共查询到20条相似文献,搜索用时 78 毫秒
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用扫描隧道显微镜(STM)研究了亚单层In原子引起的Ge(112)-(4×1)-In表面重构.结合随偏压极性不同而显著不同的STM图象和相应的“原子图象”,为这个重构提出了一个原子结构模型,供进一步研究参考.其中,In原子的吸附位置与它在Si(112)表面的吸附位置一致,但与Al原子和Ga原子在Si(112)表面的吸附位置不同.这个吸附位置的不同主要是由In原子较长的共价键键长引起的
关键词:
表面结构
In
Ge
扫描隧道显微镜(STM) 相似文献
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概述了扫描隧道显微镜(STM)的应用,讨论了扫描隧道显微镜(STM)对不同样品测试的条件,这对STM图象的分析有着重要的作用。 相似文献
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报道了利用扫描隧道显微术(STM)对金属表面氧化物层进行电子隧道谱研究的结果。在对两类铁晶体表面氧化层进行的隧道谱和势垒高度测量结果进行分析后表明,常温条件下形成的氧化层(Ⅰ类)应主要是Fe3O4;而在高温氧化条件下形成的表面层(Ⅱ类)的主要成分则应是Fe2O3。从而表明(STM)可用于研究铁表面氧化过程的不同阶段,并且由Ⅰ类氧化层的低势垒特性说明STM还可以用于观测此类氧化层的内部结构。类似研究方法还可应用到对一系列
关键词: 相似文献
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用低能电子衍射(LEED)和扫描隧道显微镜技术研究了氧气在Cu(100)表面化学吸附所形成的表面重构结构.在低覆盖度下,实验上观察到了两个有序重构的混合相,分别为c(2×2)O重构和(√2×2√2)R45°-O重构.在氧原子的覆盖度逐渐增加的过程中,c(2×2)O重构区域的面积逐渐减小.在初始氧化阶段,实验上观察到了呈条状的“锯齿”形的重构结构,这些锯齿形的结构是由相邻的局域化的c(2×2)区域的边界区域(Cu)构成的.STM实验发现,相对于其他重构区域,这些锯齿形的重构区域与有机分子之间存在更加强烈的相互作用.通过分析在不同退火温度下样品LEED衍射点的变化,研究了重构结构的热稳定性,发现三种结构的热稳定性顺序是:锯齿结构>c(2×2)O重构>(√2×2√2)R45°-O重构. 相似文献
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用扫描隧道显微镜(STM)对Cu(111)-Au和Cu(111)-Pd表面的局域功函数进行了研究.通过 测量隧道电流对针尖样品间距的响应,得到了与STM形貌图一一对应的表面局域功函数图像. 实验发现,Au/Pd覆盖层和Cu衬底间的功函数有明显的不同.Pd薄膜的功函数甚至超过了其体 本征值,且功函数在台阶处变小.用偶极子的形成解释了台阶处功函数的降低.这一工作表明 ,用测量局域功函数的方法容易区分表面上不同的元素,并具有纳米尺度的空间分辨率.
关键词:
扫描隧道显微镜
局域功函数
台阶 相似文献
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20世纪重要的发明之一就是扫描隧道显微镜 ,简称为STM .它能对金属及其他导电表面给出原子水平上的形态结构图 .最近美国科罗拉多矿学院的P .Sutter教授对STM设计了一种新的技术 ,称之为“能量过滤STM” .这项技术类似于在普通显微镜上加一个“颜色滤波片” ,使我们能方便地在摄影时分辨出想要寻找的特征 .同时 ,“能量过滤STM”也使我们能容易地区分出一些具有相似化学性质的原子 ,这类原子用其他手段常常很难分辨 .“能量过滤STM”还能确认在表面上的各种类别的化学键 .一般的STM是使用一个金属的探针 ,它对导电表面上的高能电子… 相似文献
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双成象单元扫描隧道显微镜与原子尺纳米计量技术 总被引:3,自引:3,他引:0
研制了双成象单元扫描隧道显微镜(STM),可同时对参考样品的原子晶格和被测样品扫描成象.计数原子晶格的数目,即可精确测定被测样品图象的尺度,以原子尺方式实现严格的纳米计量.本文介绍双成象单元的STM的原理和仪器系统,讨论原子尺纳米计量的可行性,给出被测样品图象的纳米计量结果. 相似文献
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本文展示了结构紧凑的(高度为66 mm,直径为25 mm)扫描隧道显微镜,配备了一套拥有原子级分辨精度的三维压电马达。其中Z方向定位依靠的是自行发明的由轴向切割的压电扫描管驱动的摩擦型步进器。X-Y方向(即样品面方向)的移动是将Z向步进器作为一个惯性滑块垂直嵌入压电扫描管内同时一端平放在压电扫描管的顶部。其设计具有在极端条件下(低温、强磁场等)从宏观尺度样品区域(平方毫米级别)搜索微观靶向(缺陷位、掺杂位、边界及纳米器件等)的能力。在室温大气下对高定向热解石墨进行测量,得到了高分辨率的原子图像. 相似文献
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Haixia Shang Huimin Xie Zhanwei Liu Haiming Guo Hongjun Gao Fulong Dai 《Optics and Lasers in Engineering》2004,41(5):498
In this paper, a new nano-moiré method using scanning tunneling microscope (STM) is proposed. This method is capable of measuring nanoscopic deformation of matter. The formation mechanism of the STM moiré fringe and the phase shifting technique used in STM moiré fringes are explained in details. Typical experiments are conducted with the crystal lattices of freshly cleaved highly oriented pyrolytic graphite, are used as specimen grating, to generate STM moiré fringe patterns. Phase shifting is realized in four steps from 0 to 2π by controlling the PZT in the STM system to shift the specimen in the vertical direction. This method provides a new way for disposal of moiré fringes pattern in the nano-moiré measurement. 相似文献
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利用第一性原理方法模拟了自由钒氧酞菁(VOPc)和钒酞菁(VPc)分子的扫描隧道显微镜(STM)图像,与实验观察结果相当符合.理论STM图像都显示出亚分子内结构,外围呈四叶状.其主要差异表现在VOPc分子中心处的钒氧离子在STM图像中为一空洞,而在VPc分子的STM图像中钒离子为突起的亮斑.通过分析VOPc和VPc分子的电子结构,对模拟结果给出自洽的理论解释.造成两者图像显著不同的物理原因是VPc分子在费米能级附近有明显含dz2成分的分子轨道,导致钒离子在STM图像中央为突起的亮斑.而在VOPc分子中dz2分态密度峰位由于氧原子的加入使之远离费米能级,使STM不能“看到”VOPc分子中钒氧离子.
关键词:
钒氧酞菁
钒酞菁
STM图像模拟
电子结构 相似文献
