复频率从几千赫兹到百千赫兹。重点介绍这些光源的发展,以及脉冲相关测量的方法。此外,以某一种光源作为例子来介绍其在多倍频超连续谱的产生,分子的电离动力学以及阿秒光源生产等方面的应用。     

Coherent fiber supercontinuum for biophotonics

Biophotonics and nonlinear fiber optics have traditionally been two independent fields. Since the discovery of fiber‐based supercontinuum generation in 1999, biophotonics applications employing incoherent light have experienced a large impact from nonlinear fiber optics, primarily because of the access to a wide range of wavelengths and a uniform spatial profile afforded by fiber supercontinuum. However, biophotonics applications employing coherent light have not benefited from the most well‐known techniques of supercontinuum generation for reasons such as poor coherence (or high noise), insufficient controllability, and inadequate portability. Fortunately, a few key techniques involving nonlinear fiber optics and femtosecond laser development have emerged to overcome these critical limitations. Despite their relative independence, these techniques are the focus of this review, because they can be integrated into a low‐cost portable biophotonics source platform. This platform can be shared across many different areas of research in biophotonics, enabling new applications such as point‐of‐care coherent optical biomedical imaging.     

非线性光学五十年

文章简要回顾了非线性光学的诞生以及早期的发展,包括二次谐波,激光和频和差频现象,受激拉曼散射,以及激光的一些自作用行为等,介绍了非线性光学的一些重要研究成果和应用,包括非线性光谱学,位相共轭和自适应光学,相干非线性光学以及高次谐波等,最后对非线性光学当前和未来研究热点作了总结和展望.     

Efficient high harmonic generation in nonlinear photonic moiré superlattice

Photonic moiré superlattice as an emerging platform of flatbands can tightly confine the light inside the cavity and has important applications not only in linear optics but also in nonlinear optics. In this paper, we numerically investigate the third- and fifth-order harmonic generation (THG and FHG) in photonic moiré superlattices fabricated by the nonlinear material silicon. The high conversion efficiency of THG and FHG is obtained at a relatively low intensity of fundamental light, e.g., the maximum conversion efficiency of THG and FHG arrives even up to be 10⁻² and 10⁻⁹ at the fundamental intensity of 30 kW/m², respectively, in the moiré superlattice of near flat band formed by the twist angle 6.01°. The results indicate the photonic moiré superlattice of a high-quality factor and flatbands is a promising platform for efficient nonlinear processes and advanced photonic devices.     

Few‐optical‐cycle light pulses with passive carrier‐envelope phase stabilization

One of the most advanced frontiers of ultrafast optics is the control of carrier‐envelope phase (CEP) ϕ of light pulses, which enables the generation of optical waveforms with reproducible electric field profile. Such control is important for pulses with few‐optical‐cycle duration, for which a CEP variation produces a strong change in the waveform, so that strongly nonlinear optical phenomena, such as multiphoton absorption, above‐threshold ionization and high‐harmonic generation become CEP‐dependent. In particular, CEP control is the prerequisite for the production of isolated attosecond pulses. Standard laser systems generate pulses that are CEP unstable; the CEP can be stabilized using either active or passive methods. Passive, all‐optical schemes rely on difference‐frequency generation (DFG) between two pulses sharing the same CEP: in this process the phases of the two pulses add up with opposite signs, leading to cancellation of the shot‐to‐shot CEP fluctuations. This paper presents an overview of passive CEP stabilization schemes, starting from the basic concepts and progressing to the details of the practical implementations of the idea. The passive approach allows the generation of CEP‐controlled few‐optical‐cycle pulses covering a very broad range of parameters in terms of carrier frequency (from visible to mid‐IR), energy (up to several mJs) and repetition rate (up to hundreds of kHz)     

