Femtosecond ultraviolet pulses generated using noncollinear optical parametric amplification and sum frequency mixing

We demonstrate the generation of ultraviolet 33-fs pulses with a shot-to-shot energy fluctuation of less than 3% using sum frequency mixing of visible pulses of a noncollinear optical parametric amplifier with sub-40-fs pulses of a 1-kHz Ti:sapphire-amplified system. The pulses are transform-limited (ΔνΔτ=0.36) and tunable in the range from 315 nm to 355 nm with energy above 1 μJ (2.6 μJ at 330 nm). Received: 21 July 2000 / Published online: 8 November 2000     

Sub-20 fs visible pulses with 750 nJ energy from a 100 kHz noncollinear optical parametric amplifier

We demonstrate the operation of a 100 kHz noncollinear optical parametric amplifier that is pumped by just a few microjoules of 800 nm pulses with 50 fs duration. The device delivers sub-20 fs pulses tunable from 460 nm to beyond 1 microm and pulse energies up to 750 nJ when it is pumped with 7 microJ of energy. The design of the single-stage amplifier has been carefully optimized, and the design considerations are discussed.     

Compact laser source for high-power white-light and widely tunable sub 65 fs laser pulses

We demonstrate an Yb:KGW femtosecond solitary mode-locked laser oscillator, which is used as a pump source for tapered fibers to generate white-light laser pulses with an average output power of up to 2.5 W and a spectral bandwidth of over 1000 nm. By spectrally filtering these pulses and subsequent compression of the filtered pulses with a prism sequence, we are able to generate ultrashort laser pulses with durations between 26 and 65 fs that are tunable from 600 to 1450 nm and with tens to several hundreds of milliwatts of average power.     

Tunable femtosecond near-infrared source based on a Yb:LYSO-laser-pumped optical parametric oscillator

We demonstrate a widely tunable near-infrared source from 767 nm to 874 nm generated by the intracavity second harmonic generation(SHG) in an optical parametric oscillator pumped by a Yb:LYSO solid-state laser. The home-made Yb:LYSO oscillator centered at 1035 nm delivers an average power of 2 W and a pulse duration as short as 351 fs. Two Mg O doped periodically poled lithium niobates(Mg O:PPLN) with grating periods of 28.5–31.5 μm in steps of 0.5 μm and19.5–21.3 μm in steps of 0.2 μm are used for the OPO and intracavity SHG, respectively. The maximum average output power of 180 m W at 798 nm was obtained and the output pulses have pulse duration of 313 fs at 792 nm if a sech2-pulse shape was assumed. In addition, tunable signal femtosecond pulses from 1428 nm to 1763 nm are also realized with the maximum average power of 355 m W at 1628 nm.     

Injection-seeded, gain-switched tunable Cr:ZnSe laser

We report a narrow-linewidth, tunable, gain-switched Cr:ZnSe laser operating between 2255 and 2455 nm. The spectral width of the laser was reduced from 125 nm to 0.3 nm by using injection seeding. Seeding was achieved with a second tunable CW Cr:ZnSe laser. The output wavelength was varied by tuning the wavelength of the seed laser. The seeded oscillator produced as high as 157 μJ pulses with 598 μJ incident pump pulse energy at a repetition rate of 1 kHz. The slope efficiency was determined to be 26%.     

Tunable phase-stabilized infrared parametric laser source

This paper reports that the tunable self-phase-stabilized infrared laser pulses have been generated from a two-stage optical parametric amplifier. With an 800 nm pump source, the output idler pulses are tunable from 1.3 μm to 2.3 μm, and the maximum output energy of the idler pulses is higher than 1 mJ at 1.6 μm by using 6 mJ pump laser. A carrier-envelope phase fluctuation of ～ 0.15 rad (rms) for the idler pulses is measured for longer than one hour by using a home build f-to-2f interferometer.     

