Generation of tunable coherent VUV radiation by anti-Stokes Raman scattering of excimer-pumped dye laser radiation

A straightforward method of generating tunable coherent VUV radiation is described. Radiation down to 1362 Å was produced by Raman shifting the output of a commercially produced, excimer-pumped dye laser system. It is shown that generation of VUV radiation at 1640 Å is more efficient using the 8th anti-Stokes line from a UV dye than by using the 10th anti-Stokes line from a visible dye which had twice the output power.     

Multi-wavelength Brillouin fiber laser using dual-cavity configuration

A simple technique for achieving multi-wavelength tunable multi-wavelength Brillouin fiber laser (BFL) based on dual-pass configuration is demonstrated. The BFL uses a piece of 10 km long non-zero dispersion shifted fiber (NZ-DSF) as a Brillouin gain medium to obtain odd-order Brillouin Stokes waves as an output with the line spacing of 0.16 nm (20 GHz) between each two consecutive waves by employing even-order Brillouin Stokes to improve output performance of the laser. With a BP of 15.3 dBm, at least 15 odd-order Brillouin Stokes and anti-Stokes lines are generated. The laser is room temperature stable, tunable over 50 nm wavelength range and has an optical signal to noise ratio of more than 30 dB at 1560 nm region. This Brillouin fiber laser can operate at any wavelength depending on the Brillouin pump (BP) wavelength used.     

Anti-stokes fluorescence of polymethine dyes excited by a titanium-sapphire laser

Fluorescence of symmetric polymethine dye solutions (λ _abs ^max ≈ 700 nm) upon anti-Stokes excitation by cw radiation of a titanium-sapphire laser (781 nm) is first investigated. A series of six compounds with analogous composition and spectral and luminescent properties is investigated. It is demonstrated that in addition to the anti-Stokes component, the Stokes component with a maximum at 820 nm (referred to the H-aggregates of initial dyes) is observed in the fluorescence spectra of solutions of the examined molecules when dye concentration increases to 10⁻³ M. Dependences of the anti-Stokes and Stokes component intensities on the exciting radiation power are obtained that confirm a linear excitation character. On examples of xanthene and polymethine dyes, the use of organic fluorophors for anti-Stokes laser cooling and some other possible applications of the anti-Stokes fluorescence are discussed. __________ Translated from Izvestiya Vysshikh Uchebnykh Zavedenii, Fizika, No. 3, pp. 63–70, March, 2007.     

Nondegenerate four-wave mixing in a birefringent optical fiber pumped by a dye laser

An efficient nondegenerate four-wave-mixing process in a highly birefringent optical fiber pumped by a dye laser is reported. The output beam from a dye laser (at ~610 nm) was found to mix with the accompanying superfluorescent light (from 575 to 600 nm) in a birefringent fiber to generate a distinct frequency-shifted beam, which could be Stokes or anti-Stokes radiation, depending on which mode of the fiber was excited. The frequency shift was comparable with that observed in the well-known pump-divided degenerate process, as confirmed by the theory.     

Polarization enhancement of anti-Stokes emission in a para-H2 Raman laser

The effect of polarization can influence the frequency conversion and enhance the anti-Stokes emission in a rotational para-H₂ Raman laser. Stokes (16 μm) and anti-Stokes (7 μm) radiations were obtained from a line tunable CO₂ laser at 10 μm.     

Continuously tunable VUV radiation (129–210 nm) by anti-Stokes Raman scattering in cooled H2

The generation of tunable vacuum ultraviolet radiation by anti-Stokes Raman scattering of tunable ultraviolet dye-laser radiation in cold hydrogen has been investigated. The scattering efficiency of XeCl laser and Nd:YAG laser pumped commercial dye lasers and the influence of different beam profiles has been studied. Up to 12 anti-Stokes orders down to 129 nm were observed with output powers between about 20 kW at =191 nm and somewhat less than 100 W at =129 nm. The efficiency of transversely pumped lasers with an intensity peaked in the center of the beam profile was found to be higher than doughnut shaped intensity distributions. The cooling of the active gas to liquid nitrogen temperatures improved the output pulse energies 3 to 5 times on average. It was found that this intensity increase was caused mainly by the narrowing of the Raman linewidth upon cooling.     

Generation of tunable cw infrared radiation by difference frequency mixing

Tunable cw infrared radiation has been generated by noncollinear difference frequency mixing in LiIO₃, using the output of an argon ion laser at 514 nm or 488 nm and the intracavity radiation of a Rhodamine 6 G dye laser. Infrared powers up to 4 μW in multimode and 0.5 μW in single-mode operation tunable in the range of 2.3 μm to 4.6 μm have been obtained. Properties and possibilities of the noncollinear mixing geometry and the intracavity mixing system are discussed.     

