激光冷却在原子束六极磁透镜技术中的应用

分析了由六极磁场构成了原子束磁透镜的原理及像差。在比较了热原子束和单色冷原子束的会聚效果后得出结论：影响它成像的主要因素是色差。应用激光冷却技术能使这一影响减小,从而使磁透镜在原子光学领域得到更广泛的应用。     

Diffraction of fast metastable atoms by micrometric reflection gratings

Diffraction of thermal velocity metastable atoms by non-magnetic and magnetic reflection gratings of micrometric period has been observed. This observation is made possible by the use of an ultra narrow beam generated by metastability exchange. Grazing incidence angles are exploited to minimise the quenching of metastable atoms on the grating surface. Potential applications are beam splitting, atom holography and probing of micro-sized solid surfaces.     

Structure formation in atom lithography using geometric collimation

Atom lithography uses standing wave light fields as arrays of lenses to focus neutral atom beams into line patterns on a substrate. Laser cooled atom beams are commonly used, but an atom beam source with a small opening placed at a large distance from a substrate creates atom beams which are locally geometrically collimated on the substrate. These beams have local offset angles with respect to the substrate. We show that this affects the height, width, shape, and position of the created structures. We find that simulated effects are partially obscured in experiments by substrate-dependent diffusion of atoms, while scattering and interference just above the substrate limit the quality of the standing wave lens. We find that in atom lithography without laser cooling the atom beam source geometry is imaged onto the substrate by the standing wave lens. We therefore propose using structured atom beam sources to image more complex patterns on subwavelength scales in a massively parallel way.     

Characterization of an oriented metastable atom source based on a magnetic hexapole

The M_J-state selection of the metastable rare-gas (Rg*) was achieved by a magnetic hexapole that is composed of permanent magnets. The performance of the magnetic hexapole was examined by characterizing the velocity distribution and the spatial profile of the state selected Rg* beam. The characterization was carried out using position resolved time-of-flight analysis and its trajectory simulation. The magnetic hexapole enhanced the beam intensity at least one order of magnitude owing to the focusing effect. In addition, the magnetic hexapole was found to act as a good velocity selector.     

Nanolithography with metastable helium atoms in a high-power standing-wave light field

We have created periodic nanoscale structures in a gold substrate with a lithography process using metastable triplet helium atoms that damage a hydrophobic resist layer on top of the substrate. A beam of metastable helium atoms is transversely collimated and guided through an intense standing-wave light field. Compared to commonly used low-power optical masks, a high-power light field (saturation parameter of 10⁷) increases the confinement of the atoms in the standing wave considerably, and makes the alignment of the experimental setup less critical. Due to the high internal energy of the metastable helium atoms (20 eV), a dose of only one atom per resist molecule is required. With an exposure time of only eight minutes, parallel lines with a separation of 542 nm and a width of 100 nm (one-eleventh of the wavelength used for the optical mask) are created.PACS 32.80.Lg; 39.25.+k; 81.16.Nd     

Change of the refractive index in PPLN waveguides due to the photorefractive effect

We present a new method for nanoscale atom lithography. We propose the use of a supersonic atomic beam, which provides an extremely high brightness and cold source of fast atoms. The atoms are to be focused onto a substrate using a thin magnetic film, into which apertures with widths on the order of 100 nm have been etched. Focused spot sizes near or below 10 nm, with focal lengths on the order of 10 μm, are predicted. Our method can be implemented in a highly parallel manner, enabling simultaneous fabrication of 10⁶ identical elements, and it is applicable both to precision patterning of surfaces with metastable atomic beams and to direct deposition of material.     

离散效应对高强度激光三次谐波转换的影响

使用分步傅里叶变换和四阶龙格库塔法(R-K) ，对高强度激光以Ⅰ/Ⅱ类角度失谐方式，在KDP晶体中的谐波转换进行了研究，详细讨论了离散效应对三次谐波转换的影响。结果表明，离散效应不但降低了三次谐波转换效率，而且使谐波光束质量显著降低；初始入射基频光束腰半径较小时，离散效应是二次谐波转换和三次谐波转换效率降低的主要因素，失谐角对三次谐波转换的影响较小；随着束腰半径的增加，离散效应的影响逐渐减小，失谐角对三次谐波转换的影响逐渐增加。     