超短激光脉冲调制上转换放大

在超短激光脉冲倍频过程中，由于调制不稳定性而产生多色圆锥辐射. 在多色圆锥辐射的任 意方向上同步注入一束宽带种子光，可以得到相应频率的调制上转换放大. 放大的光脉冲的 中心波长在500 nm时单脉冲能量最大可至150 μJ并且具有60 nm的频谱宽度. 通过改变种子 光的入射角度而实现上转换放大中心波长的连续调谐，范围约为290 nm. 关键词： 调制上转换放大 调制不稳定性 多色圆锥辐射     

Multi-color ultrafast laser platform for nonlinear optical imaging based on independently tunable optical parametric oscillators

We report on design of a multi-color laser set up that allows for high spectral, time and spatial resolution imaging based on second- and third-order optical nonlinearities in soft condensed matter. Two femtosecond optical parametric oscillators (OPOs) are pumped simultaneously to provide intrinsically synchronized pulses at more than a dozen tunable colors across visible and infrared wavelengths. We demonstrate the use of independently tunable OPOs in a variety of imaging modalities. In one useful application, we explore brain tissue in a two-photon absorption fluorescence imaging experiment with near infrared optical pulses (λ ~ 1,070 nm). We also demonstrate second and sum-frequency generation microscopies in different tissues. Results from application of time-resolved, three-color coherent anti-stokes Raman scattering in tissue are presented to demonstrate feasibility of quantitative spectroscopic imaging.     

高效率光参量转换

用一块6.5×9×20(长度)mm KTP晶体获得625nm～3575nm的皮秒可调谐激光.能量转换效率高达30%,最大信号光峰值功率34MW.     

Generation of tunable octave-spanning mid-infrared pulses by filamentation in gas media

The continued development of femtosecond mid-infrared (IR) sources with ultrabroad spectral width is critical for probing and controlling complex molecular structural dynamics on an ultrafast timescale. We report on a sub-20 fs, coherent mid-IR source with an octave-spanning spectral bandwidth (>2000 cm(-1)) tunable from 2-8 micrometers (37.5-150 THz), with energy >0.4 μJ/pulse at 1 kHz. The mid-IR pulses are generated by four-wave mixing during the filamentation of intense 800 nm and 400 nm pulses in various gas media. Spectral tunability is achieved by the choice of gas, pressure and input 800 nm pulse energy.     

Ultrabroadband phase-matched optical parametric generation in the ultraviolet by use of guided waves

We present what is believed to be the first experimental demonstration of guided-wave phase-matched frequency mixing and harmonic conversion in gases. Broad-bandwidth ultrafast pulses, tunable around 270 nm, were generated from an ultrafast Ti:sapphire amplifier system using 2? + 2? - ? parametric wave mixing in a capillary waveguide. We achieved nonresonant phase matching by coupling both the fundamental and the second-harmonic light into the lowest-order mode. The output 3? pulses have an energy of >4muJ at a 1-kHz repetition rate. Simple extensions of this method can generate higher-energy 10-20-fs pulses tunable throughout the vacuum ultraviolet.     

Tunable high-peak-power, high-energy hybrid Q-switched double-clad fiber laser

A cw laser-diode-pumped Yb-doped double-clad fiber laser operating in a hybrid Q-switched regime was demonstrated. The output pulses had a duration as short as 4.2 ns, a tunable wavelength range from 1080.8 to 1142.7 nm, and a linewidth of less than 0.05 nm. Maximum peak power of approximately 175 kW and single-pulse energy of 1.57 mJ were obtained.     

Tunable ultraviolet source from fifth and seventh harmonic generated by mid-infrared pulses filamentation in air

The seventh harmonic generation by tunable mid-infrared femtosecond pulses filamentation in air is observed first time. Pumped by a focused mid-infrared pulses, which pulse duration is ～50 fs and wavelength is tunable from 1300 to 2000 nm, the tunable region of the fifth and seventh harmonic generation can cover the near ultraviolet region from 180 to 400 nm.     

Chirped pulse amplification in single mode Tm:fiber using a chirped Bragg grating

We report femtosecond pulse generation and chirped pulse amplification in Tm:fiber. A mode-locked oscillator operating in the soliton regime produced 800 fs pulses with 5 nm spectral bandwidth, at 40 pJ pulse energy. This oscillator seeded a pre-amplifier that utilizes a Raman soliton self-frequency shift to produce wavelength tunable pulses with 3 nJ energy, reduced pulse duration of 150 fs, and increased bandwidth of 30 nm. For further amplification, the pulses were stretched up to 160 ps using a chirped Bragg grating (CBG). Stretched pulses were amplified to 85 nJ after compression in single-mode Tm:fiber and recompressed with the CBG as short as 400 fs. Compressed pulses were coupled into a highly nonlinear tellurite fiber to investigate the potential of this ultrashort pulse 2-μm fiber source as a pump for mid-IR supercontinuum generation.     

