Transient energy transfer between writing beams during hologram formation in Bi12GeO20

A large transient energy transfer between writing beams during volume phase-hologram formation in Bi₁₂GeO₂₀ has been observed. The variation of the energy transfer by applying an external field and by changing the fringe spacing of the elementary holograms have been measured and described in the framework of Kukhtarevs nonlinear theory of transient self-diffraction. The results indicate that the transient energy transfer in Bi₁₂GeO₂₀ is due to a non-stationary phase mismatch between the intensity- and refractive index grating caused by photoconductivity and that the transient energy transfer increases with increasing fringe spacing and increasing applied electric field. Up to ten-fold amplification of coherent beams has been measured, corresponding to an exponential gain of Г = 2 cm^-1. A continuous energy transfer has been observed when the phase between recording beams was changed linearly with time during recording. It is shown that light is coherently amplified for electric field strengths larger than 2.3 kV/cm and that a peak amplification factor of Г₁ = 2 cm^-1 has been reached for E₀ = 11 kV/cm.     

Transient energy transfer during hologram formation in LiNbO3 in external electric field

Volume phase hologram recording in pure LiNbO₃ crystals with applied electric field E ≈ 5 kV/cm is accompanied by considerable intensity redistribution of the writing beams by transient energy transfer. Practically the whole intensity of the donor beam may be transferred into the weak acceptor beam with initial intensity 3% from total incident intensity. This effect originates from transient phase mismatch of the recorded phase grating and fringe pattern in the applied electric field when the interacting beams have different intensities.     

The nonparaxial propagation of the TEM0l doughnut beam with the orbital angular momentum in the far field

The analytical expression for nonparaxial electric field amplitude of the TEM_0l^? doughnut beam with the orbital angular momentum quantum number l is derived in the far field by means of the angular spectrum representation and the stationary phase method. It is shown that the divergent angle of the far field of TEM_0l^? doughnut beam will be smaller with the decreasing of the orbital angular momentum quantum number l or the increasing of the beam waist width w of the initial beam. And the maximal radial intensity of the beam is decreased with its propagation at different rates for different l and w.     

Experimental study of the reaction νμ + e− → μ− + νe

The first observation of the reaction ν_μ + e^? → μ^? + ν_e has been made in the bubble chamber Gargamelle exposed to the CERN SPS wide-band neutrino beam. A signal of 26 ± 6 events has been found. This is 0.90 ± 0.20 times the prediction of the V - A theory.     

51V nuclear magnetic resonance in polycrystalline ferroelastic BiVO4

Nuclear magnetic resonance studies on polycrystalline ferroelastic BiVO₄ indicate that the ⁵¹V electric field gradient asymmetry parameter is an order parameter in the ferroelastic transition. Using ∩ = A(T?T_c)^B, B is found to be 0.48(5), in good agreement with earlier studies of this material. Near the phase transition above and below, the vanadium nuclear quadrupole coupling is constant with a value of 4.8(1) MHz.     

A study of π−π− scattering from π−p interactions at 3.93 GeV/c

A modified Chew-Low extrapolation procedure is applied to the reaction π^?p→Δ⁺⁺π^?π^? to extract the I = 2 ππ elastic cross sections from threshold to 1260 MeV. The predictions of the one-pion-exchange model are used to estimate the contributions from background processes of the type π^?p→Δ⁰?⁰. The moments of the π^?π^? angular distribution are also extrapolated to the pion pole and a phase shift analysis performed. The s-wave inelasticity is constrained using information on the inelastic cross section coming from six-body final states. The magnitude of the s-wave phase shift at the K⁰ mass is found to be 7.2⁰ ± 1.0⁰, increasing to 26.2⁰ ± 2.5⁰ at 1 GeV. d- and g-waves contribute above about 900 MeV, but the corresponding phase shifts are small compared with the s-wave. All three phase shifts have the same sign.     

