ZnGeP2 optical parametric oscillator with 3.8-12.4-mum tunability

A ZnGeP>(2) (ZGP) optical parametric oscillator (OPO) with wide mid-IR tunability has been demonstrated. The singly resonant angle-tuned ZGP OPO was pumped by 100-ns erbium laser pulses at lambda =2.93mum and yielded output that was continuously tunable from 3.8 to 12.4 mum (type I phase matching) and from 4 to 10 mum (type II phase matching). An OPO pump threshold was less than 1 mJ in the whole 4-12 mum range of the output, and the quantum conversion efficiency reached 35%. An OPO linewidth was typically a few wave numbers; however, with a single intracavity etalon (uncoated Si plate) in a type II OPO it was narrowed to <0.5cm(-1). We demonstrate the sensitive detection of N(2)O gas with the narrow-linewidth OPO.     

2.5-GHz repetition-rate singly resonant optical parametric oscillator synchronously pumped by a mode-locked diode oscillator amplifier system

We report on an optical parametric oscillator (OPO) that is synchronously pumped directly by a diode laser. This laser is an actively mode-locked master-oscillator power-amplifier system that produces 20-ps pulses at 927 nm with a repetition rate of 2.5 GHz and an average power of 0.9 W. The OPO, which is a singly resonant device based on periodically poled lithium niobate, generates 7.8-ps pulses. The OPO threshold is 300 mW of average pump power, and the maximum average idler output power is 78 mW at a wavelength of 2100 nm. By changing the crystal temperature we can wavelength tune the output in the ranges 1530-1737 nm (signal) and 1986-2348 nm (idler). Rapid wavelength tuning of the OPO over 46 nm (signal) and 74 nm (idler) is achieved through tuning the cavity length over 28 microm by use of a piezoelectric transducer.     

Wavelength-agile mid-infrared (5-10 microm) generation using a galvano-controlled KTiOPO4 optical parametric oscillator

A wavelength-agile mid-infrared (IR) ZnGeP2 (ZGP) optical parametric oscillator (OPO) using a galvano-controlled double-crystal KTiOPO4 (KTP) OPO was demonstrated. The mid-IR wavelength was tuned by varying the KTP OPO pump wavelength while the ZGP crystal angle remained fixed. Rapid tuning of the KTP OPO was achieved by changing the crystal angle by using the galvano scanner. Our mid-IR source can jump to a different wavelength without scanning through the intermediate wavelengths while also permitting continuous-wavelength scanning. The mid-IR source can be tuned from approximately 5to10 microm at a phase-matching angle of 51 degrees , while the pump wavelength is controlled in the 1.95-2.2 microm range.     

Optical parametric oscillation in quasi-phase-matched GaAs

We demonstrate an optical parametric oscillator (OPO) based on GaAs. The OPO utilizes an all-epitaxially-grown orientation-patterned GaAs crystal that is 0.5 mm thick, 5 mm wide, and 11 mm long, with a domain reversal period of 61.2 microm. Tuning either the near-IR pump wavelength between 1.8 and 2 microm or the temperature of the GaAs crystal allows the mid-IR output to be tuned between 2.28 and 9.14 microm, which is limited only by the spectral range of the OPO mirrors. The pump threshold of the singly resonant OPO is 16 microJ for the 6-ns pump pulses, and the photon conversion slope efficiency reaches 54%. We also show experimentally the possibility of pump-polarization-independent frequency conversion in GaAs.     

1.2 W中红外ZnGeP2光参量振荡器

报导了利用Tm,HoGdVO4激光器抽运双谐振ZnGeP2光参量振荡器实验研究.Tm(5%),Ho(0.5%)GdVO4晶体采用液氮制冷方式,工作在77 K温度条件下.以25 W波长为800 nm的光纤耦合激光二极管抽运,2 μm激光最大平均功率7 W,脉冲宽度小于30 ns, 脉冲重复频率5 kHz到20 kHz可调.非线性频率转换晶体ZnGeP2长15 mm,55?切割,OPO谐振腔为平平腔,腔长约25 mm.在5W的2 μm激光抽运下,脉冲重复频率10 kHz,实现了信号光3.7 μm及闲频光4.5 μm中红外激光输出,参量光脉冲宽度为15～17 ns,最大平均功率大于1.2 W,光-光转换效率为20%.测量参量光输出光束全宽度远场发散角4 mrad,光束质量M2因子小于3.     

Mid-IR frequency comb source spanning 4.4-5.4 μm based on subharmonic GaAs optical parametric oscillator

Broadband mid-IR output suitable for producing 1000-nm-wide frequency combs centered at 4.9?μm was achieved in a degenerate subharmonic optical parametric oscillator (OPO) based on 500-μm-long Brewster-angled orientation-patterned GaAs crystal. The OPO was synchronously pumped at 182 MHz repetition rate by 100 fs pulses from a Cr2?:ZnSe laser with the central wavelength of 2.45?μm and the average power of 100 mW.     