金属纳米颗粒等离激元共振增强非线性介质谐波的发展现状

随着纳米加工和制备技术的不断发展,金属纳米粒子的等离激元光学特性已得到了广泛的研究与应用。本文基于金属纳米颗粒等离激元共振特性,分析了金属纳米颗粒等离激元共振对介质谐波的增强机制,综述了该增强机制在近几年所取得的最新研究成果及其在生物成像领域的应用。金属纳米颗粒等离激元共振在增强介质非线性特性领域的发展趋势是从简单的金属纳米颗粒向复杂形状纳米颗粒和金属纳米颗粒组装体的发展,这些新型金属纳米颗粒在非线性光学、生物医学上的疾病诊断和治疗有良好的实际应用前景。     

A novel quasi-phase-matching frequency doubling technique

A new quasi-phase-matching technique for efficient second-harmonic generation is reported. It is based on the spatial periodic modulation of the light intensity along the propagation direction, rather than the conventional spatial periodic modulation of the nonlinear optical coefficients. It can be realized by using a novel dual-channel waveguide frequency doubler structure for the desired light intensity distribution. This dual-channel waveguide device has major advantages including very small beam size, high light intensity within long nonlinear-waveguide interaction length, highly efficient second-harmonic generation, ease in fabrication of the nonlinear channel waveguides without any spatially periodic poling, and low waveguide propagation losses. The new quasi-phase-matching technique can also be applied to third-harmonic generation and other nonlinear optics processes.     

Difference frequency generation in GaAs microdisks

Semiconductor-based whispering-gallery-mode microcavities are very promising for nonlinear optics applications, thanks to the high optical quality factors attainable with today's technology. We propose to exploit this advantage to generate cw light through phase-matched difference frequency generation in a triply resonant GaAs microdisk. A proper choice of the microdisk radius and thickness allows one to select the generated wavelength in the band of 2.5-2.9 mum. Besides illustrating the design features, we numerically show that temperature can be effectively used to compensate for wavelength shifts induced on the generated field by fabrication errors.     

带有自适应光学系统的ICF装置光束传输程序

 以典型的惯性约束聚变（ICF）装置为基础,根据ICF中光传输、光放大和光倍频等原理,建立了一套含自适应光学校正系统的ICF仿真软件。通过比对国内外相应的文献和专业软件的光的线性传播、非线性传播、光的增益、光的倍频等来验证软件仿真的准确性和可靠性。给出了经自适应光学系统校正前后基频光的近场强度和相位分布,3倍频光的近、远场的光强分布,说明自适应光学在提高ICF装置输出光束质量中的作用。该软件的建立将为优化ICF系统中自适应光学的设计提供参考。     

The geometric phase in nonlinear frequency conversion

The geometric phase of light has been demonstrated in various platforms of the linear optical regime, raising interest both for fundamental science as well as applications, such as flat optical elements. Recently, the concept of geometric phases has been extended to nonlinear optics, following advances in engineering both bulk nonlinear photonic crystals and nonlinear metasurfaces. These new technologies offer a great promise of applications for nonlinear manipulation of light. In this review, we cover the recent theoretical and experimental advances in the field of geometric phases accompanying nonlinear frequency conversion. We first consider the case of bulk nonlinear photonic crystals, in which the interaction between propagating waves is quasi-phase-matched, with an engineerable geometric phase accumulated by the light. Nonlinear photonic crystals can offer efficient and robust frequency conversion in both the linearized and fully-nonlinear regimes of interaction, and allow for several applications including adiabatic mode conversion, electromagnetic nonreciprocity and novel topological effects for light. We then cover the rapidly-growing field of nonlinear Pancharatnam-Berry metasurfaces, which allow the simultaneous nonlinear generation and shaping of light by using ultrathin optical elements with subwavelength phase and amplitude resolution. We discuss the macroscopic selection rules that depend on the rotational symmetry of the constituent meta-atoms, the order of the harmonic generations, and the change in circular polarization. Continuous geometric phase gradients allow the steering of light beams and shaping of their spatial modes. More complex designs perform nonlinear imaging and multiplex nonlinear holograms, where the functionality is varied according to the generated harmonic order and polarization. Recent advancements in the fabrication of three dimensional nonlinear photonic crystals, as well as the pursuit of quantum light sources based on nonlinear metasurfaces, offer exciting new possibilities for novel nonlinear optical applications based on geometric phases.