Etude par spectrometrie Mössbauer (57Fe) de FeMo2S4

We have investigated FeMo₂S₄ by transmission Mössbauer spectroscopy on the ⁵⁷Fe nucleus between 4.2 and 1037 K, using both powdered and single crystal samples.The temperature dependences of the isomer shift and the quadrupole splitting indicate the existence of ferrous ions with well localized 3d electrons. The two different crystallographic Fe sites cannot be separated over the experimental temperature range. The local symmetry of the iron site is lower than axial (η ~ 0.47) and the crystal field splittings Δ₁ and Δ₂ of the Fe²⁺ ? T_2g Orbitals, estimated by the Ingalls' method, are close to 250 and 900 cm^?1.The hyperfine field makes an angle of 14° with the normal on the plane (a, b), deviating a little from the direction of the magnetic moments determined to be perpendicular to (a, b) by neutron diffraction study.At higher temperatures, and more particularly near T_N, a line broadening is observed, and the spectra have to be fitted by a hyperfine field distribution. The broadening comes from the presence of about 7% “abnormal” Fe-sites observed in the paramagnetic spectra, and whose origin is discussed.The Néel temperature was determined to be 112 ± 1 K for the powdered sample and 106 ± l K for the single crystal.     

Crystal field splitting of Pr3+ in PrAl2 investigated by inelastic neutron scattering

We report the.results of an experimental determination of the crystal field splitting of Pr³⁺ in PrAl₂ by means of inelastic neutron scattering. For the crystal field parameters we obtain B₄ = (47.2 ± 4.0) × 10^?4 meV and B₆ = ? (156 ± 12) × 10^?6 meV.     

Ferromagnetic resonance in the randomly mixed insulating ferromagnet and antiferromagnet Rb2Mn(1-x)CrxCl4

An electron spin resonance experiment has been performed on the Cr-rich concentrations of the random mixture Rb₂Mn(_1-x)Cr_xCl₄ of an insulating ferromagnet (Rb₂CrCl₄) and an insulating antiferromagnet (Rb₂MnCl₄). The resonance fields in x = 0.6, 0.7 and 0.8 samples begin to shift towards low field side at temperatures well above the Curie temperatures, when the external field is applied in the c-plane of the crystal. The shift of the resonance field with temperature of the x = 0.7 sample agreed well with that of the x = 0.8 sample, after scaling the temperature axis, while the shift in the x = 0.6 crystal did not. From this observation, we argue that the x = 0.7 and x = 0.8 samples have a long-range ordered ferromagnetic phase below T_c, and that the low temperature phase of the x = 0.6 sample is not a truely long-range ordered one. A weak resonance line was observed in the x = 0.8 sample below about 20 K. This resonance is discussed in connection with the re-entrant spin-glass behavior of this mixed system found in the ac susceptibility measurement.     

Absorption spectra of C6H6 and C6D6 near 340 nm

The absorption spectra of C₆H₆ and C₆D₆ in the liquid phase have been studied near 340 nm. The absorption spectrophotometric mounting was a sequential double-beam attachment with linear response to energy on scanning of the spectrum before the exit slit and an electronic device which gives directly either the absorbance or the integrated absorbance of a transition and, consequently, its oscillator strength.The oscillator strength measured for the band of C₆H₆ is 8×10^?8, which corresponds to a dipole moment of 2.4×10^?3 Debye; this value is of the same order as a theoretical value calculated by Tsubomura and Mulliken (3.8×10^?3 Debye) for a transition between states ³F and ³A of an oxygen-benzene pair. This agreement corroborates the hypothetical existence of such a transition.The first vibrational band is at 28553 cm^?1 for C₆H₆; this band is not observed in the vapor or solid phase. It corresponds probably to the transition 0-0, which is considered in the literature to be near 29500 cm^?1. The isotopic shift measured for this first band is 164 cm^?1. The vibrational frequencies are, respectively, 910 cm^?1 for C₆H₆ and 889 cm^?1 for C₆D₆.     

Electron paramagnetic resonance in the system CaO-SiO2-Al2O3 containing sulfur

An EPR absorption was detected in the system CaO-SiO₂-Al₂O₃ doped with sulfur. The signal consisted of six isotropic hyperfine lines and demonstrated isotropic fine structure and forbidden doublets. The signal was attributed to an Mn²⁺ impurity displacing Ca²⁺ in fine CaS crystallites formed in the matrix of the ternary system. The spectrum was well accounted for with the parameters g = 2.0021 ± 0.0001 and A = ?77.1 ± 0.6 × 10^?4 cm^?1. Sample preparation conditions did not affect the hyperfine splitting, although the fine structure and forbidden lines proved to be dependent on the conditions of preparation. It is suggested that the appearance of the fine structure is a result of the second effect of the hyperfine structure when the cubic field parameter a approaches zero and, consequently, the structure is free of superposition caused by an anisotropic shift determined by a. We ascribe the change in fine structure to the variation in a and discuss the nature of the energy splitting of the ${}^6\text{S}{}_{\mathrm{<mtext>5</mtext><mtext>2</mtext>}}$ state in a cubic field. We also note a correlation between the fine structure and the forbidden lines. This finding suggests that a is not necessarily specific to the host lattice and, furthermore, that the consideration of superposition of axial or lower symmetry upon the original cubic field of the central Mn²⁺ ion is vital for the determination of a.     

