同位旋对用裂变截面探测鞍点前摩擦的影响

耦合了轻粒子发射的随机Langevin模型被用于计算三个Bi裂变系统因核耗散效应引起的相对于标准统计模型预计的裂变截面值的变化,σ_fdrop作为激发能的函数。发现209Bi的σ_fdrop要大于202Bi和195Bi的σ_fdrop,这表明高同位旋系统209Bi的裂变截面对摩擦强度有更大的敏感性。该结果建议,当实验上使用裂变激发函数来更精确地提取鞍点前摩擦强度时,应产生具有高同位旋的复合核。进而,通过Langevin计算拟合p+206Pb和p+209Bi反应的裂变激发函数数据,提取的鞍点前摩擦强度为（3~5）×1021 s-1。Langevin models that are coupled with particle emission are applied to calculate the drop of fission cross section caused by friction over its standard statistical-model value, σ_fdrop, as a function of excitation energy for three Bi nuclei with different isospins. We find that σ_fdrop become larger for 209Bi than for 202Bi and 195Bi, indicating a greater sensitivity of fission cross section to friction for high-isospin 209Bi. These results suggest that, to more accurately determine the presaddle dissipation strength by measuring fission excitation functions, it is best to populate those compound systems with a high isospin. Furthermore, we analyze the data of fission excitation functions measured in p + 209Bi and p + 208Pb reactions, which yield high-isospin 210Po and 209Bi systems, and extract a presaddle friction strength of (3-5)×1021 s-1 by comparing Langevin simulations with these experimental data.     

重核存活几率的N/Z效应

用Langevin方程计算了重核 194Pb, 200Pb和206Pb的蒸发残余形成几率。结果表明系统中质比(N/Z）影响了该几率大小,并且高的N/Z增加了重核存活几率。这是由于裂变位垒和鞍点前粒子发射依赖于系统N/Z的缘故。     

100,104Sn核在裂变过程中发射的轻粒子多重性

用扩散模型考察了轻的幻核¹⁰⁰Sn在裂变过程中蒸发的轻粒子多重性. 发现壳仅对质子的发射有很强的影响, 而对中子几乎没有影响, 这与¹³²Sn核的情况正好相反. 因此把这种现象归因于系统中质比(N/Z)的影响. 通过比较¹⁰⁴Sn和¹⁰⁰Sn发射的粒子, N/Z的 影响得到了进一步证实. 计算发现高激发能弱化了N/Z效应.     

重核的断前粒子发射与鞍点后摩擦的探测

基于考虑了粒子发射的随机Langevin模型,计算了重裂变核240Am在 鞍点后发射的中子、质子和$ \alpha $粒子多重性作为鞍点后摩擦强度($ \beta $)的函数。结果表明在高激发能($ E^* $)和高角动量($ \ell $)条件下,这些轻粒子发射对摩擦的敏感性变强。进而,比较了在(高$ E^* $,低$ \ell $)和(低$ E^* $,高$ \ell $)这两个不同初始条件下,240Am核在鞍点后蒸发的粒子随$ \beta $的演化。发现前者不但能增强核摩擦对粒子发射的影响,也显著提高了带电粒子对$ \beta $的敏感性。在实验方面,我们建议可以用中能重离子碰撞的方式产生高激发的重裂变系统,来更精确地用粒子发射(尤其是轻带电粒子)来探测鞍点后的摩擦强度。     

Gammasphere上裂变丰中子核核结构若干前沿领域的新进展(Ⅰ:第一和第二部分)(英文)

(第一和第二部分):使用Gammasphere多探测器系统对252Cf裂变源瞬发γ射线进行γ-γ-γ和γ-γ(θ)符合测量,裂变丰中子原子核核结构若干前沿领域的深入研究获得了新的进展。高达5.7×1011以上的三重和更高重符合事件的数据统计,以及更少压缩的三维数据为宽广未知丰中子核区的寻找和研究提供了有利的条件。在具有重要物理意义的若干丰中子核区首次建立,或显著扩展了一批包括转晕态和转晕附近能态的高自旋能级纲图。在偶-偶丰中子核110,112Ru和108Mo中鉴别出了手征对称破缺结构。丰中子110,112Ru附近核的三轴形变基态具有最低的能量,在它们之中已确认了接近最大值的三轴形变。在这些Ru和Mo同位素中观察到的手征双线能带展示出手征破缺的一切特征,特别是其理想的能量简并,表明它们在迄今已报道的手征破缺结构中,具有最好的手征特性。研究了手征结构从具有γ软度的108Ru到具有大三轴形变的110,112Ru的过渡。斜轴推转(TAC)和随机相近似(RPA)理论计算成功地拟合了在这些偶-偶丰中子核中观察到的手征双线能带的特性,并指定其为软手征振动态。在这些偶-偶核中观察到的手征破缺不可能归纳为奇-奇核中那样的简化的几何图像。前者来自闭壳外所有中子的相互作用。对双幻核132Sn附近N=83同中素链的系统研究为这个极富吸引力的核区提供了大量新的谱学信息。N=83同中素135Te(Z=52),136I(Z=53),137Xe(Z=54),138Cs(Z=55)和139Ba(Z=56)的最新能级信息,特别是首次建立的138Cs高自旋能级纲图和壳模型理论计算表明,Z=50质子闭壳外少数g7/2价质子激发同N=82中子闭壳外之唯一f7/2价中子的耦合对该核区能级结构具有关键作用。观察到了132Sn和208Pb附近核区谱学信息的相似性和相对应的三粒子和五粒子态。在135Te中观察到了磁转动,这是在双幻核132Sn附近观察到的首例磁转动。     