High-average-power mid-infrared ZnGeP2 optical parametric oscillator with a wavelength-dependent polarization rotator

A wavelength-dependent polarization rotator is used to transform the orthogonal polarizations of the signal and idler of a near-degenerate type II KTP optical parametric oscillator (OPO) into a common polarization state. This common polarization allows a single ZnGeP2 OPO to fully utilize the 2 microm signal and idler KTP OPO outputs in a mid-IR conversion. The simple design of the wavelength-dependent polarization rotator yields a compact source that simultaneously generates four mid-JR wavelengths collinearly with a total mid-IR average power of 5.5 W at a >15 kHz pulse repetition rate.     

Efficient conversion from 1 to 2 microm by a KTP-based ring optical parametric oscillator

Conversion of Q -switched 1.064-microm Nd:YAG laser pulses to the 2-2.2-mu; m region with 46% efficiency is demonstrated with a KTP-based type 2 phase-matched optical parametric oscillator (OPO) with two pairs of walk-off compensating crystals in a ring resonator. With 10 mJ of pump energy, we obtain 2.5 mJ at the 2.06-microm signal and 2.1 mJ at the 2.2-microm idler, with a beam quality of M(2) approximately 1.4 . With a ZnGeP(2) -based OPO pumped by the signal from the KTP OPO we achieved 14% conversion efficiency from 1.064microm to the 3-5-microm range.     

Laser-photofield emission from needle cathodes for low-emittance electron beams

Illumination of a ZrC needle with short laser pulses (16 ps, 266 nm) while high voltage pulses (-60 kV, 2 ns, 30 Hz) are applied, produces photo-field emitted electron bunches. The electric field is high and varies rapidly over the needle surface so that quantum efficiency (QE) near the apex can be much higher than for a flat photocathode due to the Schottky effect. Up to 150 pC (2.9 A peak current) have been extracted by photo-field emission from a ZrC needle. The effective emitting area has an estimated radius below 50 microm leading to a theoretical intrinsic emittance below 0.05 mm mrad.     

Tunable, high-repetition-rate, femtosecond pulse generation in the ultraviolet

We report efficient generation of tunable femtosecond pulses in the ultraviolet (UV) by intracavity doubling of a visible femtosecond optical parametric oscillator (OPO). The OPO, based on a 400 microm BiB3O6 crystal and pumped at 415 nm in the blue, can provide visible femtosecond signal pulses across 500-710 nm. Using a 500 microm crystal of beta-BaB2O4 internal to the OPO cavity, efficient frequency doubling of the signal pulses into the UV is achieved, providing tunable femtosecond pulses across 250-355 nm with up to 225 mW of average power at 76 MHz. Cross-correlation measurements result in UV pulses with durations down to 132 fs for 180 fs blue pump pulses.     

Broadly tunable noncritically phase-matched ZnGeP2 optical parametric oscillator with a 2-microJ pump threshold

We report a high-repetition-rate (1-10-kHz) optical parametric oscillator (OPO) based on noncritically phase-matched ZnGeP2 (ZGP). The pump source was an OPO based on periodically pole lithium niobate that was pumped in turn by a Q-switched diode-pumped 1-microm Nd:YAG laser. The ZGP OPO yielded continuously tunable output from 3.7 to 10.2 microm by tuning of the pump wavelength from 2.3 to 3.7 microm. At the optimal pump focusing, the minimum ZGP OPO threshold achieved was 2 microJ, which is to our knowledge the lowest ever reported for a singly resonant OPO. The output energy in the 6-8-microm range was > 20 microJ, and the quantum efficiency of converting 1-microm radiation to the mid IR exceeded 10%.     

Amplified Spontaneous Emision of K2Yellow Band Excimer and Its Gain Measurement by e-beam-pumpingResearch on Injection-seeded β-BaB2O4Optical Parameteric Oscillator

The design of a high temperature cell appropriate for electron beam side pumping of alkali excimer lasers is described. By using the cell, an amplified spontaneous emission (ASE) and small signal gain coefficient of 4% cm-1 of the K2 yellow band (574 nm) were observed from the e beam excited mixture of K/K2 vapor with argon buffer gas. The dissociative recombination of K+3 is discussed as an efficient formation process of upper states by electron beam pumping.It has demonstrated the feasibility of a β-BaB2O4 optical parametric oscillator(OPO) without frequency control elements that produces very narrow bandwidth, 10 ns pulses via injection seeding. It was achieved by a CW He Ne laser and the experiment threshold for injection seeding is less than 1 mW. With 25 mJ pump energy at 354.7 nm, it has obtained pulse energy of 2 mJ at 632.8 nm and the total effiency is greater than 15%.     

Generation of mid-infrared pulses by X(3) difference frequency generation in CaF(2) and BaF(2)

Tunable mid-IR pulses in the range 1300-4200 cm(-1) (7.7-2.4 microm) are generated through a phase-matched four-wave mixing process in ordinary mid-IR window materials such as CaF(2) and BaF(2) . In this process the difference frequency v(3)=2v(2)-v(1) is generated from pump fields v(1) and v(2) . The process can be phase matched to different frequencies by adjustment of the angle between the pump fields.     