Raman study of charge-density-wave phase transition in quasi-one-dimensional conductor (TaSe4)2I

Polarized Raman spectra were obtained in the quasi-one-dimensional conductor (TaSe₄)₂I above and below the charge-density-wave (CDW) transition temperature (T_c=263 K). The Raman intensities of many peaks become intenser and two of the phonon peaks shift to higher frequency with decreasing temperature. Moreover a new broad peak at about 90 cm^?1 and a new peak around 166 cm^?1 appear in the low-temperature phase. The polarization characteristic shows that the former is assigned to totally symmetric mode. The damping constant of the phonon at 90 cm^?1 increases markedly with increasing temperature. The frequency shifts to higher frequency as the temperature increases and the coupling coefficient is approximately proportional to (T_c?T)^{$\text{1}\text{2}$}. This peak becomes Raman active owing to the CDW phase transition. The temperature dependence of the damping constant and the frequency shift may have a relation to the dynamical properties of the CDW phase transition.     

Bulk magnetization study of a DyNi5 single crystal

Magnetization and susceptibility measurements were performed on a single crystal of DyNi₅ along the three main symmetry axes of the ortho-hexagonal cell. Below its ordering temperature (T_c = 11.6 K), b and c are respectively the easy and hard magnetization axes. The strong anisotropy originates from the crystalline electric field acting on the 4f electrons of the Dy³⁺ ions. A small magnetization is induced on nickel atoms by the applied field and the exchange interactions with the dysprosium atoms. The crystal field parameters, the molecular field coefficients and the susceptibility of nickel atoms are determined from the experimental data.     

Metamagnetism in ErGa2 studied on a single crystal

Magnetization measurements and neutron difrraction experiments were performed on a single crystal of ErGa₂. Because of the strong crystal field effects a huge uniaxial anisotropy imposes the Er moments to be parallel to the c-axis of the hexagonal structure. We have shown that the transition from the antiferromagnetic structure to the ferromagnetic one, when the field is applied along c, occurs through an intermediate phase. Such a behaviour is very well accounted for using a simple Ising-like model which takes into account first and second nearest neighbours exchange interactions in the hexagonal layers. A quantitative determination of the crystalline electric field effects is also presented.     

Spatial frequency dependence of the energy transfer in two-wave mixing experiments with BSO crystals

Energy transfer between two beams interfering in an electrooptic Bi₁₂SiO₂₀ crystal is analyzed as a function of the spatial frequency of the recorded hologram. We report high coefficients in a wide range of low spatial frequencies $\text{(Λ}{}^{-1}\text{?44 mm}{}^{-1}\text{)}$, when the drift length of the photocarriers becomes comparable to the fringe spacing. Exponential gain coefficients of Γ = 7 cm^-1 have been reached for high intensity beams ratio (β > 10⁴) and an optimized fringe displacement speed (moving grating recording). Application to coherent image amplification (×20) is shown.     

Analysis of the optical spectrum of Ho3+ in LiYF4

The energy levels for Ho³⁺ in single crystal LiYF₄ from 0–21,300 cm^?1 have been determined from polarized absorption and fluorescence spectra using crystals at temperatures between 4 and 300°K. Energy level assignments were made initially by comparing the crystal spectra with energy levels calculated by using crystal field parameters interpolated from previously reported analyses of Nd³⁺, Er³⁺ and Tm³⁺ in LiYF₄. The energy level scheme identifies energy levels in the 10 lowest J-multiplets and gives calculated energies for the next six higher J-multiplets. The crystal field parameters were varied to obtain a best fit between experimental and theoretical energies, and the final values B₂₀ = 410, B₄₀ = ? 615, B₄₄ = 819, B₆₀ = ? 27.9 and B₆₄ = 677 ± i32.8 cm^?1 give an r.m.s. fit of 2.78 cm^?1. The calculations were made by diagonalizing the crystal field Hamiltonian, H_x = Σ_kmB_kmC_km, in the space of ten lowest J-multiplets spanned by intermediate coupled free-ion wavefunctions calculated using the free-ion parameters of Carnall et al. for Ho in aqueous solution. The calculated g_∥ for the Γ_3.4 ground state of 13.63 compares favorably with a previously reported value of 13.3 ± 0.1.     