同位旋对断前粒子发射影响的角动量依赖性

对一个同量异位素链²⁰²Fr,²⁰²Po,²⁰²Tl和一个同位素链^189,202,212Po,用裂变扩散模型考察了角动量对裂变前粒子发射同位旋效应的影响.发现断前粒子发射的同位旋效应敏感地依赖于系统的自旋.高的角动量不但弱化了同位旋对粒子蒸发的影响,而且也降低了核耗散对粒子发射的影响.因此,为了更准确地用粒子多重性来提取核耗散系数,选择一个低自旋的复合系统是重要的     

非全熔合反应裂变角分布

采用核固体径迹探测器测量了¹⁶O+¹⁵⁹Tb、¹⁶O+¹⁹⁷)Au和¹⁶O+²⁰⁹Bi反应碎片角分布,扣除中等质量碎片(IMF)的贡献,用过渡态统计模型(TSM)和单个自旋标准理论拟合实验的裂变角分布,提取裂变核的自旋. 讨论了它随质心系入射能量的变化.     

Bi对自旋阀钉扎场的影响及机理

实验发现将Bi插入自旋阀多层膜TaNiFeCuBi(x)NiFeFeMn中可以显著地提高自旋阀的钉扎场Hex.采用XPS对Cu,Bi元素的分布情况进行了研究,发现Bi的插入明显抑制了Cu原子在自旋阀的制备过程中在NiFeFeMn界面的偏聚.进一步研究表明:自旋阀钉扎层NiFeFeMn界面中,Cu原子的存在是导致自旋阀Hex小于TaNiFeFeMn多层膜Hex的主要原因. 关键词： 自旋阀 钉扎场 交换各向异性 表面活化剂     