A ring ZnGeP2 optical parametric oscillator pumped by a Ho:LuAG laser

We have demonstrated that we believe to be the first ring ZnGeP₂ (ZGP) optical parametric oscillator (OPO) pumped by a pulsed Ho:LuAG laser. The maximum output power of the ring ZGP OPO laser was 5.51 W at 13.1 W incident Ho pump power, corresponding to a slope efficiency of 59.0 %. The ZGP OPO laser produced 14 ns mid-infrared pulses in the 3.72–4.01 and 4.37–4.75 μm spectral regions simultaneously. In addition, the continuous wave Ho:LuAG laser generated 26.5 W of linearly output at 2,094.4 nm at the absorbed Tm pump power of 49.9 W.     

Intense self-compressed, self-phase-stabilized few-cycle pulses at 2 microm from an optical filament

We report the compression of intense, carrier-envelope phase stable mid-IR pulses down to few-cycle duration using an optical filament. A filament in xenon gas is formed by using self-phase stabilized 330 microJ 55 fs pulses at 2 microm produced via difference-frequency generation in a Ti:sapphire-pumped optical parametric amplifier. The ultrabroadband 2 microm carrier-wavelength output is self-compressed below 3 optical cycles and has a 270 microJ pulse energy. The self-locked phase offset of the 2 microm difference-frequency field is preserved after filamentation. This is to our knowledge the first experimental realization of pulse compression in optical filaments at mid-IR wavelengths (lambda>0.8 microm).     

Mercury thiogallate mid-infrared femtosecond optical parametric generator pumped at 1.25 microm by a Cr:forsterite regenerative amplifier

We demonstrate a novel traveling-wave-type optical parametric generator based on 1.25-microm pumping of HgGa(2)S(4) that produces tunable, high-power, transform-limited infinity 200-fs pulses in the mid-IR from 5 to 9 microm. Output idler energies on the microjoule level are obtained with maximum conversion efficiency of 11% for the amplifier stage, which is more than two times better than the results obtained with an analogous sample of the widely spread material AgGaS(2).     

30-fs, cavity-dumped optical parametric oscillator

We demonstrate cavity dumping of a synchronously pumped optical parametric oscillator (OPO). The OPO delivers 30-fs pulses with energies as high as 13 nJ at up to 400-kHz repetition rates. The OPO's tunability ranges from 570 to 600 nm and is limited by the resonator mirror coatings. The time jitter between pulses of a Ti:sapphire laser and the cavity-dumped OPO pulses is smaller than 30 fs, permitting multicolor time-resolved spectroscopic experiments.     

High-power mid-infrared tunable optical parametric oscillator based on 3-mm-thick PPMgCLN

The experimental results of a high-power tunable mid-IR laser are presented. The optical parametric oscillator (OPO) with a 3-mm-thick PPMgCLN crystal was pumped by a 1.064 μm pulse laser. When the pump power of the 1.064 μm laser was 151 W at 10 kHz, and the operating temperature of the PPMgCLN with 5% MgO doping was 100°C, average output power of 23.7 W at 3.91 μm was obtained with a slope efficiency of 18.2% for the idler resonant OPO. The variation of the 3.91 μm output power was about ±4% in 10 min continuous operation. The beam quality factor M ² was less than 2.6. The average output power of 27.4 W at 3.91 μm was also obtained with 151 W pump power and the slope efficiency of 20.9% for the signal resonant OPO by changing the coating parameters of the OPO cavity mirrors. The mid-IR wavelength tunability of 3.7–4.0 μm can be achieved by adjusting the temperature of a 29 μm period PPMgCLN crystal from 200 to 30°C.     

Femtosecond pulse shaping directly in the mid-IR using acousto-optic modulation

Pulse shaping directly in the mid-IR is accomplished by using a germanium acousto-optic modulator (Ge AOM) capable of programmable phase and amplitude modulation for IR light between 2 and 18 microm. Shaped waveforms centered at 4.9 microm are demonstrated in both the frequency and the time domains. With a 50% throughput efficiency, the Ge AOM can generate much more intense pulses with higher resolution than can indirect shaping methods. Furthermore, the phase stability of the shaped pulse proved sufficient for cross correlation with unshaped mid-IR pulses. Thus, phase- and amplitude-tailored pulses can now be readily incorporated into phase-sensitive experiments, such as heterodyned 2D IR spectroscopy.     

Amplitude and phase measurement of mid-infrared femtosecond pulses by using cross-correlation frequency-resolved optical gating

We describe a cross-correlation-based frequency-resolved optical gating (XFROG) technique for simultaneously measuring the amplitude and phase of two ultrashort pulses that have different wavelengths but are derived from a common mode-locked oscillator. A measurement is presented in which 4.0-mum mid-IR pulses from a synchronously pumped femtosecond optical parametric oscillator (OPO) are characterized by mixing with the 770-nm OPO pump pulses. Details of the pulse-retrieval algorithm are included, together with examples of pulse data retrieved from the experimentally measured XFROG trace.