共查询到18条相似文献,搜索用时 156 毫秒
1.
利用单个原子精确的光电离散射截面和物质的复介电常数,并考虑一定的分子力学模型,可以对凝聚态物质中的原子光电离截面进行定量研究.孙卫国等最近提出了一套研究真实体系中原子光电离截面的新方法.本文首次应用它们来研究碱土金属钠在不同密度状态下的光电离截面,结果表明新的光电离截面公式比著名的孤立原子光电离截面公式更具有优越性. 相似文献
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利用单个原子精确的光电离散射截面和物质的复介电常数,并考虑一定的分子力学模型,可以对凝聚态物质中的原子光电离截面进行定量研究。孙卫国等最近提出了一套研究真实体系中原子光电离截面的新方法。本首次应用它们来研究碱土金属钠在不同密度状态下的光电离截面,结果表明新的光电离截面公式比名的孤立原子光电离截面公式更具有优越性。 相似文献
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利用我们提出的普遍适用的精确光电离截面公式和介电影响函数研究了原子光电离共振结构受粒子数密度影响的效应.结果表明用新的光电离截面公式可以直接处理宏观环境对截面的影响,明显地优于孤立原子光电离截面公式. 相似文献
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原子分子真空紫外光吸收和光电离绝对截面的精确测量 总被引:1,自引:0,他引:1
介绍了一种精确测量原子分子真空紫外光吸收和光电离绝对截面的实验方法。该方法的主要特点是使用圆筒形多级电极,有效地收集光电离产生的电子和离子,并利用高通量的同步辐射作光源,精确地测量分子(原子)的绝对光吸收、光电离和光离解截面,以及光电离量子产率和光学振子强度分布等。利用该方法获得了Xe原子和N2分子的一些实验结果。 相似文献
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实验研究了钛原子在293~321 nm波段的共振增强多光子电离. 采用激光烧蚀和超声射流相结合的实验技术来制备自由原子,由飞行时间质谱仪实现对钛原子光电离产物的检测. 从离子信号强度对和激光强度的依赖关系导出了钛原子价电子激发态的光电离截面. 实验测量的一些激发态光电离截面在0.2~6.0 Mb. 通过对46Ti、47Ti、48Ti的光电离截面测量研究,没有发现明显的同位素依赖性. 相似文献
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本文采用多组态Dirac-Hartree-Fock方法研究了温稠密等离子体环境中Al12+离子的光电离过程. 等离子体效应采用SM屏蔽势来模拟(Stanton和Murillo在2015年提出). 计算中固定标度温度1.3eV,在强耦合等离子体环境下,研究了等离子体密度对能级,连续态波函数以及光电离截面的影响. 通过与相同等离子体条件下的Debye-Hückel模型势计算的光电离截面对比,发现两种模型对应的结果中未同时出现势形共振峰,这是由于本文采用的屏蔽模型包含等离子体简并、有限温度对动能的梯度修正和量子交换关联效应,对光电离截面的大小和共振结构具有显著影响. 相似文献
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Accurate expression for photoabsorption (photoionization) cross
sections of high density system proposed recently is used to study
the photoionization of solid gold. The results show that the present
theoretical photoionization cross sections have good agreement both in
structure and in magnitude with the experimental results of gold crystal.
The studies also indicate that both the real part ε' and the imaginary part ε" of the complex dielectric constant ε, and the dielectric
influence function of a nonideal system have rich structures in low
energy side with a range about 50 eV, and suggest that the influence
of particle interactions of surrounding particles with the
photoionized particle on the photoionization cross sections
can be easily investigated using the dielectric influence function.