质子数Z分别位于Ru之上和之下的A～(100～126)丰中子原子核三轴形变在原子核形状变迁和共存中的重要作用（英文）

基于Ru(Z=44)丰中子同位素中存在最大三轴形变的理论预言和实验证据,综述了近年来Rh(Z=45),Pd(Z=46),Ag(Z=47),Cd(Z=48)(质子数Z位于Ru,Z=44之上)及Zr(Z=40),Nb(Z=41),Mo(Z=42),Tc(Z=43)(质子数Z位于Ru,Z=44之下)的A～(100～126)丰中子同位素中关于三轴形变的形状变迁和形状共存系统性研究的重要进展。252Cf自发裂变瞬发γ射线γ-γ-γ三重符合、特别是新建立的γ-γ-γ-γ四重符合数据的系统观测和研究,在Ru,Pd,Cd和Nb丰中子同位素中显著扩展或首次观测到了一系列能带,为这个核区原子核形状的研究提供了新的、重要的实验数据。联系此前报道的有关进展,使用PES,TRS,PSM,CCCSM和SCTAC理论模型计算拟合新的实验数据,在该核区沿同中素和同位素链,并随自旋和激发能变化各自由度,跟踪原子核形状渐进变化,获得了新的系统性研究成果,显著扩展和深化了人们对原子核形状变迁和形状共存的认知。对于Ru及其上的Rh(Z=45),Pd(Z=46),Ag(Z=47)和Cd(Z=48)丰中子同位素的研究表明:Rh丰中子核具有比最大值稍小的三轴形变,γ=-28°,并在103–106Rh同位素链上鉴别出了手征对称破缺;在三轴形变核112Ru和114Pd(N=68)中发现了三轴原子核的摆动运动,该摆动运动也可能在114Ru(N=70)中存在;观察到了从具有最大三轴形变的110,112Ru中手征破缺到稍小三轴形变的112,114,116Pd中扰动的手征破缺的过渡;在较软的Ag核中观察到了丰富的谱学结构,在104,105Ag中鉴别出了可能的手征对称破缺,在较重的115,117Ag中提出了趋于三轴形变的γ软度;具有小形变的Cd核的能级结构被解释为准粒子耦合、准转动和软三轴形变;最近的库伦激发的研究提供了Z=50,N=82满壳附近122,124,126Cd核中出现核集体性的实验和理论证据;上述研究成果展现出从Ru中的最大三轴形变(γ=-30°,三轴形变极小增益为0.67 Me V),经具有大三轴形变的Rh核(γ=-28°),到Pd核中的稍小、但稳定于中等自旋到高自旋区的三轴形变(γ～-41°,三轴形变极小增益为0.32 Me V),再经Ag核中的γ软度,最后到具有很小形变、但仍出现集体性质、包括软三轴形变的Cd核的过渡。对于Pd核转动带交叉系统性的研究揭示了其第一带交叉(νh11/2)2中子转动顺排的上行γ驱动,和第二带交叉(πg9/2)2质子转动顺排的下行γ驱动效应,成功地解释了114Pd中的三轴摆动运动,并给出了110-118Pd同位素链中理论早已预言、而比早期理论预言更为完整准确的形状渐进变迁和形状共存的图像。根据该核区的系统研究,发现最大三轴形变出现在112Ru,而在相邻的偶Z(Pd)同位素链,三轴形变极小的中心在114Pd,两者均为N=68。上述系统性研究沿相邻的Ru和Pd偶Z同位素链,在N=68同中素中鉴别出最大三轴形变,均比理论预言的108Ru和110Pd多4个中子。在Z值位于Ru(Z=44)之下的Zr(Z=40),Nb(Z=41),Mo(Z=42)and Tc(Z=43)丰中子同位素中,Y和Zr核具有很强的轴对称四极形变,而在较重的Zr同位素中出现了γ自由度;较重的Nb核(A=104～106)基态具有中等程度的软三轴形变和强四极形变,随着自旋和激发能的增加,过渡到接近于轴对称的强四极形变;而较轻的Nb核(A 103)基态均接近轴对称形状;在Nb同位素链上基态由球形到强四极形变的形状突变发生在100Nb(N=59),在100–106Nb同位素链中基态的软三轴形变随中子数增加而增加;在Nb核中还观察到关于软三轴形变的形状共存;Mo核具有大的三轴形变,观察到了γ振动和手征对称破缺;Tc核具有比最大值稍小的三轴形变,γ=-26°,并观察到了手征对称破缺。质子数Z从41到48的A～(100～126)丰中子同位素,特别是Pd和Nb同位素,呈现出关于三轴形变的过渡特征。     

含Hopf项和Maxwell-Chern-Simons项O(3)非线性σ模型的分数自旋和分数统计性质

研究了（2＋1）维时空中含Hopf项和Maxwell-Chern-Simons(MCS)项的非线性σ模型的分数自旋性质.根据约束Hamilton系统的Faddeev-Senjanovic(FS)路径积分量子化方案,对该系统进行量子化，由量子Noether定理给出了量子守恒角动量，说明了在量子水平上该系统仍具有分数自旋的性质. 关键词： 约束Hamilton系统 分数自旋 O(3)σ模型     

Influence of Isotope on Shell Effects of Pre-scission Particle Evaporation

The shell effects on the particle evaporation prior to fission for three Pb isotopes, 204pb, 20sPb, and 212pb,as well as three Sn isotopes, 128Sn, 132Sn, and 136Sn, are explored by a diffusion model. Calculations show that the magnitude of shell effects in the emission of particles changes with the neutron-to-proton ratio N/Z of these fissioning nuclei, and this change is affected significantly by the spin and excitation energy of the system. It is shown that high angular momentum enhances the dependence of shell effects on the N/Z while high excitation energy weakens such a dependence.     

Influence of Isotope on Shell Effects of Pre-scission Particle Evaporation

The shell effects on the particle evaporation prior to fission for three Pb isotopes, ^204Pb, ^208Pb, and ^212pb,as well as three Sn isotopes, ^128Sn, ^132Sn, and ^136Sn, are explored by a diffusion model. Calculations show that the magnitude of shell effects in the emission of particles changes with the neutron-to-proton ratio N/Z of these fissioning nuclei, and this change is affected significantly by the spin and excitation energy of the system. It is shown that high angular momentum enhances the dependence of shell effects on the N/Z while high excitation energy weakens such a dependence.     