量子模型分析激光驻波原子透镜的像差

采用量子模型对近共振激光驻波原子透镜会聚Cr原子束、形成纳米量级光栅结构的物理过程进行数值模拟。为提高原子透镜的成像质量,对各种像差,如衍射像差、球差、色差、及原子束发散角、原子磁支能级、原子同位素等因素引起的像差进行了理论分析。模拟结果表明,相比粒子光学模型,量子模型能更加精确地描述原子会聚结果,且能解释原子在驻波光场中的衍射现象。在各种像差中,原子束发散角是最主要的因素,其影响大于衍射像差、球差、色差。原子的磁支能级、同位素等因素对像差影响很小,可以忽略不计。激光冷却准直原子束的方法可以减小束发散角引起的像差,压缩原子速度Vz分布范围的方法可以减小色差。     

Atom lithography with a cold, metastable neon beam

We study different aspects of atom lithography with metastable neon atoms. Proximity printing of stencil masks is used to test suitable resists that are sensitive to the internal energy of the atoms, including dodecanethiols on gold and octadecyltrichlorosilanes grown on a SiO₂ surface. As an example of patterning the atomic beam with laser light, we create parallel line structures on the surface with a periodicity of half the laser wavelength by locally de-exciting the atoms in a standing quenching wave. Received: 29 June 1999 / Revised version: 30 August 1999 / Published online: 10 November 1999     

Enlarging lens design with f-Θ lens for real time laser lithography inspections

An enlarging lens, composed of a charge-coupled-device (CCD) lens and an f-Θ lens, has been designed for real time laser lithography visual inspection purposes. The object of this design is to enlarge the image of the working specimens in real time, which used to be done by an independent magnifying system after the lithography process. F-Θ lens has both roles in this design, being a laser lithography lens and a specimen imaging lens. A beam splitter has been inserted between the f-Θ lens and the CCD lens, which divides the UV laser beam and the visible beam to form a coaxial system. This design also reaches the image requirements in both wavelength bands, that the value of MTF is nearly diffraction-limit in UV wavelength and greater than 0.45 at 40 c/mm in visible wavelength.     

Emission characteristics of a barrier discharge in an Ar-H2O mixture

We have experimentally studied the UV radiation of a low-temperature barrier discharge plasma in an Ar-H₂O mixture. The spectral interval 300–400 nm has been examined in detail. Addition of argon with a pressure of 24 kPa to a barrier discharge in water vapor at a pressure of ～0.1 kPa leads to a ninefold increase in the UV radiation power of excited hydroxyl molecules. An increase in the duration of the UV radiation pulse of the mixture in the longitudinal discharge decay has been achieved for the first time, which may be direct evidence of energy transfer from metastable argon atoms to water molecules. An estimate of the upper boundary of the dissociative excitation rate constant of hydroxyl molecules OH*(A ²Σ⁺) upon interaction of metastable argon atoms with water molecules has been obtained.     

Spontaneous excitation of a circularly accelerated atom coupled with vacuum Dirac field fluctuations

We study the spontaneous excitation of a circularly accelerated atom coupled with vacuum Dirac field fluctuations by separately calculating the contribution to the excitation rate of vacuum fluctuations and a cross term which involves both vacuum fluctuations and radiation reaction, and demonstrate that although the spontaneous excitation for the atom in its ground state would occur in vacuum, such atoms in circular motion do not perceive a pure thermal radiation as their counterparts in linear acceleration do since the transition rates of the atom do not contain the Planckian factor characterizing a thermal bath. We also find that the contribution of the cross term that plays the same role as that of radiation reaction in the scalar and electromagnetic fields cases differs for atoms in circular motion from those in linear acceleration. This suggests that the conclusion drawn for atoms coupled with the scalar and electromagnetic fields that the contribution of radiation reaction to the mean rate of change of atomic energy does not vary as the trajectory of the atom changes from linear acceleration to circular motion is not a general trait that applies to the Dirac field where the role of radiation reaction is played by the cross term.     

Dynamics of spontaneous radiation of atoms scattered by a resonance standing light wave

The scattering of atoms by a resonance standing light wave is considered under conditions when the lower of two resonance levels is metastable, while the upper level rapidly decays due to mainly spontaneous radiative transitions to the nonresonance levels of an atom. The diffraction scattering regime is studied, when the Rabi frequency is sufficiently high and many diffraction maxima are formed due to scattering. The dynamics of spontaneous radiation of an atom is investigated. It is shown that scattering slows down substantially the radiative decay of the atom. The regions and characteristics of the power and exponential decay are determined. The adiabatic and nonadiabatic scattering regimes are studied. It is shown that the wave packets of atoms in the metastable and resonance excited states narrow down during scattering. A limiting (minimal) size of the wave packets is found, which is achieved upon nonadiabatic scattering in the case of a sufficiently long interaction time.     