The electron overlap effects are suggested to be implemented in the
future studies to improve the accuracy of theoretical photoionization
cross sections of a solid system. 相似文献
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An alternative expression for photoionization cross-section of atoms or molecules and a dielectric influence function (DIF) in a high-density system proposed recently are used to study the photoionization cross-sections of solid silver. It is suggested that a density turning point (DTP) of a photoionized system may be viewed as the critical point where the photoionization properties of atoms in a real system may have a notable change. The results show that the present theoretical photoionization cross-sections are in good agreement with the experimental results of a silver crystal both in structure and in magnitude. 相似文献
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Interference effects on the photoionization cross sections between two neighbouring atoms: nitrogen as an example 下载免费PDF全文
Interference effects on the photoionization cross sections
between two neighbouring atoms are considered based on the coherent
scattering of the ionized electrons by the two nuclei when their
separation is less than or comparable to the de Broglie wave length
of the ionized electrons. As an example, the single atomic nitrogen
ionization cross section and the total cross sections of two
nitrogen atoms with coherently added photoionization amplitudes are
calculated from the threshold to about 60~\AA (1~\AA=0.1~nm) of the
photon energy. The photoionization cross sections of atomic nitrogen
are obtained by using the close-coupling R-matrix method. In the
calculation 19 states are included. The ionization energy of the
atomic nitrogen and the photoionization cross sections agree well
with the experimental results. Based on the R-matrix results of
atomic nitrogen, the interference effects between two neighbouring
nitrogen atoms are obtained. It is shown that the interference
effects are considerable when electrons are ionized just above the
threshold, even for the separations between the two atoms are larger
than two times of the bond length of N2 molecules. Therefore, in
hot and dense samples, effects caused by the coherent interference
between the neighbours are expected to be observable for the total
photoionization cross sections. 相似文献
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Implementation of promising control schemes for the intensity and position of X-ray-laser beams with a photon energy up to several tens of kiloelectronvolts requires knowledge of the angular dependence of cross sections for photoionization of noble gas atoms by hard photons. Estimates of quadrupole corrections to the cross section for photoionization of a Kr atom by X-ray photons with an energy of about 25 keV are reported in this paper. An analytic expression for the cross section of the process is parameterized in a compact form convenient for analyzing angular distributions with an arbitrary polarization of a photon beam. 相似文献
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Mirroring doubly excited resonances in argon 总被引:1,自引:0,他引:1
Canton-Rogan SE Wills AA Gorczyca TW Wiedenhoeft M Nayandin O Liu CN Berrah N 《Physical review letters》2000,85(15):3113-3116
New features are revealed in the low-energy photoionization spectrum of Ar by critically combining high photon resolution and differential photoelectron spectroscopic techniques. Two LS-forbidden doubly excited resonances are seen in the 3p(-1)(3/2, 1/2) partial cross sections which exhibit mirroring profiles, resulting in complete cancellation in the total photoionization cross section, as was predicted by Liu and Starace [Phys. Rev. A 59, R1731 (1999)]. These results demonstrate that a new class of weakly spin-orbit induced, mirroring resonances should be observable in partial, but not in total, collisional cross sections involving atoms, molecules, and solids in general. 相似文献
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M. Ya. Agre 《Optics and Spectroscopy》2006,101(3):356-370
A compact invariant expression for the angular distribution of photoelectrons formed as a result of photoionization of axisymmetrically polarized atoms and molecules, including optically active molecules, is derived from the general symmetry considerations and using a recently developed bipolar harmonic reduction technique. In the angular distribution of photoelectrons, as well as in the total photoionization cross section, the dependence on all the geometric parameters is separated completely. The polarization of ionizing radiation can be arbitrary, with the partial polarization being specified by the Stokes parameters. The expression for the angular distribution of photoelectrons escaping from an atomic-molecular system oriented in the first order also determines the structure of the expression for the photoionization cross section of an unpolarized system with allowance for the spin polarization of a photoelectron or a photoion with the spin 1/2. The roles played by circular dichroism, chirality, etc., in the process of photoionization of oriented and aligned systems are analyzed in detail. 相似文献
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利用相对论平均自洽场理论, 研究了相对论波函数的小分量对原子光电离截面的影响。原子核尺寸效应将使波函数小分量对原子光电离截面的影响减弱。由于波函数沿径向空间被压缩, 电子离核的平均半径较小, 波函数小分量对高离化态离子光电离截面的影响比对一般原子要强得多。波函数小分量反映了相对论效应的基本特征, 从而也定性地说明了光电离过程中相对论效应的强弱。The effects of relativistic small radial component on atomic photoionization cross sections have been studied within relativistic average self consistent field theory. Relativistic effects are relatively unimportant for low photon energy, along with a review of high energy photoionization the relativistic effects are quite important. The effects of relativistic small radial component on photoionization process should show breakdown when the nuclear finite size effects is taken into account. The compression of wavefunction into the space near nucleus is so strong in highly charged ions that the electronic radius greatly decreases, and the effects of relativistic small radial component on photoionization cross sections turn to stronger than ordinary atoms. Since relativistic effects are extremely sensitive to the behavior of small radial component, the results are in good agreement with relativistic effects on photoionization cross section. 相似文献
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J. Hoszowska A. S. Kheifets M. Berset I. Bray W. Cao J.-Cl. Dousse K. Fennane M. Kav?i? Y. Kayser J. Szlachetko M. Szlachetko 《The European physical journal. Special topics》2009,169(1):23-27
We report on the investigation of the photon energy dependence of double 1s photoionization of light atoms and compare the
cross sections for hollow atom and He-like ion production. Measurements of the Kα hypersatellite x-ray spectra of Mg, Al,
and Si were carried out using the Fribourg high-resolution x-ray spectrometer installed at the ID21 and ID26 beam lines at
the ESRF. The double-to-single photoionization cross section ratios were derived as a function of the incident photon beam
energy and compared to convergent close-coupling (CCC) calculations for He-like ions. The dynamical electron-electron scattering
contribution to the DPI cross-sections was found to be more important for neutral atoms than for the He isoelectronic series. 相似文献