Tunable, high-repetition-rate, femtosecond pulse generation in the ultraviolet

We report efficient generation of tunable femtosecond pulses in the ultraviolet (UV) by intracavity doubling of a visible femtosecond optical parametric oscillator (OPO). The OPO, based on a 400 microm BiB3O6 crystal and pumped at 415 nm in the blue, can provide visible femtosecond signal pulses across 500-710 nm. Using a 500 microm crystal of beta-BaB2O4 internal to the OPO cavity, efficient frequency doubling of the signal pulses into the UV is achieved, providing tunable femtosecond pulses across 250-355 nm with up to 225 mW of average power at 76 MHz. Cross-correlation measurements result in UV pulses with durations down to 132 fs for 180 fs blue pump pulses.     

Generation of tunable multi-wavelength optical short pulses using self-seeded Fabry-Perot laser diode and tilted multimode fiber Bragg grating

We experimentally demonstrate the simultaneous generation of tunable multi-wavelength picosecond laser pulses using a self-seeding configuration that consists of a gain-switched Fabry-Perot laser diode (FPLD) with an external cavity formed by a tilted multimode fiber Bragg grating.Dualand triple-wavelength pulses are obtained and tuned in a flexible manner by changing the temperature of the FPLD.The side mode suppression ratio larger than 25 dB is achieved at different dualand triple-wavelengths and the typical pulsewidth of the output pulses is ～70 ps.In the experiment,the wavelength separation can be narrowed to 0.57 nm.     

499nm绿色激光泵浦的掺钛宝石激光输出

首次推导用ＸｅＣｌ／Ｈ２拉曼系统三阶期托克期输出作泵浦源的可调谐掺钛宝石激光输出特性在稳恒溅注浦光的波长为４９９ｎｍ，脉宽为６０ｎｓ。激光输出的斜率效率为５９％，脉宽为２０ｎｓ。最大输出能量为１．２ｍＪ。能量转换效率为４２％。采用一组调谐镜时的范围为６８０－８３４ｎｍ     

High power tunable picosecond green laser pulse generation by frequency doubling of an Yb-doped fiber power amplifier seeded by a gain switch laser diode

A compact tunable high power picosecond green laser pulse source based on frequency doubling of an Yb-doped fiber amplifier seeded by a gain switch laser diode has been developed. The fiber amplifier generates the picosecond infrared pulses with average power of 10.3 W, repetition rate of 1 MHz, pulse duration of 150 ps, and tunable range of 20 nm around 1064 nm. For underwater use, the tunable output infrared pulses are frequency doubled into picosecond green laser pulses, which can be tuned from 527 to 537 nm with average power of more than 1.1 W, corresponding to an overall conversion efficiency of 10.7% by a BBO nonlinear crystal. This kind of laser source will have potential application for underwater optical communication.     

Two-color chirped-pulse amplification in an ultrabroadband Ti:sapphire ring regenerative amplifier

We have developed a high-energy, ultrabroadband Ti:sapphire ring regenerative amplifier capable of producing in excess of 20-mJ output at a 10-Hz repetition rate. The technique of chirped-pulse amplification is used to generate two-color, time-synchronized pulses with central wavelength separations of up to approximately 120 nm and with a total energy of 10 mJ by use of a regenerative pulse-shaping technique. Mid-infrared pulses tunable from 6 to 11 microm are generated by difference frequency mixing the two-color outputs.     

High-repetition-rate picosecond pulse generation at 1.5 microm by intracavity laser frequency modulation

We propose and experimentally demonstrate generation of transform-limited pulse trains at a 2.5-GHz repetition rate from a frequency-modulated erbium-ytterbium bulk glass laser by using an intracavity lithium niobate phase modulator and an external fiber Bragg grating filter. Light pulses with durations tunable from 40 to 80 ps and 0.2-mW fiber-coupled average power at 1535 nm have been obtained.