Nanolithography with metastabile helium

We have used a self-assembling monolayer of dodecanethiole molecules as the resist for a lithography technique based on a beam of metastable helium atoms. Doses as low as 3 metastable helium atoms per 10 molecules are enough to write patterns into this resist. An edge resolution of 30 nanometers is demonstrated. The writing mechanism is based on the damage of the resist due to Penning ionization.     

Nanoscale focusing of atoms with a pulsed standing wave

We have theoretically and experimentally investigated the focusing properties of a detuned pulsed standing wave onto a beam of neutral atoms. In close analogy to the continuous-wave situation the dipole force leads to a periodic focusing of atoms with a period of λ/2, provided an adiabatic condition is fulfilled. Pulsed laser light is conveniently converted to short wavelengths and hence offers advantages in the application of atom lithography with elements of technological interest having blue or UV resonance lines. Received: 6 October 1999 / Revised version: 3 February 2000 / Published online: 5 April 2000     

Laser cooling without repumping: a magneto-optical trap for erbium atoms

We report on a novel mechanism that allows for strong laser cooling of atoms that do not have a closed cycling transition. This mechanism is observed in a magneto-optical trap (MOT) for erbium, an atom with a very complex energy level structure with multiple pathways for optical-pumping losses. We observe surprisingly high trap populations of over 10(6) atoms and densities of over 10(11) atoms cm(-3), despite the many potential loss channels. A model based on recycling of metastable and ground state atoms held in the quadrupole magnetic field of the trap explains the high trap population, and agrees well with time-dependent measurements of MOT fluorescence. The demonstration of trapping of a rare-earth atom such as erbium opens a wide range of new possibilities for practical applications and fundamental studies with cold atoms.     

Simultaneous magneto-optical trapping of a boson-fermion mixture of metastable helium atoms

We simultaneously confine fermionic metastable 3He atoms and bosonic metastable 4He atoms in a magneto-optical trap. The trapped clouds, containing up to 1.5 x 10(8) atoms of each isotope, are characterized by measuring ions and metastable helium atoms escaping from the trap. Optical pumping of 3He atoms to a nontrapped hyperfine state is investigated and it is shown that large atom numbers can be confined without additional repumping lasers. Unique possibilities for quantum degeneracy experiments with mixtures of spin-polarized metastable 3He and 4He atoms are indicated.     

一种紫外或深紫外光刻的1：1折反射式光学系统

设计了一种新的紫外或深紫外光刻物镜。该物镜与国内外现有的紫外或深紫外光刻物镜相比，既能满足大数值孔径的需要，又能充分利用物镜的视场。采用环形照明，能缓解因增大数值孔径而使焦深缩短的矛盾。     

Absolute desorption yields of metastable atoms from the surface of solid rare gases induced by exciton creation

Absolute yields of the metastable excited atoms desorbed from the surfaces of solid Ne and Ar by the creation of surface and bulk excitons have been measured using monochromated synchrotron radiation as a selective excitation source. We have obtained the absolute yields of (2.3 ± 0.7) × 10⁻³, (1.4 ± 0.4) × 10⁻³, and (7.8 ± 2.3) × 10⁻⁴ atoms/photon at the excitation of S1, B1 and S′ exciton for Ne, respectively, and 1 × 10⁻⁵ atoms/photon at S1 excitation for Ar. The probability for metastable atom desorption is found to be about 2 to 10% at the excitation of S1 exciton on the surface of solid Ne.     

辐射的相干性和熵的增加

本文讨论一个多原子辐射模型:N个有两能级的原子体系(A),与一个单模辐射(B)彼此耦合,A和B又分别同热库D和C耦合,假设在辐射场波长范围内所有原子有相同的相位,则在长波、旋转波和平均场近似下,用密度矩阵方法,引入Markov近似,便可导得A,B两体系的运动方程,这一组方程包含了单原子的自发辐射和热辐射引起的吸收、感应辐射,同时也包含了单模相干态辐射引起的N个原子的感应辐射以及这多原子体系的相干自发辐射过程。后两种过程实际上是始于Dicke模型而后曾被人们多次讨论过的两类超辐射过程,我们对上述五种过程进行 关键词：