Tunable cw infrared radiation by noncollinear difference-frequency mixing

Tunable cw infrared radiation has been generated by non-collinear difference-frequency mixing in LiJO₃, using the intracavity radiation of a Nd:YAG laser and the output of a Rhodamine 6G dye laser. Infrared powers of ∽35 μW tunable from 1.28 μm to 1.62 μm have been obtained.     

Generation of Anti-Stokes Line in Fundamental Mode of Photonic Crystal Fibre

A photonic crystal fibre （PCF） with zero-dispersion wavelength around 800 nm is designed and fabricated. Simulated results show that the zero-dispersion wavelength of fundamental mode for this PCF is at 826nm, and phase-matched four-wave mixing can be achieved in fundamental mode. Using 20ors Ti：sapphire laser with central wavelength at 810nm as pump, the anti-Stokes line around 610hm ＆ generated efficiently. The output signal has a Gaussian-like profile, which indicates that the anti-Stokes signal is in the fundamental mode of the PCF. The energy of anti-Stokes signal is higher than that of residual pump laser and the maximum ratio of the anti-Stokes signal to the pump component in the output spectrum is estimated to be 1.2.     

Generation of picoseconds stimulated Raman scattering in a BaWO4 crystal and frequency up-conversion by difference-frequency generation in BBO

The characters of stimulated Raman scattering of BaWO₄ crystal excited by a picoseconds laser at 1064 nm are studied based on optical parametric amplification (OPA). Up to six-order Stokes components and five-order anti-Stokes components are observed. The SRS components are amplified by an OPA and the wavelength tunable range from 411 to 2594 nm is achieved with a maximum conversion efficiency of 38% using the OPA stage.     

Tunable coherent radiation source covering a spectral range from 185 to 880 nm

We have studied experimentally stimulated Raman scattering and 4-wave-interaction processes occuring in hydrogen gas, which is excited by a Nd:YAG-pumped dye laser. The tuning ranges of the various Stokes and anti-Stokes lines, which are generated with high efficiency, cover the spectrum from 185 to 880 nm without a gap.     

YbVO4晶体的受激拉曼散射

采用腔外单次通过方式,研究了一种新型晶体YbVO₄的受激拉曼散射.当抽运激光为532 nm皮秒脉冲时获得了3级斯托克斯线(558.47 nm, 587.92 nm, 620.67 nm)和1级反斯托克斯线(507.58 nm),测得YbVO₄晶体1级斯托克斯受激拉曼散射的稳态增益系数为17.8±0.2 cm/GW,受激拉曼散射的整体转换效率达到37%.实现了YbVO₄晶体对355 nm皮秒激光的受激拉曼散射,观察到1级斯托克斯线(366.1 关键词： 受激拉曼散射 稳态增益系数 转换效率 4晶体')" href="#">YbVO₄晶体     

Tunable far-infrared generation by difference frequency mixing in InSb

Far-infrared radiation tunable over the range 85–105 cm^-1 and at power levels of up to 10 μW has been generated by difference frequency mixing in InSb. The infra-red radiations which are mixed are a 10.6 μm TEA-CO₂ laser line and the tunable Stokes radiation produced from it by spin-flip Raman-laser action, again in an InSb sample. It is argued that careful choice of the free-carrier concentrations in the crystals used for (a) the Stokes generation and (b) the mixing, or the application of an electric field across the mixing sample, should considerably improve the far-infrared power levels.     

Multi-wavelength Brillouin fiber laser generation using dual-pass approach

A simple and compact multi-wavelength tunable Brillouin fiber laser (BFL) in conjunction with dual-pass approach is proposed and experimentally compared with the output of a conventional single ring cavity architecture. This BFL source is demonstrated using 10 km long non-zero dispersion shifted fiber (NZ-DSF) as a Brillouin gain medium. By single ring cavity configuration, odd-order Brillouin Stokes lines appear in the backward direction with the line spacing 0.16 nm (∼20 GHz) between each two consecutive waves. However, this single ring cavity in conjunction with dual-pass configuration is able to generate Brillouin Stokes lines with 0.08 nm spacing by providing bi-directional oscillations of Brillouin waves in both forward and backward directions. With a Brillouin pump power of 15.3 dBm, approximately up to 17 Brillouin Stokes lines are generated which is tunable over 40 nm tuning range.     