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To modulate the tunneling gap with the lock-in amplifier in the scanning tunneling microscopy(STM), information of the tunneling current variation can be obtained. The local potential barrier distribution of graphite surface atoms is got by means of such technology. Compared with STM image under topography observation mode, the local potential barrier image has higher resolu tion and less influence on the tip and better anti-interference capability. Obs erved results of the graphite are given and discussed in this paper. 相似文献
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A. Busiakiewicz A. Huczko M. Puchalski M. Cichomski Z. Klusek 《Applied Surface Science》2010,256(15):4771-4776
For the first time the scanning tunneling microscopy (STM) and scanning tunneling spectroscopy (STS) are employed to investigate the morphology and the surface electronic structure of the defective silicon carbide nanowires (SiCNWs). The SiCNWs produced via combustion synthesis route are studied. The STS measurements are performed in the current imaging tunneling spectroscopy mode (CITS) that allows us to determine the correlation between STM topography and the local density of electronic states (LDOS) around the bend of an isolated SiCNW. The measurements reveal fluctuations of LDOS in the vicinity of the defect. The local graphitisation and the inhomogeneous concentration of doping impurities (e.g. nitrogen, oxygen) are considered to explain these fluctuations of metallic-like LDOS in the vicinity of the SiCNW's deformation. 相似文献
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Conductance histograms of palladium nanocontacts in ultra high vacuum (UHV) were experimentally studied at room temperature using scanning tunneling microscope (STM). Our results show that the resolution of the pure Pd peaks, at 1.8 and around 3G0, in the histograms, depends on the bias voltage and the electrodes size. The size of the electrodes should be as small as possible to achieve the higher extraction of hydrogen from them and therefore preventing the diffusion of H from the bulk to the nanocontacts during the conductance measurements, particularly at low bias voltage. This could explain why peaks have not been observed previously in the Pd histograms, using STM techniques in UHV. 相似文献
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Ilya Grigorenko J. Lee J.C. Davis H. Eisaki Alexander V. Balatsky 《Journal of Physics and Chemistry of Solids》2008,69(12):3000-3005
Superconducting excitations—Bogoliubov quasiparticles—are the quantum mechanical mixture of negatively charged electron (−e) and positively charged hole (+e). Depending on the applied voltage bias in scanning tunneling microscope (STM) one can sample the particle and hole content of such a superconducting excitation. Recent STM experiments offer a unique insight into the inner workings of the superconducting state of superconductors. We propose a new observable quantity for STM studies that is the manifestation of the particle-hole dualism of the quasiparticles. We call it a Bogoliubov angle. This angle measures the relative weight of particle and hole amplitude in the superconducting (Bogoliubov) quasiparticle. We propose that this quantity can be measured locally by comparing the ratio of tunneling currents at positive and negative biases locally. This Bogoliubov angle allows one to measure directly the energy and position dependent particle-hole admixture and therefore visualize robustness of superconducting state locally. It may also allow one to measure the particle-hole admixture of excitations in normal state above critical temperature and thus may be used to measure superconducting correlations in pseudogap state. 相似文献