Optical decoherence and persistent spectral hole burning in Tm:LiNbO3

We report studies of decoherence and spectral hole burning for the 794 nm optical transition of thulium-doped lithium niobate. In addition to transient spectral holes due to the ³H₄ and ³F₄ excited states of Tm³⁺, persistent spectral holes with lifetimes of up to minutes were observed when a magnetic field of a few hundred Gauss was applied. The observed anti-hole structure identified the hole burning mechanism as population storage in the ¹⁶⁹Tm nuclear hyperfine levels. In addition, the magnetic field was effective in suppressing spectral diffusion, increasing the phase memory lifetime from 11 μs at zero field to 23 μs in a field of 320 Gauss applied along the crystal’s c-axis. Coupling between Tm³⁺ and the ⁷Li and ⁹³Nb spins in the host lattice was also observed and a quadrupole shift of 22 kHz was measured for ⁷Li at 1.7 K. A Stark shift of 18 kHz cm/V was measured for the optical transition with the electric field applied parallel to the c-axis.     

Self-pulsation and optical chaos in self-pumped photorefractive BaTiO3

Sinusoidal intensity oscillations of the phase conjugated wave reflected from a self-pumped photorefractive BaTiO₃ crystal have been observed. The oscillation amplitude is shown to be increased by providing optical feedback of the light scattered during grating formation. The oscillation frequency ? can be tuned from 0.024 Hz to 2 Hz by changing the light intensity I₀ of the object beam from 0.7 W/cm² to 100 W/cm². A power law ? ∝ I^β₀ ∝ σ with β = 0.89 was observed over this range of intensities (σ = photoconductivity). Transitions to a chaotically oscillating or a stable reflecting state have been observed at higher power levels or with increased optical feedback. An additional pump beam near the entrance face of the signal beam can decrease the build-up time for the self-pumping process by a factor of five or more.     

激光辐照非晶Fe73.5Cu1Nb3Si13.5B 9微量晶化的穆斯堡尔谱研究

在激光功率为40—160W、扫描速度为10mm/s、激光光斑为20mm照射条件下,用CO ₂激 光辐照非晶Fe_73.5Cu₁Nb₃Si_13.5B_{9< /sub>产生微量晶化.利用透射穆斯堡尔谱 （TMS）技术分析了原始态和晶化后样品的超精细结构.确定了穆斯堡尔谱的基本参数——化 学位移(IS)、四极分裂(QS)、内磁场(Hhf)随激光功率变化的规律.分析表明，CO2关键词： 激光辐照 微量晶化 73.5Cu1Nb3 Si13.5B9')" href="#">非晶Fe73.5Cu1Nb3 Si13.5B9 穆斯堡尔谱}     

Light-induced charge transfer processes in Mn-doped Bi12GeO20 and Bi12SiO20 single crystals

The optical absorption and ESR spectra of Bi₁₂GeO₂₀ and B₁₂SiO₂₀ doped with Mn have been measured before and after illumination with visible light. Uniaxial stress measurements on a sharp line observed at 8026 cm^?1 were performed. The observed ESR spectrum is a superposition of six lines resulting from the hyperfine interaction of manganese ions in tetrahedral positions. The g-factor and hyperfine constant are g = 1.999 ± 0.003 and A = 78 Gs. Analysis of the light-induced absorption spectrum leads to the conclusion that a small hole polaron bound to an Mn impurity at a tetrahedral site is responsible for the very broad absorption band which appears after illumination. The sharp line is interpreted as due to a transition inside the Mn⁺ center in tetrahedral coordination. Bands in the region 10,000–16,000 cm^?1 are due to Mn³⁺ centers in interstitial positions, whose symmetry can be treated to a first approximation as tetragonal. The following crystal field parameters for this center were found: B = 565 cm^?1, Dq = 1400 cm^?1, Dt = ?330 cm^?1, Ds = 4170 cm^?1 and C = 2260 cm^?1. The illumination conditions which are needed for homogeneous coloration of the sample are also discussed.