Role of N/Z in Pre-scission Neutrons as an Observable of Nuclear Friction

A dynamical Langevin model is employed to evaluate the excess of the neutron emission in the fission of heavy nuclei ²⁴⁰Cf, ²⁴⁶Cf, ²⁵⁴Cf, ²⁴⁰U relative to the standard statistical-model prediction at various saddle-to-scission friction strengths. It is shown that when the neutron-to-proton ratio N/Z of the system increases, the sensitivity of the excess to the friction decreases substantially, and it almostdisappears for ²⁴⁰U. We suggest that using those compound systems with low N/Z favors an accurate determination for the saddle-to-scission friction strength based on the measurement of the pre-scission neutron multiplicity.     

激发能相关的能级密度参数和重核衰变性质(英文)

基于裂变的随机模型,研究了能级密度参数在鞍点与其基态处的比值a_f/a_n在热核衰变过程中的作用。计算表明,a_f/a_n的大小能显著影响蒸发剩余截面及其自旋分布的大小以及裂变过程中热核的耗散行为。发现,能级密度参数对激发能的依赖性a_f/a_n(E*) 能改变断点处的激发能对摩擦强度的敏感性。最后指出了a_f/a_n随E* 的变化对超重核的稳定性和散裂反应退激阶段描述的意义。Based on the stochastic approach to fission, we have demonstrated that the ratio of level-density parameters at saddle to that at ground-state configuration, af/an, plays a significant role in the decay of an excited nucleus. It modifies not only the sensitivity of evaporation residue cross section and its spin distributionsto nuclear friction, but also the dissipation properties of hot nuclei. Furthermore, we find that af/an as a function of excitation energy appreciably affects the evolution of excitation energy at scission with the friction strength. A consequence of a change of af /an with E* on the stability of superheavy nuclei and on modelling de-excitation processes of spallation reactions is indicated.     

MEASUREMENTS OF ANGULAR MOMENTUM EFFECT OF FISSION BARRIER

The fission cross sections and the evaporation residue cross sections for ¹²C+²⁰⁹Bi and ¹⁴N+Pb reactions were measured with the gold surface barrier silicon detectors and the mica nuclear track detectors.The critical angular momentum l_er was deduced from the measured evaporation residue cross section σ_er on the basis of the sharp-off model.The fission barrier with the particular angular momentum i derived from the condition Γ_f/Γ_n=1 at l=l_e The angular momentum effect of the fission barrier was studied experimentally.     

Effects of N/Z on survival probability of heavy nuclei

The excitation functions of the evaporation residue formation probability of three heavy nuclei 194Pb, 200Pb and 206Pb are calculated by using a Langevin equation coupled with a statistical decay model.The results show that the neutron-to-proton ratio (N/Z) of a compound nucleus has an effect on survival probability and this effect becomes larger with increasing N/Z. This is because the fission barrier and the pre-saddle particle emission depend on the N/Z ratio of the system.     

裂变路径对断点前粒子发射的影响

用扩散模型研究了裂变系统从鞍点到断点的时间演化, 以及在此间的粒子发射与鞍点前粒子发射的比随着裂变系统质量的变化. 解释了实验上发现的断点前粒子多重性随裂变碎片质量不对称性的变化趋势. 结果表明上述两种变化趋势都可以归因于裂变演化路程长短的影响.     

New type of asymmetric fission in proton-rich nuclei

A very exotic process of β-delayed fission of 180Tl is studied in detail by using resonant laser ionization with subsequent mass separation at ISOLDE (CERN). In contrast to common expectations, the fission-fragment mass distribution of the post-β-decay daughter nucleus 180Hg (N/Z=1.25) is asymmetric. This asymmetry is more surprising since a mass-symmetric split of this extremely neutron-deficient nucleus would lead to two 90Zr fragments, with magic N=50 and semimagic Z=40. This is a new type of asymmetric fission, not caused by large shell effects related to fragment magic proton and neutron numbers, as observed in the actinide region. The newly measured branching ratio for β-delayed fission of 180Tl is 3.6(7) × 10(-3)%, approximately 2 orders of magnitude larger than in an earlier study.     

Fusion-fission angular distributions: A new probe of fast fission fractionation in nucleus-nucleus collisions

Fragment angular distributions in heavy ion-induced fission reactions have been analysed in terms of a two component model—fission following compound nucleus formation and fast fission events. It is seen that, contrary to the general assumption, fast fission competes with compound nucleus fission even when the composite system is formed with a spin less than the rotating liquid drop model limit for vanishing fission barrier.