Generation of multiorder Stokes and anti-Stokes lines in a Brillouin erbium-fiber laser with a Sagnac loop mirror

We have demonstrated a novel multiwavelength lasing scheme in which a Brillouin erbium-fiber laser with a Sagnac loop mirror and a metal-coated planar mirror were used. The Sagnac loop permitted the simultaneous presence of a stimulated Brillouin scattering (SBS) pump and Stokes lines within the loop and thus generated high-order Stokes and anti-Stokes waves through a four-wave mixing (FWM) process. A total of 34 lines of Stokes and anti-Stokes waves with 0.08-nm line spacing was generated through the SBS and FWM processes with 1.5-mW SBS pump power at 1561 nm and 80-mW erbium-doped-fiber pump power.     

Enhanced stimulated Raman scattering in H<Subscript>2</Subscript> by seeding an SRS line into an H-ɛ Balmer line: Amplification-coupled laser wavelength shifter

The stimulated Raman scattering (SRS) in H₂ gas above the dissociation energy limit was recorded using a 266-nm UV laser. All of the observed Stokes and anti-Stokes SRS lines showed a normal behavior except the third Stokes SRS lines at 397.8 nm, which showed a substantial intensity enhancement of about a 36%-conversion efficiency of the pump energy. This enhancement in the SRS line is attributed to the seeding of the SRS line into the Balmer H-? line at 397 nm in molecular hydrogen. To the best of our knowledge, there is no report of any work on enhanced stimulated Raman scattering in H₂ by the seeding of the H-? Balmer line into the SRS line and attaining a very high intensity at the third Stokes SRS lines at 397.8 nm. The cell pressure and the laser pulse energy dependence of these SRS lines substantiate our explanation.     

Generation of continuous-wave 243-nm radiation by sum-frequency mixing

We have generated tunable cw radiation near 243 nm with a linewidth of less than 4 MHz by sum-frequency mixing the 351 nm radiation from an argon-ion laser with the 789 nm radiation from a ring dye laser in a crystal of ammonium dihydrogen phosphate held at moderate temperature. An external ring cavity, resonant with the dye laser, gives a power enhancement of about 12 in the sum-frequency generated radiation. Thermal lensing due to laser heating of the nonlinear crystal, distorded the 351 nm mode structure. This effect could limit the efficiency of the sum frequency mixing process.     

Continuous wave stimulated Raman scattering of benzene by fluorescence enhancement in hollow fused silica fiber

We present continuous wave stimulated Raman scattering (SRS) of benzene (C₆H₆) influenced by the fluorescent dye m‐cresol purple in a hollow fused silica fiber (HFSF). Because of the transmission loss of the HFSF filled with C₆H₆, the SRS occurs when the Stokes gain equals the transmission loss, with the loss taken at the Stokes wavelength. The 992 cm⁻¹ stimulated Stokes line has been obtained at the pump wavelength 658 nm, which cannot be obtained at 532 nm because the Stokes wavelength (562 nm) does not locate in the transmission loss. Also, the pump power is 35 mW with m‐cresol purple which is much lower than 800 mW without the dye. The profile of the 992 cm⁻¹ stimulated Stokes is changed, and the weak shoulders of the profile are amplified by fluorescence. These results are expected to be of relevance in applications on the tunable Raman laser at new wavelengths. Copyright © 2011 John Wiley & Sons, Ltd.     

在BBO中获得230.8—223.2nm高功率和频输出

用Q-YAG泵浦的Rh·6G染料激光在一块45°切割的β-BaB₂O₄(BBO)晶体中倍频,产生294.8—282.5nm范围的连续调谐输出,其能量为8mJ(在285nm处)。用这个倍频光与泵浦染料后剩余基波(1064nm)在另一块45°切割的BBO中和频,已获得230.8—223.2nm范围的连续调谐输出,其能量为120μJ,相应的峰值功率为12kW。还简述了获得高功率和频输出的关键技术。     

Efficient generation of tunable VUV laser radiation below 205 nm by SFM in BBO

Design and performance characteristics of a tunable dye laser system for sum frequency mixing (SFM) in a BBO crystal are presented. The system is composed of two tunable pulsed dye lasers pumped synchronously by the second harmonic of a commercial Nd:YAG laser. The radiation produced by the first dye laser is frequency doubled by second-harmonic generation (SHG) in KDP and subsequently mixed by SFM in BBO with the light of the second dye laser. The interest was focussed on generation of tunable laser radiation below 205 nm with high output power and long-time wavelength stability. High conversion efficiencies enable output energies of 100 J (20 kW) at 196 nm using only moderate Nd:YAG pump energies of 67 mJ. Altogether, a laser system with very good specifications for analytical application in the near VUV spectral region is reported.